Advanced Functional Materials最新文献_第8页

Polyphenol-Regulated Bimetallic Artificial Metalloproteinases with Broad-Spectrum RONS Scavenging Activities for Diabetic Wound Repair

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202501438

Minghui Ou, Ke Zhang, Guangneng Liao, Zhiwei Wei, Li Yang, Shengqiu Chen, Xinnian Fan, Yi Xie, Changsheng Zhao

{"title":"Polyphenol-Regulated Bimetallic Artificial Metalloproteinases with Broad-Spectrum RONS Scavenging Activities for Diabetic Wound Repair","authors":"Minghui Ou, Ke Zhang, Guangneng Liao, Zhiwei Wei, Li Yang, Shengqiu Chen, Xinnian Fan, Yi Xie, Changsheng Zhao","doi":"10.1002/adfm.202501438","DOIUrl":"https://doi.org/10.1002/adfm.202501438","url":null,"abstract":"Although numerous enzyme-mimicking nanomaterials have been developed to regulate the highly reactive oxygen species (ROS)-rich microenvironment of diabetic wounds for improving its healing, the poor broad-spectrum ROS-scavenging capacity and biological toxicity resulting from side reactions of nanomaterials still require improvement. To tackle these challenges, a polyphenol-mediated copper-bismuth bimetallic artificial metalloproteinases, CuBi-TA@BSA, based on a protein-scaffold design strategy, is conceptually engineered. The Bi and polyphenols can cooperatively enhance the loading capacity of Cu ions and regulate their coordination microenvironment within the BSA scaffold. The CuBi-TA@BSA exhibits remarkable scavenging activity against various ROS via effectively donating electrons, as well as the reaction pathway specificity of catalytic H2O2 decomposition without POD-like activity. Moreover, in vitro and in vivo studies further confirm that the CuBi-TA@BSA can protect cells from oxidative damage, inhibit the onset and progression of inflammation, and promote diabetic wound healing. This work presents a simple strategy for biocatalysts to effectively scavenge ROS and accelerate the diabetic wound-healing process, also provides a strategy for designing artificial metalloproteinases for antioxidative therapy.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"32 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745520","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Homogenized Current Collector Surface for High Reversibility Anode-Free Zinc Metal Batteries

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202504042

Yuanhao Shen, Yuzhou Jiao, Chenyang Wang, Juan Zou, Peng Li, Shengli Chen, Mengqi Zeng, Lei Fu

{"title":"Homogenized Current Collector Surface for High Reversibility Anode-Free Zinc Metal Batteries","authors":"Yuanhao Shen, Yuzhou Jiao, Chenyang Wang, Juan Zou, Peng Li, Shengli Chen, Mengqi Zeng, Lei Fu","doi":"10.1002/adfm.202504042","DOIUrl":"https://doi.org/10.1002/adfm.202504042","url":null,"abstract":"The advancement of anode-free batteries (AFBs) presents a promising approach to enhance the energy density of secondary batteries. Nonetheless, a prevalent challenge associated with AFBs is the low Coulombic efficiency (CE), which arises from the surface inhomogeneity of the current collector. Conventional strategies load a variety of metalophile materials on its surface to enhance CE. However, without the solution of the intrinsic inhomogeneity of the current collector, the modification cannot be absolutely uniform, resulting in defect generation and even interface failures. Herein, anode-free zinc metal batteries employing copper foil as a representative are used to eliminate the inhomogeneity of the oxide layer on the commercial copper foil surface while simultaneously adhering a homogenized thin chlorine (Cl) atomic layer with 100% conformal coverage (modified-Cu) by a one-step method. The homogenized Cl atomic layer exhibits a 3D diffusion for Zn atoms and induces dense growth of Zn (100) crystal plane, promoting reversible Zn plating/stripping. Additionally, the modified-Cu||ZnxMnO2 anode-free full battery exhibits superior cycling stability (500 cycles with 80% capacity retention). In addition to this, meter-level modified-Cu is produced in large quantities through a roll-to-roll system. This innovative strategy for constructing homogenized surfaces can promote the development of high-energy-density anode-free metal batteries toward practical applications.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"8 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745721","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Helical Phononic Modes Induced by a Screw Dislocation

