Nano Convergence最新文献

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Materials descriptors of machine learning to boost development of lithium-ion batteries 利用机器学习的材料描述符促进锂离子电池的开发
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2024-02-26 DOI: 10.1186/s40580-024-00417-6
Zehua Wang, Li Wang, Hao Zhang, Hong Xu, Xiangming He
{"title":"Materials descriptors of machine learning to boost development of lithium-ion batteries","authors":"Zehua Wang,&nbsp;Li Wang,&nbsp;Hao Zhang,&nbsp;Hong Xu,&nbsp;Xiangming He","doi":"10.1186/s40580-024-00417-6","DOIUrl":"10.1186/s40580-024-00417-6","url":null,"abstract":"<div><p>Traditional methods for developing new materials are no longer sufficient to meet the needs of the human energy transition. Machine learning (ML) artificial intelligence (AI) and advancements have caused materials scientists to realize that using AI/ML to accelerate the development of new materials for batteries is a powerful potential tool. Although the use of certain fixed properties of materials as descriptors to act as a bridge between the two separate disciplines of AI and materials chemistry has been widely investigated, many of the descriptors lack universality and accuracy due to a lack of understanding of the mechanisms by which AI/ML operates. Therefore, understanding the underlying operational mechanisms and learning logic of AI/ML has become mandatory for materials scientists to develop more accurate descriptors. To address those challenges, this paper reviews previous work on AI, machine learning and materials descriptors and introduces the basic logic of AI and machine learning to help materials developers understand their operational mechanisms. Meanwhile, the paper also compares the accuracy of different descriptors and their advantages and disadvantages and highlights the great potential value of accurate descriptors in AI/machine learning applications for battery research, as well as the challenges of developing accurate material descriptors.</p><h3>Graphical Abstract</h3>\u0000<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"11 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2024-02-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://nanoconvergencejournal.springeropen.com/counter/pdf/10.1186/s40580-024-00417-6","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139967788","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of gut microbiota-derived metabolites and extracellular vesicles on neurodegenerative disease in a gut-brain axis chip 肠道微生物群衍生代谢物和细胞外囊泡对肠脑轴芯片神经退行性疾病的影响
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2024-02-10 DOI: 10.1186/s40580-024-00413-w
Na Yeon Kim, Ho Yeon Lee, Yoon Young Choi, Sung Jun Mo, Soomin Jeon, Jang Ho Ha, Soo Dong Park, Jae-Jung Shim, Jaehwan Lee, Bong Geun Chung
{"title":"Effect of gut microbiota-derived metabolites and extracellular vesicles on neurodegenerative disease in a gut-brain axis chip","authors":"Na Yeon Kim,&nbsp;Ho Yeon Lee,&nbsp;Yoon Young Choi,&nbsp;Sung Jun Mo,&nbsp;Soomin Jeon,&nbsp;Jang Ho Ha,&nbsp;Soo Dong Park,&nbsp;Jae-Jung Shim,&nbsp;Jaehwan Lee,&nbsp;Bong Geun Chung","doi":"10.1186/s40580-024-00413-w","DOIUrl":"10.1186/s40580-024-00413-w","url":null,"abstract":"<div><p>A new perspective suggests that a dynamic bidirectional communication system, often referred to as the microbiome-gut-brain axis, exists among the gut, its microbiome, and the central nervous system (CNS). This system may influence brain health and various brain-related diseases, especially in the realms of neurodevelopmental and neurodegenerative conditions. However, the exact mechanism is not yet understood. Metabolites or extracellular vesicles derived from microbes in the gut have the capacity to traverse the intestinal epithelial barrier or blood–brain barrier, gaining access to the systemic circulation. This phenomenon can initiate the physiological responses that directly or indirectly impact the CNS and its function. However, reliable and controllable tools are required to demonstrate the causal effects of gut microbial-derived substances on neurogenesis and neurodegenerative diseases. The integration of microfluidics enhances scientific research by providing advanced in vitro engineering models. In this study, we investigated the impact of microbe-derived metabolites and exosomes on neurodevelopment and neurodegenerative disorders using human induced pluripotent stem cells (iPSCs)-derived neurons in a gut-brain axis chip. While strain-specific, our findings indicate that both microbial-derived metabolites and exosomes exert the significant effects on neural growth, maturation, and synaptic plasticity. Therefore, our results suggest that metabolites and exosomes derived from microbes hold promise as potential candidates and strategies for addressing neurodevelopmental and neurodegenerative disorders.</p></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"11 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2024-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://nanoconvergencejournal.springeropen.com/counter/pdf/10.1186/s40580-024-00413-w","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139715711","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Polymeric DNase-I nanozymes targeting neutrophil extracellular traps for the treatment of bowel inflammation 针对中性粒细胞胞外捕获物的聚合 DNase-I 纳米酶用于治疗肠道炎症。
