Plasma Chemistry and Plasma Processing最新文献

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Integrated Transport Model for Controlled Delivery of Short-Lived Reactive Species via Plasma-Activated Liquid with Practical Applications in Plant Disease Control 通过等离子激活液控制短效活性物质传输的综合传输模型及其在植物病害控制中的实际应用
IF 3.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-06-08 DOI: 10.1007/s11090-024-10461-z
Toshiro Kaneko, K. Takashima, S. Sasaki
{"title":"Integrated Transport Model for Controlled Delivery of Short-Lived Reactive Species via Plasma-Activated Liquid with Practical Applications in Plant Disease Control","authors":"Toshiro Kaneko, K. Takashima, S. Sasaki","doi":"10.1007/s11090-024-10461-z","DOIUrl":"https://doi.org/10.1007/s11090-024-10461-z","url":null,"abstract":"","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":3.6,"publicationDate":"2024-06-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141369360","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The Biosafety of Periodontal Ligament Fibroblasts Induced by Cold Atmospheric Plasma in vitro: Cytotoxicity, Genotoxicity and Mechanisms 冷大气等离子体体外诱导牙周韧带成纤维细胞的生物安全性:细胞毒性、遗传毒性和机制
IF 2.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-06-08 DOI: 10.1007/s11090-024-10482-8
Xiaojiao Zhang, Yinglong Li, Ruonan Ma, Zhitong Chen, Ruixue Wang, Zuomin Wang
{"title":"The Biosafety of Periodontal Ligament Fibroblasts Induced by Cold Atmospheric Plasma in vitro: Cytotoxicity, Genotoxicity and Mechanisms","authors":"Xiaojiao Zhang,&nbsp;Yinglong Li,&nbsp;Ruonan Ma,&nbsp;Zhitong Chen,&nbsp;Ruixue Wang,&nbsp;Zuomin Wang","doi":"10.1007/s11090-024-10482-8","DOIUrl":"10.1007/s11090-024-10482-8","url":null,"abstract":"<div><p>Cold atmospheric plasma (CAP) has been reported as a promising technique in dentistry. The biosafety and mechanisms on periodontal tissue are especially important in clinical practice. This study aims to evaluate the cytotoxicity, genotoxicity and mechanisms of human periodontal ligament fibroblasts (hPDLFs) induced by CAP. The antimicrobial effect on <i>Porphyromonas gingivalis (P. gingivalis)</i> was evaluated using the colony-forming unit methods (CFU). Human periodontal ligament fibroblasts were treated with CAP for variable times (1, 2, 4, 8, and 16 min). CCK-8 assays were performed to detect cell viability and flow cytometry was performed to measure the cell cycle and apoptosis. Cell migration ability was determined by scratch assays. The physicochemical properties of plasma activated medium were evaluated, including the pH values, H<sub>2</sub>O<sub>2</sub> and NO levels. DCF-DA staining and analysis were performed to evaluate intracellular ROS levels inside cells using flow cytometry. Immunofluorescence of DNA double-strand breaks (DSBs) marker, phosphorylated γH2AX was used to establish the genotoxicity of plasma. The results showed that CAP has a significant inhibition effect of <i>P. gingivalis</i> after 6 min treatment. It has significantly dose-dependent effects that ranging from increasing cell proliferation to inducing apoptosis. A low doses (1, 2, 4, and 8 min) could enhance the cell proliferation. A high dose (16 min) resulted in the inhibition of cell proliferation (<i>p</i> &lt; 0.01). It is also shown that these effects are primarily due to the formation of reactive oxygen and nitrogen species (RONS).</p></div>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":2.6,"publicationDate":"2024-06-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141369930","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Plasma-Liquid Synthesis as a New Method for the Production of MXenes 等离子体-液体合成法作为生产 MXenes 的新方法
IF 2.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-06-08 DOI: 10.1007/s11090-024-10483-7
Nikolay Sirotkin, Anna Khlyustova, Alexander Agafonov
