Advanced Materials Interfaces最新文献_第7页

Nitrogen-Doped Amorphous Carbon Film for Enhanced Cu2+ Electrochemical Sensing in Marine Environments 海洋环境中增强Cu2+电化学传感的氮掺杂非晶碳膜

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-29 DOI: 10.1002/admi.202500583

Xueqing Zhao, Silong Zhang, Shuyuan Wang, Peng Guo, Zhenyu Wang, Guanshui Ma, Aiying Wang

{"title":"Nitrogen-Doped Amorphous Carbon Film for Enhanced Cu2+ Electrochemical Sensing in Marine Environments","authors":"Xueqing Zhao, Silong Zhang, Shuyuan Wang, Peng Guo, Zhenyu Wang, Guanshui Ma, Aiying Wang","doi":"10.1002/admi.202500583","DOIUrl":"https://doi.org/10.1002/admi.202500583","url":null,"abstract":"Amorphous carbon (a-C) is a promising material for electrochemical sensing due to its wide potential window and chemical stability. However, its high resistance and limited surface activity hinder performance. Nitrogen (N) doping can improve conductivity while maintaining a low background current, but precise control of N content remains challenging. In this study, N-doped a-C films are fabricated using a high-ionization anode-layer ion source by adjusting the C2H2/N2 gas ratio. The influence of N concentration on Cu2⁺ detection performance is systematically evaluated. Moderate N doping (≈12.9 at.%) facilitates the formation of sp2-hybridized carbon and nitrogen-containing functional groups, significantly enhancing electrochemical activity. The optimized electrode exhibits a wide linear detection range from 8 × 10−3 to 5 mM and a low detection limit of 8 × 10−3 mM in 3.5 wt% NaCl solution, sufficient for monitoring copper alloy crevice corrosion (≈0.1 mm). The electrodes also show excellent repeatability, reproducibility, and long-term stability. Theoretical calculations indicate that increased sp2 content and C─N bonds enhance Cu2⁺ adsorption and electron transfer, thereby improving sensor performance via N doping.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 18","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500583","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145129470","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Local Femtosecond Pulsed Laser Decoating of Superhydrophobic Paper Coating for Enhanced Fog Harvesting Efficiency 超疏水纸涂层局部飞秒脉冲激光消光提高雾收集效率

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-27 DOI: 10.1002/admi.202500332

Martin Kahlmeyer, Carina Breuer, Andreas Winkel, Markus Biesalski, Camilo Florian-Baron, Stefan Böhm

{"title":"Local Femtosecond Pulsed Laser Decoating of Superhydrophobic Paper Coating for Enhanced Fog Harvesting Efficiency","authors":"Martin Kahlmeyer, Carina Breuer, Andreas Winkel, Markus Biesalski, Camilo Florian-Baron, Stefan Böhm","doi":"10.1002/admi.202500332","DOIUrl":"10.1002/admi.202500332","url":null,"abstract":"Superhydrophobic paper has demonstrated significant potential for efficient water harvesting. Previous studies have indicated that the incorporation of pinning structures on superhydrophobic surfaces can enhance water collection efficiency. This study explores the feasibility of creating such pinning structures through femtosecond laser ablation of wax-based superhydrophobic coatings. Static contact angle measurements and the roll-off behavior of droplets on laser-treated surfaces are conducted to evaluate the effects of laser ablation. Additionally, fogging tests are performed to assess the water collection performance, revealing an improvement of above 10% in comparison to unmodified superhydrophobic paper without localized pinning structures. Notably, the laser ablation process minimally affects the load-bearing capacity of the paper, ensuring that its structural integrity is preserved. The ability to design laterally resolved pinning structures opens new possibilities for further optimization, such as the creation of flow paths, ultimately enhancing the overall efficiency of water harvesting systems.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 17","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500332","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145032303","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Dynamic Wettability Behavior of Emerging Ultrawhite Radiative Cooling Paints 新兴超白辐射冷却涂料的动态润湿性

