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Single particle trace element analysis of uranium oxide standards with laser-induced breakdown spectroscopy 用激光诱导击穿光谱法分析氧化铀标准品中的单颗粒微量元素
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-29 DOI: 10.1007/s10967-025-09994-0
Gregory Hull, Joanna S. Denton, Jeremy D. Inglis, Matthew E. Sanborn
{"title":"Single particle trace element analysis of uranium oxide standards with laser-induced breakdown spectroscopy","authors":"Gregory Hull,&nbsp;Joanna S. Denton,&nbsp;Jeremy D. Inglis,&nbsp;Matthew E. Sanborn","doi":"10.1007/s10967-025-09994-0","DOIUrl":"10.1007/s10967-025-09994-0","url":null,"abstract":"<div><p>Femtosecond Laser-Induced Breakdown Spectroscopy (LIBS) was used to analyze over 1000 individual particles of uranium oxide trace element standard CRM124. Intra-granular analysis showed elemental concentrations were consistent across different surface locations on each uranium grain. However, inter-granular comparison revealed large heterogeneity between different grains of the same sample. By comparing the distribution of elemental concentrations across the particle populations, we were able to correctly identify a manufacturing process involving wet chemistry, rather than a dry mixing of two powders to give an overall chemical average. This demonstrates the utility of LIBS as a large-scale single particle analysis tool for nuclear forensics.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 3","pages":"2353 - 2367"},"PeriodicalIF":1.5,"publicationDate":"2025-01-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707185","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Assessment of tritium radioactivity and the health risks associated with its consumption in various drinking waters from Bursa, Türkiye 评估来自土耳其布尔萨市的各种饮用水中的氚放射性和与食用氚有关的健康风险
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-29 DOI: 10.1007/s10967-025-10000-w
Serdar Dizman, Kübra Memişoğlu, Ali Erdem Özçelik
{"title":"Assessment of tritium radioactivity and the health risks associated with its consumption in various drinking waters from Bursa, Türkiye","authors":"Serdar Dizman,&nbsp;Kübra Memişoğlu,&nbsp;Ali Erdem Özçelik","doi":"10.1007/s10967-025-10000-w","DOIUrl":"10.1007/s10967-025-10000-w","url":null,"abstract":"<div><p>In this study, tritium levels in some water sources frequently used by the public in the Bursa province were investigated using Liquid Scintillation Counter. The minimum detectable activity concentration (MDA) for the employed method was established at 1.31 Bq/L. The mean tritium concentration for the 21 samples was calculated as 2.05 ± 0.47 Bq/L (17.36 ± 3.98 TU). Additionally, the annual effective dose rates and lifetime cancer risk values associated with the consumption of the studied water samples were calculated. The results show that consumption of these water samples does not pose a health risk to individuals in terms of tritium radioisotope.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 3","pages":"2219 - 2226"},"PeriodicalIF":1.5,"publicationDate":"2025-01-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10967-025-10000-w.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707183","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Elemental identification of sealed cargo based on fast neutron activation analysis and artificial neural network 基于快中子活化分析和人工神经网络的密封货物元素识别
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-29 DOI: 10.1007/s10967-025-09991-3
Hadi Shahabinejad, Davorin Sudac, Karlo Nad, Isabelle Espagnon, Clotilde de Sainte Foy, Bertrand Perot, Cedric Carasco, Alix Sardet, Edwin Friedmann, Jean Philippe Poli, Jessica Delgado, Felix Pino, Sandra Moretto, Christine Mer, Guillaume Sannie, Jasmina Obhodas
{"title":"Elemental identification of sealed cargo based on fast neutron activation analysis and artificial neural network","authors":"Hadi Shahabinejad,&nbsp;Davorin Sudac,&nbsp;Karlo Nad,&nbsp;Isabelle Espagnon,&nbsp;Clotilde de Sainte Foy,&nbsp;Bertrand Perot,&nbsp;Cedric Carasco,&nbsp;Alix Sardet,&nbsp;Edwin Friedmann,&nbsp;Jean Philippe Poli,&nbsp;Jessica Delgado,&nbsp;Felix Pino,&nbsp;Sandra Moretto,&nbsp;Christine Mer,&nbsp;Guillaume Sannie,&nbsp;Jasmina Obhodas","doi":"10.1007/s10967-025-09991-3","DOIUrl":"10.1007/s10967-025-09991-3","url":null,"abstract":"<div><p>Securing global trade requires efficient screening of containers for threat materials. This work demonstrates a novel approach combining fast neutron activation analysis and artificial neural network (ANN) to identify elemental composition of sealed cargo, in particular elements carbon, oxygen, and nitrogen, which are the main components of explosives. This study shows that Rapidly Relocatable Tagged Neutron Inspection System in combination with ANN is a potential promising solution for the inspection of sealed containers, allowing precise identification of elements and detection of potential threats without the need to open the containers.