Ultrasonics Sonochemistry最新文献

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Enhancing the efficacy of sonodynamic therapy through modulation of autophagy 通过调节自噬增强声动力治疗的疗效
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-25 DOI: 10.1016/j.ultsonch.2025.107527
Meng-Ying Wang , Xiang-Nan Deng , Hao Dong , Xiao-Ying Feng , Fu-Rong Zhu , Dan Yin , Chen Hong , Zhi-Yuan Chen , Ling Wang , Xiao-Ming Zhu
{"title":"Enhancing the efficacy of sonodynamic therapy through modulation of autophagy","authors":"Meng-Ying Wang ,&nbsp;Xiang-Nan Deng ,&nbsp;Hao Dong ,&nbsp;Xiao-Ying Feng ,&nbsp;Fu-Rong Zhu ,&nbsp;Dan Yin ,&nbsp;Chen Hong ,&nbsp;Zhi-Yuan Chen ,&nbsp;Ling Wang ,&nbsp;Xiao-Ming Zhu","doi":"10.1016/j.ultsonch.2025.107527","DOIUrl":"10.1016/j.ultsonch.2025.107527","url":null,"abstract":"<div><div>Sonodynamic therapy (SDT), a noninvasive treatment modality that combines low intensity ultrasound with sonosensitizers, has shown significant potential in the treatment of cancer and metabolic diseases. However, SDT induced autophagy plays a dual role in disease progression, as it can promote either cell survival or cell death, and its effects are highly dependent on cell type and pathological context. This complexity underscores the urgent need for regulation of autophagy to optimize the therapeutic efficacy of SDT. Therefore, this review summarizes emerging regulatory strategies aimed at enhancing SDT efficacy through the induction or inhibition of autophagy. These encompass pharmacological approaches utilizing classic autophagy inhibitors/inducers, as well as nanomaterial-based strategies involving the design of nanocarriers or smart nano-sonosensitizers endowed with capabilities for targeted delivery and stimuli-responsive release. This review aims to provide a comprehensive theoretical framework for understanding the dual roles of autophagy in SDT and for achieving its precise and efficient regulation, thereby offering valuable insights for the development of more effective SDT based therapeutic strategies.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"121 ","pages":"Article 107527"},"PeriodicalIF":9.7,"publicationDate":"2025-08-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144912467","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Programmable ultrasonic modulation of viscoelasticity in polymer-based elastomers: Experiments and constitutive modeling 聚合物基弹性体粘弹性的可编程超声调制:实验和本构建模
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-24 DOI: 10.1016/j.ultsonch.2025.107517
Ying Geng , Guoyan Sun , Sheng Wang , Qingliang Zhao
{"title":"Programmable ultrasonic modulation of viscoelasticity in polymer-based elastomers: Experiments and constitutive modeling","authors":"Ying Geng ,&nbsp;Guoyan Sun ,&nbsp;Sheng Wang ,&nbsp;Qingliang Zhao","doi":"10.1016/j.ultsonch.2025.107517","DOIUrl":"10.1016/j.ultsonch.2025.107517","url":null,"abstract":"<div><div>One of the central challenges in soft matter mechanics is to achieve reversible and programmable modulation of viscoelasticity in polymer-based elastomers at small strains, which is crucial for precision engineering and advanced functional devices. Conventional approaches are constrained by irreversibility and lack of dynamic control. In this study, it is demonstrated that ultrasonic vibration (19–22 kHz) enables dynamic, reversible, and tunable modulation of the mechanical response in such materials. Uniaxial compression experiments combined with constitutive and inverse modeling reveal a reversible transition from viscoelastic, dissipative behavior to an elastic-dominated, stable state. The standard linear solid (SLS) model links macroscopic mechanical changes to molecular-level dynamics, such as chain alignment and mobility. Experimentally, ultrasonic vibration suppresses viscoelastic relaxation and energy dissipation, induces negative hysteresis, and enables tunable, reversible hardening, all strongly dependent on vibration frequency and power. Quantitatively, a typical 20% increase in the instantaneous elastic modulus and over 80% reduction in the delayed elastic modulus and viscosity are achieved under ultrasonic vibration. These results clarify the mechanism by which ultrasonic vibration regulates viscoelasticity and provide practical guidance for designing adaptive polymer systems in applications such as ultrasonic-assisted polishing, soft robotics, and flexible electronics.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"121 ","pages":"Article 107517"},"PeriodicalIF":9.7,"publicationDate":"2025-08-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144912469","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Sonochemical oxidation activity in 20-kHz probe systems: The effects of vessel shape, vessel wall thickness, and probe position 20 khz探针系统中的声化学氧化活性:血管形状、血管壁厚度和探针位置的影响
