Advanced Materials Interfaces最新文献

Wide-Field Bond Quality Evaluation Using Frequency Domain Thermoreflectance with Deep Neural Network Feature Reconstruction (Adv. Mater. Interfaces 13/2025) 基于频域热反射和深度神经网络特征重构的宽场键合质量评价。接口13/2025)

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70057

Amun Jarzembski, Siddharth Nair, Wyatt Hodges, Matthew Jordan, Anthony McDonald, Logan Antiporda, Greg W. Pickrell, Timothy Walsh, Fabio Semperlotti, Jason Neely, Luke Yates

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Mechanistic Insights Into Proton and Oxygen Transport Through Ultrathin Amorphous Al2O3 and Al2O3-SiO2 Electrocatalyst Overlayers (Adv. Mater. Interfaces 13/2025) 超薄无定形Al2O3和Al2O3- sio2电催化层中质子和氧传输的机理研究（Adv. Mater.）。接口13/2025)

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70055

Dalia Leon-Chaparro, Minh Duc Nguyen, Christoph Baeumer, Guido Mul, Georgios Katsoukis

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Nanohybrid of Silver-MXene: A Promising Sorbent for Iodine Gas Capture from Nuclear Waste (Adv. Mater. Interfaces 13/2025) 银- mxene纳米杂化材料：一种有前途的核废料碘气体捕集剂。接口13/2025)

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70056

Karamullah Eisawi, Elham Loni, Saehwa Chong, Martin Liezers, Ming Tang, Kyle S. Brinkman, Brian J. Riley, Michael Naguib

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Improved ORR Performance of Precious Metal-Free Fe Single-Atom Catalysts by Heteroatom Doping 杂原子掺杂改善无贵金属铁单原子催化剂的ORR性能

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-01 DOI: 10.1002/admi.202500253

Zhexin Pan, Yiming Zhu, Yihong Liu, Wei-Hsiang Huang, Yujie Cui, Yang Zhao, Menghao Yang, Hongfei Cheng, Nicolas Alonso-Vante, Jiwei Ma

{"title":"Improved ORR Performance of Precious Metal-Free Fe Single-Atom Catalysts by Heteroatom Doping","authors":"Zhexin Pan, Yiming Zhu, Yihong Liu, Wei-Hsiang Huang, Yujie Cui, Yang Zhao, Menghao Yang, Hongfei Cheng, Nicolas Alonso-Vante, Jiwei Ma","doi":"10.1002/admi.202500253","DOIUrl":"https://doi.org/10.1002/admi.202500253","url":null,"abstract":"The development of platinum group metal (PGM)-free catalysts is essential to advance the wide application of fuel cells. Single-atom Fe─N─C catalysts are one type of promising PGM-free catalysts that can replace the expensive Pt/C catalyst for the electrocatalytic oxygen reduction reaction. However, Fe─N─C catalysts still suffer from poor stability due to the inevitable Fenton reaction. In this work, a doping strategy is demonstrated to alter the electronic structure around the catalytic sites and significantly improve their catalytic activity. In particular, the phosphorous-doped Fe─N─C catalyst (P─Fe─N─C) achieves a half-wave potential of 0.885 V versus RHE in 0.1 m KOH and demonstrates excellent stability, with only a 7 mV decay in the half-wave potential after 10 000 cyclic voltammetry cycles, superior to that of boron-doped one (B─Fe─N─C). Density functional theory (DFT) calculations further confirm that heteroatom doping favors the ORR process, highlighting the potential of this catalyst for advanced energy applications.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 13","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500253","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144646905","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Effective Manipulation of Water Droplets on Open Superhydrophobic Glass Surfaces by Using a Triboelectrically Charged Polytetrafluoroethylene Rod on the Back Side of These Surfaces (Adv. Mater. Interfaces 12/2025) 在开放的超疏水玻璃表面上使用摩擦带电聚四氟乙烯棒对水滴的有效操纵。接口12/2025)

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-06-30 DOI: 10.1002/admi.70038

Wei Chen Huang, Ming Yen Chang, Jiann Shieh, Chun Hung Lin, Chin Chi Hsu

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Ferrofluid-Based Bioink for 3D Printed Skeletal Muscle Tissues with Enhanced Force and Magnetic Response 基于铁流体的生物链接，用于增强力和磁响应的3D打印骨骼肌组织

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-06-25 DOI: 10.1002/admi.202400824

Judith Fuentes, Maria Guix, Zoran M. Cenev, Anna C. Bakenecker, Noelia Ruiz-González, Grégory Beaune, Jaakko V.I. Timonen, Samuel Sanchez, Veronika Magdanz

