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Front Cover: Steric hindrance induced low exciton binding energy enables low-driving-force organic solar cells 封面：立体阻碍诱导的低激子结合能可实现低驱动力有机太阳能电池
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-10-20 DOI: 10.1002/agt2.681
Tianyu Hu, Xufan Zheng, Ting Wang, Aziz Saparbaev, Bowen Gao, Jingnan Wu, Jingyi Xiong, Ming Wan, Tingting Cong, Yuda Li, Ergang Wang, Xunchang Wang, Renqiang Yang
{"title":"Front Cover: Steric hindrance induced low exciton binding energy enables low-driving-force organic solar cells","authors":"Tianyu Hu,&nbsp;Xufan Zheng,&nbsp;Ting Wang,&nbsp;Aziz Saparbaev,&nbsp;Bowen Gao,&nbsp;Jingnan Wu,&nbsp;Jingyi Xiong,&nbsp;Ming Wan,&nbsp;Tingting Cong,&nbsp;Yuda Li,&nbsp;Ergang Wang,&nbsp;Xunchang Wang,&nbsp;Renqiang Yang","doi":"10.1002/agt2.681","DOIUrl":"https://doi.org/10.1002/agt2.681","url":null,"abstract":"<p>This article focuses on the regulation of steric hindrance effect on the exciton binding energy of Y-series non-fullerene acceptors. The introduction of bulk cyclohexyl group in the side chains modulates inter- and intramolecular interactions of acceptors, thereby influencing the exciton binding energy and ultimately enhancing the energy conversion efficiency of organic solar cells (e632).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-10-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.681","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142540836","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Back Cover: Lysine aggregates-based nanostructured antimicrobial peptides for cariogenic biofilm microenvironment-activated caries treatment 封底：基于赖氨酸聚合体的纳米结构抗菌肽用于致龋生物膜微环境激活型龋病治疗
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-10-20 DOI: 10.1002/agt2.684
Siyuan Li, Feng Wang, Yang Chen, Wanrui Shi, Dashuai Liu, Mingyang Lv, Bin Zhao, Yi Liu, Hao Zhang
{"title":"Back Cover: Lysine aggregates-based nanostructured antimicrobial peptides for cariogenic biofilm microenvironment-activated caries treatment","authors":"Siyuan Li,&nbsp;Feng Wang,&nbsp;Yang Chen,&nbsp;Wanrui Shi,&nbsp;Dashuai Liu,&nbsp;Mingyang Lv,&nbsp;Bin Zhao,&nbsp;Yi Liu,&nbsp;Hao Zhang","doi":"10.1002/agt2.684","DOIUrl":"https://doi.org/10.1002/agt2.684","url":null,"abstract":"<p>Aggregated lysine mimics antimicrobial peptides (AMPs) by disrupting bacterial membranes, interfering with metabolism, and inhibiting protein synthesis. With Fe<sup>3+</sup> hydrolysis, lysine coordination, and ultrasmall Au nanoparticle deposition, FeOOH@Fe-Lysine@Au shows AMP-like antibacterial activity and reactive oxygen species generation, providing an effective approach for cariogenic biofilm microenvironment-activated caries treatment (e578).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-10-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.684","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142540837","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inside Front Cover: Stimuli-responsive photoluminescent copper(I) halides for scintillation, anticounterfeiting, and light-emitting diode applications 封面内页：用于闪烁、防伪和发光二极管的刺激响应型光致发光铜（I）卤化物
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-10-20 DOI: 10.1002/agt2.682
Dilruba A. Popy, Yashpal Singh, Yauhen Tratsiak, Abby M. Cardoza, John M. Lane, Luis Stand, Mariya Zhuravleva, Neeraj Rai, Bayram Saparov
{"title":"Inside Front Cover: Stimuli-responsive photoluminescent copper(I) halides for scintillation, anticounterfeiting, and light-emitting diode applications","authors":"Dilruba A. Popy,&nbsp;Yashpal Singh,&nbsp;Yauhen Tratsiak,&nbsp;Abby M. Cardoza,&nbsp;John M. Lane,&nbsp;Luis Stand,&nbsp;Mariya Zhuravleva,&nbsp;Neeraj Rai,&nbsp;Bayram Saparov","doi":"10.1002/agt2.682","DOIUrl":"https://doi.org/10.1002/agt2.682","url":null,"abstract":"<p>Near unity photoluminescence efficiency has been achieved in green emitting (TEP)<sub>2</sub>Cu<sub>2</sub>Br<sub>4</sub> and orange emitting (TEP)<sub>2</sub>Cu<sub>4</sub>Br<sub>6</sub>. In both cases, emission originates from self-trapped excitons localized on the copper(I) halide structural units. The sensitivity of these compounds to the external stimuli coupled with their ultrabright emission allows their consideration for applications such as solid-state lighting, scintillation, sensing, information storage, and anticounterfeiting (e602).