{"title":"Plasma-Liquid Synthesis as a New Method for the Production of MXenes","authors":"Nikolay Sirotkin,&nbsp;Anna Khlyustova,&nbsp;Alexander Agafonov","doi":"10.1007/s11090-024-10483-7","DOIUrl":"10.1007/s11090-024-10483-7","url":null,"abstract":"<div><p>In this work, the successful synthesis of nanostructures based on MXenes by initiating a pulse discharge between titanium wires immersed in carbon tetrachloride is presented. By choosing carbon tetrachloride as the environment, the formation of oxide structures in the synthesized samples could be avoided. The characterization of the obtained structures was carried out using various techniques, including scanning electron microscopy, X-ray phase analysis, EDS, Raman and FTIR spectroscopy. The results confirmed the successful formation of MXenes with a Cl<sup>−</sup> occupying the interlayer space. The properties of the discharge initiated in CCl<sub>4</sub> were also determined. The results suggest the potential of this plasma-liquid method for the synthesis of high-purity MXenes without impurities commonly found in conventionally prepared samples.</p></div>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":2.6,"publicationDate":"2024-06-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141368780","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Experimental Study of the Discharge Characteristics of a Stepped-Nozzle Arc Plasma Torch 阶跃喷嘴电弧等离子炬放电特性的实验研究
IF 2.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-06-07 DOI: 10.1007/s11090-024-10481-9
Kuan Li, Cheng Zhu, Yunfei Zhang, Zhaoyu Yu, Yuan Tian, Weidong Xia, Cheng Wang
{"title":"Experimental Study of the Discharge Characteristics of a Stepped-Nozzle Arc Plasma Torch","authors":"Kuan Li,&nbsp;Cheng Zhu,&nbsp;Yunfei Zhang,&nbsp;Zhaoyu Yu,&nbsp;Yuan Tian,&nbsp;Weidong Xia,&nbsp;Cheng Wang","doi":"10.1007/s11090-024-10481-9","DOIUrl":"10.1007/s11090-024-10481-9","url":null,"abstract":"<div><p>The stepped-nozzle arc plasma torch (SNAPT) is a promising arc source due to the advantages of high stability and high energy density, but the micro-time scale discharge characteristics have not yet been adequately investigated. In this study, a SNAPT was designed and studied, in order to investigate the effects of discharge current, gas flow rate, and nozzle morphology on the discharge characteristics. The results show that the volt-ampere characteristics of the SNAPT have an increasing curve when the gas flow rate is greater than 4 Nm<sup>3</sup>/h, and a decreasing curve when the gas flow rate is 3 Nm<sup>3</sup>/h. This result is related to the position of the arc root, and an arc constriction phenomenon occurs at high current and low gas flow rate. The thermal efficiency of the SNAPT decreases with the increasing current and decreasing gas flow rate, ranging from 69.6 to 82.3% within the experimental parameters. The optical emission spectroscopy results show that there are many active particles inside the plasma. The experimental parameters of the heavy particle temperature of 4851.5 to 9189.3 K and the electron temperature of 7846.9 to 10185.6 K both correspond to the Boltzmann distribution and are close to the local thermodynamic equilibrium state. Comparative experimental results show that the cylindrical-nozzle has the decreasing volt-ampere characteristics and higher voltages, but has large voltage fluctuations and poor stability compared with the stepped-nozzle. The results of the study are of guiding significance for design, selection of operating parameters, and application scenarios for this type of plasma torch.</p></div>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":2.6,"publicationDate":"2024-06-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141372554","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of Argon in Nitrogen Gliding Arc Plasma for Ammonium Ions Enrichment in Water 氮滑弧等离子体中的氩对水中铵离子富集的影响
IF 3.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-05-28 DOI: 10.1007/s11090-024-10473-9
Indumathy Balakrishnan, Ananthanarasimhan Jayanarasimhan, Lakshminarayana Rao, Suraj Kumar Sinha, Yugeswaran Subramaniam
{"title":"Effect of Argon in Nitrogen Gliding Arc Plasma for Ammonium Ions Enrichment in Water","authors":"Indumathy Balakrishnan, Ananthanarasimhan Jayanarasimhan, Lakshminarayana Rao, Suraj Kumar Sinha, Yugeswaran Subramaniam","doi":"10.1007/s11090-024-10473-9","DOIUrl":"https://doi.org/10.1007/s11090-024-10473-9","url":null,"abstract":"<p>This work investigates the effect of Ar addition on N<sub>2</sub> gliding arc plasma to enhance ammonium ions concentration in water. The concentration of ammonium ion <span>(left({text{N}text{H}}_{4}^{+}right))</span> increased by 50.2% when Ar gas was added upto 40% by volume to the N<sub>2</sub> gliding arc plasma, thus indicating the significant contribution of Ar in <span>({text{N}text{H}}_{4}^{+})</span> synthesis. Adding 20% Ar in N<sub>2</sub> resulted in a maximum <span>({ text{N}text{H}}_{4}^{+})</span> concentration of 16.5 ppm and a production rate of 1.31 mg hr<sup>-1</sup>. While adding 40% Ar into N<sub>2</sub> plasma, the highest energy efficiency of 0.036 g-<span>({text{N}text{H}}_{4}^{+})</span>KWh<sup>−1</sup>was obtained with a specific energy input of 742.5 J/L. The mechanisms of <span>({ text{N}text{H}}_{4}^{+})</span> enrichment with Ar addition were investigated by studying the electrical properties, vibrational, rotational and electron temperature of the gliding arc plasma with respect to the addition of Ar concentration in N<sub>2</sub> plasma. Results show that the addition of Ar raises the vibrational and electron temperatures, and decreases the rotational temperature of the gliding arc plasma. (As per the reviewer-2 suggestion, this line has been removed from the abstract). Particularly, the presence of 26.5% Ar by volume in N<sub>2</sub> plasma results in a significant ion current, which generates high ionization of <span>({text{N}}_{2}^{+})</span>.</p>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":3.6,"publicationDate":"2024-05-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141172070","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Metastable Helium Atom Creation Dynamics in High-Voltage Pulsed Discharge with Transverse Magnetic Field Effects 具有横向磁场效应的高压脉冲放电中氦原子的可迁移生成动力学
IF 2.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-05-28 DOI: 10.1007/s11090-024-10478-4
K. M. Rabadanov, N. A. Ashurbekov, K. O. Iminov, G. Sh. Shakhsinov, M. Z. Zakaryaeva, A. A. Murtazaeva
{"title":"Metastable Helium Atom Creation Dynamics in High-Voltage Pulsed Discharge with Transverse Magnetic Field Effects","authors":"K. M. Rabadanov,&nbsp;N. A. Ashurbekov,&nbsp;K. O. Iminov,&nbsp;G. Sh. Shakhsinov,&nbsp;M. Z. Zakaryaeva,&nbsp;A. A. Murtazaeva","doi":"10.1007/s11090-024-10478-4","DOIUrl":"10.1007/s11090-024-10478-4","url":null,"abstract":"<div><p>In this work, we investigate the effect of an external transverse weak magnetic field on the creation of metastable helium atoms and excited helium molecules in a high-voltage pulsed discharge in helium at medium pressure. A two-dimensional fluid model is used to describe a high-voltage pulsed discharge in helium in the external transverse weak magnetic field. The dynamics of discharge development in the high-voltage pulsed discharge in helium at a pressure of 30 Torr in the presence and absence of the magnetic field is studied. The effect of the external magnetic field on the behavior of the density of charged particles, metastable helium atoms, and excited helium molecules in the high-voltage pulsed helium discharge has been investigated. It is shown that in the discharge region, the density of metastable atoms decreases when a transverse magnetic field is applied, which is a consequence of an increase in the frequency of stepwise ionization.</p></div>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":2.6,"publicationDate":"2024-05-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141172217","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Influence of Gas Type on Reactive Species Formation, Antimicrobial Activity, and Cytotoxicity of Plasma-Activated Water Produced in a Coaxial DBD Reactor 气体类型对同轴 DBD 反应器中产生的等离子活化水的反应物形成、抗菌活性和细胞毒性的影响
IF 2.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-05-24 DOI: 10.1007/s11090-024-10475-7
F. S. Miranda, V. K. F. Tavares, D. M. Silva, N. V. M. Milhan, N. F. Azevedo Neto, M. P. Gomes, R. S. Pessoa, C. Y. Koga-Ito
{"title":"Influence of Gas Type on Reactive Species Formation, Antimicrobial Activity, and Cytotoxicity of Plasma-Activated Water Produced in a Coaxial DBD Reactor","authors":"F. S. Miranda,&nbsp;V. K. F. Tavares,&nbsp;D. M. Silva,&nbsp;N. V. M. Milhan,&nbsp;N. F. Azevedo Neto,&nbsp;M. P. Gomes,&nbsp;R. S. Pessoa,&nbsp;C. Y. Koga-Ito","doi":"10.1007/s11090-024-10475-7","DOIUrl":"10.1007/s11090-024-10475-7","url":null,"abstract":"<div><p>In this study, a coaxial dielectric barrier discharge (DBD) reactor was employed using various gases: compressed air (CA), helium (He), or argon (Ar) to produce plasma-activated water (PAW) from deionized water. The influence of these gases on the generation and quantification of reactive