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202417313

Yun Zhou, Robert Davis, Li Chen, Erda Wen, Prabhakar Bandaru, Daniel Sievenpiper

引用次数: 0

Recent Progress on Flexible Silicon Nanomembranes for Advanced Electronics and Optoelectronics

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202502191

Ziyu Zhang, Yang Wang, Tianjun Cai, Binmin Wu, Bofan Hu, Xing Li, Enming Song, Gaoshan Huang, Ziao Tian, Zengfeng Di, Yongfeng Mei

{"title":"Recent Progress on Flexible Silicon Nanomembranes for Advanced Electronics and Optoelectronics","authors":"Ziyu Zhang, Yang Wang, Tianjun Cai, Binmin Wu, Bofan Hu, Xing Li, Enming Song, Gaoshan Huang, Ziao Tian, Zengfeng Di, Yongfeng Mei","doi":"10.1002/adfm.202502191","DOIUrl":"https://doi.org/10.1002/adfm.202502191","url":null,"abstract":"Silicon nanomembranes, an emerging material with ultrathin thickness, combine the electrical properties of semiconductors with the flexibility that bulk materials lack. These nanomembranes can impart enhanced functionality to devices, supporting development needs for next-generation technologies “more-than-Moore” Law. In recent years, as research of fabrication techniques and fundamental principles have advanced, the focus of silicon nanomembrane studies has evolved from material preparation and component processing to functionalization and system-level integration. This review begins with an overview of silicon nanomembrane preparation methods and formation principles. In terms of device advancements and applications, developments in optoelectronic devices, sensors, biomedicine, energy harvesting, and integrated circuits are covered. Finally, the review discusses the current challenges in silicon nanomembrane technology and the potential of silicon nanomembrane devices and systems in future optoelectronics, biomedicine, energy harvesting, and advanced integrated circuit architectures.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"22 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745766","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

A Bipartite Synergistic Strategy for All-Weather Sodium-Ion Fiber Supercapacitor with Excellent Energy Density and Temperature Adaptability 具有优异能量密度和温度适应性的全天候钠离子纤维超级电容器的两方协同策略

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202506540

Fuquan Ma, Ling Li, Xiumei Chen, Xuexia He, Qi Li, Jie Sun, Ruibin Jiang, Zhibin Lei, Zong-Huai Liu

{"title":"A Bipartite Synergistic Strategy for All-Weather Sodium-Ion Fiber Supercapacitor with Excellent Energy Density and Temperature Adaptability","authors":"Fuquan Ma, Ling Li, Xiumei Chen, Xuexia He, Qi Li, Jie Sun, Ruibin Jiang, Zhibin Lei, Zong-Huai Liu","doi":"10.1002/adfm.202506540","DOIUrl":"https://doi.org/10.1002/adfm.202506540","url":null,"abstract":"Sodium-ion fiber supercapacitor (AFSIC) are promising candidates for wearable devices. However, their practical implementation is hindered by the absence of cathodes with fast Na-ion diffusion kinetics to match the anode and the poor temperature adaptability of conventional electrolytes. To address these challenges, a carbon-coated NaV3O8 nanowires (NaNVO@C10) with low diffusion energy barriers of Na-ion are designed, enabling rapid and reversible Na-ion intercalation/de-intercalation. By leveraging the liquid crystalline phase induced characteristic of graphene oxide (GO), NaNVO@C10/rGO fiber cathode is fabricated using wet spinning. This fiber achieves a large volume capacitive of 565 F cm−3. In parallel, a novel dual co-solvent electrolyte (SLPHNa) is developed by introducing sulfolane and ethylphosphate as co-solvent. This electrolyte synergistically reshape the Na-ion solvation sheath, thereby improving the cycle stability and enhancing temperature adaptability from −60 to 80 °C of AFSIC. The resulting NaNVO@C10/rGO//MXene AFSIC exhibits a remarkable energy density of 35 mWh cm−3, and maintains 9.3 mWh cm−3 even at −60 °C, along with an ultra-long lifespan of 10 000 cycles under all-weather condition. Moreover, the device maintains 82% of its initial capacitance after 1000 bending cycles, showing excellent mechanical durability. This work offers new insights into the development of high performance all-weather sodium-ion fiber supercapacitors.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"27 19 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745515","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Dragonfly Wing-Inspired Reticular Hierarchical Structure Enables Strong and Tough Supramolecular Elastomers

