Joule最新文献_第5页

Acidified gas phase enables long-term stable CO2 electrolysis 酸化气相可实现长期稳定的CO2电解

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102095

Yixin Chen , Xingyu Ding , Zuxin Wen , Xianbiao Fu

引用次数: 0

Efficient electroreduction of CO2 to C3+ chemicals by a formaldehyde condensation mechanism 用甲醛缩合机理将CO2有效电还原为C3+化学物

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102094

Yuanyuan Xue , Gengfeng Zheng

引用次数: 0

Diagnostic-free onboard battery health assessment 无诊断的机载电池健康评估

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102010

Yunhong Che , Vivek N. Lam , Jinwook Rhyu , Joachim Schaeffer , Minsu Kim , Martin Z. Bazant , William C. Chueh , Richard D. Braatz

{"title":"Diagnostic-free onboard battery health assessment","authors":"Yunhong Che , Vivek N. Lam , Jinwook Rhyu , Joachim Schaeffer , Minsu Kim , Martin Z. Bazant , William C. Chueh , Richard D. Braatz","doi":"10.1016/j.joule.2025.102010","DOIUrl":"10.1016/j.joule.2025.102010","url":null,"abstract":"<div><div><span>Diverse usage patterns induce complex and variable aging behaviors in lithium-ion batteries, complicating accurate health diagnosis and prognosis. In this work, we leverage portions of operational measurements from charging or dynamic discharging in combination with an interpretable machine learning model to enable rapid, onboard battery health diagnostics and prognostics without offline diagnostic testing and access to </span>historical data<span>. We integrate mechanistic constraints derived from differential voltage analysis within an encoder-decoder to extract electrode health states in a physically interpretable latent space, which enables improved reconstruction of the degradation path with onboard aging mechanisms tracking. The diagnosis model can be flexibly applied across diverse applications with slight fine-tuning. We demonstrate the model’s versatility by applying it to three battery-cycling datasets consisting of 422 cells under different operating conditions, with a mean absolute error of less than 2% for health diagnosis under varying conditions, highlighting the utility of an interpretable, diagnostic-free model.</span></div></div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"9 8","pages":"Article 102010"},"PeriodicalIF":35.4,"publicationDate":"2025-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144516176","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Bottlenecks of commercializing anion exchange membranes for energy devices 能源装置用阴离子交换膜商业化的瓶颈

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102051

Wanjie Song , Xiaolin Ge , Liang Wu , Zhengjin Yang , Tongwen Xu

引用次数: 0

Monolithic integration of radiative cooling and solar heating functionalities by laser-induced pyrolysis 激光诱导热解的辐射冷却和太阳能加热功能的整体集成

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102007

Yeongju Jung , Seongmin Jeong , Gyu Heo , Kyung Rok Pyun , Seok Hwan Choi , Junhyuk Bang , Jae Gun Lee , Hongchan Kim , Jaeho Shin , Sukjoon Hong , Jinwoo Lee , Daeyeon Won , Jaeman Song , Seung Hwan Ko

{"title":"Monolithic integration of radiative cooling and solar heating functionalities by laser-induced pyrolysis","authors":"Yeongju Jung , Seongmin Jeong , Gyu Heo , Kyung Rok Pyun , Seok Hwan Choi , Junhyuk Bang , Jae Gun Lee , Hongchan Kim , Jaeho Shin , Sukjoon Hong , Jinwoo Lee , Daeyeon Won , Jaeman Song , Seung Hwan Ko","doi":"10.1016/j.joule.2025.102007","DOIUrl":"10.1016/j.joule.2025.102007","url":null,"abstract":"<div><div>Conventional thermal management systems contribute significantly to environmental challenges, motivating the exploration of zero-energy techniques such as radiative cooling and solar heating. In this study, an innovative strategy is introduced to transform transparent polydimethylsiloxane into a versatile material via laser-induced pyrolysis. By precisely controlling laser intensity, the material is engineered for multi-thermal management, exhibiting high reflectivity and thermal emission for effective cooling under high-energy processing and strong solar absorption for notable heating under low-energy conditions. Simulation results indicate that applying this material to building roofs could reduce annual energy consumption by up to 26.5%. Moreover, its capability to form Janus structures and all-laser-patterned solar thermoelectric devices highlights its potential for sustainable technologies. This work represents a pioneering strategy in sustainable thermal management for cooling and heating, demonstrating a novel use of a monolith material and a facile fabrication technique and offering a promising solution to global environmental challenges.</div></div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"9 8","pages":"Article 102007"},"PeriodicalIF":35.4,"publicationDate":"2025-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144516180","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Deuterium-substituted cations enhance perovskite solar cell efficiency and stability 氘取代阳离子提高钙钛矿太阳能电池的效率和稳定性