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2024-02-08 DOI: 10.1186/s40580-024-00414-9
Chi-Pin James Wang, Ga Ryang Ko, Yun Young Lee, Juwon Park, Wooram Park, Tae-Eun Park, Yoonhee Jin, Se-Na Kim, Jung Seung Lee, Chun Gwon Park
{"title":"Polymeric DNase-I nanozymes targeting neutrophil extracellular traps for the treatment of bowel inflammation","authors":"Chi-Pin James Wang,&nbsp;Ga Ryang Ko,&nbsp;Yun Young Lee,&nbsp;Juwon Park,&nbsp;Wooram Park,&nbsp;Tae-Eun Park,&nbsp;Yoonhee Jin,&nbsp;Se-Na Kim,&nbsp;Jung Seung Lee,&nbsp;Chun Gwon Park","doi":"10.1186/s40580-024-00414-9","DOIUrl":"10.1186/s40580-024-00414-9","url":null,"abstract":"<div><p>Inflammatory bowel disease (IBD), including Crohn’s disease and ulcerative colitis, is a family of chronic disorders along the gastrointestinal tract. Because of its idiopathic nature, IBD does not have a fundamental cure; current available therapies for IBD are limited to prolonged doses of immunomodulatory agents. While these treatments may reduce inflammation, limited therapeutic efficacy, inconsistency across patients, and adverse side effects from aggressive medications remain as major drawbacks. Recently, excessive production and accumulation of neutrophil extracellular traps (NETs) also known as NETosis have been identified to exacerbate inflammatory responses and induce further tissue damage in IBD. Such discovery invited many researchers to investigate NETs as a potential therapeutic target. DNase-I is a natural agent that can effectively destroy NETs and, therefore, potentially reduce NETs-induced inflammations even without the use of aggressive drugs. However, low stability and rapid clearance of DNase-I remain as major limitations for further therapeutic applications. In this research, polymeric nanozymes were fabricated to increase the delivery and therapeutic efficacy of DNase-I. DNase-I was immobilized on the surface of polymeric nanoparticles to maintain its enzymatic properties while extending its activity in the colon. Delivery of DNase-I using this platform allowed enhanced stability and prolonged activity of DNase-I with minimal toxicity. When administered to animal models of IBD, DNase-I nanozymes successfully alleviated various pathophysiological symptoms of IBD. More importantly, DNase-I nanozyme administration successfully attenuated neutrophil infiltration and NETosis in the colon compared to free DNase-I or mesalamine.</p></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"11 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2024-02-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://nanoconvergencejournal.springeropen.com/counter/pdf/10.1186/s40580-024-00414-9","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139705749","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Formation techniques for upper active channel in monolithic 3D integration: an overview 单片三维集成中的上部主动通道形成技术:概述。
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2024-01-29 DOI: 10.1186/s40580-023-00411-4
An Hoang-Thuy Nguyen, Manh-Cuong Nguyen, Anh-Duy Nguyen, Seung Joon Jeon, Noh-Hwal Park, Jeong-Hwan Lee, Rino Choi
{"title":"Formation techniques for upper active channel in monolithic 3D integration: an overview","authors":"An Hoang-Thuy Nguyen,&nbsp;Manh-Cuong Nguyen,&nbsp;Anh-Duy Nguyen,&nbsp;Seung Joon Jeon,&nbsp;Noh-Hwal Park,&nbsp;Jeong-Hwan Lee,&nbsp;Rino Choi","doi":"10.1186/s40580-023-00411-4","DOIUrl":"10.1186/s40580-023-00411-4","url":null,"abstract":"<div><p>The concept of three-dimensional stacking of device layers has attracted significant attention with the increasing difficulty in scaling down devices. Monolithic 3D (M3D) integration provides a notable benefit in achieving a higher connection density between upper and lower device layers than through-via-silicon. Nevertheless, the practical implementation of M3D integration into commercial production faces several technological challenges. Developing an upper active channel layer for device fabrication is the primary challenge in M3D integration. The difficulty arises from the thermal budget limitation for the upper channel process because a high thermal budget process may degrade the device layers below. This paper provides an overview of the potential technologies for forming active channel layers in the upper device layers of M3D integration, particularly for complementary metal-oxide-semiconductor devices and digital circuits. Techniques are for polysilicon, single crystal silicon, and alternative channels, which can solve the temperature issue for the top layer process.