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1157 - 1166"},"PeriodicalIF":1.5,"publicationDate":"2025-01-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481037","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Novel probe with iRGD integrated graphene oxide nanoparticles and labeled with 131I for detection of thyroid papillary carcinoma cells 新型iRGD集成氧化石墨烯纳米颗粒并标记131I的探针用于检测甲状腺乳头状癌细胞
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-29 DOI: 10.1007/s10967-025-09985-1
Pinghui Li, Jiaojiao Feng, Tingting Wang, Shici Yang, Xiaoming Cai, Yaohui Zhang, Jinming Cai, Gaohong Zhu
{"title":"Novel probe with iRGD integrated graphene oxide nanoparticles and labeled with 131I for detection of thyroid papillary carcinoma cells","authors":"Pinghui Li,&nbsp;Jiaojiao Feng,&nbsp;Tingting Wang,&nbsp;Shici Yang,&nbsp;Xiaoming Cai,&nbsp;Yaohui Zhang,&nbsp;Jinming Cai,&nbsp;Gaohong Zhu","doi":"10.1007/s10967-025-09985-1","DOIUrl":"10.1007/s10967-025-09985-1","url":null,"abstract":"<div><p>Integrating multiple targets and hence bio-distribution effectively for papillary thyroid carcinoma (PTC) treatment remains a significant challenge, which can be addressed by using suitable nano-scale materials. Herein, iRGD-modified graphene oxide (GO) loaded <sup>131</sup>I are developed for the specific treatment of PTC strengthened integrin targeting. Fine structural characteristics of GO and GO-iRGDs were characterized by fourier transform infrared spectroscopy (FT-IR), scanning electron microscope (SEC), Raman spectrum and X-ray photoelectron spectroscopy (XPS). The results showed that there were characteristic peaks and chemical bonds on GO and GO-iRGDs by FT-IR, the D-peak and G-peak of GO disappeared by Raman spectrum and C-N bond with iRGD of GO-iRGDs were strong by XPS. These <sup>131</sup>I-GO-iRGDs and <sup>131</sup>I-GOs were taken up by PTC cell (TPC-1, BCPAP, and IHH-4) through endocytosis after 48 h and 72 h in cell uptake test, especially the uptake rate of <sup>131</sup>I-GO50-iRGD was the highest. The CCK-8 cytotoxicity test of <sup>131</sup>I-GO-iRGDs and <sup>131</sup>I-GOs showed that these nanoparticles toxicity were higher than that of Na<sup>131</sup>I and finally promoted PTC death. In vitro data verified the targeting mechanism of GO and <sup>131</sup>I for PTC cell line is based on the relevant advantages of binding cell, followed by iRGD-endowed cell surface transport. The tailored design of GO-iRGDs validates a promising paradigm for radioisotope (131-iodine) delivery to combat PTC resistance and metastasis resulting from poor target access for effective combination therapy.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1577 - 1587"},"PeriodicalIF":1.5,"publicationDate":"2025-01-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10967-025-09985-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481038","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Phosphorus functionalized carbon nitride for rapid adsorption of uranium from aqueous solution 磷功能化氮化碳对水溶液中铀的快速吸附
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-29 DOI: 10.1007/s10967-025-09992-2
Youkui Zhang, Ruojing Deng, Junbo Zeng, Fanyue Shi, Sanquan Yang, Yingshuo Wu, Tao Duan
{"title":"Phosphorus functionalized carbon nitride for rapid adsorption of uranium from aqueous solution","authors":"Youkui Zhang,&nbsp;Ruojing Deng,&nbsp;Junbo Zeng,&nbsp;Fanyue Shi,&nbsp;Sanquan Yang,&nbsp;Yingshuo Wu,&nbsp;Tao Duan","doi":"10.1007/s10967-025-09992-2","DOIUrl":"10.1007/s10967-025-09992-2","url":null,"abstract":"<div><p>In this work, a novel phosphorus functionalized carbon nitride (PCN) was designed and synthesized by a pyrolysis method for rapid adsorption of uranium. The optimized sample obtained at 600 °C (marked as PCN-600) exhibited the highest ability for uranium adsorption with efficiency of over 96% in only 1 min. The PCN-600 also exhibited high selectivity for uranium adsorption from simulated wastewater containing multiple interfering ions. The characterization results further revealed that the main adsorption mechanism of the uranium on PCN-600 is chemisorption. This work provides newly insight into adsorbent design for uranium removal from wastewater.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 3","pages":"2227 - 2236"},"PeriodicalIF":1.5,"publicationDate":"2025-01-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10967-025-09992-2.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707015","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A heat and mass transfer model for evaluation of damaged cesium chloride radiological sources 一种评价氯化铯放射源损伤的传热传质模型