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-23 DOI: 10.1016/j.ultsonch.2025.107519
Chaewoon Hwang , Iseul Na , Younggyu Son
{"title":"Sonochemical oxidation activity in 20-kHz probe systems: The effects of vessel shape, vessel wall thickness, and probe position","authors":"Chaewoon Hwang ,&nbsp;Iseul Na ,&nbsp;Younggyu Son","doi":"10.1016/j.ultsonch.2025.107519","DOIUrl":"10.1016/j.ultsonch.2025.107519","url":null,"abstract":"<div><div>As a follow-up to our previous studies aimed at optimizing the use of the 20 kHz probe system in chemical and environmental engineering processes, the effects of vessel shape, vessel wall thickness, and probe position on sonochemical oxidation activity in circular and rectangular acrylic vessels were investigated. Electrical and calorimetric powers were obtained, and the sonochemical oxidation activity was quantified using KI dosimetry (pseudo-zero-order reaction kinetics) under 42 geometric conditions. All the geometric conditions of vessel shape, wall thickness, and probe position significantly affected the magnitudes and trends of the sonochemical activity. The average power conversion efficiencies from electrical to calorimetric power were 47.9 ± 3.0 % and 50.3 ± 6.1 % for circular and rectangular vessels, respectively. Overall, much higher activity was obtained when the probe was placed close to the bottom of the circular and rectangular vessels. Average volume-modified zero-order reaction rate constants were 0.20 ± 0.09 and 0.29 ± 0.08 μmol/min for the circular vessels with wall thicknesses of 5 and 10 mm and rectangular vessels with wall thicknesses of 5, 10, 15, and 20 mm. However, the probe positions for the highest activity moved toward to the liquid surface as the thickness increased in the rectangular vessels. The variation in the sonochemical activity was well visualized in the sonochemiluminescence (SCL) image (side and bottom views) analysis, and a higher intensity was observed in the SCL images when the probe was positioned adjacent to the vessel bottom. Thus, the total intensities of the SCL matched well with those of the sonochemical activity using KI dosimetry. Significantly different trends were observed in the BPA degradation tests, which may be attributed to the difference between the zero-order and first-order reactions.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"121 ","pages":"Article 107519"},"PeriodicalIF":9.7,"publicationDate":"2025-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144896389","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Grain refining in copper foil induced by ultrasonic field during the electrodeposition process 电沉积过程中超声场对铜箔晶粒细化的影响
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-22 DOI: 10.1016/j.ultsonch.2025.107526
Chengwen Wu , Xiaolong Ren , Lin Xie , Wenhua Wu , Zhiwei Liu , Wei Zhai , Jianyuan Wang
{"title":"Grain refining in copper foil induced by ultrasonic field during the electrodeposition process","authors":"Chengwen Wu ,&nbsp;Xiaolong Ren ,&nbsp;Lin Xie ,&nbsp;Wenhua Wu ,&nbsp;Zhiwei Liu ,&nbsp;Wei Zhai ,&nbsp;Jianyuan Wang","doi":"10.1016/j.ultsonch.2025.107526","DOIUrl":"10.1016/j.ultsonch.2025.107526","url":null,"abstract":"<div><div>Electrodeposition is a key technique for fabricating ultra-thin copper foils, where grain refinement plays a critical role in determining their mechanical performance. In recent years, the unique cavitation effects associated with ultrasonic fields have demonstrated significant potential in modulating metal deposition. This study quantitatively investigates the influence of ultrasonic amplitude on the nucleation behavior of copper electrodeposited on a Co–Ni alloy substrate. At amplitudes of 18–24 μm, ultrasound enhances ion transport and activation via cavitation and agitation, thereby accelerating nucleation. As the amplitude increases, high amplitudes (30–42 μm) intensify acoustic streaming and cavitation bubble clustering, inducing strong fluid perturbations at the cathode interface. That brings local current pulsation and intermittent deposition. These dynamic effects promote finer grain structures and more uniform grain distribution. Notably, at 42 μm amplitude, the grain size is reduced by nearly an order of magnitude. These findings provide quantitative insights into ultrasonic regulation, offering guidance for high-efficiency, uniform copper foil deposition.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"121 ","pages":"Article 107526"},"PeriodicalIF":9.7,"publicationDate":"2025-08-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144908833","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A review of microcavitation bubbles dynamics in biological systems and their mechanical applications 生物系统中的微空化气泡动力学及其力学应用综述