</p></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"11 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2024-01-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://nanoconvergencejournal.springeropen.com/counter/pdf/10.1186/s40580-023-00411-4","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139569447","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
How to improve the structural stabilities of halide perovskite quantum dots: review of various strategies to enhance the structural stabilities of halide perovskite quantum dots 如何提高卤化物包晶量子点的结构稳定性:综述提高卤化物包晶量子点结构稳定性的各种策略。
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2024-01-27 DOI: 10.1186/s40580-024-00412-x
Dokyum Kim, Taesun Yun, Sangmin An, Chang-Lyoul Lee
{"title":"How to improve the structural stabilities of halide perovskite quantum dots: review of various strategies to enhance the structural stabilities of halide perovskite quantum dots","authors":"Dokyum Kim,&nbsp;Taesun Yun,&nbsp;Sangmin An,&nbsp;Chang-Lyoul Lee","doi":"10.1186/s40580-024-00412-x","DOIUrl":"10.1186/s40580-024-00412-x","url":null,"abstract":"<div><p>Halide perovskites have emerged as promising materials for various optoelectronic devices because of their excellent optical and electrical properties. In particular, halide perovskite quantum dots (PQDs) have garnered considerable attention as emissive materials for light-emitting diodes (LEDs) because of their higher color purities and photoluminescence quantum yields compared to conventional inorganic quantum dots (CdSe, ZnSe, ZnS, etc.). However, PQDs exhibit poor structural stabilities in response to external stimuli (moisture, heat, etc<i>.</i>) owing to their inherent ionic nature. This review presents recent research trends and insights into improving the structural stabilities of PQDs. In addition, the origins of the poor structural stabilities of PQDs and various methods to overcome this drawback are discussed. The structural degradation of PQDs is mainly caused by two mechanisms: (1) defect formation on the surface of the PQDs by ligand dissociation (<i>i.e.,</i> detachment of weakly bound ligands from the surface of PQDs), and (2) vacancy formation by halide migration in the lattices of the PQDs due to the low migration energy of halide ions. The structural stabilities of PQDs can be improved through four methods: (1) ligand modification, (2) core–shell structure, (3) crosslinking, and (4) metal doping, all of which are presented in detail herein. This review provides a comprehensive understanding of the structural stabilities and opto-electrical properties of PQDs and is expected to contribute to future research on improving the device performance of perovskite quantum dot LEDs (PeLEDs).</p></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"11 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2024-01-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10821855/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139569448","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advances in nanobiosensors during the COVID-19 pandemic and future perspectives for the post-COVID era COVID-19 大流行期间纳米生物传感器的进展以及后 COVID 时代的未来展望。
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2024-01-11 DOI: 10.1186/s40580-023-00410-5
Young Jun Kim, Junhong Min
{"title":"Advances in nanobiosensors during the COVID-19 pandemic and future perspectives for the post-COVID era","authors":"Young Jun Kim,&nbsp;Junhong Min","doi":"10.1186/s40580-023-00410-5","DOIUrl":"10.1186/s40580-023-00410-5","url":null,"abstract":"<div><p>The unprecedented threat of the highly contagious virus, severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2), which causes exponentially increased infections of coronavirus disease 2019 (COVID-19), highlights the weak spots of the current diagnostic toolbox. In the midst of catastrophe, nanobiosensors offer a new opportunity as an alternative tool to fill a gap among molecular tests, rapid antigen tests, and serological tests. Nanobiosensors surpass the potential of antigen tests because of their enhanced sensitivity, thus enabling us to see antigens as stable and easy-to-access targets. During the first three years of the COVID-19 pandemic, a substantial number of studies have reported nanobiosensors for the detection of SARS-CoV-2 antigens. The number of articles on nanobiosensors and SARS-CoV-2 exceeds the amount of nanobiosensor research on detecting previous infectious diseases, from influenza to SARS-CoV and MERS-CoV. This unprecedented publishing pace also implies the significance of SARS-CoV-2 and the present pandemic. In this review, 158 studies reporting nanobiosensors for detecting SARS-CoV-2 antigens are collected to discuss the current challenges of nanobiosensors using the criteria of point-of-care (POC) diagnostics along with COVID-specific issues. These advances and lessons during the pandemic pave the way for preparing for the post-COVID era and potential upcoming infectious diseases.