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-28 DOI: 10.1007/s10967-024-09911-x
Kellis Kincaid, David Abrecht, Shawn Sasser, Nate See, Charles Weber
{"title":"A heat and mass transfer model for evaluation of damaged cesium chloride radiological sources","authors":"Kellis Kincaid,&nbsp;David Abrecht,&nbsp;Shawn Sasser,&nbsp;Nate See,&nbsp;Charles Weber","doi":"10.1007/s10967-024-09911-x","DOIUrl":"10.1007/s10967-024-09911-x","url":null,"abstract":"<div><p>Radiological sources are vital to many applications, and typically contain byproducts from waste streams which decay over time to form complex mixtures of elements. Daughter products resulting from these decay processes can introduce complicating factors to the integrity and safety of the vessel that contains the radiological material. Sources containing cesium 137 (<span>(^{137})</span>Cs) are of particular interest, because the decay of this isotope produces barium metal which reacts readily and exothermically with oxygen. This work employs physics-based numerical tools to examine the thermal response of a radiological source containing a mixture of cesium and barium in the event that vessel walls are damaged and atmospheric gases contact source material. A parametric study was conducted to determine the sensitivity of the response to various factors, including vessel geometry, source material age, the degree of vessel damage, and other parameters. It was found that the peak temperatures that occurred within the source material strongly depend on these parameters, particularly vessel geometry and age, which determine whether a breach would be a relatively minor accident or a catastrophic incident. Finally, the model’s sensitivity to uncertain thermophysical properties is discussed.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 3","pages":"2061 - 2071"},"PeriodicalIF":1.5,"publicationDate":"2025-01-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707013","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High energy radiation induced degradation of poly(lactic acid) (PLLA) film: radiation chemical yield, kinetics, mechanism and radioracemization evidences 高能辐射诱导聚乳酸（PLLA）膜降解：辐射化学产率、动力学、机理和辐射去离子化证据
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-28 DOI: 10.1007/s10967-025-09979-z
Franco Cataldo, Ransel Barzaga, D. Aníbal García-Hernández, Arturo Manchado, Ilaria Di Sarcina, Alessia Cemmi
{"title":"High energy radiation induced degradation of poly(lactic acid) (PLLA) film: radiation chemical yield, kinetics, mechanism and radioracemization evidences","authors":"Franco Cataldo,&nbsp;Ransel Barzaga,&nbsp;D. Aníbal García-Hernández,&nbsp;Arturo Manchado,&nbsp;Ilaria Di Sarcina,&nbsp;Alessia Cemmi","doi":"10.1007/s10967-025-09979-z","DOIUrl":"10.1007/s10967-025-09979-z","url":null,"abstract":"<div><p>The chain scission radiation chemical yield G(S) of irradiated PLLA films has been calculated directly from the ketone absorption band of its FT-IR spectra recorded at different absorbed dose. The maximum value G(S) = 2.85 ± 0.1 scission/100 eV was determined at 100 kGy, in excellent agreement with previously reported G(S) but determined from CO<sub>2</sub> and CO gas analysis. Furthermore, from the FT-IR spectra, the rate constant of PLLA radiolityc degradation was determined in the range of 4.2–4.5 × 10<sup>–3</sup> h<sup>−1</sup> at a dose rate of 3 kGy/h. The optical rotatory dispersion analysis of the irradiated PLLA films has shown that the complete radioracemization is reached at 100 kGy. The irradiated PLLA films were also analyzed by thermal analysis (both DSC and TGA) and spectrophotometrically.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 4","pages":"2875 - 2885"},"PeriodicalIF":1.5,"publicationDate":"2025-01-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143888771","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Parameters affecting skin decontamination using wet reagents 使用湿试剂影响皮肤去污的参数