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-21 DOI: 10.1016/j.ultsonch.2025.107521
Ahmed K. Abu-Nab , Adel M. Morad , Ehab S. Selima , Tetsuya Kanagawa , Ali F. Abu-Bakr
{"title":"A review of microcavitation bubbles dynamics in biological systems and their mechanical applications","authors":"Ahmed K. Abu-Nab ,&nbsp;Adel M. Morad ,&nbsp;Ehab S. Selima ,&nbsp;Tetsuya Kanagawa ,&nbsp;Ali F. Abu-Bakr","doi":"10.1016/j.ultsonch.2025.107521","DOIUrl":"10.1016/j.ultsonch.2025.107521","url":null,"abstract":"<div><div>In this review, the theoretical studies are presented for the microcavitation bubble dynamics problems, which mainly depend on the microcavitation models, such as the Rayleigh-Plesset model, the Church model, the diffusion-concentration model, and the Keller-Miksis model in biological systems. The various solutions to these models, which were formulated based on basic mathematical and physical concepts, are schematically presented. Moreover, these models are employed in many different physical problems, such as the treatment of cancerous tumours via a technique known as histotripsy and lipid shells of membrane cells, that employ focused ultrasonic therapy as a non-invasive tissue ablation method. Using the mechanical action of bubble clouds, historic triumph destroys tissue differently than the thermally ablative techniques of therapeutic ultrasonography. Also, lipid-coated microbubbles are used in different therapeutic applications. Besides, the effect of different physical coefficients on Newtonian, non-Newtonian fluids, and viscoelastic media studied by numerical and analytical methods with external fields is examined for incompressible fluid states, and the Navier-Stokes hydrodynamic equations are investigated. It is anticipated that this work will serve as a valuable guide for the use of microcavitations in many medicinal applications, such as histotripsy, lipid shells in membrane cells and diver’s tissue.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"121 ","pages":"Article 107521"},"PeriodicalIF":9.7,"publicationDate":"2025-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144904649","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ultrasonic pretreatment assisted enzymolysis for preparation of low molecular weight osteogenic collagen peptides: Kinetics, thermodynamics, and osteogenic activity 超声预处理辅助酶解制备低分子量成骨胶原肽:动力学,热力学和成骨活性
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-21 DOI: 10.1016/j.ultsonch.2025.107525
Liwei Qi , Lishuang Mao , Xiaojie Qin , Yujie Guo , Chunhui Zhang
{"title":"Ultrasonic pretreatment assisted enzymolysis for preparation of low molecular weight osteogenic collagen peptides: Kinetics, thermodynamics, and osteogenic activity","authors":"Liwei Qi ,&nbsp;Lishuang Mao ,&nbsp;Xiaojie Qin ,&nbsp;Yujie Guo ,&nbsp;Chunhui Zhang","doi":"10.1016/j.ultsonch.2025.107525","DOIUrl":"10.1016/j.ultsonch.2025.107525","url":null,"abstract":"<div><div>To prepare low molecular weight (LMW) osteogenic collagen peptides, ultrasonic (US) pretreatment was used to enhance the enzymolysis efficiency of bovine bone collagen (BBC). Therefore, this study analyzed the enzymolysis kinetics, thermodynamics, and osteogenic activity. The kinetic results indicated that US pretreatment increased the association constant (K<sub>a</sub>) by 19.30 % and decreased the Michaelis constant (K<sub>m</sub>) by 11.14 %. The thermodynamic results indicated that US pretreatment reduced the activation energy (<em>E</em><sub>a</sub>), enthalpy (Δ<em>H</em>), and entropy (Δ<em>S</em>) by 25.73 %, 27.69 %, and 15.39 %, respectively, and Gibbs free energy (Δ<em>G</em>) was reduced by 1.86 (298 K), 1.51 (308 K), 1.18 (318 K), and 0.88 % (328 K), and the reaction rate constant (k) was increased by 89.87 (298 K), 71.54 (308 K), 39.53 (318 K), and 38.44 % (328 K). Structural characterization demonstrated that the shear force, microflow, turbulent force, and cavitation effects produced by US disrupted the compact spatial structure of BBC. Additionally, it resulted in a more uniform distribution of BBC with smaller particles in the solution, that exposed more enzyme cleavage sites. The molecular weight distribution demonstrated that the proportion of collagen peptides less than 1000 Da in UP-BBCP was 83.67 %, which was 14.21 % higher than that (69.46 %) in BBCP. MC3T3-E1 cell experiments demonstrated that UP-BBCP exhibited stronger pro-osteogenic activity than that of BBCP, including proliferation activity (increased by 27.26 %) and calcium deposition level (increased by 35.05 %). In conclusion, US pretreatment may be a potential strategy to enhance enzymolysis efficiency for preparing LMW osteogenic collagen peptides.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"120 ","pages":"Article 107525"},"PeriodicalIF":9.7,"publicationDate":"2025-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144889607","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ultrasound-responsive diagnostic and therapeutic micro-/nanoplatforms for biomedical applications and clinical translation 用于生物医学应用和临床翻译的超声响应诊断和治疗微/纳米平台