</p><h3>Graphical Abstract</h3>\u0000<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"11 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2024-01-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://nanoconvergencejournal.springeropen.com/counter/pdf/10.1186/s40580-023-00410-5","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139416054","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Rapid assays of SARS-CoV-2 virus and noble biosensors by nanomaterials 用纳米材料快速检测 SARS-CoV-2 病毒和贵族生物传感器。
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2024-01-08 DOI: 10.1186/s40580-023-00408-z
Yang Liu, Yilong Li, Yuteng Hang, Lei Wang, Jinghan Wang, Ning Bao, Youngeun Kim, Ho Won Jang
{"title":"Rapid assays of SARS-CoV-2 virus and noble biosensors by nanomaterials","authors":"Yang Liu,&nbsp;Yilong Li,&nbsp;Yuteng Hang,&nbsp;Lei Wang,&nbsp;Jinghan Wang,&nbsp;Ning Bao,&nbsp;Youngeun Kim,&nbsp;Ho Won Jang","doi":"10.1186/s40580-023-00408-z","DOIUrl":"10.1186/s40580-023-00408-z","url":null,"abstract":"<div><p>The COVID-19 outbreak caused by SARS-CoV-2 in late 2019 has spread rapidly across the world to form a global epidemic of respiratory infectious diseases. Increased investigations on diagnostic tools are currently implemented to assist rapid identification of the virus because mass and rapid diagnosis might be the best way to prevent the outbreak of the virus. This critical review discusses the detection principles, fabrication techniques, and applications on the rapid detection of SARS-CoV-2 with three categories: rapid nuclear acid augmentation test, rapid immunoassay test and biosensors. Special efforts were put on enhancement of nanomaterials on biosensors for rapid, sensitive, and low-cost diagnostics of SARS-CoV-2 virus. Future developments are suggested regarding potential candidates in hospitals, clinics and laboratories for control and prevention of large-scale epidemic.</p><h3>Graphical Abstract</h3>\u0000<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"11 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2024-01-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://nanoconvergencejournal.springeropen.com/counter/pdf/10.1186/s40580-023-00408-z","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139376989","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Upconverting-photon quenching-mediated perforation influx as an intracellular delivery method using posAuNP@UCNPs nanocomposites for osteoarthritis treatment 利用posAuNP@UCNPs纳米复合材料的上转换-光子淬灭介导的穿孔流入作为细胞内给药方法治疗骨关节炎
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2024-01-03 DOI: 10.1186/s40580-023-00409-y
Hye Jin Kim, Hui Bang Cho, Hye-Ryoung Kim, Sujeong Lee, Ji-in Park, Keun-Hong Park
{"title":"Upconverting-photon quenching-mediated perforation influx as an intracellular delivery method using posAuNP@UCNPs nanocomposites for osteoarthritis treatment","authors":"Hye Jin Kim,&nbsp;Hui Bang Cho,&nbsp;Hye-Ryoung Kim,&nbsp;Sujeong Lee,&nbsp;Ji-in Park,&nbsp;Keun-Hong Park","doi":"10.1186/s40580-023-00409-y","DOIUrl":"10.1186/s40580-023-00409-y","url":null,"abstract":"<div><p>Photoporation techniques based on plasmonic nanoparticles such as gold nanoparticles have been extensively studied for the intracellular delivery of substances via cell membrane disruption. However, the clinical application of AuNP is challenging due to its absorption in the 500 nm region of the light spectrum. To overcome this challenge, upconversion nanoparticles were employed to stimulate AuNP at NIR wavelengths. posAuNP@UCNPs nanocomposites were produced by coating 30 nm UCNPs on 80 nm AuNPs using DOPA-PEI, which were then irradiated with 980 nm NIR light to facilitate their intracellular delivery. TEM and DLS confirmed that posAuNP and UCNP combine to form nanocomposites. Additionally, multiphysics simulation was used to analyze the distribution of the posAuNP electric field based on morphological differences that change as the UCNP ratio increases. Next, effective LED irradiation conditions were established by applying upconverting-photon quenching-mediated perforation influx to C28/I2 cells as suspensions or spheroids. posAuNP@UCNP nanocomposites were confirmed to be effective for the delivery of baricitinib as a treatment for osteoarthritis in a three-dimensional osteoarthritis model. Finally, chondrocyte differentiation was induced through intracellular delivery of baricitinib using posAuNP@UCNPs. The findings suggest that posAuNP@UCNPs have great potential as a tool for non-invasive drug delivery via UCPPin.