Advanced Materials Interfaces最新文献_第8页

Mechanistic Insights Into Proton and Oxygen Transport Through Ultrathin Amorphous Al2O3 and Al2O3-SiO2 Electrocatalyst Overlayers (Adv. Mater. Interfaces 13/2025) 超薄无定形Al2O3和Al2O3- sio2电催化层中质子和氧传输的机理研究（Adv. Mater.）。接口13/2025)

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70055

Dalia Leon-Chaparro, Minh Duc Nguyen, Christoph Baeumer, Guido Mul, Georgios Katsoukis

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Nanohybrid of Silver-MXene: A Promising Sorbent for Iodine Gas Capture from Nuclear Waste (Adv. Mater. Interfaces 13/2025) 银- mxene纳米杂化材料：一种有前途的核废料碘气体捕集剂。接口13/2025)

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70056

Karamullah Eisawi, Elham Loni, Saehwa Chong, Martin Liezers, Ming Tang, Kyle S. Brinkman, Brian J. Riley, Michael Naguib

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Thickness and Morphology Control in Laser-Assisted Zone Casting of Ultrathin, Polycrystalline Films 激光辅助区域铸造超薄、多晶薄膜的厚度和形貌控制

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.202500275

Adam Kiersnowski, Krzysztof Janus, Michał Wyskiel

{"title":"Thickness and Morphology Control in Laser-Assisted Zone Casting of Ultrathin, Polycrystalline Films","authors":"Adam Kiersnowski, Krzysztof Janus, Michał Wyskiel","doi":"10.1002/admi.202500275","DOIUrl":"10.1002/admi.202500275","url":null,"abstract":"Film morphology control and adaptability of the coating process to substrate size or shape (scalability) are valid issues in thin film fabrication technologies. Overcoming technological limitations in the morphology control or the scalability stimulates development in thin film technologies and therefore drives progress in related fields of materials science. This paper demonstrates laser-assisted zone casting (LAZEC): a contactless thin-film fabrication method utilizing laser heating in a setup resembling meniscus-guided coating. LAZEC is based on thermally induced near-the-surface flows and permits the fabrication of films with thicknesses ranging from a few to several tens of nanometers on flat or curved surfaces. The film thickness can be controlled by solution viscosity, coating speed, and laser power. LAZEC enables the fabrication of polymer and small molecule films with uniform polycrystalline morphologies. Tuning the coating speed and laser power permits tailoring crystal domain sizes as well as their orientation. The latter can be translated to, e.g., planar anisotropy of field-effect charge carrier transport. Owing to its advantages, LAZEC can contribute to the development in the fields of printed electronics, photovoltaics, or thermoelectrics.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 16","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500275","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144894227","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Rapid and Scalable Lubrication Coating for Industrial and Medical Applications via Sequential Dip-Coating 快速和可扩展的润滑涂层工业和医疗应用通过顺序浸涂

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-16 DOI: 10.1002/admi.202500353

Yeontaek Lee, Kayoung Son, Yejin Jo, Seung Hyun Lee, Jeuhee Lee, Tae Young Kim, Seonghyeon Eom, Youn-Hoo Hwang, Dae-Eun Kim, Inhee Choi, Jung Seung Lee, Jungmok Seo

{"title":"Rapid and Scalable Lubrication Coating for Industrial and Medical Applications via Sequential Dip-Coating","authors":"Yeontaek Lee, Kayoung Son, Yejin Jo, Seung Hyun Lee, Jeuhee Lee, Tae Young Kim, Seonghyeon Eom, Youn-Hoo Hwang, Dae-Eun Kim, Inhee Choi, Jung Seung Lee, Jungmok Seo","doi":"10.1002/admi.202500353","DOIUrl":"10.1002/admi.202500353","url":null,"abstract":"Surface coatings have been widely studied and applied in industrial and biomedical fields to give functionalities such as friction reduction, anti-fouling, and enhanced biocompatibility. However, conventional coating techniques often suffer from limited material compatibility, non-uniform coverage on complex geometries, labor-intensive fabrication, and dependence on specialized equipment. In this study, Swift Lubrication is introduced for Industrial and Medical Equipment (SLIME), a rapid (≈10 s) two-step dip-coating method that employs an UV perfluoropolyether base coat followed by a slippery activation layer. SLIME enables the formation of ultra-low friction surfaces, robust anti-fouling properties, and effective diffusion barrier functionality without requiring intricate fabrication processes or specialized equipment. The versatility of SLIME coatings is demonstrated through their application on 3D-printed molds, high-viscosity storage containers, and various biomedical devices, highlighting their material-independent applicability, excellent biocompatibility, and superior anti-adhesion performance. This is envision that SLIME coatings will serve as a practical and scalable solution for an advanced surface lubrication method, significantly enhancing device durability, operational efficiency, and performance across industrial and biomedical applications.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 14","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500353","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144740186","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Exploring the Role of Stent Strut Geometry in Cellular Behavior: An In Vitro Chip Model to Understand In-Stent Restenosis 探索支架支撑几何形状在细胞行为中的作用：一个了解支架内再狭窄的体外芯片模型

