Advanced Materials Interfaces最新文献

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Ultrafast Photocatalytic Wettability Switching in Substrate-Interface Tailored Titanium Dioxide Thin Films 衬底-界面定制二氧化钛薄膜的超快光催化润湿性切换
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-04-07 Epub Date: 2026-02-24 DOI: 10.1002/admi.202500986
Rucha A. Deshpande, Jesper Navne, David C. B. Nielsen, Mathias Adelmark, Radu Malureanu, Ole Hansen, Rafael Taboryski
{"title":"Ultrafast Photocatalytic Wettability Switching in Substrate-Interface Tailored Titanium Dioxide Thin Films","authors":"Rucha A. Deshpande,&nbsp;Jesper Navne,&nbsp;David C. B. Nielsen,&nbsp;Mathias Adelmark,&nbsp;Radu Malureanu,&nbsp;Ole Hansen,&nbsp;Rafael Taboryski","doi":"10.1002/admi.202500986","DOIUrl":"10.1002/admi.202500986","url":null,"abstract":"<p>In this study, we investigate the ultrafast photocatalytic wettability switching in titanium dioxide (TiO<sub>2</sub>) thin films, tailored at the substrate-interface level. We explore the effects of silicon substrate doping and the introduction of interface oxides on the photocatalytic contact angle switching rate. Our findings demonstrate that higher silicon substrate doping levels decrease the active layer thickness, reducing the switching rate, while the presence of interface oxides enhances the switching rate by preventing electron-hole pair transfer into the substrate. Additionally, we examine the photocatalytic liquid spreading effects on nanostructured TiO<sub>2</sub> surfaces, revealing that conformally TiO<sub>2</sub> coated silica nanostructures strongly support photocatalytic hemiwicking. These results are supported by theoretical predictions and provide insights into optimizing TiO<sub>2</sub> thin films for advanced photocatalytic applications.</p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 7","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-04-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500986","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147668681","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enabling Real-Time, Non-Ionizing 3D Imaging of Implantable Magnetic Cements Using Magnetic Particle Imaging 利用磁颗粒成像技术实现可植入磁性水泥的实时、非电离三维成像
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-04-07 Epub Date: 2025-11-02 DOI: 10.1002/admi.202500757
Gabriel C. Pinto, João M. Costa, Simão P. Fernandes, Gabriela F. Resende, Eduardo T. C. Coimbra, Patrick Vogel, Mariana B. Oliveira, Marco Giardiello, Ricardo M. Silva, Armando A.C.S. Lourenço, Nuno J. O. Silva
{"title":"Enabling Real-Time, Non-Ionizing 3D Imaging of Implantable Magnetic Cements Using Magnetic Particle Imaging","authors":"Gabriel C. Pinto,&nbsp;João M. Costa,&nbsp;Simão P. Fernandes,&nbsp;Gabriela F. Resende,&nbsp;Eduardo T. C. Coimbra,&nbsp;Patrick Vogel,&nbsp;Mariana B. Oliveira,&nbsp;Marco Giardiello,&nbsp;Ricardo M. Silva,&nbsp;Armando A.C.S. Lourenço,&nbsp;Nuno J. O. Silva","doi":"10.1002/admi.202500757","DOIUrl":"10.1002/admi.202500757","url":null,"abstract":"<p>Magnetic Particle Imaging (MPI) is a non-ionizing tomographic technique capable of real-time 3D imaging with unmatched temporal resolution, reaching up to 46 vol/s. These features make MPI a promising tool for the monitoring of implantable resin composites, particularly in scenarios requiring frequent safe, and dynamic assessment. However, integrating magnetic responsiveness into medical materials without compromising their structural and biological integrity remains a challenge. In this study, it is presented the first strategy to enable MPI signal generation in a commercial implantable cement by depositing a continuous iron thin film onto its surface. This structured magnetic layer introduces directional magnetic anisotropy, resulting in an angle-dependent MPI signal. This directional dependence can be explored to noninvasively track for the position and orientation of the implant, potentially benefiting applications in confined anatomical regions. In vitro assays confirmed that the incorporation of the magnetic layer does not compromise cytocompatibility. Altogether, these findings demonstrate that magnetic thin films can serve as anisotropic contrast sources for MPI, expanding the range of new possibilities for imaging implantable materials with orientation-sensitive contrast and without ionizing radiation.</p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 7","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-04-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500757","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147668060","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Spin-Crossover Confinement in Mesoporous Matrices Enables Tunable Porosity for Molecular Sensing 介孔矩阵的自旋交叉限制使分子传感的孔隙度可调
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-04-07 Epub Date: 2026-03-12 DOI: 10.1002/admi.202501103