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-10-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.682","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142540834","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inside Back Cover: Supramolecular self-assembled nanoparticles for targeted therapy of myocardial infarction by enhancing cardiomyocyte mitophagy 封底内页超分子自组装纳米粒子通过增强心肌细胞有丝分裂靶向治疗心肌梗死
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-10-20 DOI: 10.1002/agt2.683
Yang Jiao, Haimang Wang, Xiechuan Weng, Jihang Wang, Ying Li, Jian Shen, Weiwei Zhao, Qing Xi, Hongyu Zhang, Zhenhong Fu
{"title":"Inside Back Cover: Supramolecular self-assembled nanoparticles for targeted therapy of myocardial infarction by enhancing cardiomyocyte mitophagy","authors":"Yang Jiao,&nbsp;Haimang Wang,&nbsp;Xiechuan Weng,&nbsp;Jihang Wang,&nbsp;Ying Li,&nbsp;Jian Shen,&nbsp;Weiwei Zhao,&nbsp;Qing Xi,&nbsp;Hongyu Zhang,&nbsp;Zhenhong Fu","doi":"10.1002/agt2.683","DOIUrl":"https://doi.org/10.1002/agt2.683","url":null,"abstract":"<p>In this study, supramolecular self-assembled nanoparticles were developed with multi-functional properties of macrophage escape, cardiac targeting, and drug release for the treatment of myocardial infarction. The nanoparticles reduced cardiomyocyte apoptosis, alleviated myocardial interstitial fibrosis, and enhanced cardiac function based on the mechanism of the enhancement in mitophagy and alleviation in mitochondrial damage (e563).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-10-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.683","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142540835","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Back Cover: Special RCA based sensitive point-of-care detection of HPV mRNA for cervical cancer screening 封底：基于特殊 RCA 的宫颈癌筛查 HPV mRNA 床旁灵敏检测技术
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-08-20 DOI: 10.1002/agt2.656
Yi Long, Shurui Tao, Dongni Shi, Xingyu Jiang, Tian Yu, Yingxi Long, Libing Song, Guozhen Liu
{"title":"Back Cover: Special RCA based sensitive point-of-care detection of HPV mRNA for cervical cancer screening","authors":"Yi Long,&nbsp;Shurui Tao,&nbsp;Dongni Shi,&nbsp;Xingyu Jiang,&nbsp;Tian Yu,&nbsp;Yingxi Long,&nbsp;Libing Song,&nbsp;Guozhen Liu","doi":"10.1002/agt2.656","DOIUrl":"https://doi.org/10.1002/agt2.656","url":null,"abstract":"<p>In the newly developed MSS-RCA technique, a circular template with minimal secondary structure was designed to achieve the higher amplification efficiency compared with conventional RCA technique. The linear structure of the MSS-RCA product provides the highest signal binding efficiency. Integration with a blood glucose meter, MSS-RCA technique was suitable for point-of-care detection of HPV mRNA for cervical cancer screening (e569).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.656","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142013562","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inside Back Cover: Aggregation and aging of nanoparticle–protein complexes at interfaces studied by evanescent-light scattering microscopy 封底内页：用渐变光散射显微镜研究纳米粒子-蛋白质复合物在界面上的聚集和老化现象
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-08-20 DOI: 10.1002/agt2.655
Wei Liu, Yuwei Zhu, Hang Jiang, Lidan Zhou, Yinan Li, Jiahao Wu, Jie Han, Cheng Yang, Jianzhong Jiang, To Ngai