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-24 DOI: 10.1002/admi.202500288

Orlando G. Rivera González, Abdulrahman K. Aljwirah, Andrea L. Felicelli, Xiulin Ruan, Justin A. Weibel

{"title":"Dynamic Wettability Behavior of Emerging Ultrawhite Radiative Cooling Paints","authors":"Orlando G. Rivera González, Abdulrahman K. Aljwirah, Andrea L. Felicelli, Xiulin Ruan, Justin A. Weibel","doi":"10.1002/admi.202500288","DOIUrl":"10.1002/admi.202500288","url":null,"abstract":"Outdoor radiative cooling surfaces passively lose heat by reflecting solar irradiation and emitting infrared radiation to cold deep space through the atmospheric sky window (8–13 µm), thereby achieving sub-ambient temperature. Ultrawhite radiative cooling paints are an emerging technology offering scalable solutions for cooling and passive water harvesting wherein surface wettability plays a key role. This work, examines how radiative cooling paint pigment and binder formulations affect surface morphology, roughness, and dynamic wettability. Samples are prepared with three different nanoparticulate pigments, calcium carbonate (CaCO3), barium sulfate (BaSO4), and hexagonal boron nitride (hBN); two binders, including an acrylic and a waterborne silicone-modified polyurethane dispersion (SILIKOPUR 8081); and pigment solid volume concentrations from 0% to 80% v/v. The CaCO3 and BaSO4 pigments produced paints with rougher textures and higher contact angles due to their pigment particle morphology. While high solar reflectance was achieved across various pigment and binder combinations, wettability exhibited a complex trend with pigment concentration, indicating that maximizing reflectance does not necessarily optimize wetting behavior. This expanded understanding on how pigment type, binder and concentration influence wettability, offering pathways to design coatings with tailored spectral and wetting properties for both self-cleaning paints and passive water harvesting applications","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 16","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500288","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144894400","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Laser-Induced Nano-Functional Surfaces for Enhanced SERS Performance 增强SERS性能的激光诱导纳米功能表面

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-18 DOI: 10.1002/admi.202500366

Hardik Vaghasiya, Paul-Tiberiu Miclea

{"title":"Laser-Induced Nano-Functional Surfaces for Enhanced SERS Performance","authors":"Hardik Vaghasiya, Paul-Tiberiu Miclea","doi":"10.1002/admi.202500366","DOIUrl":"10.1002/admi.202500366","url":null,"abstract":"Nanostructured metal surfaces play a crucial role in sensing applications, particularly in Surface-Enhanced Raman Spectroscopy (SERS). In this study, laser-induced periodic surface structures (LIPSS) are fabricated on silicon substrates using femtosecond laser irradiation to investigate their formation mechanisms and impact on Raman signal enhancement. By systematically varying the laser fluence and pulse number, their effects are examined on LIPSS periodicity and, consequently, SERS performance. The results reveal that increasing laser fluence from 0.80 to 1.40 J/cm2 significantly reduces LIPSS periodicity due to enhanced Surface Plasmon Polaritons (SPPs) excitation and energy redistribution. LIPSS exhibit elongated elliptical structures at lower pulse numbers, which gradually transition into circular patterns with increasing pulses, driven by electric field redistribution and interference effects. The influence of LIPSS on SERS is systematically analyzed using a thiophenol solution to evaluate Raman signal sensitivity. The results demonstrate that precisely tuned periodicity and depth of LIPSS significantly enhance SERS signals by optimizing localized electromagnetic fields and plasmonic resonance effects. Notably, LIPSS with a periodicity of ∼795 nm exhibited the highest enhancement due to the resonant coupling of SPPs with the excitation laser, while optimal depths (∼352–547 nm) balanced hotspot density and plasmonic efficiency.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 14","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500366","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144740456","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Wide-Field Bond Quality Evaluation Using Frequency Domain Thermoreflectance with Deep Neural Network Feature Reconstruction (Adv. Mater. Interfaces 13/2025) 基于频域热反射和深度神经网络特征重构的宽场键合质量评价。接口13/2025)