Lucia B. Pizarro, Matias Rafti, Annette Andrieu-Brunsen, Marcelo Ceolín
{"title":"Spin-Crossover Confinement in Mesoporous Matrices Enables Tunable Porosity for Molecular Sensing","authors":"Lucia B. Pizarro,&nbsp;Matias Rafti,&nbsp;Annette Andrieu-Brunsen,&nbsp;Marcelo Ceolín","doi":"10.1002/admi.202501103","DOIUrl":"10.1002/admi.202501103","url":null,"abstract":"<p>Bistable spin crossover (SCO) complexes are promising functional materials for microscale and nanoscale sensing applications due to their ability to reversibly switch physical properties in response to external stimuli such as temperature or molecular adsorption. Nevertheless, their practical integration into responsive devices is often limited by the poor accessibility of active sites in typically nonporous solids. Herein, we report a hierarchically structured hybrid platform in which mesoporous silica networks are supported within cellulose-paper microfibers and subsequently loaded with the SCO complex [Fe(II)(Trz)<sub>3</sub>]BF<sub>4</sub> (Trz = 1,2,4-triazole). This multiscale architecture establishes a continuous structural connection from the microscopic paper scaffold down to the molecular level, enabling confinement-driven coupling between architecture and bistability. We show that confinement within the mesoporous framework not only modulates the thermodynamic behavior of the spin transition but also promotes cooperative interactions between the SCO material and the porous matrix, where molecular self-assembly increases accessible surface area. The confined SCO domains exhibit guest-responsive spin transitions, as molecular uptake induces measurable shifts in the transition temperature. These combined effects reveal a cooperative mechanism linking nanoscale confinement and microscale hierarchy, providing a versatile pathway toward flexible, paper-based materials for responsive and sensing technologies.</p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 7","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-04-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202501103","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147668392","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
3D-Printed Arch-Structured Tribolayer with Conducting Polymer Coating for Enhanced Triboelectric Energy Harvesting 具有导电聚合物涂层的3d打印拱形结构摩擦层用于增强摩擦电能收集
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-04-07 Epub Date: 2026-03-11 DOI: 10.1002/admi.202500963
Mariam E. Alhosani, Bushara Fatma, Reem B. Irshaid, Kyriaki Katsikari, Maryam Aljaberi, Israr Ud Din, Seoyoung Kang, Young Pyo Jeon, Kamran A. Khan, Charalampos Pitsalidis
{"title":"3D-Printed Arch-Structured Tribolayer with Conducting Polymer Coating for Enhanced Triboelectric Energy Harvesting","authors":"Mariam E. Alhosani,&nbsp;Bushara Fatma,&nbsp;Reem B. Irshaid,&nbsp;Kyriaki Katsikari,&nbsp;Maryam Aljaberi,&nbsp;Israr Ud Din,&nbsp;Seoyoung Kang,&nbsp;Young Pyo Jeon,&nbsp;Kamran A. Khan,&nbsp;Charalampos Pitsalidis","doi":"10.1002/admi.202500963","DOIUrl":"10.1002/admi.202500963","url":null,"abstract":"<p>Three-dimensional printed (3DP) triboelectric nanogenerators (TENGs) provide a versatile approach for complex and customizable microstructures tailored for efficient energy harvesting and sensing. Here, we demonstrate the fabrication of flexible microstructured TENGs produced via stereolithography 3D printing and subsequently coated with a conducting polymer, PEDOT:PSS (P:P). Three geometries are investigated: pillars, pyramids, and arches, with the arch configuration emerging as a new design combining enhanced mechanical adaptability and improved triboelectric performance. The arch-shaped TENGs exhibit superior flexibility, structural stability, and a high active surface area, which collectively facilitate efficient energy conversion under repetitive deformation. Furthermore, the incorporation of P:P coating substantially enhances performance, resulting in a more than twentyfold increase in voltage output compared to uncoated counterparts. Among the 3DP structures, the arch geometry consistently delivers better performance, confirming the geometry-driven performance of 3DP-TENGs. The optimized arch configuration is found to yield a peak voltage output of ∼101 V, corresponding to a maximum power output of ∼193.6 mW/m<sup>2</sup>. By exploiting the spring-like behavior of the arch-shaped tribolayer, a “zero-gap” TENG architecture is presented, offering a compact and adaptable energy-harvesting platform as well as pressure-sensing capabilities. Finally, a wireless pressure-sensing platform configured as a vehicle parking counter is demonstrated, showcasing the potential of this development for integration into smart infrastructure and environmental monitoring systems.</p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 7","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-04-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500963","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147668650","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Tunable Plasmonic Response of Silver Nanoparticles Entangled in Detonation Nanodiamond Network via Colloidal Self-Assembly (Adv. Mater. Interfaces 6/2026) 基于胶体自组装的银纳米粒子在爆轰纳米金刚石网络中的可调谐等离子体响应。接口6/2026)