{"title":"Ferrofluid-Based Bioink for 3D Printed Skeletal Muscle Tissues with Enhanced Force and Magnetic Response","authors":"Judith Fuentes, Maria Guix, Zoran M. Cenev, Anna C. Bakenecker, Noelia Ruiz-González, Grégory Beaune, Jaakko V.I. Timonen, Samuel Sanchez, Veronika Magdanz","doi":"10.1002/admi.202400824","DOIUrl":"https://doi.org/10.1002/admi.202400824","url":null,"abstract":"3D printing has emerged as a transformative technology in several manufacturing processes, being of particular interest in biomedical research for allowing the creation of 3D structures that mimic native tissues. The process of tissue 3D printing entails the construction of functional, 3D tissue structures. In this article, the integration of ferrofluid consisting of iron oxide nanoparticles into muscle cell-laden bioink is presented to obtain a 3D printed magnetically responsive muscle tissue, i.e., the ferromuscle. Using extrusion-based methods, the seamless integration of biocompatible ferrofluids are achieved to cell-laden hydrogels. The resulting ferromuscle tissue exhibits improved tissue differentiation demonstrated by the increased force output upon electrical stimulation compared to muscle tissue prepared without ferrofluid. Moreover, the magnetic component originating from the iron oxide nanoparticles allows magnetic guidance, as well as good cytocompatibility and biodegradability in cell culture. These findings offer a new versatile fabrication approach to integrate magnetic components into living constructs, with potential applications as bioactuators and for future integration in smart, functional muscle implants.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 13","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-06-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202400824","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144647841","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Latest Strategies Promoting Stable and Efficient Perovskite, Organic, and Perovskite-Organic Tandem Solar Cells 促进稳定和高效的钙钛矿、有机和钙钛矿-有机串联太阳能电池的最新策略

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-06-23 DOI: 10.1002/admi.202500204

Hongrui Zhang, Yongmin Luo, Dr Top Archie Dela Peña, Dr Ruijie Ma, Prof He Yan, Prof Mingjie Li, Prof Mahesh Suryawanshi, Prof Jiaying Wu, Prof Ashraf Uddin

{"title":"Latest Strategies Promoting Stable and Efficient Perovskite, Organic, and Perovskite-Organic Tandem Solar Cells","authors":"Hongrui Zhang, Yongmin Luo, Dr Top Archie Dela Peña, Dr Ruijie Ma, Prof He Yan, Prof Mingjie Li, Prof Mahesh Suryawanshi, Prof Jiaying Wu, Prof Ashraf Uddin","doi":"10.1002/admi.202500204","DOIUrl":"https://doi.org/10.1002/admi.202500204","url":null,"abstract":"Developing solution-processable photovoltaic materials is expected to foster cheaper solar cell technology through high-throughput printing-based fabrications. In recent years, solution-based organic solar cells (OSCs) and perovskite solar cells (PSCs) have demonstrated great potential. However, achieving reliable stability and commercially competitive device efficiency remains a great challenge. Specifically, although Sn-based narrow bandgap perovskites have shown significant advancements, the stability development for wide bandgap perovskites remains more promising, indicating its advantage for UV applications. Meanwhile, OSCs have made good progress in catching up with the PSC's device efficiency. However, most organic photoabsorbers demonstrate intrinsic photo-degradation from UV exposure while having excellent stability for near-infrared (NIR) applications. Imperatively, constructing perovskite-organic tandems is anticipated to bear synergistic benefits for long-term operation stability, in addition to higher device efficiency. On the other hand, this notion remains primarily theoretical. Accordingly, there is a rapid evolution of material designs and device engineering strategies, extending the limits of both organic and perovskite absorbers. Likewise, novel ideas for intermediate layers, i.e., constructing the interconnecting layer to join perovskites and organic subcells, are emerging. Hence, this review revisits and gives insightful comments on these latest developments, highlighting the existing challenges and providing key research ideas for future research explorations.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 13","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500204","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144647758","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Interfacial Strength in Hierarchical Carbon Fiber Composites: Interplay of Interphase Modulus and Roughness 分层碳纤维复合材料的界面强度：界面模量和粗糙度的相互作用

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-06-23 DOI: 10.1002/admi.202500135

Nihal Kanbargi, Sumit Gupta, Sargun Singh Rohewal, Logan T. Kearney, Amit K. Naskar

