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Front Cover: A Novel Family of Luminescent Pyrenyl-(N-Heterocyclic Carbene)- Halogenated Coinage Metal Complexes: Synthesis, Crystal Structures, and Optical Properties (Eur. J. Inorg. Chem. 27/2024)
IF 2.2 4区 化学
European Journal of Inorganic Chemistry Pub Date : 2024-09-27 DOI: 10.1002/ejic.202482701
Yaping Cheng, Geoffrey Gontard, Marie Noelle Rager, Abderrahim Khatyr, Michael Knorr, Hani Amouri
{"title":"Front Cover: A Novel Family of Luminescent Pyrenyl-(N-Heterocyclic Carbene)- Halogenated Coinage Metal Complexes: Synthesis, Crystal Structures, and Optical Properties (Eur. J. Inorg. Chem. 27/2024)","authors":"Yaping Cheng,&nbsp;Geoffrey Gontard,&nbsp;Marie Noelle Rager,&nbsp;Abderrahim Khatyr,&nbsp;Michael Knorr,&nbsp;Hani Amouri","doi":"10.1002/ejic.202482701","DOIUrl":"https://doi.org/10.1002/ejic.202482701","url":null,"abstract":"<p><b>The Front Cover</b> illustrates the synthesis of a family of pyrenyl-(NHC)MCl coinage metal complexes, M=Cu<sup>I</sup>, Ag<sup>I</sup> and Au<sup>I</sup>, (NHC=<i>N</i>-heterocyclic carbene). These compounds are stable and were obtained in high yields. The molecular structures of all complexes were ascertained by X-ray diffraction studies. The use of the chromophoric-(NHC) ligand endows these complexes with emissive properties in the blue region at a similar wavelength to the magical natural blue light created by phytoplankton on the surface of the ocean at nightfall. More information can be found in the Research Article by H. Amouri and co-workers.\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure>\u0000 </p>","PeriodicalId":38,"journal":{"name":"European Journal of Inorganic Chemistry","volume":null,"pages":null},"PeriodicalIF":2.2,"publicationDate":"2024-09-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ejic.202482701","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142328456","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Changes in the Editorial Team at ACS Sensors ACS 传感器编辑部的变化
IF 8.2 1区 化学
ACS Sensors Pub Date : 2024-09-27 DOI: 10.1021/acssensors.4c0238610.1021/acssensors.4c02386
J. Justin Gooding, 
{"title":"Changes in the Editorial Team at ACS Sensors","authors":"J. Justin Gooding,&nbsp;","doi":"10.1021/acssensors.4c0238610.1021/acssensors.4c02386","DOIUrl":"https://doi.org/10.1021/acssensors.4c02386https://doi.org/10.1021/acssensors.4c02386","url":null,"abstract":"","PeriodicalId":24,"journal":{"name":"ACS Sensors","volume":null,"pages":null},"PeriodicalIF":8.2,"publicationDate":"2024-09-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142326078","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hiroaki Misawa Festschrift: Frontiers in Photochemistry Hiroaki Misawa Festschrift：光化学前沿
IF 3.3 3区 化学
The Journal of Physical Chemistry C Pub Date : 2024-09-26 DOI: 10.1021/acs.jpcc.4c0553810.1021/acs.jpcc.4c05538
Kosei Ueno*, Hong-Bo Sun, Paul Mulvaney, Stephan Link and Johan Hofkens, 
{"title":"Hiroaki Misawa Festschrift: Frontiers in Photochemistry","authors":"Kosei Ueno*,&nbsp;Hong-Bo Sun,&nbsp;Paul Mulvaney,&nbsp;Stephan Link and Johan Hofkens,&nbsp;","doi":"10.1021/acs.jpcc.4c0553810.1021/acs.jpcc.4c05538","DOIUrl":"https://doi.org/10.1021/acs.jpcc.4c05538https://doi.org/10.1021/acs.jpcc.4c05538","url":null,"abstract":"","PeriodicalId":61,"journal":{"name":"The Journal of Physical Chemistry C","volume":null,"pages":null},"PeriodicalIF":3.3,"publicationDate":"2024-09-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142318180","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The Trail of Challenges: Autobiographical Notes of Hiroaki Misawa 挑战的足迹三泽宏明自传笔记
IF 3.3 3区 化学
The Journal of Physical Chemistry C Pub Date : 2024-09-26 DOI: 10.1021/acs.jpcc.4c0553910.1021/acs.jpcc.4c05539
Hiroaki Misawa*, 
{"title":"The Trail of Challenges: Autobiographical Notes of Hiroaki Misawa","authors":"Hiroaki Misawa*,&nbsp;","doi":"10.1021/acs.jpcc.4c0553910.1021/acs.jpcc.4c05539","DOIUrl":"https://doi.org/10.1021/acs.jpcc.4c05539https://doi.org/10.1021/acs.jpcc.4c05539","url":null,"abstract":"","PeriodicalId":61,"journal":{"name":"The Journal of Physical Chemistry C","volume":null,"pages":null},"PeriodicalIF":3.3,"publicationDate":"2024-09-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142318170","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Editorial─Excellence in Review Awards 2024 社论──2024 年卓越回顾奖
IF 3.8 3区 工程技术
