Matter最新文献 - Book学术

Electrostatic breakdown at liquid-solid-gas triple-phase interfaces owing to contact electrification

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-26 DOI: 10.1016/j.matt.2025.102007

Cuiying Ye, Di Liu, Yikui Gao, Fan Liu, Hongxuan Xu, Tao Jiang, Zhong Lin Wang

引用次数: 0

Sustained exposure to multivalent antigen-decorated nanoparticles generates broad anti-coronavirus responses

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-25 DOI: 10.1016/j.matt.2025.102006

Julie Baillet, John H. Klich, Ben S. Ou, Emily L. Meany, Jerry Yan, Theodora U.J. Bruun, Ashley Utz, Carolyn K. Jons, Sebastien Lecommandoux, Eric A. Appel

{"title":"Sustained exposure to multivalent antigen-decorated nanoparticles generates broad anti-coronavirus responses","authors":"Julie Baillet, John H. Klich, Ben S. Ou, Emily L. Meany, Jerry Yan, Theodora U.J. Bruun, Ashley Utz, Carolyn K. Jons, Sebastien Lecommandoux, Eric A. Appel","doi":"10.1016/j.matt.2025.102006","DOIUrl":"https://doi.org/10.1016/j.matt.2025.102006","url":null,"abstract":"The threat of future coronavirus pandemics requires developing effective vaccine technologies that provide broad and long-lasting protection against circulating and emerging strains. Here, we report a multivalent liposomal hydrogel depot vaccine technology comprising the receptor binding domain (RBD) of up to four relevant coronavirus strains from severe acute respiratory syndrome (SARS) and Middle East respiratory syndrome (MERS) non-covalently displayed on the surface of the liposomes within the hydrogel structure. The multivalent presentation and sustained exposure of RBD antigens improved the potency, neutralizing activity, durability, and consistency of antibody responses across homologous and heterologous coronavirus strains in a naive murine model. When administrated in animals pre-exposed to wild-type SARS-CoV-2 antigens, liposomal hydrogels elicited durable antibody responses against the homologous SARS and MERS strains for more than 6 months and elicited neutralizing activity against the immune-evasive SARS-CoV-2 variant Omicron BA.4/BA.5. Overall, the tunable liposomal hydrogel platform we report here generates robust responses against diverse coronaviruses, supporting global efforts to respond to future viral outbreaks.","PeriodicalId":388,"journal":{"name":"Matter","volume":"32 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-02-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143486394","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

A thermal transfer-enhanced zinc anode for stable and high-energy-density zinc-ion batteries

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-25 DOI: 10.1016/j.matt.2025.102013

Shaofei La, Yong Gao, Qinghe Cao, Jingzhu Chen, Abdelnaby M. Elshahawy, Yingyi Cui, Fan Bu, Salah A. Makhlouf, Pei Song Chee, Cao Guan

{"title":"A thermal transfer-enhanced zinc anode for stable and high-energy-density zinc-ion batteries","authors":"Shaofei La, Yong Gao, Qinghe Cao, Jingzhu Chen, Abdelnaby M. Elshahawy, Yingyi Cui, Fan Bu, Salah A. Makhlouf, Pei Song Chee, Cao Guan","doi":"10.1016/j.matt.2025.102013","DOIUrl":"https://doi.org/10.1016/j.matt.2025.102013","url":null,"abstract":"Achieving a Zn anode with simultaneous excellent cycling stability and high Zn utilization rate still remains a huge challenge for practical rechargeable zinc-ion batteries. Here, thermal transfer-enhanced layers are coated on both sides of Zn foil, where the top layer enables uniform Zn2+ flux and temperature distribution, and the bottom coating improves local heat diffusion and mechanical stability. With such dual thermal protection, thermodynamically driven dendrite growth and side reactions are effectively suppressed. The Zn anode can be stably cycled for 440 h at 5 mA cm−2/5 mAh cm−2 (corresponding to a high Zn utilization rate of 85.5%), which is superior to previously reported results for protective layer-coated zinc anodes. A V2O3/N-doped carbon (NC)-based full cell exhibits stable performance for 200 cycles with a high specific energy density (174 Wh kg−1, based on the whole mass of electrodes) and high volumetric energy density (218 Wh L−1, based on the whole cell), which is promising for practical applications.","PeriodicalId":388,"journal":{"name":"Matter","volume":"14 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-02-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143486602","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Sub-nm kinetically controlled liquid metal printing of ternary antimony indium oxide transistors

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-24 DOI: 10.1016/j.matt.2025.102003

