Jason Lynch, Tzu-Yu Peng, Jing-Wei Yang, Ben R. Conran, Bongjun Choi, Cindy Yueli Chen, Zahra Fakhraai, Clifford McAleese, Yu-Jung Lu, Deep Jariwala
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High-temperature-resilient hyperbolicity in a mixed-dimensional superlattice
Hyperbolic superlattices are used for subwavelength focusing, cloaking, and optical thermal management. Typically, these superlattices are constructed of layers of noble metals and insulators. Despite these systems displaying excellent optical performance, the poor thermal stability of noble metals prevents their application in high-temperature environments. Instead, CMOS-compatible transition-metal nitrides are often substituted for noble metals in plasmonic systems since they have high thermal stability at the expense of optical properties. Here, we fabricate hyperbolic titanium nitride (TiN)/hexagonal boron nitride (hBN) superlattices with 3D-2D interfaces. The mixed-dimensional nature of the interfaces prevents atoms from diffusing across the interface at high temperatures. The hyperbolicity of the superlattice is found to be unaffected by annealing at high temperature (800°C for 5 days), and TiN/hBN is found to have a larger hyperbolic figure of merit than similar superlattices.
期刊介绍:
Matter, a monthly journal affiliated with Cell, spans the broad field of materials science from nano to macro levels,covering fundamentals to applications. Embracing groundbreaking technologies,it includes full-length research articles,reviews, perspectives,previews, opinions, personnel stories, and general editorial content.
Matter aims to be the primary resource for researchers in academia and industry, inspiring the next generation of materials scientists.