{"title":"Inside Back Cover: Aggregation and aging of nanoparticle–protein complexes at interfaces studied by evanescent-light scattering microscopy","authors":"Wei Liu,&nbsp;Yuwei Zhu,&nbsp;Hang Jiang,&nbsp;Lidan Zhou,&nbsp;Yinan Li,&nbsp;Jiahao Wu,&nbsp;Jie Han,&nbsp;Cheng Yang,&nbsp;Jianzhong Jiang,&nbsp;To Ngai","doi":"10.1002/agt2.655","DOIUrl":"https://doi.org/10.1002/agt2.655","url":null,"abstract":"<p>Aggregation and aging of nanoparticle–protein complexes at interfaces are resolved via an evanescent-light scattering microscopy. Time- and space-resolved measurements by correlation functions show that aging of such soft materials is out-of-equilibrium, stretched and compressed exponential decays can coexist in one aging process. Corona formation, inner stress and inter-connection are key for the aggregation and aging dynamics (e538).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.655","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142013561","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inside Front Cover: Exploring and leveraging aggregation effects on reactive oxygen species generation in photodynamic therapy 封面内页：探索和利用光动力疗法中活性氧生成的聚集效应
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-08-20 DOI: 10.1002/agt2.654
Zeyan Zhuang, Jianqing Li, Pingchuan Shen, Zujin Zhao, Ben Zhong Tang
{"title":"Inside Front Cover: Exploring and leveraging aggregation effects on reactive oxygen species generation in photodynamic therapy","authors":"Zeyan Zhuang,&nbsp;Jianqing Li,&nbsp;Pingchuan Shen,&nbsp;Zujin Zhao,&nbsp;Ben Zhong Tang","doi":"10.1002/agt2.654","DOIUrl":"https://doi.org/10.1002/agt2.654","url":null,"abstract":"<p>This paper focuses on the aggregation effects on the reactive oxygen species generation, highlighting the significant variations among isolated and various nano-aggregated states. It provides a consolidated overview on the fundamental principles, discusses current research methodologies, and reviews present research status concerning the aggregation effects on ROS generation, aiming to drive continuous progress in aggregate-level phototheranostic platforms (e540).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.654","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142013630","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Front Cover: Rhein-based Pickering emulsion for hepatocellular carcinoma: Shaping the metabolic signaling and immunoactivation in transarterial chemoembolization 封面：治疗肝细胞癌的莱茵基皮克林乳剂：塑造经动脉化疗栓塞术中的代谢信号和免疫激活作用
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-08-20 DOI: 10.1002/agt2.653
Xiaoliu Liang, Hui Liu, Hu Chen, Xuqi Peng, Zhenjie Li, Minglei Teng, Yisheng Peng, Jiwei Li, Linyu Ding, Jingsong Mao, Chengchao Chu, Hongwei Cheng, Gang Liu
{"title":"Front Cover: Rhein-based Pickering emulsion for hepatocellular carcinoma: Shaping the metabolic signaling and immunoactivation in transarterial chemoembolization","authors":"Xiaoliu Liang,&nbsp;Hui Liu,&nbsp;Hu Chen,&nbsp;Xuqi Peng,&nbsp;Zhenjie Li,&nbsp;Minglei Teng,&nbsp;Yisheng Peng,&nbsp;Jiwei Li,&nbsp;Linyu Ding,&nbsp;Jingsong Mao,&nbsp;Chengchao Chu,&nbsp;Hongwei Cheng,&nbsp;Gang Liu","doi":"10.1002/agt2.653","DOIUrl":"https://doi.org/10.1002/agt2.653","url":null,"abstract":"<p>This study identifies metabolic reprogramming and immunosuppression as key factors in transarterial chemoembolization (TACE) refractoriness. Rhein is optimized as a glycolytic inhibitor and immunoactivator to enhance tumor response to TACE. An oil-in-water lipiodol emulsion stabilized with Rhein nanogel holds enhanced mechanical stability, ensuring effective embolization, prolonged drug release, and potent anti-tumor immunity, presenting a new approach for TACE (e552).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.653","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142013629","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Photo-induced Bacillus subtilis-spore transformation for bowel disease therapy and therapeutic outcome visualization 光诱导枯草芽孢杆菌孢子转化用于肠道疾病治疗和疗效可视化
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-07-02 DOI: 10.1002/agt2.597
Lin Kong, Wei He, Junyi Gong, Zijie Qiu, Zheng Zhao, Ben Zhong Tang