Industrial & Engineering Chemistry Research Pub Date : 2024-09-25 DOI: 10.1021/acs.iecr.4c0307010.1021/acs.iecr.4c03070
Michael Baldea, 
{"title":"Editorial─Excellence in Review Awards 2024","authors":"Michael Baldea,&nbsp;","doi":"10.1021/acs.iecr.4c0307010.1021/acs.iecr.4c03070","DOIUrl":"https://doi.org/10.1021/acs.iecr.4c03070https://doi.org/10.1021/acs.iecr.4c03070","url":null,"abstract":"","PeriodicalId":39,"journal":{"name":"Industrial & Engineering Chemistry Research","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142318158","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Oxygen Self-Doping Bi2S3@C Spheric Successfully Enhanced Long-Term Performance in Lithium-Ion Batteries. 氧自掺杂 Bi2S3@C Spheric 成功提高了锂离子电池的长期性能。
IF 8.3 2区 材料科学
ACS Applied Materials & Interfaces Pub Date : 2024-09-24 DOI: 10.1021/acsami.4c11172
Xiaojing Zhang, Jing Xie, Yakun Tang, Zhenjiang Lu, Jindou Hu, Yang Wang, Yali Cao
{"title":"Oxygen Self-Doping Bi<sub>2</sub>S<sub>3</sub>@C Spheric Successfully Enhanced Long-Term Performance in Lithium-Ion Batteries.","authors":"Xiaojing Zhang, Jing Xie, Yakun Tang, Zhenjiang Lu, Jindou Hu, Yang Wang, Yali Cao","doi":"10.1021/acsami.4c11172","DOIUrl":"https://doi.org/10.1021/acsami.4c11172","url":null,"abstract":"<p><p>High theoretical capacity of Bi<sub>2</sub>S<sub>3</sub> propels it toward an ideal anode material for lithium-ion batteries (LIBs); however, rapid capacity attenuation and poor long-term stability are major barriers to widespread application. In this work, an oxygen self-doping strategy was utilized to synthesize O-Bi<sub>2</sub>S<sub>3</sub>@C, significantly increasing the amount of active sites for lithium-ion storage. Meanwhile, sulfur vacancies were formed to improve the electrical conductivity and ionic transport efficiency, enhance the long-term stability, and accelerate the electrochemical kinetics of Bi<sub>2</sub>S<sub>3</sub>@C. O-BSC-S1:3 anode exhibits a reversible capacity of 673.1 mAh g<sup>-1</sup> at 0.2 A g<sup>-1</sup>. It retains a long-term capacity of 596.3 mAh g<sup>-1</sup> over 1100 cycles at a high density of 3 A g<sup>-1</sup> in LIBs. Moreover, the installed O-Bi<sub>2</sub>S<sub>3</sub>@C//LiCoO<sub>2</sub> full battery offers exceptional reversible capacity and remarkable cyclability (325.2 mAh g<sup>-1</sup> after 200 cycles) at 0.2 A g<sup>-1</sup>. The combined strategy of oxygen self-doping and sulfur vacancy effectively enhances the reversible capacity and cycling life of Bi<sub>2</sub>S<sub>3</sub>, providing an approach for the design of high-performance transition metal sulfide anodes for LIBs.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":null,"pages":null},"PeriodicalIF":8.3,"publicationDate":"2024-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142306544","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhancing Performances of Enzyme/Metal-Organic Polyhedra Composites by Mixed-Protein Co-Immobilization. 通过混合蛋白协同固定提高酶/金属有机多面体复合材料的性能
IF 8.3 2区 材料科学
ACS Applied Materials & Interfaces Pub Date : 2024-09-24 DOI: 10.1021/acsami.4c10146
Yuri Kanzaki, Ryosuke Minami, Koshiro Ota, Junya Adachi, Yuichiro Hori, Ryo Ohtani, Benjamin Le Ouay, Masaaki Ohba
{"title":"Enhancing Performances of Enzyme/Metal-Organic Polyhedra Composites by Mixed-Protein Co-Immobilization.","authors":"Yuri Kanzaki, Ryosuke Minami, Koshiro Ota, Junya Adachi, Yuichiro Hori, Ryo Ohtani, Benjamin Le Ouay, Masaaki Ohba","doi":"10.1021/acsami.4c10146","DOIUrl":"https://doi.org/10.1021/acsami.4c10146","url":null,"abstract":"<p><p>Protein immobilization using water-soluble ionic metal-organic polyhedra (MOPs) acting as porous spacers has recently been demonstrated as a potent strategy for the preparation of biocatalysts. In this article, we describe a mixed-protein approach to achieve biocomposites with adjustable enzyme contents and excellent immobilization efficiencies, in a systematic and well-controlled manner. Self-assembly of either cationic or anionic MOPs with bovine serum albumin or egg white lysozyme combined with enzymes (alkaline phosphatase, laccase or cytochrome c) led to solid-state catalysts with a high retention of enzyme activity. Furthermore, for all these systems, the dilution of enzymes within the solid-state composite led to noticeably improved catalytic performances, with both higher specific activity and affinity for substrate.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":null,"pages":null},"PeriodicalIF":8.3,"publicationDate":"2024-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142306522","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Graphene-Metal Nanocrystal Hybrid Materials for Bioapplications. 用于生物应用的石墨烯-金属纳米晶混合材料。
