Matter最新文献_第2页

Giant berry curvature in amorphous ferromagnet Co2MnGa

IF 18.9 1区材料科学

Matter Pub Date : 2025-02-10 DOI: 10.1016/j.matt.2025.101988

Weiyao Zhao, Yao Zhang, Yuefeng Yin, Kaijian Xing, Shengqiang Zhou, Abdulhakim Bake, Golrokh Akhgar, David Cortie, Lei Chen, Xiaolin Wang, Kirrily C. Rule, Nikhil V. Medkehar, Simon Granville, Julie Karel

{"title":"Giant berry curvature in amorphous ferromagnet Co2MnGa","authors":"Weiyao Zhao, Yao Zhang, Yuefeng Yin, Kaijian Xing, Shengqiang Zhou, Abdulhakim Bake, Golrokh Akhgar, David Cortie, Lei Chen, Xiaolin Wang, Kirrily C. Rule, Nikhil V. Medkehar, Simon Granville, Julie Karel","doi":"10.1016/j.matt.2025.101988","DOIUrl":"https://doi.org/10.1016/j.matt.2025.101988","url":null,"abstract":"In amorphous materials, long-range translational order breaks down, and <em>k</em> is no longer a good quantum number; however, some of the phenomena, for instance ferromagnetic interactions and a mechanism similar to the Berry curvature, can be preserved. Here, we demonstrate a giant Berry-curvature-induced anomalous Hall effect and anomalous Hall angle in amorphous Co<sub>2</sub>MnGa (a-CMG) thin films. Remarkably, the effect presents the same magnitude as high-quality crystalline CMG with the L2<sub>1</sub> structure. The elastic neutron scattering peak in a-CMG is centered close to the crystalline phase, indicating that the amorphous material presents similar local atomic environments and magnetic interactions. First-principles density functional theory calculations further show that the anomalous Hall conductivity arises only when the local environments in the amorphous structure are similar to the L2<sub>1</sub> phase. Our work strongly points to the application of low-cost, industry-compatible, and thermally stable amorphous topological materials in emerging electronic and spintronic applications.","PeriodicalId":388,"journal":{"name":"Matter","volume":"51 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143375159","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

A ferroelectric living interface for fine-tuned exosome secretion toward physiology-mimetic neurovascular remodeling 用于微调外泌体分泌以实现仿生学神经血管重塑的铁电活界面

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.10.019

Mingxing Peng , Qilong Zhao , Anping Chai , Yutian Wang , Min Wang , Xuemin Du

{"title":"A ferroelectric living interface for fine-tuned exosome secretion toward physiology-mimetic neurovascular remodeling","authors":"Mingxing Peng , Qilong Zhao , Anping Chai , Yutian Wang , Min Wang , Xuemin Du","doi":"10.1016/j.matt.2024.10.019","DOIUrl":"10.1016/j.matt.2024.10.019","url":null,"abstract":"<div><div>Establishing vascular neural networks is critical for tissue regeneration. However, none of the existing approaches can replicate the physiological processes that varying extracellular cues sequentially play parts in different phases, thus hindering synergistic neurovascular remodeling. Here, we report a ferroelectric living interface for fine-tuned exosome secretion (LIFES) that harnesses unique topographical and electric (piezoelectric and photopyroelectric) signals and sustained generation of bioactive exosomes by rationally constructing a ferroelectric layer and a living cell layer. The LIFES exhibits physiology-mimicking paracrine effects, including sustained (∼192 h), phase-specific exosome secretion with tunable contents (∼8-fold increases) and programmable microRNA (miRNA) cargoes (initially pro-angiogenic and later pro-neurogenic), which overcome the limitations of the existing exosome delivery systems, such as short lifetime (∼24–48 h), difficult-to-preserve bioactivity, and non-changeable cargoes. LIFES allows for enhanced effectiveness in promoting neurovascular remodeling both <em>in vitro</em> and in challenging diabetic wound models, opening new avenues for next-generation intelligent materials and biomedical devices.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101901"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142678451","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Mixed-dimensional heterojunction by 3D CdS nanowire arrays bridged with 2D WSe2 for ultrafast photoelectric gas sensor 三维CdS纳米线阵列与二维WSe2桥接用于超快光电气体传感器的混维异质结

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.008

Wei Zheng , Guocai Lu , Xianghong Liu , Shilei Fan , Yinhua Hu , Nicola Pinna , Jun Zhang

{"title":"Mixed-dimensional heterojunction by 3D CdS nanowire arrays bridged with 2D WSe2 for ultrafast photoelectric gas sensor","authors":"Wei Zheng , Guocai Lu , Xianghong Liu , Shilei Fan , Yinhua Hu , Nicola Pinna , Jun Zhang","doi":"10.1016/j.matt.2024.11.008","DOIUrl":"10.1016/j.matt.2024.11.008","url":null,"abstract":"<div><div>Heterojunctions are of essential importance for electronic sensors due to their unique properties at the junctions. However, a planar junction made of two-dimensional (2D) materials commonly suffers from slow response and irreversible recovery because of slow physisorption and desorption rates. Herein, we present a unique design of a mixed-dimensional heterojunction built from patterned growth of 3D n-type CdS nanowire arrays and p-type 2D WSe<sub>2</sub> nanosheets for photoelectric gas sensors. This heterojunction sensor showed highly selective and reversible responses to NO<sub>2</sub> and NH<sub>3</sub> with detection limits of 60 and 54 ppb, respectively, under UV illumination at room temperature. Notably, the sensor exhibited an ultrafast response time of less than 1 s to 1 ppm NO<sub>2</sub> and NH<sub>3</sub>, which outperforms most previous reports. The hybrid junction structure proposed herein will pave the way for engineering new electronic devices from a broad selection of materials to achieve improved sensing performances at room temperature.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101914"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142763890","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Smart liquid crystal elastomer fibers