oxygen and nitrogen species (RONS) was examined. Their impact on PAW's physicochemical properties, including pH, oxygen reduction potential (ORP), and conductivity, was also assessed. In parallel, the efficacy of produced PAW against microbial species such as <i>Staphylococcus aureus</i>, <i>Escherichia coli</i>, and <i>Candida albicans</i> was evaluated, in addition to their cytotoxicity to mammalian cells. Notably, after a 10-min contact, a 99.99% reduction in <i>S. aureus</i> and <i>E. coli</i> was observed when CA and Ar were used, and reductions of 99.96% and 99.95% were seen when He was employed, respectively. For <i>C. albicans</i>, reductions of 12.05% with CA, 22.89% with Ar, and 39.76% with He was observed. After 30 min, a reduction of up to 53.41% was achieved with Ar. Additionally, PAW generated with all the gases were classified as non-cytotoxic. These findings underscore the potential of the coaxial DBD reactor system in PAW production, emphasizing its significant antimicrobial properties and low toxicity to mammalian cells.</p></div>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":2.6,"publicationDate":"2024-05-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141100802","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of Transient Spark Discharge and Plasma Activated Water Treatments against Fusarium graminearum Infected Wheat Grains under Laboratory Conditions 实验室条件下瞬态火花放电和等离子体活化水处理对禾谷镰刀菌感染小麦谷粒的影响
IF 2.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-05-17 DOI: 10.1007/s11090-024-10479-3
Pratik Doshi, Vladimír Scholtz, Alexandra Oplíštilová, Josef Khun, Myron Klenivskyi, Jaroslav Julák, Michal Šerý, Božena Šerá
{"title":"Effect of Transient Spark Discharge and Plasma Activated Water Treatments against Fusarium graminearum Infected Wheat Grains under Laboratory Conditions","authors":"Pratik Doshi,&nbsp;Vladimír Scholtz,&nbsp;Alexandra Oplíštilová,&nbsp;Josef Khun,&nbsp;Myron Klenivskyi,&nbsp;Jaroslav Julák,&nbsp;Michal Šerý,&nbsp;Božena Šerá","doi":"10.1007/s11090-024-10479-3","DOIUrl":"10.1007/s11090-024-10479-3","url":null,"abstract":"<div><p>Over the last decade, more and more attention has been paid to applications of non-thermal plasma in agriculture, where it is used to decontaminate various microorganisms and to improve the seed germination. In this study, we present the results of a newly developed point-to-ring NTP transient spark discharge apparatus (NTP), plasma activated water (PAW) and their combined treatment on Durum wheat and Common wheat grains under laboratory conditions. Transient spark discharge treatment was used as direct treatment while indirect treatment of wheat grains was performed by PAW produced in point-to-plane NTP transient spark apparatus. We found that the degree of grain surface decontamination was in order NTP &gt; PAW &gt; combined treatment. In the case of Durum wheat grain germination, all treatments increased germination with increasing exposure times, while in the case of Common wheat, PAW treatment and combined treatment did not significantly increase the grain germination. In conclusion, plasma treatment has enormous potential for use in agriculture and its possibilities need to be fully explored.</p></div>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":2.6,"publicationDate":"2024-05-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s11090-024-10479-3.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140965715","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Study on Synergy Between Plasma and Composite Industry Wastes in Catalyzing HC Removal in Diesel Exhaust 等离子体与复合材料工业废料在催化去除柴油机废气中 HC 方面的协同作用研究
IF 2.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-05-16 DOI: 10.1007/s11090-024-10477-5
Sakshi Vijay, B. S. Rajanikanth
