Advanced Materials Interfaces最新文献

Atomic Layer Deposition of ZnO Coating on Biodegradable Fe-Based Alloys (Adv. Mater. Interfaces 11/2025) 可生物降解铁基合金（Adv. Mater）上ZnO涂层的原子层沉积。接口11/2025)

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-06-09 DOI: 10.1002/admi.202570033

Birgit Paul, Amin Bahrami, Veronika Hahn, Antje Quade, Amit Datye, Konrad Kosiba, Stefan Pilz, Phil Goldberg, Udo D. Schwarz, Frank Hempel, Julia Hufenbach, Kornelius Nielsch

引用次数: 0

Challenges of Soft Tissue Integration Around Dental Implants and Strategies Based on Material Surface Modification 牙种植体周围软组织整合的挑战及基于材料表面修饰的策略

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-26 DOI: 10.1002/admi.202500025

Shasha Jia, Hanqing Zhao, Yingliang Song, Yong Sun, Guowei Wang, Xiaojing Wang

{"title":"Challenges of Soft Tissue Integration Around Dental Implants and Strategies Based on Material Surface Modification","authors":"Shasha Jia, Hanqing Zhao, Yingliang Song, Yong Sun, Guowei Wang, Xiaojing Wang","doi":"10.1002/admi.202500025","DOIUrl":"https://doi.org/10.1002/admi.202500025","url":null,"abstract":"The stability and long-term survival of dental implants depend not only on osseointegration, but also on complete and rigid soft tissue integration (STI) in the transgingival area. Excellent STI prevents the peri-implant hard and soft tissues from being disturbed by bacteria and other external stimuli. However, peri-implant STI is weaker and more susceptible to damage than natural teeth, which may increase the incidence of peri-implant disease. The surface properties of materials in the gingival region of dental implants play a crucial role in modulating the biological response of the surrounding soft tissues. Therefore, different surface modifications have been made to enhance peri-implant STI. This review provides an in-depth analysis of the challenges of STI around dental implants, comprehensively reviews the effects of different implant/abutment modification strategies, including materials, surface characteristics, coatings, summarizes the availability and limitations of the current research, suggests possible future directions to provide feasible ideas for exploring the most optimal implant/abutment design to increase STI, and provides a reference for the clinical translation of the surface modifications to dental implants.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 11","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-05-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500025","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144245115","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Facile Fabrication of Antibacterial 3D Fibrous Sponge via In Situ Protonation-Induced Direct Electrospinning 原位质子诱导直接静电纺丝制备抗菌三维纤维海绵

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-24 DOI: 10.1002/admi.202400935

Altangerel Amarjargal, Olga Miler, Viraj P. Nirwan, Rebecca Hengsbach, Pawel Sajkiewicz, Amir Fahmi

{"title":"Facile Fabrication of Antibacterial 3D Fibrous Sponge via In Situ Protonation-Induced Direct Electrospinning","authors":"Altangerel Amarjargal, Olga Miler, Viraj P. Nirwan, Rebecca Hengsbach, Pawel Sajkiewicz, Amir Fahmi","doi":"10.1002/admi.202400935","DOIUrl":"https://doi.org/10.1002/admi.202400935","url":null,"abstract":"A versatile, straightforward approach for direct fabrication of three-dimensional (3D) nanofibrous sponges via electrospinning is reported. The fabrication of porous 3D nanofibrous sponges is facilitated due to the protonation of dimethylamino ethyl (DMAE) groups in Eudragit E100 (EE). The generated 3D sponges are characterized by microscopy, thermal analysis, light scattering, and contact angle measurements to reveal their physicochemical properties. Additionally, antibacterial properties are confirmed via a colony-forming unit assay. Microscopy analysis demonstrated that the obtained nanofibers possessed uniform conformation without beads, and their overall diameter varies depending on the fraction of the blend composition. The protonation of DMAE groups is investigated via infrared spectroscopy and further confirmed via zeta potential measurements. The charged electrospun 3D sponges exhibited significant antibacterial properties, effectively combating E. coli even at a diluted extract of samples. Owing to their morphology, electrostatically charged surface, and significant antibacterial properties, these 3D nanofibrous sponges present themselves as an effective material for integration in filtering membranes or cartridges, which may minimize harmful substances suspended in the air.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 11","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-05-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202400935","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144245094","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

ESCRT III Regulates Lysosomal Perinuclear Clustering by Inhibiting Kinesin 1 Leading to Agnps Cytotoxicity in Human Cells (Adv. Mater. Interfaces 10/2025) ESCRT III通过抑制激酶1导致人类细胞Agnps细胞毒性调控溶酶体核周聚集（Adv. Mater.）。接口10/2025)

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-22 DOI: 10.1002/admi.202570030

Tiantian Liu, Aiguo Xie, Chao Xing, RuiZhe He, Wei Ni, Yinbo Peng, Peng Xu, Yong Fang