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70057

Amun Jarzembski, Siddharth Nair, Wyatt Hodges, Matthew Jordan, Anthony McDonald, Logan Antiporda, Greg W. Pickrell, Timothy Walsh, Fabio Semperlotti, Jason Neely, Luke Yates

引用次数: 0

Bioinspired Spider Silk Fiber of MOF-Based Zwitterionic Hydrogel for Low-Humidity Atmospheric Water Harvesting 生物灵感蜘蛛丝纤维mof基两性离子水凝胶用于低湿度大气集水

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.202500421

Hengyu Pan, Lingmei Zhu, Huijie Wei, Chang Gao, Maolin Zhou, Tiance Zhang, Qiang Luo, Boyang Tian, Jianhua Wang, Yongping Hou, Yongmei Zheng

{"title":"Bioinspired Spider Silk Fiber of MOF-Based Zwitterionic Hydrogel for Low-Humidity Atmospheric Water Harvesting","authors":"Hengyu Pan, Lingmei Zhu, Huijie Wei, Chang Gao, Maolin Zhou, Tiance Zhang, Qiang Luo, Boyang Tian, Jianhua Wang, Yongping Hou, Yongmei Zheng","doi":"10.1002/admi.202500421","DOIUrl":"https://doi.org/10.1002/admi.202500421","url":null,"abstract":"A bioinspired spider silk fiber (i.e., PCLC) is presented by introducing the zwitterionic hydrogel poly-[2-(methacryloyloxy)ethyl] dimethyl-(3-sulfopropyl)ammonium hydroxide (PDMAPS) and CAU-10-H used as carriers of hygroscopic salt Lithium chloride (LiCl), and the addition of carbon black (CB) nanoparticles makes the prepared fibers have photothermal effect. PCLC fiber achieves the moisture absorption capacity of ≈1.49 – 1.99 g g−1 after 2 h adsorption at ≈40% relative humidity (RH). The temperature of a single PCLC knot can rise to 46.4 °C for ≈3600 s, and the temperature of a batch of PCLC spider knot fibers can rise to 112.1 °C for ≈3600 s (under ≈1 sun illumination), which has excellent photothermal effect. Water collection is conducted for five consecutive days with a daily collected amount of ≈1.87 g g−1. The PCLC fiber shows good water vapor adsorption reversibility after 10 consecutive adsorption-desorption cycles, the moisture absorption can be stabilized at ≈1.9 g g−1, and the water vapor desorption capacity reaches ≈1.73 g g−1 (under ≈1 sun illumination, exhibiting water vapor desorption efficiency of ≈92.1%).","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 15","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500421","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145146260","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Mechanistic Insights Into Proton and Oxygen Transport Through Ultrathin Amorphous Al2O3 and Al2O3-SiO2 Electrocatalyst Overlayers (Adv. Mater. Interfaces 13/2025) 超薄无定形Al2O3和Al2O3- sio2电催化层中质子和氧传输的机理研究（Adv. Mater.）。接口13/2025)

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70055

Dalia Leon-Chaparro, Minh Duc Nguyen, Christoph Baeumer, Guido Mul, Georgios Katsoukis

引用次数: 0

Nanohybrid of Silver-MXene: A Promising Sorbent for Iodine Gas Capture from Nuclear Waste (Adv. Mater. Interfaces 13/2025) 银- mxene纳米杂化材料：一种有前途的核废料碘气体捕集剂。接口13/2025)

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70056

Karamullah Eisawi, Elham Loni, Saehwa Chong, Martin Liezers, Ming Tang, Kyle S. Brinkman, Brian J. Riley, Michael Naguib

引用次数: 0

Rapid and Scalable Lubrication Coating for Industrial and Medical Applications via Sequential Dip-Coating 快速和可扩展的润滑涂层工业和医疗应用通过顺序浸涂

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-16 DOI: 10.1002/admi.202500353