IF 8.3 2区 材料科学
ACS Applied Materials & Interfaces Pub Date : 2024-09-24 DOI: 10.1021/acsami.4c11442
Xiaoxu Cao, Shengkai Li, Shen Wang, Rongshen Guo, Qian Dong, Long Chen, Zhuo Chen
{"title":"Graphene-Metal Nanocrystal Hybrid Materials for Bioapplications.","authors":"Xiaoxu Cao, Shengkai Li, Shen Wang, Rongshen Guo, Qian Dong, Long Chen, Zhuo Chen","doi":"10.1021/acsami.4c11442","DOIUrl":"https://doi.org/10.1021/acsami.4c11442","url":null,"abstract":"<p><p>The development of functional nanomaterials is crucial for advancing personalized and precision medicine. Graphene-metal nanocrystal hybrid materials not only possess the intrinsic advantages of graphene-based materials but also exhibit additional optical, magnetic, and catalytic properties of various metal nanocrystals, showing great synergies in bioapplications, including biosensing, bioimaging, and disease treatments. In this Perspective, we discuss the advantages and design principles of graphene-metal nanocrystal hybrid materials and provide an overview of their applications in biological fields. Finally, we highlight the challenges and future directions for their practical implementation.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":null,"pages":null},"PeriodicalIF":8.3,"publicationDate":"2024-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142306538","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Recycling Materials for Sustainable DNA Origami Manufacturing. 可持续 DNA 折纸制造的回收材料。
IF 9.6 1区 材料科学
Nano Letters Pub Date : 2024-09-24 DOI: 10.1021/acs.nanolett.4c02695
Michael J Neuhoff, Yuchen Wang, Nicholas J Vantangoli, Michael G Poirier, Carlos E Castro, Wolfgang G Pfeifer
{"title":"Recycling Materials for Sustainable DNA Origami Manufacturing.","authors":"Michael J Neuhoff, Yuchen Wang, Nicholas J Vantangoli, Michael G Poirier, Carlos E Castro, Wolfgang G Pfeifer","doi":"10.1021/acs.nanolett.4c02695","DOIUrl":"https://doi.org/10.1021/acs.nanolett.4c02695","url":null,"abstract":"<p><p>DNA origami nanotechnology has great potential in multiple fields including biomedical, biophysical, and nanofabrication applications. However, current production pipelines lead to single-use devices incorporating a small fraction of initial reactants, resulting in a wasteful manufacturing process. Here, we introduce two complementary approaches to overcome these limitations by recycling the strand components of DNA origami nanostructures (DONs). We demonstrate reprogramming entire DONs into new devices, reusing scaffold strands. We validate this approach by reprogramming DONs with complex geometries into each other, using their distinct geometries to verify successful scaffold recycling. We reprogram one DON into a dynamic structure and show both pristine and recycled structures display similar properties. Second, we demonstrate the recovery of excess staple strands postassembly and fold DONs with these recycled strands, showing these structures exhibit the expected geometry and dynamic properties. Finally, we demonstrate the combination of both approaches, successfully fabricating DONs solely from recycled DNA components.</p>","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":9.6,"publicationDate":"2024-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142306621","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Boosting Med Chem Education: Integrating Biology for Drug Discovery Talents. 促进医学化学教育：整合生物学，培养药物发现人才。
IF 6.8 1区 医学
Journal of Medicinal Chemistry Pub Date : 2024-09-24 DOI: 10.1021/acs.jmedchem.4c02208
Qiu Sun, Liang Ouyang
{"title":"Boosting Med Chem Education: Integrating Biology for Drug Discovery Talents.","authors":"Qiu Sun, Liang Ouyang","doi":"10.1021/acs.jmedchem.4c02208","DOIUrl":"https://doi.org/10.1021/acs.jmedchem.4c02208","url":null,"abstract":"","PeriodicalId":46,"journal":{"name":"Journal of Medicinal Chemistry","volume":null,"pages":null},"PeriodicalIF":6.8,"publicationDate":"2024-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142306580","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"医学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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