</p><h3>Graphical Abstract</h3>\u0000<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"11 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2024-01-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://nanoconvergencejournal.springeropen.com/counter/pdf/10.1186/s40580-023-00409-y","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139082742","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nanoscale inhomogeneity and the evolution of correlation strength in FeSe(_{1-x})S(_x) FeSe[式中:见正文]S[式中:见正文]中的纳米级不均匀性和相关强度的演变。
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2023-12-22 DOI: 10.1186/s40580-023-00405-2
Yu Liu, Aifeng Wang, Qianheng Du, Lijun Wu, Yimei Zhu, Cedomir Petrovic
{"title":"Nanoscale inhomogeneity and the evolution of correlation strength in FeSe(_{1-x})S(_x)","authors":"Yu Liu,&nbsp;Aifeng Wang,&nbsp;Qianheng Du,&nbsp;Lijun Wu,&nbsp;Yimei Zhu,&nbsp;Cedomir Petrovic","doi":"10.1186/s40580-023-00405-2","DOIUrl":"10.1186/s40580-023-00405-2","url":null,"abstract":"<div><p>We report a comprehensive study of the nanoscale inhomogeneity and disorder on the thermoelectric properties of FeSe<span>(_{1-x})</span>S<span>(_x)</span> (<span>(0 le x le 1)</span>) single crystals and the evolution of correlation strength with S substitution. A hump-like feature in temperature-dependent thermpower is enhanced for <i>x</i> = 0.12 and 0.14 in the nematic region with increasing in orbital-selective electronic correlations, which is strongly suppressed across the nematic critical point and for higher S content. Nanoscale Se/S atom disorder in the tetrahedral surroundings of Fe atoms is confirmed by scanning transmission electron microscopy measurements, providing an insight into the nanostructural details and the evolution of correlation strength in FeSe<span>(_{1-x})</span>S<span>(_x)</span>.</p></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"10 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2023-12-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10746694/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138827607","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Filament-free memristors for computing 用于计算的无灯丝忆阻器
IF 11.7 2区 材料科学
Nano Convergence Pub Date : 2023-12-19 DOI: 10.1186/s40580-023-00407-0
Sanghyeon Choi, Taehwan Moon, Gunuk Wang, J. Joshua Yang
{"title":"Filament-free memristors for computing","authors":"Sanghyeon Choi,&nbsp;Taehwan Moon,&nbsp;Gunuk Wang,&nbsp;J. Joshua Yang","doi":"10.1186/s40580-023-00407-0","DOIUrl":"10.1186/s40580-023-00407-0","url":null,"abstract":"<div><p>Memristors have attracted increasing attention due to their tremendous potential to accelerate data-centric computing systems. The dynamic reconfiguration of memristive devices in response to external electrical stimuli can provide highly desirable novel functionalities for computing applications when compared with conventional complementary-metal–oxide–semiconductor (CMOS)-based devices. Those most intensively studied and extensively reviewed memristors in the literature so far have been filamentary type memristors, which typically exhibit a relatively large variability from device to device and from switching cycle to cycle. On the other hand, filament-free switching memristors have shown a better uniformity and attractive dynamical properties, which can enable a variety of new computing paradigms but have rarely been reviewed. In this article, a wide range of filament-free switching memristors and their corresponding computing applications are reviewed. Various junction structures, switching properties, and switching principles of filament-free memristors are surveyed and discussed. Furthermore, we introduce recent advances in different computing schemes and their demonstrations based on non-filamentary memristors. This Review aims to present valuable insights and guidelines regarding the key computational primitives and implementations enabled by these filament-free switching memristors.</p></div>","PeriodicalId":712,"journal":{"name":"Nano Convergence","volume":"10 1","pages":""},"PeriodicalIF":11.7,"publicationDate":"2023-12-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://nanoconvergencejournal.springeropen.com/counter/pdf/10.1186/s40580-023-00407-0","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138739644","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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