Advanced Materials Interfaces最新文献_第7页

Sugars in Antimicrobial Polymers – The Impact of Sugar-Lectin Binding in Membrane Interaction of Cationic Glycopolymers 抗菌聚合物中的糖-糖-凝集素结合对阳离子糖共聚物膜相互作用的影响

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-27 DOI: 10.1002/admi.202500273

Alain M. Bapolisi, Steffen Tank, Anne-Catherine Lehnen, Antje Stindt, Rujuta Athavale, Jan A. M. Kurki, Sany Chea, Sophia Rosencrantz, Ruben R. Rosencrantz, Katja M. Arndt, Matthias Hartlieb

{"title":"Sugars in Antimicrobial Polymers – The Impact of Sugar-Lectin Binding in Membrane Interaction of Cationic Glycopolymers","authors":"Alain M. Bapolisi, Steffen Tank, Anne-Catherine Lehnen, Antje Stindt, Rujuta Athavale, Jan A. M. Kurki, Sany Chea, Sophia Rosencrantz, Ruben R. Rosencrantz, Katja M. Arndt, Matthias Hartlieb","doi":"10.1002/admi.202500273","DOIUrl":"10.1002/admi.202500273","url":null,"abstract":"Membrane-active antimicrobial polymers (APs) are promising alternatives for treating infectious diseases as they are less susceptible to antimicrobial resistance development. However, their non-specific cytotoxicity limits their clinical application. One interesting strategy to improve cytocompatibility is the incorporation of sugar units into APs. This approach takes advantage of specific interactions between sugars and protein receptors, such as lectins, on the surface of bacteria, potentially allowing for discrimination between different bacterial types. However, there is limited research on how sugar addition to cationic APs affects their selectivity and interactions with lectins. Herein, a library of acrylamide-based cationic glycopolymers is synthesized by a xanthate-supported photo-initiated Reversible Additon-Fragmentation chain Trasnfer (XPI-RAFT) polymerization. Diverse sugars are added to this cationic scaffold by either chain extension with glycomonomers (based on fucose, glucose, mannose, and polyhydroxy acrylamide) or simply by reductive amination (lactose and melibiose). Various analytical techniques are used to probe the interaction of (glyco)polymers with bacteria, membrane models, and lectins. In general, (glyco)polyhydroxy incorporation proves to reduce the hydrophobicity of the cationic APs and consequently enhances hemocompatibility while maintaining the antimicrobial activity. Although sugar-protein-specific recognition may contribute to selectivity, the results demonstrate that electrostatic interaction predominantly drives the binding efficacy of cationic glycopolymers to bacterial membranes.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 16","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500273","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144894482","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Local Femtosecond Pulsed Laser Decoating of Superhydrophobic Paper Coating for Enhanced Fog Harvesting Efficiency 超疏水纸涂层局部飞秒脉冲激光消光提高雾收集效率

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-27 DOI: 10.1002/admi.202500332

Martin Kahlmeyer, Carina Breuer, Andreas Winkel, Markus Biesalski, Camilo Florian-Baron, Stefan Böhm

{"title":"Local Femtosecond Pulsed Laser Decoating of Superhydrophobic Paper Coating for Enhanced Fog Harvesting Efficiency","authors":"Martin Kahlmeyer, Carina Breuer, Andreas Winkel, Markus Biesalski, Camilo Florian-Baron, Stefan Böhm","doi":"10.1002/admi.202500332","DOIUrl":"10.1002/admi.202500332","url":null,"abstract":"Superhydrophobic paper has demonstrated significant potential for efficient water harvesting. Previous studies have indicated that the incorporation of pinning structures on superhydrophobic surfaces can enhance water collection efficiency. This study explores the feasibility of creating such pinning structures through femtosecond laser ablation of wax-based superhydrophobic coatings. Static contact angle measurements and the roll-off behavior of droplets on laser-treated surfaces are conducted to evaluate the effects of laser ablation. Additionally, fogging tests are performed to assess the water collection performance, revealing an improvement of above 10% in comparison to unmodified superhydrophobic paper without localized pinning structures. Notably, the laser ablation process minimally affects the load-bearing capacity of the paper, ensuring that its structural integrity is preserved. The ability to design laterally resolved pinning structures opens new possibilities for further optimization, such as the creation of flow paths, ultimately enhancing the overall efficiency of water harvesting systems.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 17","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500332","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145032303","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Advancing Methylene Blue Adsorption Approach for More Precise Measurement of Specific Surface Area of Graphene Oxide 推进亚甲基蓝吸附法更精确测量氧化石墨烯比表面积

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-24 DOI: 10.1002/admi.202500233