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-16 DOI: 10.1002/admi.202500170

Emmie J.D. Schoutens, Juul Verbakel, Heleen M.M. van Beusekom, Jaap M.J. den Toonder, Olaf van der Sluis, Jan de Boer

{"title":"Exploring the Role of Stent Strut Geometry in Cellular Behavior: An In Vitro Chip Model to Understand In-Stent Restenosis","authors":"Emmie J.D. Schoutens, Juul Verbakel, Heleen M.M. van Beusekom, Jaap M.J. den Toonder, Olaf van der Sluis, Jan de Boer","doi":"10.1002/admi.202500170","DOIUrl":"10.1002/admi.202500170","url":null,"abstract":"Stent-based balloon angioplasty is commonly used to treat occluded arteries, but patients still suffer from in-stent restenosis (ISR), a recurrent lumen narrowing. Stent design plays a crucial role in ISR, yet current clinical research cannot isolate the effects of geometry alone. To tackle this problem and allow studying the underlying mechanobiological mechanisms, an in vitro platform containing geometries closely mimicking representative stent strut cross-sectional designs are designed and fabricated. This paper presents the fabrication and a biological validation of the in vitro platform. Morphological analysis revealed that strut-like geometries alter cellular morphology. This analysis further revealed that sharp cornered geometries (rectangle, triangle, trapezium) induced cell proliferation and extracellular matrix isotropy compared to smooth, rounded geometries (circle, oval, hexagon). Rho/ROCK-inhibition suggests intracellular tension as essential force for these responses. The outcomes are in line with clinical trials, where sharp strut shapes show increased neointimal tissue formation. The platform holds great potential for the development of improved stent designs with reduced ISR risk.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 16","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500170","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144894377","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Exploring the Potential of Silicon Clathrate Films with NiOx-Based Selective Contacts for Optoelectronic Devices 探索具有niox基选择性触点的硅包合物薄膜在光电器件中的潜力

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-15 DOI: 10.1002/admi.202500301

Charif Tamin, Anil Kumar Bharwal, Céline Chevalier, Alain Fave, Erwann Fourmond, Stéphane Roques, Aziz Dinia, Abdelilah Slaoui, Thomas Fix

{"title":"Exploring the Potential of Silicon Clathrate Films with NiOx-Based Selective Contacts for Optoelectronic Devices","authors":"Charif Tamin, Anil Kumar Bharwal, Céline Chevalier, Alain Fave, Erwann Fourmond, Stéphane Roques, Aziz Dinia, Abdelilah Slaoui, Thomas Fix","doi":"10.1002/admi.202500301","DOIUrl":"10.1002/admi.202500301","url":null,"abstract":"Silicon clathrates are a unique class of materials with a cage-like structure that offer significant advantages for optoelectronic applications, particularly in indoor photovoltaics (IPV). Their direct bandgaps and tunable electronic properties from metal-like to semiconductor-like behavior enable a wide range of optoelectronic functionalities. In this study, a photovoltaic device is demonstrated based on semiconducting silicon clathrate films (SCF) synthesized from crystalline silicon (c-Si) wafers, with NiOx incorporated as hole selective contact. XPS and Auger spectroscopy confirmed the incorporation of Na within the SCF framework, in agreement with the type-II clathrate structure revealed by XRD analysis. Optical and electronic measurements indicate that the SCF exhibits intrinsic-like behavior with a bandgap of 1.72 eV. Integration of SCF with NiOx resulted in rectification and a clear photovoltaic response under illumination, confirming device functionality. Band alignment analysis suggested efficient hole transport and secondary charge generation from the c-Si substrate. These results highlight the importance of selective contact engineering for efficient charge extraction and demonstrate the potential for further optimization of SCF photovoltaic devices.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 17","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500301","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145032308","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Computational and Experimental Analysis of Drug-Coated Microneedle Skin Insertion: The Mode of Administration Matters 药物包被微针皮肤插入的计算和实验分析：给药方式的问题