引用次数: 0

Extracellular Vesicle Crosslinkers Constructing Hydrogels with Stress-Relaxation and Bioactive Protein Modification (Adv. Mater. Interfaces 10/2025) 细胞外囊泡交联剂构建应力松弛和生物活性蛋白修饰水凝胶。接口10/2025)

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-22 DOI: 10.1002/admi.202570032

Lufeng Shi, Yanzhen Jing, Haowen Lu, Fanxuan Zhao, Mengying An, Shuiling Jin, Chang Gao, Yongdong Dai, Yinxin Zhu, Shuxu Yang, Songying Zhang, Xuesong Ye, Xiujun Cai, Yifan Wang, Shangjing Xin

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Learning and Controlling Silicon Dopant Transitions in Graphene Using Scanning Transmission Electron Microscopy 利用扫描透射电子显微镜学习和控制石墨烯中的硅掺杂过渡

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-20 DOI: 10.1002/admi.202400998

Max Schwarzer, Jesse Farebrother, Joshua Greaves, Ekin Dogus Cubuk, Rishabh Agarwal, Aaron Courville, Marc G. Bellemare, Sergei Kalinin, Igor Mordatch, Pablo Samuel Castro, Kevin M. Roccapriore

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Coupled Solid-State Diffusion of Li+ and O2 − During Fabrication of Ni-Rich NMC Thin-Film Cathodes Resulting in the Formation of Inactive Ni2O3 and NiO Phases 富镍NMC薄膜阴极制备过程中Li+和O2−的耦合固态扩散导致非活性Ni2O3和NiO相的形成

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-19 DOI: 10.1002/admi.202400911

Sameer Rodrigues, Louis De Taeye, Philippe M. Vereecken

{"title":"Coupled Solid-State Diffusion of Li+ and O2 − During Fabrication of Ni-Rich NMC Thin-Film Cathodes Resulting in the Formation of Inactive Ni2O3 and NiO Phases","authors":"Sameer Rodrigues, Louis De Taeye, Philippe M. Vereecken","doi":"10.1002/admi.202400911","DOIUrl":"https://doi.org/10.1002/admi.202400911","url":null,"abstract":"Ni-rich Li(Ni1−x−yMnxCoy)O2 (NMC) is an attractive cathode material for Li-ion batteries due to its high practical capacity (>200 mAh g−1). However, it is plagued by stability issues that, over multiple cycles or prolonged storage in air, degrade the material and decreases its electrochemical performance. A thin-film model system can be used to simplify the cathode by omitting all passive components and electrode porosity and allow for an in-depth analysis on the interfacial reactions that initiate the material degradation. In this work, the reactions occurring during the fabrication of thin film NMC are investigated. A lot of these reactions stemmed from the loss of active material from the film toward the substrate during annealing. Methods are then devised to reduce the unwanted reactions occurring during annealing. These included lowering the annealing temperature, compensating for material loss, as well as depositing a diffusion barrier between the substrate and NMC film. The findings in this paper outline the various conditions that affect the preparation of thin-film NMC and give readers an overview of reactions to consider when developing thin-film battery materials.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 11","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-05-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202400911","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144245023","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Integration of Plasmonic Nanoheaters for Rapid and Tunable Light-Driven Phase Transitions in VO₂ Nanocomposites 集成等离子体纳米加热器用于VO 2纳米复合材料的快速可调谐光驱动相变

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-19 DOI: 10.1002/admi.202500035

Shankar Acharya, Aaron Hutchins, Opeyemi Akanbi, Hong Tang, Yingjie Zhang, Hualiang Zhang, Wei Guo

{"title":"Integration of Plasmonic Nanoheaters for Rapid and Tunable Light-Driven Phase Transitions in VO₂ Nanocomposites","authors":"Shankar Acharya, Aaron Hutchins, Opeyemi Akanbi, Hong Tang, Yingjie Zhang, Hualiang Zhang, Wei Guo","doi":"10.1002/admi.202500035","DOIUrl":"https://doi.org/10.1002/admi.202500035","url":null,"abstract":"The synthesis, and characterization of vanadium dioxide (VO₂) nanopowders mixed with gold nanoparticles (AuNP) are presented, enabling phase transition under visible light illumination at ambient temperature via AuNP plasmonic heating. The inclusion of AuNP enhances the thermal sensitivity of VO₂, allowing precise control of its metal-insulator transition (MIT). The MIT behavior is analyzed using Fourier transform infrared (FTIR) spectroscopy in the mid-infrared spectrum under varying external light power densities. VO₂ nanoparticles are synthesized with different AuNP particle number ratios, ranging from 1:5 to 1:20. The illumination power density threshold for MIT ranges from 3.7 to 7.9 mW mm−2, depending on the particle ratio. Time-resolved analysis of VO2 reveals a two-stage process, with rise times of 40 and 250 ms, and fall times of 12 and 140 ms, respectively. This rapid thermal response enables efficient phase modulation, achieving frequencies up to 1 kHz and a modulation depth of 10%.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 11","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-05-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500035","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144245024","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