Pei Lay Yap, Deyu Wang, Dusan Losic

{"title":"Advancing Methylene Blue Adsorption Approach for More Precise Measurement of Specific Surface Area of Graphene Oxide","authors":"Pei Lay Yap, Deyu Wang, Dusan Losic","doi":"10.1002/admi.202500233","DOIUrl":"10.1002/admi.202500233","url":null,"abstract":"The industrial production of graphene oxide (GO) using various oxidizing precursors and processing conditions results in substantial variability in their composition of oxygen-containing groups, structures, and specific surface area (SSA), which are critical to its performance in diverse applications. Spectrophotometric methylene blue (MB) adsorption has emerged as a promising alternative to the conventional nitrogen physisorption method. However, this method still lacks a standardized and optimized protocol, limiting its reliability and consistency in SSA determination. To address this gap, this study systematically evaluates the uncertainties in the MB-based SSA characterization by revealing the influence of key experimental parameters and their optimization, including adsorption time, GO and MB concentration, MB/GO ratio, and the methods for determining maximum MB adsorption capacity on GO using both single-point and multi-point Langmuir isotherm approaches. A series of commercial and lab-prepared GOs materials in different forms (powders, aerogels, films, and dispersions) are used as model systems. The study confirms the optimized parameters, including adsorption time (24 h), concentrations of MB (0.005–0.02 mg mL−1), GO (0.5–2.0 mg mL−1), MB/GO weight ratio (0.4–0.44), and single-point MB adsorption. This refined protocol offers a robust, rapid, low-cost, and reliable characterization and quality control of manufactured GO materials.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 17","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500233","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145032322","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Dynamic Wettability Behavior of Emerging Ultrawhite Radiative Cooling Paints 新兴超白辐射冷却涂料的动态润湿性

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-24 DOI: 10.1002/admi.202500288

Orlando G. Rivera González, Abdulrahman K. Aljwirah, Andrea L. Felicelli, Xiulin Ruan, Justin A. Weibel

{"title":"Dynamic Wettability Behavior of Emerging Ultrawhite Radiative Cooling Paints","authors":"Orlando G. Rivera González, Abdulrahman K. Aljwirah, Andrea L. Felicelli, Xiulin Ruan, Justin A. Weibel","doi":"10.1002/admi.202500288","DOIUrl":"10.1002/admi.202500288","url":null,"abstract":"Outdoor radiative cooling surfaces passively lose heat by reflecting solar irradiation and emitting infrared radiation to cold deep space through the atmospheric sky window (8–13 µm), thereby achieving sub-ambient temperature. Ultrawhite radiative cooling paints are an emerging technology offering scalable solutions for cooling and passive water harvesting wherein surface wettability plays a key role. This work, examines how radiative cooling paint pigment and binder formulations affect surface morphology, roughness, and dynamic wettability. Samples are prepared with three different nanoparticulate pigments, calcium carbonate (CaCO3), barium sulfate (BaSO4), and hexagonal boron nitride (hBN); two binders, including an acrylic and a waterborne silicone-modified polyurethane dispersion (SILIKOPUR 8081); and pigment solid volume concentrations from 0% to 80% v/v. The CaCO3 and BaSO4 pigments produced paints with rougher textures and higher contact angles due to their pigment particle morphology. While high solar reflectance was achieved across various pigment and binder combinations, wettability exhibited a complex trend with pigment concentration, indicating that maximizing reflectance does not necessarily optimize wetting behavior. This expanded understanding on how pigment type, binder and concentration influence wettability, offering pathways to design coatings with tailored spectral and wetting properties for both self-cleaning paints and passive water harvesting applications","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 16","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500288","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144894400","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Surface Performance of Bioactive Glass–Polycaprolactone–Gelatin Nanocomposite Coating on Anodized Ti6Al4V Alloy 氧化Ti6Al4V合金生物活性玻璃-聚己内酯-明胶纳米复合涂层的表面性能

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-22 DOI: 10.1002/admi.202500179

Sharareh Mehrnoush, Sheyda Labbaf, Abdoulmajid Eslami, Majid Goli

{"title":"Surface Performance of Bioactive Glass–Polycaprolactone–Gelatin Nanocomposite Coating on Anodized Ti6Al4V Alloy","authors":"Sharareh Mehrnoush, Sheyda Labbaf, Abdoulmajid Eslami, Majid Goli","doi":"10.1002/admi.202500179","DOIUrl":"https://doi.org/10.1002/admi.202500179","url":null,"abstract":"In this study, a polycaprolactone-gelatin composite coating containing 0, 5, 15, and 25 wt.% bioactive glass nanoparticles (with a size of 96 ± 12 nm) is electrosprayed onto the surface of anodized Ti6Al4V alloy to improve surface properties. Hydrophilicity increased with higher bioactive glass content, with the 15 wt% coating achieving a contact angle of 53.66°. Corrosion testing indicated that all coatings enhanced substrate protection, with the 15 wt% showing superior passivation.The bioactivity results show that a higher amount of hydroxyapatite have formed on the 15 wt.% sample, with a calcium-to-phosphorus ratio of 1.65. All coated groups revealed a non-cytotoxic behavior upon exposure to MG63 cells, with 15 wt.% demonstrating a better performance in terms of cell adhesion and proliferation. This group also presents antibacterial properties, forming halos with diameters of 13.92 and 10.57 mm for Escherichia coli and Staphylococcus aureus, respectively. The findings support its potential as an advanced surface modification technique for orthopedic implants offering significant improvements over conventional methods.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 15","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500179","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145146275","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Empirical Analysis of Frictional Forces in Advancing and Receding Triple-Phase Contact Lines: Effect of Surface Roughness 进退三相接触线摩擦力的实证分析：表面粗糙度的影响