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-15 DOI: 10.1002/admi.202500202

Wenting Shu, Thomas Lijnse, Fiona McCartney, David J. Brayden, Aisling Ní Annaidh, Eoin D. O'Cearbhaill

{"title":"Computational and Experimental Analysis of Drug-Coated Microneedle Skin Insertion: The Mode of Administration Matters","authors":"Wenting Shu, Thomas Lijnse, Fiona McCartney, David J. Brayden, Aisling Ní Annaidh, Eoin D. O'Cearbhaill","doi":"10.1002/admi.202500202","DOIUrl":"10.1002/admi.202500202","url":null,"abstract":"Due to an incomplete understanding of the biomechanics of microneedle skin insertion for therapeutic delivery, translating microneedle device performance to clinical use remains challenging. For drug-coated microneedles, it is hypothesized that the mode of skin insertion plays a significant role in how efficiently the drug is released and diffuses. By modeling application pressure magnitude and duration, both computationally and experimentally, the influence of both factors on drug delivery is evaluated. Building on the previously described computational modeling approaches, the development of a Franz Diffusion Cell assay customized with 3D-printed components for use with microneedle patches with adjustable boundary conditions that capture strain-dependent drug diffusion in porcine skin is described. Findings demonstrate that the modified Franz Diffusion Cells accurately simulate microneedle-skin interactions under load, correlating with computational trends. Specifically, leaving microneedle patches in situ for 10 h reduced drug diffusion by ≈14%, compared to removal after 6 h. Prolonged application pressure may negatively impact on diffusion of the drug from the coated patch due to localized strain on surrounding skin tissue. These findings enhance understanding of how microneedle application mode influences drug delivery and the reliability of ex vivo transdermal testing, enabling more effective predictive pre-clinical assessment of microneedle performance.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 17","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500202","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145032307","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Coaxial Electrospun ZIF-8@PAN Nanofiber Membranes for Tetracycline and Doxycycline Adsorption in Wastewater 同轴静电纺丝ZIF-8@PAN纳米纤维膜对废水中四环素和强力霉素的吸附

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-15 DOI: 10.1002/admi.202500364

Pu Wang, Yanan Liu, Wei He, Yaoning Chen, Jianfeng Zhou, Deng-Guang Yu

{"title":"Coaxial Electrospun ZIF-8@PAN Nanofiber Membranes for Tetracycline and Doxycycline Adsorption in Wastewater","authors":"Pu Wang, Yanan Liu, Wei He, Yaoning Chen, Jianfeng Zhou, Deng-Guang Yu","doi":"10.1002/admi.202500364","DOIUrl":"10.1002/admi.202500364","url":null,"abstract":"In this study, polyacrylonitrile (PAN) nanofibers functionalized with ZIF-8 (ZIF-8@PAN), exhibiting a core-shell structure, are produced via coaxial electrospinning for removing tetracycline (TC) and doxycycline (DC). This approach aims to enhance the recoverability and stability of metal-organic framework (MOF)-based adsorbents while effectively minimizing the embedding of ZIF-8 within the polymer in blend electrospinning. It is found that the highest removal efficiencies for TC and DC, obtained with 5% (w/v) ZIF-8 (PZ-5), are 72.2% and 94.1%. The maximum adsorption capacities are 83.4 and 150.2 mg g−1, respectively. Kinetics, isotherms, and thermodynamic studies indicated adsorption is endothermic and conformed to pseudo-second-order kinetic and Sips models. Mechanisms such as electrostatic attraction, coordination bonding, hydrogen bonding, and π–π stacking are primarily responsible. DFT calculations revealed PZ-5 exhibited superior adsorption performance for DC compared to TC. Additionally, PZ-5 showed good resistance to various ions and exhibited high antibiotic removal efficiency in real water. It also exhibited excellent stability and reusability after three cycles. The ZIF-8@PAN nanofiber membrane developed in this study offers a novel approach for the efficient, stable, and easy separation of antibiotic from wastewater, as well as offers new insights into the application of MOF-based materials in environmental remediation.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 16","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500364","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144894085","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Enhancing Diffraction Efficiency in Polarization Volume Gratings via Polymer-Stabilized Cholesteric Liquid Crystal Bilayers 聚合物稳定胆甾液晶双分子层提高极化体积光栅的衍射效率

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-15 DOI: 10.1002/admi.202500396

