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A soft and fatigue-resistant material that mimics heart valves 一种柔软且抗疲劳的材料,模仿心脏瓣膜
IF 17.3 1区 材料科学
Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.020
Xi Chen , Fengkai Liu , Qifeng Yu , Meng Yang , Zhigang Suo , Jingda Tang
{"title":"A soft and fatigue-resistant material that mimics heart valves","authors":"Xi Chen ,&nbsp;Fengkai Liu ,&nbsp;Qifeng Yu ,&nbsp;Meng Yang ,&nbsp;Zhigang Suo ,&nbsp;Jingda Tang","doi":"10.1016/j.matt.2024.11.020","DOIUrl":"10.1016/j.matt.2024.11.020","url":null,"abstract":"<div><div>Bovine pericardium, a tissue commonly used to make artificial heart valves, fulfills two fundamental mechanical requirements: a low modulus to ensure opening and closing in cyclic pulsatile flow and a high fatigue threshold to prevent crack growth. The tissue consists of a soft matrix and crimped fibers. Inspired by this architecture, we develop a composite of a soft polymer matrix and a knitted fabric. When the stretch is small to modest, the knitted fabric is easily stretched, so that the composite is soft. When the stretch is large, the knitted fabric is stiff and strong, so that the composite resists fatigue crack growth. The mechanical behavior of the composite is comparable to that of bovine pericardium. The composite has an exceptionally long fatigue life, enduring 25 million cycles of pulsatile flow, two orders of magnitude longer than the polymer matrix. This soft and fatigue-resistant composite may find broad applications in biomedicine.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101926"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142816241","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Massively multiplexed optical recording with polychromatic DNA frameworks 利用多色 DNA 框架进行大规模复用光学记录
IF 17.3 1区 材料科学
Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.10.020
Lu Song , Ruiyan Guo , Li Pan , Yishakejiang Saimaiti , Shaopeng Wang , Fan Li , Xiuhai Mao , Fei Wang , Qi Li , Dekai Ye , Sisi Jia , Gang Liu , Min Li , Xiaolei Zuo , Chunhai Fan
{"title":"Massively multiplexed optical recording with polychromatic DNA frameworks","authors":"Lu Song ,&nbsp;Ruiyan Guo ,&nbsp;Li Pan ,&nbsp;Yishakejiang Saimaiti ,&nbsp;Shaopeng Wang ,&nbsp;Fan Li ,&nbsp;Xiuhai Mao ,&nbsp;Fei Wang ,&nbsp;Qi Li ,&nbsp;Dekai Ye ,&nbsp;Sisi Jia ,&nbsp;Gang Liu ,&nbsp;Min Li ,&nbsp;Xiaolei Zuo ,&nbsp;Chunhai Fan","doi":"10.1016/j.matt.2024.10.020","DOIUrl":"10.1016/j.matt.2024.10.020","url":null,"abstract":"<div><div>Rapid data growth highlights the increasing demand for high-density storage solutions. Multiplexed optical recording based on synthetic inorganic nanoparticles represents the next generation of data storage. However, diverse photophysical properties of nanoparticles reduce their reliability and information density. Here, we present a highly programmable polychromatic DNA tetrahedral framework (PDTF) that enables precise control over their optical performances. By programming the size of PDTFs, we reduce the feature size of the recording medium to 3.4 nm, which was 41-fold smaller than that of commercially available Blu-ray technology. PDTF chains with up to 47 million distinct color codes further enhance optical storage with higher information capacity. Additionally, nanopatterning technology integrates the PDTFs into on-chip architectures, achieving an impressive density of 25.9 Gb/cm<sup>2</sup>. Finally, the PDTFs demonstrate excellent re-writability and long-term stability (10,826 years at room temperature), exhibiting promising potential in high-density and secure data storage applications.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101902"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142673718","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Atomic sulfur-bonded titanium carbide nanosheets for flexible piezoresistive sensor in monitoring sleep apnea syndrome 原子硫键合碳化钛纳米片用于监测睡眠呼吸暂停综合征的柔性压阻传感器
IF 17.3 1区 材料科学
Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.021
Yan Bai , Longlu Wang , Xiang Zou , Ning Ding , Yuhui Feng , Zhen You , Weiwei Zhao , Weikang Wang , Feifei Lin , Yuzhe Chen , Yijie Zhang , Jianmin Li , Fangyi Guan , Shujuan Liu , Wei Huang , Qiang Zhao