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-27 DOI: 10.1007/s10967-024-09886-9
Jaleh Semmler, Zahid Khan, Arshad Toor
{"title":"Parameters affecting skin decontamination using wet reagents","authors":"Jaleh Semmler,&nbsp;Zahid Khan,&nbsp;Arshad Toor","doi":"10.1007/s10967-024-09886-9","DOIUrl":"10.1007/s10967-024-09886-9","url":null,"abstract":"<div><p>This paper reports the results of tests performed to evaluate the effects of key parameters on the effectiveness of several wet decontamination processes for removal of <sup>60</sup>Co, <sup>137</sup>Cs and <sup>241</sup>Am from pig skin. Parameters tested included decontamination reagent composition, radionuclide deposition solution composition, the time between contamination and decontamination, and skin thickness and moisture content. Gamma-spectroscopy was used to determine the percentage activity removed and to quantify radionuclide permeation. The composition of the solution used for radionuclide deposition affected radionuclide removal, especially <sup>241</sup>Am. Radionuclide permeation showed a strong effect of skin hydration; <sup>137</sup>Cs permeated quickly through the samples while <sup>241</sup>Am showed no permeation.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1359 - 1373"},"PeriodicalIF":1.5,"publicationDate":"2025-01-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143480988","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Sparse restoration of fractal self-similar data and its application in uranium distribution 分形自相似数据的稀疏恢复及其在铀分布中的应用
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-25 DOI: 10.1007/s10967-024-09950-4
Jianyun Wang, Chenkai He, Zhenghua Xu, Yifan Chen, Yong Liu
{"title":"Sparse restoration of fractal self-similar data and its application in uranium distribution","authors":"Jianyun Wang,&nbsp;Chenkai He,&nbsp;Zhenghua Xu,&nbsp;Yifan Chen,&nbsp;Yong Liu","doi":"10.1007/s10967-024-09950-4","DOIUrl":"10.1007/s10967-024-09950-4","url":null,"abstract":"<div><p>Uranium is a rare and important energy mineral. In order to study the distribution characteristics of uranium deposits, we establish a data restoration algorithm with fractal features and sparse known point data. The algorithm ensures the accuracy of the restoration and the retention of fractal features through the steps of determining the basis function, preserving the dimension invariant restoration, and dimension greedy optimization. By comparing the numerical test with the Kriging interpolation method, it is proved that the algorithm is better in accuracy error and dimension error when restoring the fractal feature data.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1205 - 1215"},"PeriodicalIF":1.5,"publicationDate":"2025-01-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481216","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Optimizing Prussian blue synthesis: exploring the influence of synthesis parameters on maximum binding capacity of Prussian blue for thallium 优化普鲁士蓝合成：探索合成参数对普鲁士蓝对铊的最大结合能力的影响
IF 1.5 3区 化学
Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2025-01-25 DOI: 10.1007/s10967-024-09940-6
Vivek Kumar, Riya Mahar, Nidhi Sandal
{"title":"Optimizing Prussian blue synthesis: exploring the influence of synthesis parameters on maximum binding capacity of Prussian blue for thallium","authors":"Vivek Kumar,&nbsp;Riya Mahar,&nbsp;Nidhi Sandal","doi":"10.1007/s10967-024-09940-6","DOIUrl":"10.1007/s10967-024-09940-6","url":null,"abstract":"<div><p>This study optimized Prussian Blue (PB) synthesis parameters to enhance its binding capacity for thallium (Tl(I)). Using direct (PB-1) and indirect (PB-2) methods, key parameters such as stirring time, drying conditions, oxidant concentration, and iron content were evaluated. For PB-1, the optimal conditions were 12-h stirring, 4-h drying at 60 °C, resulting in a maximum binding capacity (MBC) of 200 mg/g. For PB-2, the optimal parameters included 2-h drying at 80 °C, 20 mL oxidant, and 2-h aging at 60 °C, yielding an MBC of 208.33 mg/g. These findings ensure improved therapeutic efficacy of PB as an active pharmaceutical ingredient. Yes, the street name for the affiliation one is correct</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 2","pages":"1311 - 1322"},"PeriodicalIF":1.5,"publicationDate":"2025-01-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143481215","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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