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-03-16 DOI: 10.1002/admi.70394
Vendula Hrnčířová, Markéta Šlapal Bařinková, Muhammad Qamar, Kateřina Kolářová, Bohuslav Rezek
{"title":"Tunable Plasmonic Response of Silver Nanoparticles Entangled in Detonation Nanodiamond Network via Colloidal Self-Assembly (Adv. Mater. Interfaces 6/2026)","authors":"Vendula Hrnčířová,&nbsp;Markéta Šlapal Bařinková,&nbsp;Muhammad Qamar,&nbsp;Kateřina Kolářová,&nbsp;Bohuslav Rezek","doi":"10.1002/admi.70394","DOIUrl":"https://doi.org/10.1002/admi.70394","url":null,"abstract":"<p><b>Plasmonic Nanodiamonds</b></p><p>The cover depicts self-assembled nanocomplexes in colloidal mixtures as stars: detonation nanodiamond networks (white) trapping silver particles (yellow), resulting in altered plasmonic resonance (glow) depending on silver concentration. Mountains symbolize a nanocomplex optical absorption showing a shifted and enhanced plasmonic peak. More details can be found in the Research Article by Vendula Hrnčířová and co-workers (DOI: 10.1002/admi.202500461).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 6","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-03-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.70394","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147566164","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Interfacial Behavior of Methane in Methane/p-Xylene/Water Systems: First Principles Inspected Using Neutron Imaging and Molecular Dynamics Simulations 甲烷在甲烷/对二甲苯/水体系中的界面行为:用中子成像和分子动力学模拟检验第一原理
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-03-16 Epub Date: 2026-01-26 DOI: 10.1002/admi.202500786
Martin Melčák, Tereza-Markéta Durďáková, Petr Číhal, Jonatan Šercl, Jongmin Lee, Pierre Boillat, Jan Heyda, Pavel Trtik, Ondřej Vopička
{"title":"Interfacial Behavior of Methane in Methane/p-Xylene/Water Systems: First Principles Inspected Using Neutron Imaging and Molecular Dynamics Simulations","authors":"Martin Melčák,&nbsp;Tereza-Markéta Durďáková,&nbsp;Petr Číhal,&nbsp;Jonatan Šercl,&nbsp;Jongmin Lee,&nbsp;Pierre Boillat,&nbsp;Jan Heyda,&nbsp;Pavel Trtik,&nbsp;Ondřej Vopička","doi":"10.1002/admi.202500786","DOIUrl":"https://doi.org/10.1002/admi.202500786","url":null,"abstract":"<p>Pressurized gases adsorb on the gas-liquid (<i>g</i>-<i>l</i>) interfaces, thus reducing the interfacial tension (IFT). Gas-saturated liquid–liquid (<i>l</i>-<i>l</i>) emulsions occur in oil and gas wells, possible IFT changes due to saturation remain unclear. We study if the IFT reduction occurs for the model system of methane, <i>p-</i>xylene, and water. The neutron imaging (NI) observations of bulk (<i>g</i>-<i>l</i>-<i>l</i>) systems at 100 bar provide several quantities simultaneously from each experimental run, e.g., IFT for <i>g</i>-<i>l</i> and methane diffusivity for the <i>p-</i>xylene rich phase, but does not sensitively provide IFT for the <i>l</i>-<i>l</i> interface. The quantities derived for the <i>p-</i>xylene-rich phase using NI allows us to calibrate molecular dynamics (MD) simulation, which is used for the predictions of IFT for <i>l</i>-<i>l</i>, literature data for binary benzene/water (<i>l</i>-<i>l</i>) system are used as the reference. Overall, no, or very minor effect (±1 mN m<sup>−</sup><sup>1</sup>) on IFT is robustly found up to methane saturation at 100 bar. Variation of partial charges on the <i>p</i>-xylene model from zero to quantum calculation-based modulate the fine structure of <i>p</i>-xylene/water interface and has small, yet qualitative effect on IFT, resulting in a weak adsorption (−1 mN m<sup>−1</sup>), or weak depletion (+1 mN m<sup>−1</sup>) of methane from <i>l-l</i>.</p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 6","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-03-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500786","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147569783","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Development of Artificial Sebaceous Gland-Integrated In Vitro Human Skin Model 人造皮脂腺整合人体外皮肤模型的建立
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-03-16 Epub Date: 2026-02-10 DOI: 10.1002/admi.202501055
Daeun Ryu, Hyewon Noh, Jimin Son, Haejung Lee, Bo Mi Kang, Chong Won Choi, Jong Hwan Sung, Jae Jung Kim