{"title":"Study on Synergy Between Plasma and Composite Industry Wastes in Catalyzing HC Removal in Diesel Exhaust","authors":"Sakshi Vijay,&nbsp;B. S. Rajanikanth","doi":"10.1007/s11090-024-10477-5","DOIUrl":"10.1007/s11090-024-10477-5","url":null,"abstract":"<div><p>The increased usage of diesel in the past 20 years, particularly in developing countries like India, has resulted in serious concerns in abating gaseous pollutants such as oxides of nitrogen (NO<sub>X</sub>) and hydrocarbons (HC). On the other hand, the growing metallurgical processing industries leave behind tons of solid waste, making waste management a bigger issue. In the current work several industry wastes have been tested under discharge plasma environment for their catalytic properties in the removal of HCs from diesel exhaust. To explore the benefit of metal oxide components, present in industry wastes, a new approach was proposed in this work wherein two industrial wastes were blended to form a composite waste which was then powdered and bound to form pellets. Four such composite waste-based pellets, namely <i>red mud</i> + <i>iron tailing, iron tailing</i> + <i>lignite ash, lignite ash</i> + <i>copper slag and red mud</i> + <i>oyster shells,</i> were tested for their catalytic properties under plasma environment. Exhaust emanating from a 6 HP engine is sampled and studied for HC removal in a pulsed plasma reactor embedded with composite wastes. The pellets being porous in nature, studies were also conducted for HC adsorption by cascading composite wastes with plasma alone while treating the exhaust. All the composite wastes exhibited good plasma catalysis in HC removal (58–73%) when compared to that with plasma alone (31%). Further, there is a marked difference between plasma adsorption and plasma catalysis by a factor of 1.75–2.2 indicating synergy between plasma and metal oxides present in composite wastes while catalysing HC removal.</p></div>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":2.6,"publicationDate":"2024-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140967719","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dielectric-Boosted Gliding Arc Discharge for N2 Fixation into NOx 用于将 N2 固定为氮氧化物的介质增压滑动电弧放电
IF 2.6 3区 物理与天体物理
Plasma Chemistry and Plasma Processing Pub Date : 2024-05-13 DOI: 10.1007/s11090-024-10474-8
Xiangyi Meng, Na Lu, Kefeng Shang, Nan Jiang
{"title":"Dielectric-Boosted Gliding Arc Discharge for N2 Fixation into NOx","authors":"Xiangyi Meng,&nbsp;Na Lu,&nbsp;Kefeng Shang,&nbsp;Nan Jiang","doi":"10.1007/s11090-024-10474-8","DOIUrl":"10.1007/s11090-024-10474-8","url":null,"abstract":"<div><p>Plasma nitrogen fixation technology is of great significance in solving the problem of nitrogen fertilizer resource shortage, saving energy and reducing carbon emission, promoting sustainable development of agriculture and promoting resource recycling. To enhance the efficiency and treatment capacity of the two-dimensional, blade-type gliding arc nitrogen fixation reaction, a dielectric-boosted gliding arc discharge reactor with a 50-mm-diameter quartz dielectric (DBGAD<sub><i>Φ</i>50</sub>) was used to conduct N<sub>2</sub> fixation into NO<sub><i>x</i></sub>. The impact of reactor parameters and gas parameters on the nitrogen fixation reaction was systematically investigated in this study. The findings revealed that the DBGAD<sub><i>Φ</i>50</sub> significantly improved the nitrogen fixation effect. At a specific input energy of 2.7 kJ/L, the concentration of NO<sub><i>x</i></sub> generated by the dielectric-boosted gliding arc air discharge was 1.12 times that of the conventional gliding arc discharge (GAD). By utilizing the DBGAD<sub><i>Φ</i>50</sub> reactor, the energy efficiency of 6.83 g/kW h was achieved at a gas flow rate of 5.6 L/min. Appropriately increasing O<sub>2</sub> concentration favors the production of NO<sub><i>x</i></sub>. In the DBGAD<sub><i>Φ</i>50</sub>, the NO<sub><i>x</i></sub> concentration was 1.33 times higher than that in the air atmosphere when the added O<sub>2</sub> volume fraction reached 30%. Performance can be further enhanced by adding TiO<sub>2</sub> catalyst particles to the surface of the quartz dielectric to form a catalyst layer approximately 5 mm thick. At an O<sub>2</sub> concentration of 30%, the DBGAD<sub><i>Φ</i>50</sub> reactor loaded with TiO<sub>2</sub> increased NO<sub><i>x</i></sub> concentration by 26% and energy efficiency by 49%, respectively, resulting in an efficiency of 14.9 g/kW h compared to the case without catalyst.</p></div>","PeriodicalId":734,"journal":{"name":"Plasma Chemistry and Plasma Processing","volume":null,"pages":null},"PeriodicalIF":2.6,"publicationDate":"2024-05-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140927034","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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