{"title":"Interfacial Strength in Hierarchical Carbon Fiber Composites: Interplay of Interphase Modulus and Roughness","authors":"Nihal Kanbargi, Sumit Gupta, Sargun Singh Rohewal, Logan T. Kearney, Amit K. Naskar","doi":"10.1002/admi.202500135","DOIUrl":"https://doi.org/10.1002/admi.202500135","url":null,"abstract":"A facile, direct deposition approach that exploits van der Waals interactions between carbonaceous materials is utilized to create unidirectional hybrid carbon fiber composites. Two small molecule crosslinkers, a trifunctional aromatic (TL) and a difunctional aliphatic (DL) acyl chloride, are first utilized to create a crosslinked interphase with a softer and stiffer modulus respectively. TL crosslinked interphase with a higher modulus improved the tensile strength by 50%, despite non-covalent linking between fiber and matrix, elucidating the critical role of the interphase in alleviating modulus mismatch between the high modulus carbon fiber and the rubbery matrix. Fractional quantities of carbon nanotubes are additionally dispersed in the small molecule crosslinkers which behaved as a dispersant, helping introduce nanoasperities on the carbon fiber surface. Strong “pi-pi” interactions between CNTs and CF contributed to tensile properties, which are increased by 66% compared to the control. A cohesive zone model suggests that a stiffer interphase is better able to exploit surface heterogeneities and roughness on the fiber, synergistically enhancing interfacial strength.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 13","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500135","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144647741","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications 纳米和微材料在聚合物基板上的图案化使用喷涂，选择性激光处理，以及用于传感应用的粘合剂分层

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-06-19 DOI: 10.1002/admi.202500027

Mehraneh Tavakkoli Gilavan, Oluwawemimo Igun, Md Ali Akbar, Shayan Jahangirifard, Peter Kruse, Ponnambalam Ravi Selvaganapathy

{"title":"Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications","authors":"Mehraneh Tavakkoli Gilavan, Oluwawemimo Igun, Md Ali Akbar, Shayan Jahangirifard, Peter Kruse, Ponnambalam Ravi Selvaganapathy","doi":"10.1002/admi.202500027","DOIUrl":"https://doi.org/10.1002/admi.202500027","url":null,"abstract":"Integrating conductive nanomaterials with polymer substrates in a scalable and low-cost way is crucial for developing flexible electronics. This work presents a scalable process for integrating high-quality nanomaterials with polymer films to fabricate flexible electrical devices by combining simple yet effective techniques. Various conductive patterns on polymer substrates are successfully created by utilizing a combination of nanomaterial spraying, laser treatment, and adhesive delamination. The laser treatment embeds the sprayed nanoparticles onto the polymer surface by partially melting the polymer and significantly enhancing their adhesion selectively in places where it traces a path. This method incorporates single-walled carbon nanotubes, graphene, and molybdenum disulfide onto polymers such as polypropylene, polyvinylidene fluoride, and nylon, achieving a minimum line width of 350 µm. The versatility of this technique is demonstrated by fabricating a range of devices, including microheaters, temperature sensors, chemiresistive sensors, and electrochemical sensors. The fabricated devices exhibit excellent durability and stable performance, addressing the limitations of integrating nanomaterials into polymer films. Additionally, this method allows for precise control of conductivity and pattern complexity, making it suitable for various applications. This work contributes to the advancement of flexible electronics, providing a scalable and adaptable method for creating high-performance devices.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 13","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-06-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500027","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144647176","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Water Nanofilms Mediate Adhesion and Heat Transfer at Hematite-Hydrocarbon Interfaces 水纳米膜介导赤铁矿-碳氢化合物界面的粘附和传热

IF 4.3 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-06-17 DOI: 10.1002/admi.202500267

Fionn Carman, Fernando Bresme, Billy Wu, Daniele Dini, James P. Ewen

{"title":"Water Nanofilms Mediate Adhesion and Heat Transfer at Hematite-Hydrocarbon Interfaces","authors":"Fionn Carman, Fernando Bresme, Billy Wu, Daniele Dini, James P. Ewen","doi":"10.1002/admi.202500267","DOIUrl":"https://doi.org/10.1002/admi.202500267","url":null,"abstract":"A detailed understanding of nanoscale heat transport at metal oxide-hydrocarbon interfaces is critical for many applications that require efficient thermal management. Under ambient conditions, water nanofilms are expected to form at these interfaces, but these are rarely accounted for in simulations. Using molecular dynamics simulations, it is shown that water nanofilms at the hydroxylated hematite/poly-α-olefin (PAO) interface significantly affect wettability and thermal transport. Including water nanofilms improves agreement with experimental work of adhesion, which cannot be replicated with anhydrous systems using realistic solid–liquid interactions. For water films thicker than one monolayer, interfacial thermal resistance (ITR) converges to a consistent value, independent of solid–liquid interaction strength. This value is dominated by the ITR at the water/PAO interface. The ITR at the water/PAO interface is dependent on the surface area between the water film and the PAO and the magnitude of the interfacial potential. These simulations provide a more precise estimate of ITR at the hematite/PAO interface by accounting for surface hydration expected in experiments under ambient conditions. This study offers crucial insights into the roles of surface hydroxylation and water nanofilms in controlling wettability and thermal transport at industrially important interfaces.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 13","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500267","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144647524","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0