{"title":"Development of Artificial Sebaceous Gland-Integrated In Vitro Human Skin Model","authors":"Daeun Ryu,&nbsp;Hyewon Noh,&nbsp;Jimin Son,&nbsp;Haejung Lee,&nbsp;Bo Mi Kang,&nbsp;Chong Won Choi,&nbsp;Jong Hwan Sung,&nbsp;Jae Jung Kim","doi":"10.1002/admi.202501055","DOIUrl":"https://doi.org/10.1002/admi.202501055","url":null,"abstract":"<p>Sebum plays a critical role in maintaining skin homeostasis, but its overproduction is associated with pore enlargement, acne, and other dermatological conditions. Acne causes physiological stress and reduced quality of life, contributing to social burden. Although various sebaceous gland models exist, including 2D, explant-based, and in vivo/ex vivo systems, each has limitations in longevity or physiological relevance. While in vitro 3D sebocyte models would be more suitable for screening, they still fall short in recapitulating interactions with key skin components like fibroblasts and keratinocytes. Here, a 3D skin model was developed to mimic the epidermis and dermal layer including sebaceous glands. Uniform 3D collagen-based artificial sebaceous glands, termed SebaSpheres, were produced using microfluidic technology. These SebaSpheres successfully accumulated lipids and expressed the differentiation marker, Blimp-1. SebaSpheres were integrated into the microwell-shaped dermal layer populated with fibroblasts, followed by the addition of keratinocytes (HaCaT) to establish an epidermis of the skin model. During co-culture, live/dead imaging indicated that all three cell types maintained viability. Involucrin expression was observed in HaCaT cells under co-culture conditions, indicating compatibility with sebocyte integration. This in vitro skin model provides a platform for future studies aimed at evaluating acne-related stimuli and cosmetic compounds targeting oily skin.</p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 6","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-03-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202501055","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147564588","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Integrating Direct Air Capture Technology and Plasma Based Calcination for Sustainable Syngas and Concrete – An Experimental Investigation 将直接空气捕获技术与等离子体煅烧相结合用于可持续合成气和混凝土的实验研究
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-03-16 Epub Date: 2026-02-20 DOI: 10.1002/admi.202500992
Valentin Benedikt Seithümmer, Samuel Jaro Kaufmann, Felix Jonathan Brucker, Resul Çağtay Sahin, Kai Peter Birke, Paul Rößner
{"title":"Integrating Direct Air Capture Technology and Plasma Based Calcination for Sustainable Syngas and Concrete – An Experimental Investigation","authors":"Valentin Benedikt Seithümmer,&nbsp;Samuel Jaro Kaufmann,&nbsp;Felix Jonathan Brucker,&nbsp;Resul Çağtay Sahin,&nbsp;Kai Peter Birke,&nbsp;Paul Rößner","doi":"10.1002/admi.202500992","DOIUrl":"https://doi.org/10.1002/admi.202500992","url":null,"abstract":"&lt;p&gt;The persistent reliance of the cement sector on fossil fuels for CaO production and the high energy demand for DAC sorbent regeneration pose a significant barrier to reaching sustainable industrial production. Herein, a novel process concept is presented, establishing an integrated, fully electrified &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;CO&lt;/mi&gt;\u0000 &lt;mn&gt;2&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm CO}_2$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt;-loop driven by gliding arc plasma technology. Atmospheric &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;CO&lt;/mi&gt;\u0000 &lt;mn&gt;2&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm CO}_2$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt; is captured in an alkaline absorption unit, where the pH value serves as a reliable performance parameter for system predictability. Subsequent liquid-solid conversion solidifies the captured &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;CO&lt;/mi&gt;\u0000 &lt;mn&gt;2&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm CO}_2$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt; as &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;CaCO&lt;/mi&gt;\u0000 &lt;mn&gt;3&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm CaCO}_3$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt;, achieving a high yield with high phase purity. Rotating gliding arc plasma experiments successfully demonstrate the electric calcination for CaO regeneration and the &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;CO&lt;/mi&gt;\u0000 &lt;mn&gt;2&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm CO}_2$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt; release to close the carbon and calcium loop. With the ability of simultaneous plasma-based &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;CO&lt;/mi&gt;\u0000 &lt;mn&gt;2&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm CO}_2$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt; splitting the process enables the use of the resulting CO as a precursor for