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102031

Jiazhi Meng , Yu Gao , Junnan Hu , Chengcheng Wu , Yuan Li , Si-Wei Zhang , Yuou Chen , Ross A. Kerner , Jing Ma , Yang Shen , Xuan Zhang , Feiyu Kang , Barry P. Rand , Guodan Wei

{"title":"Deuterium-substituted cations enhance perovskite solar cell efficiency and stability","authors":"Jiazhi Meng , Yu Gao , Junnan Hu , Chengcheng Wu , Yuan Li , Si-Wei Zhang , Yuou Chen , Ross A. Kerner , Jing Ma , Yang Shen , Xuan Zhang , Feiyu Kang , Barry P. Rand , Guodan Wei","doi":"10.1016/j.joule.2025.102031","DOIUrl":"10.1016/j.joule.2025.102031","url":null,"abstract":"<div><div><span><span><span>Halide </span>perovskite solar cells<span> with mixed-cation compositions often face instabilities under continuous illumination due to the </span></span>deprotonation<span> of methylammonium (CH</span></span><sub>3</sub>NH<sub>3</sub><sup>+</sup><span>, MA</span><sup>+</sup>) cations. To address this, we systematically evaluate the partial and complete deuteration of MA<sup>+</sup><span><span> cations. This approach inhibits deprotonation and degradation, reduces the formation energy of the </span>perovskite<span> phase, improves grain growth, passivates defects, and restrains ion migration. As a result, perovskite solar cells incorporating this deuteration strategy achieve exceptional performance, including a high fill factor (FF) of 82.6% and a power conversion efficiency (PCE) of 25.6%. Their modules with a device area of 56 cm</span></span><sup>2</sup><span> demonstrate remarkable stability, maintaining over 93.7% of their initial PCE after 1,000 h at the maximum power point under continuous illumination at 40°C. This novel deuteration strategy presents a promising approach to enhance both the efficiency and stability of perovskite solar cells.</span></div></div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"9 8","pages":"Article 102031"},"PeriodicalIF":35.4,"publicationDate":"2025-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144578101","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

A rational lens on prioritizing emission reductions via removal versus abatement 一个理性的视角，优先考虑通过移除和减少来减少排放

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102040

Matthias Mersch , Marwan Sendi , Christos N. Markides , Niall Mac Dowell

{"title":"A rational lens on prioritizing emission reductions via removal versus abatement","authors":"Matthias Mersch , Marwan Sendi , Christos N. Markides , Niall Mac Dowell","doi":"10.1016/j.joule.2025.102040","DOIUrl":"10.1016/j.joule.2025.102040","url":null,"abstract":"<div><div>Matthias Mersch is a postdoctoral researcher in the Clean Energy Processes (CEP) Laboratory in the Department of Chemical Engineering at Imperial College London. He holds an MSc in energy engineering from RWTH Aachen University and a PhD in chemical engineering from Imperial College London, working in collaboration with the Centre for Environmental Policy. Matthias works at the interface between detailed technology modeling and whole-energy system optimization.</div><div>Marwan Sendi is a senior engineer in the Life Cycle Assessment Group at Saudi Aramco’s Technology Strategy and Planning Department, where he focuses on technology assessment and net-zero strategy. He holds a PhD from Imperial College London, where his research centered on geospatial modeling of chemical processes and energy systems, including direct air capture systems.</div><div>Christos N. Markides is a professor of clean energy technologies and head of the Clean Energy Processes (CEP) Laboratory at Imperial College London, with an interest in the development of next-generation energy technologies and systems. He is editor-in-chief of the journal <em>Applied Thermal Engineering</em> and founding editor-in-chief of the journal <em>AI Thermal Fluids</em>. Professor Markides has authored over 400 journal articles and books.</div><div>Niall Mac Dowell is a professor of future energy systems at Imperial College London. He is a chartered engineer and is a fellow of both the Institution of Chemical Engineers and the Royal Society of Chemistry. Professor Mac Dowell has 20 years of experience in the energy transition and has published more than 200 books, papers, and technical reports on this subject. He has consulted widely for a range of public and private organizations who are active in implementing the net-zero transition.</div></div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"9 8","pages":"Article 102040"},"PeriodicalIF":35.4,"publicationDate":"2025-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144652589","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Large language models for batteries 用于电池的大型语言模型