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.101950

Jiazhe Ma , Zhongqiang Yang

引用次数: 0

Direct observation of structural disorder effects on iridium dioxide nanocrystal dissolution 直接观察结构紊乱对二氧化铱纳米晶体溶解的影响

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.003

Matteo Fratarcangeli , S. Avery Vigil , Ziqing Lin , Conner J. Soderstedt , Ivan A. Moreno-Hernandez

{"title":"Direct observation of structural disorder effects on iridium dioxide nanocrystal dissolution","authors":"Matteo Fratarcangeli , S. Avery Vigil , Ziqing Lin , Conner J. Soderstedt , Ivan A. Moreno-Hernandez","doi":"10.1016/j.matt.2024.11.003","DOIUrl":"10.1016/j.matt.2024.11.003","url":null,"abstract":"<div><div>The current state-of-the-art electrocatalyst for the oxygen evolution reaction (OER) is iridium dioxide, providing a compromise between activity and stability. The low elemental abundance of iridium, coupled with the dissolution of iridium dioxide under operating conditions, prevents the global-scale implementation of electrolyzers. Understanding the origin of iridium dioxide dissolution at the nanoscale is crucial for the development of next-generation electrocatalysts that efficiently utilize iridium to meet energy demands. Herein, we report the influence of structural disorder, modulated by synthesis temperature, on the nanoscale dissolution dynamics and electrocatalytic activity of iridium dioxide nanocrystals. Our observations of dissolution on single nanocrystals revealed that structural disorder destabilized the OER-inactive (111) facets and had no substantial effect on the stability of the OER-active (110) facets. These findings highlight the importance of understanding nanoscale dynamic restructuring and suggest the possibility of developing highly active and stable (110)-based iridium dioxide electrocatalysts for water oxidation.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101909"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142713356","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Artificially engineered red blood cells for universal blood transfusion

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.029

Ying Zhang , Jun Xu , Ben Wang

引用次数: 0

Polyfunctional eutectogels with multiple hydrogen-bond-shielded amorphous networks for soft ionotronics

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2025.101993

Yizhe Shao, Chao Dang, Haobo Qi, Ziyang Liu, Haoran Pei, Tongqing Lu, Wei Zhai

引用次数: 0

Bio-inspiration or bio-obfuscation? 生物启发还是生物混淆？

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.10.012

Steve Cranford

引用次数: 0

In-plane compressive strain stabilized formamidinium-based perovskite 面内压缩应变稳定的甲脒基钙钛矿

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.014

Xuechun Sun , Pengju Shi , Jiahui Shen , Jichuang Shen , Liuwen Tian , Jiazhe Xu , Qingqing Liu , Yuan Tian , Donger Jin , Xiaohe Miao , Jingjing Xue , Rui Wang

{"title":"In-plane compressive strain stabilized formamidinium-based perovskite","authors":"Xuechun Sun , Pengju Shi , Jiahui Shen , Jichuang Shen , Liuwen Tian , Jiazhe Xu , Qingqing Liu , Yuan Tian , Donger Jin , Xiaohe Miao , Jingjing Xue , Rui Wang","doi":"10.1016/j.matt.2024.11.014","DOIUrl":"10.1016/j.matt.2024.11.014","url":null,"abstract":"<div><div>Compressive strain is often considered as a key factor in stabilizing formamidinium (FA)-based perovskites. However, the compression along which direction stabilizes perovskite remains unclear due to the presence of non-uniform strain within the material. Here, we introduce a metal encapsulation method to apply compressive strain along the in-plane or out-of-plane direction of perovskite film. According to the grazing-incidence wide-angle X-ray scattering (GIWAXS) results, in-plane compression enhances the stability of perovskites, whereas out-of-plane compression has a detrimental effect. Specifically, out-of-plane compression can lead to the formation of an inactive δ-phase, which compromises the stability of the perovskite. Finally, we develop a general process to integrate in-plane compression into perovskite solar cell (PSC) devices, thereby improving their stability. Our study clarifies the mechanism by which compressive strain affects perovskite stability, offering valuable guidance for strain engineering to optimize perovskite performance.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101920"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142793479","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Biomimetic conductor from viscoelastic polymer composite gels for smart soft electronics 用于智能软电子器件的粘弹性聚合物复合凝胶仿生导体

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.022

Jingyun Lan , Yan Peng , Hao Peng , Jiuyang Zhang

{"title":"Biomimetic conductor from viscoelastic polymer composite gels for smart soft electronics","authors":"Jingyun Lan , Yan Peng , Hao Peng , Jiuyang Zhang","doi":"10.1016/j.matt.2024.11.022","DOIUrl":"10.1016/j.matt.2024.11.022","url":null,"abstract":"<div><div>The neural system in living organisms has achieved highly optimized features in perception, response, and learning, which are extremely desirable for modern soft robots. Today’s soft robots generally utilize flexible conductors to fabricate their sensory systems. Such a system usually exhibits instantaneous response behaviors upon external stimuli without signal persistence or environmental adaptability to protect living organisms. This work provides a bio-conductor based on viscoelastic polymer gels and metal microfibers. The flexible bio-conductor can achieve critical sensory persistence and adaptation via efficient control over the electrical conductive network through relaxation of metal microfibers and polymer chains. The signal transmission in the bio-conductor can be conveniently mediated through the parameters of the composites, exhibiting unique responses to diverse environmental conditions. An aerial vehicle integrated with the bio-conductor, and a microcontroller unit (MCU) was successfully fabricated for a robot system to simulate the signal transmission, processing, and response in biological nervous systems.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101928"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142832468","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0