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-21 DOI: 10.1002/admi.202500258

Sreya Sarkar, Arani Mukhopadhyay, Anish Pal, Constantine M. Megaridis

{"title":"Empirical Analysis of Frictional Forces in Advancing and Receding Triple-Phase Contact Lines: Effect of Surface Roughness","authors":"Sreya Sarkar, Arani Mukhopadhyay, Anish Pal, Constantine M. Megaridis","doi":"10.1002/admi.202500258","DOIUrl":"10.1002/admi.202500258","url":null,"abstract":"Predicting the open-surface movement of liquids on solids requires a fundamental understanding of adhesion and the interplay of frictional forces at the moving contact line. Frictional forces are commonly studied in two main contexts: (1) static and kinetic friction acting on droplets subjected to lateral forces, and (2) resisting (frictional) forces opposing the motion of advancing or receding liquid contact lines on solid surfaces. While conventional studies assume identical advancing and receding frictional forces for any liquid–solid pair, recent studies have challenged this notion, emphasizing the need for deeper insight into these forces, especially when the solid is rough. This study employs sessile-droplet experiments for unpinned Wenzel (penetrating) states to quantify frictional forces at the triple-phase contact line, revealing an empirical relationship between frictional force ratio and surface roughness. Contact angle (CA) measurements at constant contact-line speeds under negligible viscous effects (Capillary number, Cα < <1) demonstrate that the advancing-to-receding friction force ratio scales solely with Wenzel roughness, being independent of liquid surface tension, viscosity, or chemical composition. This relationship enables accurate predictions of intrinsic CAs (<2% error) for wetting scenarios where experimental determination is challenging. The findings provide a predictive framework for characterizing new materials and their surface energies, while promoting the understanding and application of wetting dynamics on realistic (rough) surfaces.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 14","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500258","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144740073","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Laser-Induced Nano-Functional Surfaces for Enhanced SERS Performance 增强SERS性能的激光诱导纳米功能表面

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-18 DOI: 10.1002/admi.202500366

Hardik Vaghasiya, Paul-Tiberiu Miclea

{"title":"Laser-Induced Nano-Functional Surfaces for Enhanced SERS Performance","authors":"Hardik Vaghasiya, Paul-Tiberiu Miclea","doi":"10.1002/admi.202500366","DOIUrl":"10.1002/admi.202500366","url":null,"abstract":"Nanostructured metal surfaces play a crucial role in sensing applications, particularly in Surface-Enhanced Raman Spectroscopy (SERS). In this study, laser-induced periodic surface structures (LIPSS) are fabricated on silicon substrates using femtosecond laser irradiation to investigate their formation mechanisms and impact on Raman signal enhancement. By systematically varying the laser fluence and pulse number, their effects are examined on LIPSS periodicity and, consequently, SERS performance. The results reveal that increasing laser fluence from 0.80 to 1.40 J/cm2 significantly reduces LIPSS periodicity due to enhanced Surface Plasmon Polaritons (SPPs) excitation and energy redistribution. LIPSS exhibit elongated elliptical structures at lower pulse numbers, which gradually transition into circular patterns with increasing pulses, driven by electric field redistribution and interference effects. The influence of LIPSS on SERS is systematically analyzed using a thiophenol solution to evaluate Raman signal sensitivity. The results demonstrate that precisely tuned periodicity and depth of LIPSS significantly enhance SERS signals by optimizing localized electromagnetic fields and plasmonic resonance effects. Notably, LIPSS with a periodicity of ∼795 nm exhibited the highest enhancement due to the resonant coupling of SPPs with the excitation laser, while optimal depths (∼352–547 nm) balanced hotspot density and plasmonic efficiency.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 14","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500366","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144740456","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Wide-Field Bond Quality Evaluation Using Frequency Domain Thermoreflectance with Deep Neural Network Feature Reconstruction (Adv. Mater. Interfaces 13/2025) 基于频域热反射和深度神经网络特征重构的宽场键合质量评价。接口13/2025)