{"title":"Atomic sulfur-bonded titanium carbide nanosheets for flexible piezoresistive sensor in monitoring sleep apnea syndrome","authors":"Yan Bai ,&nbsp;Longlu Wang ,&nbsp;Xiang Zou ,&nbsp;Ning Ding ,&nbsp;Yuhui Feng ,&nbsp;Zhen You ,&nbsp;Weiwei Zhao ,&nbsp;Weikang Wang ,&nbsp;Feifei Lin ,&nbsp;Yuzhe Chen ,&nbsp;Yijie Zhang ,&nbsp;Jianmin Li ,&nbsp;Fangyi Guan ,&nbsp;Shujuan Liu ,&nbsp;Wei Huang ,&nbsp;Qiang Zhao","doi":"10.1016/j.matt.2024.11.021","DOIUrl":"10.1016/j.matt.2024.11.021","url":null,"abstract":"<div><div>Flexible piezoresistive sensors have attracted great attention for the real-time monitoring of sleep apnea syndrome (SAS) through respiratory airflow. Although two-dimensional ultrathin Ti<sub>3</sub>C<sub>2</sub> is regarded as a promising piezoresistive material, its poor structural compressibility and antioxidation limit its practical applications. Here, an innovative atomic sulfur-bonded strategy is proposed to fabricate large-sized, crumpled, and antioxidative Ti<sub>3</sub>C<sub>2</sub>/Na<sub>2</sub>S (TS) flakes for preparing flexible piezoresistive sensors. The fundamental mechanism is rooted in the synergistic effect of lateral boundary assembly of Ti<sub>3</sub>C<sub>2</sub> nanosheets into large flakes (∼7 μm), lattice distortion to induce crumpled structures, and edge passivation by S<sup>2−</sup> ions to mitigate oxidation (105 days). The crumpled microstructure provides abundant voids for enhanced compressibility and contact site variability, resulting in a 5-fold sensitivity improvement over the Ti<sub>3</sub>C<sub>2</sub> sensor and an ultralow detection limit of 0.2 Pa. We demonstrate the practical application of highly sensitive and stable piezoresistive sensors integrated into a respiratory monitoring system for SAS detection.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101927"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142832467","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Multi-band luminescence from a rare earth-based two-dimensional material 基于稀土的二维材料的多波段发光
IF 17.3 1区 材料科学
Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.023
Rahul Rao , Emmanuel Rowe , Ryan Siebenaller , Jonathan T. Goldstein , Adam Alfieri , Bongjun Choi , Ryan Selhorst , Andrea N. Giordano , Jie Jiang , Christopher E. Stevens , Thuc T. Mai , Tyson C. Back , Ruth Pachter , Joshua R. Hendrickson , Deep Jariwala , Michael A. Susner
{"title":"Multi-band luminescence from a rare earth-based two-dimensional material","authors":"Rahul Rao ,&nbsp;Emmanuel Rowe ,&nbsp;Ryan Siebenaller ,&nbsp;Jonathan T. Goldstein ,&nbsp;Adam Alfieri ,&nbsp;Bongjun Choi ,&nbsp;Ryan Selhorst ,&nbsp;Andrea N. Giordano ,&nbsp;Jie Jiang ,&nbsp;Christopher E. Stevens ,&nbsp;Thuc T. Mai ,&nbsp;Tyson C. Back ,&nbsp;Ruth Pachter ,&nbsp;Joshua R. Hendrickson ,&nbsp;Deep Jariwala ,&nbsp;Michael A. Susner","doi":"10.1016/j.matt.2024.11.023","DOIUrl":"10.1016/j.matt.2024.11.023","url":null,"abstract":"<div><div>Photoluminescence (PL) emission in two-dimensional (2D) materials is of great interest for nanophotonics applications. While excitonic emission has been observed in numerous 2D materials, tunable multi-band luminescence is rare. Here, we present single-crystalline AgErP<sub>2</sub>Se<sub>6</sub>, a 2D material that exhibits bright, multi-band PL emission from Er<sup>3+</sup> ions within the lattice. The emission bands cover a wide range (350–1,550 nm), with ultra-narrow (as low as 0.5 nm at room temperature) emission peaks and room temperature lifetimes up to ∼4 μs. The intensities of the PL emission bands from the single crystals depend strongly on temperature and pressure, enabling sensing over a wide temperature and pressure range. Furthermore, the PL persists in exfoliated flakes down to at least 11 nm thick and demonstrates thickness-dependent Purcell enhancement. This work establishes 2D AgErP<sub>2</sub>Se<sub>6</sub> as a multi-band luminescent emitter and sensor, poised to enable integration into a number of optoelectronic and nanophotonic applications.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101929"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142833036","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Leveraging biomimetic materials for bioelectronics
IF 17.3 1区 材料科学
Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2025.101961
Junyi Yin , Shaolei Wang , Xiao Xiao , Farid Manshaii , Kamryn Scott , Jun Chen
{"title":"Leveraging biomimetic materials for bioelectronics","authors":"Junyi Yin ,&nbsp;Shaolei Wang ,&nbsp;Xiao Xiao ,&nbsp;Farid Manshaii ,&nbsp;Kamryn Scott ,&nbsp;Jun Chen","doi":"10.1016/j.matt.2025.101961","DOIUrl":"10.1016/j.matt.2025.101961","url":null,"abstract":"<div><div>The exploration of biomimetic materials for bioelectronics is driving transformative advancements in medical technology and beyond. Drawing inspiration from nature’s intricate designs, these materials hold immense potential for creating bioelectronics that integrate seamlessly with living tissues. This work highlights three key biomimetic strategies in the current bioelectronics community: structural design, material properties, and natural processes. We demonstrate how these approaches significantly enhance the bioelectronic performance in the aspects of bio-signal acquisition, transduction, and analysis, addressing critical challenges in current biomedical technologies. By incorporating these principles, biomimetic materials and technologies are poised to revolutionize the conventional medical model, fostering the development of more intelligent, efficient, and biocompatible bioelectronic devices.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101961"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143124567","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Modulating hydration states of polymer micropores for ion-selective transport 调节聚合物微孔的水合状态以实现离子选择性传输
IF 17.3 1区 材料科学
Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.101953
Jing Guo , Yanqiu Zhang , Lu Shao
{"title":"Modulating hydration states of polymer micropores for ion-selective transport","authors":"Jing Guo ,&nbsp;Yanqiu Zhang ,&nbsp;Lu Shao","doi":"10.1016/j.matt.2024.101953","DOIUrl":"10.1016/j.matt.2024.101953","url":null,"abstract":"<div><div>Precise ion-selective transport through membranes plays pivotal roles in electrochemical processes. Recently, in <em>Nature</em>, Song and coworkers reported the fine-tuning of pore hydration states by designing hydrophobic pendant groups in functional polymer membranes. Consequently, interconnecting pore networks with narrow gate sizes and optimal chemical environments were constructed in polymer membranes, resulting in superior performance in electrochemical devices.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101953"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143124566","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Unlocking the potential hidden in MXene layers through lignin-mediated intercalation
IF 17.3 1区 材料科学
Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2025.101960
Qingxiao Zhang , Qinghua Yu , Xiuxia Meng , Naitao Yang , Hui Li
{"title":"Unlocking the potential hidden in MXene layers through lignin-mediated intercalation","authors":"Qingxiao Zhang ,&nbsp;Qinghua Yu ,&nbsp;Xiuxia Meng ,&nbsp;Naitao Yang ,&nbsp;Hui Li","doi":"10.1016/j.matt.2025.101960","DOIUrl":"10.1016/j.matt.2025.101960","url":null,"abstract":"<div><div>MXene nanosheets feature tunable interlayer structures, but achieving continuous tuning remains a challenge. Pan et al. reported an intercalation strategy using lignin that allows for precise control of the MXene interlayer spacing and enhances the material’s oxidation stability.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101960"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143124564","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Establishing an elastic electron/lithium-ion transport network via in situ crosslinking for stabilizing interphases in SiOx electrodes 通过原位交联建立弹性电子/锂离子输运网络以稳定SiOx电极的界面相
IF 18.9 1区 材料科学
Matter Pub Date : 2025-01-21 DOI: 10.1016/j.matt.2024.101952
Lu Wang, Zhibo Song, Yongsheng Li, Yuxiang Huang, Hao Zhang, Zuwei Yin, Jinlin Xiao, Chen Zhu, Yiqian Zhao, Meng Zhang, Tongchao Liu, Feng Pan, Luyi Yang