{"title":"Photo-induced Bacillus subtilis-spore transformation for bowel disease therapy and therapeutic outcome visualization","authors":"Lin Kong,&nbsp;Wei He,&nbsp;Junyi Gong,&nbsp;Zijie Qiu,&nbsp;Zheng Zhao,&nbsp;Ben Zhong Tang","doi":"10.1002/agt2.597","DOIUrl":"10.1002/agt2.597","url":null,"abstract":"<p>Efficient strategies for transforming <i>Bacillus subtilis</i> vegetative cells into spores (BtS transformation) are still limited, although they show promise for the treatment of inflammatory bowel disease (IBD). A novel, simple, and rapid photo-induced BtS transformation mechanism is now presented that utilizes a novel aggregation-induced emission luminogen (AIEgen) photosensitizer, triphenylamine-benzothiadiazole-pyridine-p-tolylboronic acid bromine salt (TBPBB), that generates reactive oxygen species (ROS) when exposed to light. The ROS selectively target and damage the membranes of <i>Bacillus subtilis</i> and trigger their transformation into spores. These spores demonstrate considerable promise for the effective treatment of IBD in a mouse disease model. Furthermore, the fluorescence signal generated by TBPBB can be used to directly visualize the recovery of damaged intestinal tissue. This is a valuable tool for monitoring the healing process and gaining insights into therapeutic efficacy. This study highlights the remarkable practical value of AIEgen-induced BtS transformation for identifying, localizing, and visualizing the therapeutic outcomes of IBD treatments.</p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-07-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.597","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141551768","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Steric hindrance induced low exciton binding energy enables low-driving-force organic solar cells 立体阻碍诱导的低激子结合能可实现低驱动力有机太阳能电池
IF 13.9
Aggregate (Hoboken, N.J.) Pub Date : 2024-07-02 DOI: 10.1002/agt2.632
Tianyu Hu, Xufan Zheng, Ting Wang, Aziz Saparbaev, Bowen Gao, Jingnan Wu, Jingyi Xiong, Ming Wan, Tingting Cong, Yuda Li, Ergang Wang, Xunchang Wang, Renqiang Yang
{"title":"Steric hindrance induced low exciton binding energy enables low-driving-force organic solar cells","authors":"Tianyu Hu,&nbsp;Xufan Zheng,&nbsp;Ting Wang,&nbsp;Aziz Saparbaev,&nbsp;Bowen Gao,&nbsp;Jingnan Wu,&nbsp;Jingyi Xiong,&nbsp;Ming Wan,&nbsp;Tingting Cong,&nbsp;Yuda Li,&nbsp;Ergang Wang,&nbsp;Xunchang Wang,&nbsp;Renqiang Yang","doi":"10.1002/agt2.632","DOIUrl":"10.1002/agt2.632","url":null,"abstract":"<p>Exciton binding energy (<i>E</i><sub>b</sub>) has been regarded as a critical parameter in charge separation during photovoltaic conversion. Minimizing the <i>E</i><sub>b</sub> of the photovoltaic materials can facilitate the exciton dissociation in low-driving force organic solar cells (OSCs) and thus improve the power conversion efficiency (PCE); nevertheless, diminishing the <i>E</i><sub>b</sub> with deliberate design principles remains a significant challenge. Herein, bulky side chain as steric hindrance structure was inserted into Y-series acceptors to minimize the <i>E</i><sub>b</sub> by modulating the intra- and intermolecular interaction. Theoretical and experimental results indicate that steric hindrance-induced optimal intra- and intermolecular interaction can enhance molecular polarizability, promote electronic orbital overlap between molecules, and facilitate delocalized charge transfer pathways, thereby resulting in a low <i>E</i><sub>b</sub>. The conspicuously reduced <i>E</i><sub>b</sub> obtained in Y-ChC5 with pinpoint steric hindrance modulation can minimize the detrimental effects on exciton dissociation in low-driving-force OSCs, achieving a remarkable PCE of 19.1% with over 95% internal quantum efficiency. Our study provides a new molecular design rationale to reduce the <i>E</i><sub>b</sub>.</p>","PeriodicalId":72127,"journal":{"name":"Aggregate (Hoboken, N.J.)","volume":null,"pages":null},"PeriodicalIF":13.9,"publicationDate":"2024-07-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/agt2.632","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141551767","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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