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.70057

Amun Jarzembski, Siddharth Nair, Wyatt Hodges, Matthew Jordan, Anthony McDonald, Logan Antiporda, Greg W. Pickrell, Timothy Walsh, Fabio Semperlotti, Jason Neely, Luke Yates

引用次数: 0

Bioinspired Spider Silk Fiber of MOF-Based Zwitterionic Hydrogel for Low-Humidity Atmospheric Water Harvesting 生物灵感蜘蛛丝纤维mof基两性离子水凝胶用于低湿度大气集水

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.202500421

Hengyu Pan, Lingmei Zhu, Huijie Wei, Chang Gao, Maolin Zhou, Tiance Zhang, Qiang Luo, Boyang Tian, Jianhua Wang, Yongping Hou, Yongmei Zheng

{"title":"Bioinspired Spider Silk Fiber of MOF-Based Zwitterionic Hydrogel for Low-Humidity Atmospheric Water Harvesting","authors":"Hengyu Pan, Lingmei Zhu, Huijie Wei, Chang Gao, Maolin Zhou, Tiance Zhang, Qiang Luo, Boyang Tian, Jianhua Wang, Yongping Hou, Yongmei Zheng","doi":"10.1002/admi.202500421","DOIUrl":"https://doi.org/10.1002/admi.202500421","url":null,"abstract":"A bioinspired spider silk fiber (i.e., PCLC) is presented by introducing the zwitterionic hydrogel poly-[2-(methacryloyloxy)ethyl] dimethyl-(3-sulfopropyl)ammonium hydroxide (PDMAPS) and CAU-10-H used as carriers of hygroscopic salt Lithium chloride (LiCl), and the addition of carbon black (CB) nanoparticles makes the prepared fibers have photothermal effect. PCLC fiber achieves the moisture absorption capacity of ≈1.49 – 1.99 g g−1 after 2 h adsorption at ≈40% relative humidity (RH). The temperature of a single PCLC knot can rise to 46.4 °C for ≈3600 s, and the temperature of a batch of PCLC spider knot fibers can rise to 112.1 °C for ≈3600 s (under ≈1 sun illumination), which has excellent photothermal effect. Water collection is conducted for five consecutive days with a daily collected amount of ≈1.87 g g−1. The PCLC fiber shows good water vapor adsorption reversibility after 10 consecutive adsorption-desorption cycles, the moisture absorption can be stabilized at ≈1.9 g g−1, and the water vapor desorption capacity reaches ≈1.73 g g−1 (under ≈1 sun illumination, exhibiting water vapor desorption efficiency of ≈92.1%).","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 15","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500421","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145146260","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

High-Throughput Design of Epitaxial Orientation for Functional Thin Films 功能薄膜外延取向的高通量设计

IF 4.4 3区材料科学

Advanced Materials Interfaces Pub Date : 2025-07-17 DOI: 10.1002/admi.202500382

Liyufen Dai, Mingqiang Cheng, Mingqiang Huang, Xiangli Zhong, Gaokuo Zhong

{"title":"High-Throughput Design of Epitaxial Orientation for Functional Thin Films","authors":"Liyufen Dai, Mingqiang Cheng, Mingqiang Huang, Xiangli Zhong, Gaokuo Zhong","doi":"10.1002/admi.202500382","DOIUrl":"10.1002/admi.202500382","url":null,"abstract":"The structure and properties of functional thin films are highly sensitive to their epitaxial orientations. However, the orientation of the thin film is typically constrained by that of the substrate, making it challenging to achieve distinct orientations between the thin film and the substrate. The use of buffer layers is an effective approach to manipulate the epitaxial orientations of functional thin films. Nevertheless, this method requires precise screening of buffer layer parameters that may influence the orientation of the overlying functional layer, making the process labor-intensive and time-consuming. Here, a high-throughput strategy is proposed for screening buffer layer parameters. Taking the epitaxial growth of PbZr1-xTixO3 ferroelectric films as a model system, the optimal thickness of the CoFe2O4 buffer layer is successfully determined, enabling the epitaxial growth of [111]-oriented PbZr0.2Ti0.8O3 on a [001]-oriented Mica substrate. Furthermore, a composite buffer layer structure consisting of SrRuO3 and CoFe2O4 is screened, which facilitated the epitaxial growth of [111]-oriented PbZr1-xTixO3 films on a [001]-oriented SrTiO3 substrate. This work establishes an efficient approach for the high-throughput screening of buffer layer structures and provides valuable insights into the design of epitaxial functional thin films beyond conventional substrate constraints.","PeriodicalId":115,"journal":{"name":"Advanced Materials Interfaces","volume":"12 16","pages":""},"PeriodicalIF":4.4,"publicationDate":"2025-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admi.202500382","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144894229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0