synthesis gas. The observation of internal temperature gradients facilitates the definition of a suitable reaction volume for calcination. XRD and TGA/DSC analyses confirm the formation of pure Ca-products, validating the concept. This work provides a foundational material-flow validation for this novel DAC Power-to-X pathway, substituting fossil fuels for calcination and DAC-operation entirely with electrical energy. The process offers a crucial opportunity for the decarbonization of the construction and transport sectors, with future work focusing on optimizing reactor design","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 6","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-03-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500992","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147567449","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Tunable Sensitivity in PAN/CNF/PEDOT:PSS Nanofiber-Based Piezocapacitive Sensors PAN/CNF/PEDOT:PSS纳米纤维压电容传感器的灵敏度可调
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-03-16 Epub Date: 2026-01-29 DOI: 10.1002/admi.202500913
Alireza Gholamhoseini, Sheyda Mirjalali, Aisan Nouri, David Payne, Noushin Nasiri
{"title":"Tunable Sensitivity in PAN/CNF/PEDOT:PSS Nanofiber-Based Piezocapacitive Sensors","authors":"Alireza Gholamhoseini,&nbsp;Sheyda Mirjalali,&nbsp;Aisan Nouri,&nbsp;David Payne,&nbsp;Noushin Nasiri","doi":"10.1002/admi.202500913","DOIUrl":"https://doi.org/10.1002/admi.202500913","url":null,"abstract":"<p>Flexible piezocapacitive pressure sensors are poised to underpin next-generation wearable electronics; however, the concurrent attainment of high sensitivity, mechanical endurance, and structural tunability within a scalable fabrication framework remains a formidable challenge. Here, a class of robust and tunable capacitive pressure sensors engineered from electrospun polyacrylonitrile (PAN) nanofibers incorporating functional conductive fillers: carbon nanofibers (CNF) and poly(3,4-ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS) is presented. Systematic optimization of filler composition and nanofiber mat thickness yields pronounced enhancements in electromechanical responsiveness. Notably, incorporation of 0.2 wt.% CNF and 2 wt.% PEDOT:PSS delivers sensitivities of 27 and 47 MPa<sup>−1</sup> in the low-pressure regime, representing improvements of 94% and 237% relative to pristine PAN, respectively. A clear thickness-dependent behavior is observed, with ultrathin nanofiber mats (0.5 mL electrospun volume) consistently achieving the highest sensitivity through superior compressibility and dielectric modulation. Continuous loading reveals nonlinearities associated with air entrapment in the porous matrix, while cyclic testing over 2000 cycles confirms exceptional mechanical resilience with &lt;3% signal degradation. These findings delineate a scalable strategy for the fabrication of robust, tunable, and sensitive pressure sensors, advancing their deployment in wearable biomedical monitoring and soft human–machine interfaces.</p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 6","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-03-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500913","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147570124","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The Vegan Villain Sets Out to The End of Summer: Functionalized Coatings as Biohybrid UV-Sensors (Adv. Mater. Interfaces 6/2026) 素食主义者恶棍出发到夏末:功能化涂层作为生物混合紫外线传感器(Adv. Mater)。接口6/2026)
IF 4.4 3区 材料科学
Advanced Materials Interfaces Pub Date : 2026-03-16 DOI: 10.1002/admi.70395
Amelie Skopp, Matea Marosevic, Broder Rühmann, Volker Sieber
{"title":"The Vegan Villain Sets Out to The End of Summer: Functionalized Coatings as Biohybrid UV-Sensors (Adv. Mater. Interfaces 6/2026)","authors":"Amelie Skopp,&nbsp;Matea Marosevic,&nbsp;Broder Rühmann,&nbsp;Volker Sieber","doi":"10.1002/admi.70395","DOIUrl":"https://doi.org/10.1002/admi.70395","url":null,"abstract":"<p><b>Biohybrid Sensor</b></p><p>The cover playfully depicts our biohybrid UV sensor's transition from its initial “Vegan Villain” green to its photoconverted “End of Summer” red. It features the <i>E. coli</i>–based system, the photoconvertible mEosFP triad, and a dynamic interplay with UV light, visually capturing both the biological design and the light-driven mechanism underlying the sensor's function. More details can be found in the Research Article by Volker Sieber and co-workers (DOI: 10.1002/admi.202500125).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"13 6","pages":""},"PeriodicalIF":4.4,"publicationDate":"2026-03-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.70395","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147566461","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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