Yeontaek Lee, Kayoung Son, Yejin Jo, Seung Hyun Lee, Jeuhee Lee, Tae Young Kim, Seonghyeon Eom, Youn-Hoo Hwang, Dae-Eun Kim, Inhee Choi, Jung Seung Lee, Jungmok Seo

{"title":"Rapid and Scalable Lubrication Coating for Industrial and Medical Applications via Sequential Dip-Coating","authors":"Yeontaek Lee, Kayoung Son, Yejin Jo, Seung Hyun Lee, Jeuhee Lee, Tae Young Kim, Seonghyeon Eom, Youn-Hoo Hwang, Dae-Eun Kim, Inhee Choi, Jung Seung Lee, Jungmok Seo","doi":"10.1002/admi.202500353","DOIUrl":"10.1002/admi.202500353","url":null,"abstract":"Surface coatings have been widely studied and applied in industrial and biomedical fields to give functionalities such as friction reduction, anti-fouling, and enhanced biocompatibility. However, conventional coating techniques often suffer from limited material compatibility, non-uniform coverage on complex geometries, labor-intensive fabrication, and dependence on specialized equipment. In this study, Swift Lubrication is introduced for Industrial and Medical Equipment (SLIME), a rapid (≈10 s) two-step dip-coating method that employs an UV perfluoropolyether base coat followed by a slippery activation layer. SLIME enables the formation of ultra-low friction surfaces, robust anti-fouling properties, and effective diffusion barrier functionality without requiring intricate fabrication processes or specialized equipment. The versatility of SLIME coatings is demonstrated through their application on 3D-printed molds, high-viscosity storage containers, and various biomedical devices, highlighting their material-independent applicability, excellent biocompatibility, and superior anti-adhesion performance. This is envision that SLIME coatings will serve as a practical and scalable solution for an advanced surface lubrication method, significantly enhancing device durability, operational efficiency, and performance across industrial and biomedical applications.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 14","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500353","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144740186","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Exploring the Potential of Silicon Clathrate Films with NiOx-Based Selective Contacts for Optoelectronic Devices 探索具有niox基选择性触点的硅包合物薄膜在光电器件中的潜力

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-15 DOI: 10.1002/admi.202500301

Charif Tamin, Anil Kumar Bharwal, Céline Chevalier, Alain Fave, Erwann Fourmond, Stéphane Roques, Aziz Dinia, Abdelilah Slaoui, Thomas Fix

{"title":"Exploring the Potential of Silicon Clathrate Films with NiOx-Based Selective Contacts for Optoelectronic Devices","authors":"Charif Tamin, Anil Kumar Bharwal, Céline Chevalier, Alain Fave, Erwann Fourmond, Stéphane Roques, Aziz Dinia, Abdelilah Slaoui, Thomas Fix","doi":"10.1002/admi.202500301","DOIUrl":"10.1002/admi.202500301","url":null,"abstract":"Silicon clathrates are a unique class of materials with a cage-like structure that offer significant advantages for optoelectronic applications, particularly in indoor photovoltaics (IPV). Their direct bandgaps and tunable electronic properties from metal-like to semiconductor-like behavior enable a wide range of optoelectronic functionalities. In this study, a photovoltaic device is demonstrated based on semiconducting silicon clathrate films (SCF) synthesized from crystalline silicon (c-Si) wafers, with NiOx incorporated as hole selective contact. XPS and Auger spectroscopy confirmed the incorporation of Na within the SCF framework, in agreement with the type-II clathrate structure revealed by XRD analysis. Optical and electronic measurements indicate that the SCF exhibits intrinsic-like behavior with a bandgap of 1.72 eV. Integration of SCF with NiOx resulted in rectification and a clear photovoltaic response under illumination, confirming device functionality. Band alignment analysis suggested efficient hole transport and secondary charge generation from the c-Si substrate. These results highlight the importance of selective contact engineering for efficient charge extraction and demonstrate the potential for further optimization of SCF photovoltaic devices.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 17","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500301","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145032308","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0