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102037

Wenhua Zuo , Huihuo Zheng , Tanjin He , Venkatram Vishwanath , Maria K.Y. Chan , Rick L. Stevens , Khalil Amine , Gui-Liang Xu

{"title":"Large language models for batteries","authors":"Wenhua Zuo , Huihuo Zheng , Tanjin He , Venkatram Vishwanath , Maria K.Y. Chan , Rick L. Stevens , Khalil Amine , Gui-Liang Xu","doi":"10.1016/j.joule.2025.102037","DOIUrl":"10.1016/j.joule.2025.102037","url":null,"abstract":"<div><div>Large language models (LLMs) are advanced artificial intelligence systems capable of solving diverse tasks using language, reasoning, and external tools. Despite their growing deployment in academia and industry, their potential remains underexplored in battery research. This review presents a comprehensive overview of existing and emerging applications of LLMs in the battery field, addressing two critical questions: what can LLMs offer to support battery-related tasks, and how can more effective models be developed for this purpose? We begin by outlining the principles of LLMs and criteria for selecting appropriate models and tools for battery research and development. We then explore the roles of LLMs in text mining, data interpretation, and the development of intelligent battery systems. In parallel, we discuss technical challenges, such as data standardization and sharing, model evaluation, and tool integration. Finally, we propose future research directions with short-, medium-, and long-term goals and highlight more broad perspectives for connecting experts and cross-disciplinary collaborations.</div></div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"9 8","pages":"Article 102037"},"PeriodicalIF":35.4,"publicationDate":"2025-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144863287","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Bio-morphogenesis relieves pressure in all-solid-state batteries 生物形态发生减轻了全固态电池的压力

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102093

Myeong Gyun Nam , Yuan Yang

引用次数: 0

A low-cost, fluorine-free electrolyte for improved sodium batteries 用于改进钠电池的低成本、无氟电解质

IF 35.4 1区材料科学

Joule Pub Date : 2025-08-20 DOI: 10.1016/j.joule.2025.102045

Evan Summerwill Flitz , Nicholas Ryan Singstock , Seoung-Bum Son , Cooper Tezak , Marcos Lucero , Xiaolin Li , Charles Musgrave , Chunmei Ban

{"title":"A low-cost, fluorine-free electrolyte for improved sodium batteries","authors":"Evan Summerwill Flitz , Nicholas Ryan Singstock , Seoung-Bum Son , Cooper Tezak , Marcos Lucero , Xiaolin Li , Charles Musgrave , Chunmei Ban","doi":"10.1016/j.joule.2025.102045","DOIUrl":"10.1016/j.joule.2025.102045","url":null,"abstract":"<div><div><span><span>Sodium batteries are an attractive alternative to lithium-ion technologies due to sodium’s lower cost and natural abundance—over 1,000 times greater than lithium, comprising approximately 2.4% of the Earth’s crust. However, most current electrolytes rely on fluorine-containing components, which raise economic and environmental concerns. This study explores fluorine-free, borate-based electrolytes that offer improved cycling stability and significant cost and sustainability benefits. We demonstrate stable </span>sodium<span><span> metal stripping and plating on aluminum foil, enabling anode-free cell configurations with over 50% capacity retention after 700 cycles. Spectroscopic and </span>electrochemical analyses<span> reveal the effects of solvents and salt composition on </span></span></span>solvation<span><span>, ionic conductivity, and </span>oxidative stability<span>. In full-cell configurations, the fluorine-free electrolyte maintains more than 98% capacity retention after 400 cycles. These findings represent a critical step toward the development of cost-effective, environmentally friendly, and high-performance sodium battery systems suitable for future electrification.</span></span></div></div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"9 8","pages":"Article 102045"},"PeriodicalIF":35.4,"publicationDate":"2025-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144578521","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0