Yu-Chieh Chang, Ting-Wei Gu, Yu-Chieh Li, Ta-Lung Chang, Chun-Ta Wang

{"title":"Enhancing Diffraction Efficiency in Polarization Volume Gratings via Polymer-Stabilized Cholesteric Liquid Crystal Bilayers","authors":"Yu-Chieh Chang, Ting-Wei Gu, Yu-Chieh Li, Ta-Lung Chang, Chun-Ta Wang","doi":"10.1002/admi.202500396","DOIUrl":"10.1002/admi.202500396","url":null,"abstract":"Polarization volume gratings (PVGs), formed using patterned cholesteric liquid crystals (CLCs), offer high diffraction efficiency, polarization selectivity, and broad angular bandwidth—making them ideal for advanced photonic applications. However, traditional CLC-based PVGs are intrinsically limited to a maximum reflectivity of 50% for unpolarized light, capping their diffraction efficiency. To overcome this limitation, a recently proposed approach is presented that achieves hyper-reflectivity in a single polymer-stabilized cholesteric liquid crystals CLC (PSCLC) cell using a bilayer helical structure fabricated via photo-polymerization-enforced stratification (PES). This method enables the coexistence of two CLC layers with orthogonal helical handedness, facilitating reflection of both left- and right-handed circularly polarized light. Experimental results confirm that through precise material composition and photo-polymerization processing, PVGs with either multi-band reflection or high diffraction efficiency can be realized. Moreover, the bilayer architecture exhibits tunable optical behavior under electric fields and temperature variation, underscoring its potential in adaptive and reconfigurable optical systems.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 17","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500396","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145028446","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Enhancing X-Ray Detection Sensitivity Through Hybrid Active Layers of PBDB-T:ITIC and CdSe Core 2D Nanoplatelets 利用PBDB-T:ITIC和CdSe核心二维纳米血小板混合有源层增强x射线探测灵敏度

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-15 DOI: 10.1002/admi.202500069

Jaewon Son, Jehoon Lee, Chanyeol Lee, Jungwon Kang

{"title":"Enhancing X-Ray Detection Sensitivity Through Hybrid Active Layers of PBDB-T:ITIC and CdSe Core 2D Nanoplatelets","authors":"Jaewon Son, Jehoon Lee, Chanyeol Lee, Jungwon Kang","doi":"10.1002/admi.202500069","DOIUrl":"10.1002/admi.202500069","url":null,"abstract":"In this study a high-performance hybrid X-ray detector incorporating CdSe nanoplatelets (NPLs) is presented into a PBDB-T(Poly[[4,8-bis[5-(2-ethylhexyl)-2-thienyl]benzo[1,2-b:4,5-b′]dithiophene-2,6-diyl]-2,5-thiophenediyl[5,7-bis(2-ethylhexyl)-4,8-dioxo-4H,8H-benzo[1,2-c:4,5-c′]dithiophene-1,3-diyl]]polymer):ITIC (2,2′-[[6,6,12,12-Tetrakis(4-hexylphenyl)-6,12-dihydrodithieno[2,3-d:2′,3′-d′]-s-indaceno[1,2-b:5,6-b′]dithiophene-2,8-diyl]bis[methylidyne(3-oxo-1H-indene-2,1(3H)-diylidene)]]bis[propanedinitrile])organic semiconductor matrix. Organic semiconductors offer advantages such as flexibility and low-cost fabrication, but their limited X-ray sensitivity restricts their application in radiation detection. To overcome this, hybrid active layers incorporating inorganic nanomaterials such as CdSe nanoplatelets have emerged as promising candidates for enhancing performance. The 5-monolayer CdSe NPLs are synthesized with precise thickness control, exhibiting strong absorption and photoluminescence at 556 nm, which effectively matches the emission spectrum of CsI(Tl) scintillators. The hybrid active layer is optimized by investigating various PBDB-T:ITIC ratios and CdSe NPLs concentrations. The optimal device configuration, achieved with a 1:1 ratio of PBDB-T:ITIC and 1.5 mg of CdSe NPLs, demonstrates a power conversion efficiency of 7.18% and a photocurrent density of 18.74 mA/cm−2. The incorporation of CdSe NPLs enhanced the X-ray detector's sensitivity by 31.9% compared to the pure organic device, reaching 1.86 mA/Gy cm−2. The enhanced performance is attributed to the improved light absorption and charge transport properties of the hybrid active layer, despite a slight increase in surface roughness. This work demonstrates the potential of organic–inorganic hybrid systems for next-generation X-ray detection applications.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 16","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500069","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144894084","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0