Samuel W. Ong, Simon A. Agnew, Md Saifur Rahman, William J. Scheideler

{"title":"Sub-nm kinetically controlled liquid metal printing of ternary antimony indium oxide transistors","authors":"Samuel W. Ong, Simon A. Agnew, Md Saifur Rahman, William J. Scheideler","doi":"10.1016/j.matt.2025.102003","DOIUrl":"https://doi.org/10.1016/j.matt.2025.102003","url":null,"abstract":"Two-dimensional (2D) metal oxide semiconductors offer a superlative combination of high electron mobility and visible-range transparency uniquely suitable for flexible transparent electronics. Synthesis of these ultrathin (<3 nm) semiconductors by Cabrera-Mott oxidation of liquid metals could enable emerging device applications but requires the precise design of their electrostatics at the nanoscale. This study demonstrates sub-nanometer-level control over the thickness of semiconducting 2D antimony-doped indium oxide (AIO) by manipulating the kinetics of Cabrera-Mott oxidation through variable-speed liquid metal printing at plastic-compatible temperatures (175°C). By modulating both the growth kinetics and doping, we engineer the conductivity and crystallinity of AIO for integration in ultrathin channel transistors exhibiting exceptional steep turn-on, on-off ratios > 106 and an outstanding average mobility of 34.7 ± 12.9 cm2/Vs. This result shows the potential for kinetically controlling 2D oxide synthesis for various high-performance optoelectronic device applications.","PeriodicalId":388,"journal":{"name":"Matter","volume":"36 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-02-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143477768","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Lattice distortion boosted exceptional electromagnetic wave absorption in high-entropy diborides 晶格畸变促进高熵二硼化物对特殊电磁波的吸收

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-18 DOI: 10.1016/j.matt.2025.102004

Fangchao Gu, Wu Wang, Hong Meng, Yiwen Liu, Lei Zhuang, Hulei Yu, Yanhui Chu

引用次数: 0

Open-air spray deposition of PCBM/BCP electron transport layer for inverted perovskite solar cells

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-17 DOI: 10.1016/j.matt.2025.101990

Justin P. Chen, Thomas W. Colburn, Juliet Risner-Jamtgaard, Arturas Vailionis, Andrew Barnum, Margarita Golding, Abigail Carbone, Austin C. Flick, Reinhold H. Dauskardt

{"title":"Open-air spray deposition of PCBM/BCP electron transport layer for inverted perovskite solar cells","authors":"Justin P. Chen, Thomas W. Colburn, Juliet Risner-Jamtgaard, Arturas Vailionis, Andrew Barnum, Margarita Golding, Abigail Carbone, Austin C. Flick, Reinhold H. Dauskardt","doi":"10.1016/j.matt.2025.101990","DOIUrl":"https://doi.org/10.1016/j.matt.2025.101990","url":null,"abstract":"A [6,6]-phenyl C61 butyric acid methyl ester (PCBM) and bathocuproine (BCP) electron transport layer (ETL) is spray deposited in open air directly on top of a perovskite at linear speeds of 9 m/min. The PCBM precursor ink contains a binary mixture of 1:1 chlorobenzene:chloroform, which optimizes spray wettability on the perovskite surface and allows quick solvent evaporation. A near-infrared heating module additionally provides a flash cure (<5 s) for the formation of smooth, large-area PCBM films (∼20 cm2). A BCP solution in isopropanol is subsequently sprayed to form an ultrathin (<5 nm) film and characterized with a suite of high-resolution metrologies. The spray-deposition processing and near-infrared treatment do not damage the underlying perovskite. Inverted architecture devices containing the sprayed ETL achieve a champion efficiency of 20.3% and demonstrate stable performance without additional interlayers or surface treatments. The technoeconomic cost of the open-air spray process is compared against traditional vacuum-based evaporation, resulting in a decrease in manufacturing costs by 26%.","PeriodicalId":388,"journal":{"name":"Matter","volume":"35 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-02-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143427248","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Sustainable conversion of husk into viscoelastic hydrogels for value-added biomedical applications

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-17 DOI: 10.1016/j.matt.2025.102002

Changxu Sun, Jiping Yue, Pengju Li, Wen Li, Jingcheng Ma, Chuanwang Yang, Saehyun Kim, Bozhi Tian