{"title":"Establishing an elastic electron/lithium-ion transport network via in situ crosslinking for stabilizing interphases in SiOx electrodes","authors":"Lu Wang, Zhibo Song, Yongsheng Li, Yuxiang Huang, Hao Zhang, Zuwei Yin, Jinlin Xiao, Chen Zhu, Yiqian Zhao, Meng Zhang, Tongchao Liu, Feng Pan, Luyi Yang","doi":"10.1016/j.matt.2024.101952","DOIUrl":"https://doi.org/10.1016/j.matt.2024.101952","url":null,"abstract":"The significant volumetric fluctuations experienced by high-capacity silicon-based electrodes during cycling lead to the disintegration of conductive frameworks and destabilization of the solid-electrolyte interphase (SEI). To overcome these challenges, an <em>in situ</em> thiol-ene click reaction is employed to fabricate an elastic electron/lithium-ion (e<sup>−</sup>/Li<sup>+</sup>)-conducting polymer network that uniformly binds SiO<sub><em>x</em></sub> active materials. The proposed polymer incorporates rigid backbone segments that enhance electron conduction, along with flexible linkers that facilitate Li<sup>+</sup> transport and stress dissipation within the SiO<sub><em>x</em></sub> electrode, thereby stabilizing the interfacial charge transfer on SiO<sub><em>x</em></sub>. By reducing the initial expansion rate of the SiO<sub><em>x</em></sub> electrode from 157% to 65%, the stable polymeric network effectively mitigates SEI degradation during cycling. As a result, the <em>in</em>-<em>situ</em>-crosslinked polymer framework enables improved capacity retention (82.7% after 250 cycles) and rate performance. By simultaneously strengthening the ion and electron transport pathways, this work offers new avenues for the future design of high-capacity negative electrodes.","PeriodicalId":388,"journal":{"name":"Matter","volume":"32 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-01-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142991240","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Brilliant colorful daytime radiative cooling coating mimicking scarab beetle 模仿猩红甲虫的绚丽多彩的日间辐射冷却涂层
IF 17.3 1区 材料科学
Matter Pub Date : 2025-01-08 DOI: 10.1016/j.matt.2024.10.016
Xiaoyu Hou , Kaiyue Zhang , Xintao Lai , Liwei Hu , Florian Vogelbacher , Yanlin Song , Lei Jiang , Mingzhu Li
{"title":"Brilliant colorful daytime radiative cooling coating mimicking scarab beetle","authors":"Xiaoyu Hou ,&nbsp;Kaiyue Zhang ,&nbsp;Xintao Lai ,&nbsp;Liwei Hu ,&nbsp;Florian Vogelbacher ,&nbsp;Yanlin Song ,&nbsp;Lei Jiang ,&nbsp;Mingzhu Li","doi":"10.1016/j.matt.2024.10.016","DOIUrl":"10.1016/j.matt.2024.10.016","url":null,"abstract":"<div><div>Passive daytime radiative cooling is regarded as a promising technology to achieve all-day subambient cooling without energy consumption and pollution. The installation of monotonous white radiative cooling coating on the facades of buildings poses challenges in terms of aesthetic integration. Fabricating radiative cooling coatings with different colors and high cooling efficiency at a low cost is an optimal solution for their broad adoption and commercialization. Here, inspired by the elytra of the scarab beetle, we design a hierarchically porous nested structured radiative cooling film with high subambient cooling efficiency and flexible color tunability. This film exhibits both high solar reflectance (93.4%) and superior thermal emissivity (92.3%), realizing subambient cooling of ∼10.2°C at night and ∼7.2°C at midday. Its color is brilliant, stable, and flexible. Additionally, this film is self-cleaning and can reduce noise, which suggests possibilities for the development of multifunctional radiative cooling surfaces in building envelopes, automobile coatings, and clothes.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 1","pages":"Article 101898"},"PeriodicalIF":17.3,"publicationDate":"2025-01-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142637609","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Citations are not a card game 引文不是纸牌游戏
IF 17.3 1区 材料科学
Matter Pub Date : 2025-01-08 DOI: 10.1016/j.matt.2024.10.014
Yan Li, Steve Cranford
{"title":"Citations are not a card game","authors":"Yan Li,&nbsp;Steve Cranford","doi":"10.1016/j.matt.2024.10.014","DOIUrl":"10.1016/j.matt.2024.10.014","url":null,"abstract":"","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 1","pages":"Article 101896"},"PeriodicalIF":17.3,"publicationDate":"2025-01-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142936133","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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