High-throughput Photocatalytic Reactor With in Operando Characterisation for Fast Screening of Materials for the Photodegradation of Water-Borne Pollutants 高通量光催化反应器的运行特性及其对水中污染物光降解材料的快速筛选

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-19 DOI: 10.1002/admi.202401000

Elisante Maloda Maloda, Likius Shipwiisho Daniel, Dmitry Busko, Andrey Turshatov, Justine Sageka Nyarige, Bryce Sydney Richards

{"title":"High-throughput Photocatalytic Reactor With in Operando Characterisation for Fast Screening of Materials for the Photodegradation of Water-Borne Pollutants","authors":"Elisante Maloda Maloda, Likius Shipwiisho Daniel, Dmitry Busko, Andrey Turshatov, Justine Sageka Nyarige, Bryce Sydney Richards","doi":"10.1002/admi.202401000","DOIUrl":"https://doi.org/10.1002/admi.202401000","url":null,"abstract":"A novel fast-screening photocatalytic reactor system (FaS-PhoReS) using simulated terrestrial sunlight is conceived and demonstrated. The instrument is capable of screening, automated data measurement and recording 32 samples at once with no external characterisation devices (e.g., spectrophotometer) required. The capabilities of the system are validated in operando via i) photolysis tests of 12 water-soluble organic dyes to investigate the photostability under simulated sunlight; and ii) photocatalytic degradation of the four most photostable dyes – methylene orange, tartrazine 85, rhodamine B and direct black 38 identified from the photolysis results – using TiO2 thin films prepared by atomic layer deposition. The applicability of the instrument is also demonstrated: i) using alternate photocatalysts – ZnO films and TiO2 nano-powders; and ii) for the in situ detection of reactive oxygen species. The findings indicate that FaS-PhoReS exhibits consistent and repeatable results without being affected by factors such as i) non-uniformity of light intensity; ii) temperature and humidity; and iii) artefacts due to evaporation of the dye solution. Methylene orange and tartrazine 85 dyes are chosen to evaluate photocatalytic degradation, TiO2 thin films annealed at 500 to 600 °C and TiO2 nano-powders of 0.1 to 0.3 mg exhibiting better performance.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 11","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-05-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202401000","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144245106","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Self-Recovery of Carbonate-Contaminated Strontium Titanate (100) Vicinal Surfaces Imaged by Tip-Enhanced Raman Spectroscopy 碳酸盐污染的钛酸锶（100）邻近表面自恢复的尖端增强拉曼光谱成像

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-05-16 DOI: 10.1002/admi.202401024

Mohammad Bakhtbidar, Daniel Gueckelhorn, Marivi Fernández-Serra, Yon Leandro Leibas López, Alexandre Merlen, Andreas Ruediger

{"title":"Self-Recovery of Carbonate-Contaminated Strontium Titanate (100) Vicinal Surfaces Imaged by Tip-Enhanced Raman Spectroscopy","authors":"Mohammad Bakhtbidar, Daniel Gueckelhorn, Marivi Fernández-Serra, Yon Leandro Leibas López, Alexandre Merlen, Andreas Ruediger","doi":"10.1002/admi.202401024","DOIUrl":"https://doi.org/10.1002/admi.202401024","url":null,"abstract":"Strontium titanate (SrTiO3) as a model perovskite has significant applications in catalysis, carbon capture, and advanced electronics. On SrO-terminated (100) surfaces, carbon dioxide (CO2) is a common chemisorption, altering the electronic and chemical properties. This study employed tip-enhanced Raman spectroscopy (TERS) and density functional theory (DFT) simulations to explore this CO2 chemisorption. The (100) surface of SrTiO3 exhibits two distinct terminations, SrO and TiO2 with nominally almost the same heights (0.2 nm). Height scans of hydrothermally treated (100) SrTiO3, show values closer to 0.3 and 0.1 nm, where we attribute the difference in height to the selective adsorption of ambient CO2 on one of the terminations. The TERS analysis shows the presence of a 1071 cm−1 Raman peak (characteristic of carbonate vibration), localized exclusively at the SrO terrace, confirming that CO2 preferentially adsorbs onto SrO. Both experimental and DFT results indicate that this CO2 monolayer alters the binding energy between the SrO and TiO2 terminations. This leads to spontaneous yet slow delamination of SrO and the emergence of SrCO3 nanograins on a purely TiO2-terminated crystal surface. The interpretation is in quantitative agreement with respective volumes of layers and grains throughout the process.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 11","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202401024","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144244836","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0