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-21 DOI: 10.1016/j.ultsonch.2025.107524
Wei Guo , Siying Gao , Yiran Hao , Zijing Li , Haoyuan Hu , Huijun Wu, Changhao Hu, Xueqin Cheng, Weiwen Zhao, Yuxuan Kong, Hong Jiang, Songyun Wang
{"title":"Ultrasound-responsive diagnostic and therapeutic micro-/nanoplatforms for biomedical applications and clinical translation","authors":"Wei Guo ,&nbsp;Siying Gao ,&nbsp;Yiran Hao ,&nbsp;Zijing Li ,&nbsp;Haoyuan Hu ,&nbsp;Huijun Wu,&nbsp;Changhao Hu,&nbsp;Xueqin Cheng,&nbsp;Weiwen Zhao,&nbsp;Yuxuan Kong,&nbsp;Hong Jiang,&nbsp;Songyun Wang","doi":"10.1016/j.ultsonch.2025.107524","DOIUrl":"10.1016/j.ultsonch.2025.107524","url":null,"abstract":"<div><div>Ultrasound is a widely utilized diagnostic and therapeutic tool in biomedicine due to its non-invasiveness, biocompatibility, cost-effectiveness, and high tissue penetration depth. With the continuous development of materials science and nanomedicine, ultrasound-based diagnosis and treatment have achieved significant advancements. By combining ultrasound as a trigger with responsive biomaterials, platforms with diagnostic and therapeutic performance for specific diseases could be established, offering a promising approach for the development of precise medicine. Through various synthesis and material modification techniques, diverse biomaterials are endowed with diagnostic or therapeutic properties. While ensuring their biocompatibility and biosafety, their tissue targeting specificity is enhanced, thereby minimizing adverse drug reactions. In this review, we introduce the biological effects of ultrasound and the classification of ultrasound-responsive micro-/nanoplatforms, and systematically describe the relevant applications in the diagnostic imaging and treatment of tumors, cardiovascular diseases, infectious diseases, neurological diseases, and metabolic diseases. Finally, we summarized relevant clinical trials in this field and proposed challenges and solutions in the process of clinical translation to better promote the widespread clinical application of this technology and provide novel avenues for the development of clinical diagnostic and therapeutic technologies.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"121 ","pages":"Article 107524"},"PeriodicalIF":9.7,"publicationDate":"2025-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144933272","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Sonochemistry in light of third reactivity paradigm 第三反应性范式下的声化学
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-21 DOI: 10.1016/j.ultsonch.2025.107523
Sergey I. Nikitenko
{"title":"Sonochemistry in light of third reactivity paradigm","authors":"Sergey I. Nikitenko","doi":"10.1016/j.ultsonch.2025.107523","DOIUrl":"10.1016/j.ultsonch.2025.107523","url":null,"abstract":"<div><div>Large number of chemical reactions can be described rigorously using classical thermodynamics and classical kinetics. However, there are an increasing number of examples of chemical reactions that deviate from “classical” behavior. Describing them requires considering quantum effects. The purpose of this review is to emphasize the importance of such “non-classical” reactions in sonochemistry. Quantum effects in sonochemistry are a direct consequence of the formation of nonequilibrium plasma inside collapsing bubbles. Spectroscopic studies of multibubble sonoluminescence revealed that intrabubble processes cannot be described by a single gas temperature. Rather, vibrational excitation and ionization must also be considered. Most clearly, quantum effects in sonochemistry, like those in “classical” chemistry, appeared for kinetic isotope effects, KIE. The anomalous H/D KIE during water sonolysis in the presence of noble gases can be understood in terms of electron quantum tunneling during the heterolytic splitting of a water molecule. In addition, the inverse <sup>13</sup>C/<sup>12</sup>C KIE observed during water sonolysis in the presence of CO indicated a similarity with a non-equilibrium plasma generated by CO excitation in a gas phase. This KIE originated from the quantum vibration–vibration pumping mechanism. In the concluding part of the review, some perspective research directions are discussed.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"121 ","pages":"Article 107523"},"PeriodicalIF":9.7,"publicationDate":"2025-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144908910","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ultrasonication-driven optimization of cricket protein nanoemulsions: influence of pH and rheological stabilizers 超声驱动蟋蟀蛋白纳米乳的优化:pH和流变稳定剂的影响