{"title":"Sustainable conversion of husk into viscoelastic hydrogels for value-added biomedical applications","authors":"Changxu Sun, Jiping Yue, Pengju Li, Wen Li, Jingcheng Ma, Chuanwang Yang, Saehyun Kim, Bozhi Tian","doi":"10.1016/j.matt.2025.102002","DOIUrl":"https://doi.org/10.1016/j.matt.2025.102002","url":null,"abstract":"Natural plants provide a wealth of valuable materials for healthcare, with much of their potential often overlooked in what is commonly considered waste. This study focuses on the Malva nut tree (Sterculia lychnophora Hance), whose fruit, Pangdahai (PDH), has long been used in traditional Chinese medicine. By investigating the swelling behavior of PDH husk, we efficiently extracted its polysaccharides without harsh chemicals. Using micro-compression, we developed a viscoelastic hydrogel, and through electrostatic crosslinking with chitosan, we further enhanced its mechanical properties. The hydrogel exhibited biocompatibility and accelerated wound healing by promoting keratinocyte migration. Additionally, it outperformed commercial patches as a skin-attached interfacial material for electrocardiography (ECG), demonstrating superior signal-to-noise ratios. Integrated into a 16-channel mesh electronic device, the hydrogel provided stable performance for in vivo epicardial ECG recording on a beating heart. This research highlights the potential of rigid polysaccharide waste, presenting a sustainable approach to converting plant waste into valuable healthcare materials.","PeriodicalId":388,"journal":{"name":"Matter","volume":"47 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-02-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143427250","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

High-performance 2D perovskite-based flexible photodetectors for optical communication and information encryption

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-13 DOI: 10.1016/j.matt.2025.101998

Kaijia Feng, Ying Li, Yancheng Chen, Zhongming Wei, Guozhen Shen

{"title":"High-performance 2D perovskite-based flexible photodetectors for optical communication and information encryption","authors":"Kaijia Feng, Ying Li, Yancheng Chen, Zhongming Wei, Guozhen Shen","doi":"10.1016/j.matt.2025.101998","DOIUrl":"https://doi.org/10.1016/j.matt.2025.101998","url":null,"abstract":"Flexible optical wireless communication is significant for major strategic needs due to its safety, portability, and precision. As a core component in optical communication systems, photodetectors (PDs) are plagued by stringent requirements, including high detectivity, stability, and flexibility. Herein, an optical wireless communication system based on flexible two-dimensional (2D) Ruddlesden-Popper (RP) perovskite PDs is presented. The thickness-optimized PD with outstanding thermal stability and flexibility has a high responsivity over the visible light range with two peaks at 488 and 532 nm. Based on these advancements, a multiplexing encrypted communication system is presented by exploiting the 488 and 532 nm light as independent information transmission channels to improve information security. Moreover, the flexible PD is integrated into the integrated circuit to simulate an optical wireless communication system for visible light positioning and bidirectional information transmission, which realizes the real-time positioning of the vehicle and the real-time presentation of the user interface.","PeriodicalId":388,"journal":{"name":"Matter","volume":"23 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-02-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143401226","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Exploring the soft cradle effect and ionic transport mechanisms in the LiMXCl4 superionic conductor family

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-13 DOI: 10.1016/j.matt.2025.102001

KyuJung Jun, Grace Wei, Xiaochen Yang, Yu Chen, Gerbrand Ceder

{"title":"Exploring the soft cradle effect and ionic transport mechanisms in the LiMXCl4 superionic conductor family","authors":"KyuJung Jun, Grace Wei, Xiaochen Yang, Yu Chen, Gerbrand Ceder","doi":"10.1016/j.matt.2025.102001","DOIUrl":"https://doi.org/10.1016/j.matt.2025.102001","url":null,"abstract":"LiMXCl4, a recently discovered lithium superionic conductor, achieves Li conductivity up to 12.4 mS/cm at room temperature. Notably, LiNbOCl4 features flexible, rotating polyhedra, potentially explaining its high ionic conductivity. However, the generalizability of these findings across different chemistries and the direct link between polyhedra rotations and Li-ion mobility remain unclear. In this study, we explore various M-cation and X-anion substitutions in the LiMXCl4 system, identifying fluoro-chlorides as promising for enhancing electrochemical stability while maintaining high ionic conductivity. Meyer-Neldel analysis on ab initio simulations reveals that LiMXCl4 outperforms existing halide conductors, with projected conductivities of 10–100 mS/cm. Our probabilistic analysis of lithium-ion hops and small-angle tilting events reveals a “soft cradle effect,” where weakly bound M-octahedra tilt in conjunction with Li-ion hops, optimizing the energy landscape. This work provides fundamental insights into the factors driving high ionic conductivity in non-close-packed oxyhalide systems and suggests exciting directions for further improving these materials.","PeriodicalId":388,"journal":{"name":"Matter","volume":"30 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-02-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143401222","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

3D printing of alloys with AB reaction at room temperature

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-13 DOI: 10.1016/j.matt.2025.101999

Weicheng Kong, Yuling Lu, Ximin Yuan, Meng Zhu, Qilin Wu, Ke Yao, Tao Fu, Yong He

引用次数: 0