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-19 DOI: 10.1016/j.ultsonch.2025.107522
Rosa María Sánchez-García , Azahara Rodríguez-Luna , Jenifer Santos , Luis A. Trujillo-Cayado
{"title":"Ultrasonication-driven optimization of cricket protein nanoemulsions: influence of pH and rheological stabilizers","authors":"Rosa María Sánchez-García ,&nbsp;Azahara Rodríguez-Luna ,&nbsp;Jenifer Santos ,&nbsp;Luis A. Trujillo-Cayado","doi":"10.1016/j.ultsonch.2025.107522","DOIUrl":"10.1016/j.ultsonch.2025.107522","url":null,"abstract":"<div><div>This study investigates the formulation of sustainable nanoemulsions using cricket protein as a natural emulsifier and linseed oil as the dispersed phase, emphasizing the effects of pH, ultrasonication, and rheological modifiers on emulsion stability and structure. Surface and interfacial tension analyses revealed significant reductions with increasing protein concentration, stabilizing at ≥1 g/L. At alkaline pH (≥12), interfacial tension became unmeasurable due to complete phase merging, attributed to enhanced protein solubility and surface activity. Droplet size distribution exhibited bimodal patterns across all pH levels, with the smallest Sauter diameter (0.54 μm) and optimal span (1.91) achieved at pH 12.5.</div><div>Ultrasonication parameters (amplitude and sonication time) were optimized using response surface methodology. The smallest droplet size (0.365 μm) was predicted at 63 % amplitude and 9.6 min of sonication. However, higher energy inputs also increased polydispersity, likely due to droplet recoalescence in the absence of sufficient emulsifier. To enhance stability, guar gum (GG) and advanced performance xanthan gum (APXG) were tested. APXG, particularly at ≥0.25 wt%, significantly improved viscoelasticity (G′ &gt; G″) and increased consistency (K = 9.87 Pa·s<sup>n</sup> at 0.5 wt%), forming gel-like structures and reducing the Turbiscan Stability Index (TSI) over a 21-day period.</div><div>These results underscore the critical roles of pH, ultrasonic processing, and rheological modification in designing robust nanoemulsions. The integration of cricket protein and APXG under optimized conditions offers a promising platform for stable, eco-friendly emulsions in functional food and nutraceutical applications.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"120 ","pages":"Article 107522"},"PeriodicalIF":9.7,"publicationDate":"2025-08-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144889668","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hydrogen production via water ultrasonication: A review 水超声制氢技术研究进展
IF 9.7 1区 化学
Ultrasonics Sonochemistry Pub Date : 2025-08-18 DOI: 10.1016/j.ultsonch.2025.107515
Slimane Merouani , Aissa Dehane , Oualid Hamdaoui
{"title":"Hydrogen production via water ultrasonication: A review","authors":"Slimane Merouani ,&nbsp;Aissa Dehane ,&nbsp;Oualid Hamdaoui","doi":"10.1016/j.ultsonch.2025.107515","DOIUrl":"10.1016/j.ultsonch.2025.107515","url":null,"abstract":"<div><div>This review thoroughly examines the potential of water ultrasonication (US) for producing hydrogen. First, it discusses ultrasonication reactor designs and techniques for measuring ultrasonication power and optimizing energy. Then, it explores the results of hydrogen production via ultrasonication experiments, focusing on the impact of processing factors such as ultrasonication frequency, acoustic intensity, dissolved gases, pH, temperature, and static pressure on the process. Additionally, it examines advanced ultrasonication techniques, such as US/photolysis, US/catalysis, and US/photocatalysis, emphasizing how these techniques could increase hydrogen production. Lastly, to progress the efficacy and scalability of hydrogen generation through ultrasonication, the review identifies existing challenges, proposes solutions, and suggests areas for future research.</div></div>","PeriodicalId":442,"journal":{"name":"Ultrasonics Sonochemistry","volume":"120 ","pages":"Article 107515"},"PeriodicalIF":9.7,"publicationDate":"2025-08-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144866369","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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