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202506282

Qingchuang Lu, Lei Duan, Yao Liu, Chenrui Zhang, Zebo Zhang, Zhenyang Luo, Cheng-Hui Li, Yanlong Luo

{"title":"Dragonfly Wing-Inspired Reticular Hierarchical Structure Enables Strong and Tough Supramolecular Elastomers","authors":"Qingchuang Lu, Lei Duan, Yao Liu, Chenrui Zhang, Zebo Zhang, Zhenyang Luo, Cheng-Hui Li, Yanlong Luo","doi":"10.1002/adfm.202506282","DOIUrl":"https://doi.org/10.1002/adfm.202506282","url":null,"abstract":"Dragonfly wings possess exceptionally high strength, toughness, and fatigue resistance due to their unique hierarchical structure from the micro to macro scale. Inspired by this, mismatched supramolecular interactions (MMSIs) are introduced into the dynamic acylsemicarbazide groups, constructing an interconnected hybrid network of soft and hard segments in the SPUU-DS elastomer. This design, featuring a dense array of hydrogen bonds, achieves exceptional mechanical properties: a true stress at breaks of 1.1 GPa comparable to that of typical spider silk (0.8–1.5 GPa); toughness of 325.54 MJ m−3, twice that of typical spider silk (≈160 MJ m−3); and a fracture energy of 232.83 kJ m−2, surpassing many metals and alloys. Furthermore, a monitoring device with a “hamburger” structure is developed by integrating SPUU-DS with a conductive graphene film. When placed inside a tire, this device enhances the tire's puncture resistance by approximately twofold. By correlating the resistance signals with puncture angles, the system enables the detection of damage at various locations on the tire, allowing for timely repair of damage and preventing traffic accidents. This novel biomimetic approach, inspired by dragonfly wings, provides valuable insights for designing healable elastomers with superior mechanical properties.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"50 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745332","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Ultrafast Room-Temperature Nanofabrication via Ozone-Based Gas-Phase Metal-Assisted Chemical Etching for High-Performance Silicon Photodetectors

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202502010

Hyein Cho, Yejin Han, Geonhwi Kim, Jihwan Jeong, Seongmin Lee, Yebin Ahn, Sang Beom Hong, Soohyeok Park, Inkyeong Park, So Eun Jang, Duck Hyun Youn, Han-Don Um

{"title":"Ultrafast Room-Temperature Nanofabrication via Ozone-Based Gas-Phase Metal-Assisted Chemical Etching for High-Performance Silicon Photodetectors","authors":"Hyein Cho, Yejin Han, Geonhwi Kim, Jihwan Jeong, Seongmin Lee, Yebin Ahn, Sang Beom Hong, Soohyeok Park, Inkyeong Park, So Eun Jang, Duck Hyun Youn, Han-Don Um","doi":"10.1002/adfm.202502010","DOIUrl":"https://doi.org/10.1002/adfm.202502010","url":null,"abstract":"High-aspect-ratio silicon nanostructures are essential building blocks for next-generation electronics, but their fabrication remains challenging due to process complexities and structural instabilities. Here, this study presents an unprecedented gas-phase metal-assisted chemical etching (GP-MACE) strategy using high-purity ozone (O3) as an oxidizing agent. This approach achieves remarkable etching rates of ≈1 µm min−1 at room temperature—70 times faster than conventional oxygen-based processes—while maintaining superior structural integrity. The enhanced oxidation potential of O3 (E0 = 2.08 V) enables precise control over the etching mechanism, yielding vertical nanowires with minimal surface defects, as confirmed by the unity critical-depth-to-maximum-depth ratio and three-fold reduction in surface porosity compared to liquid-phase processes. Leveraging this exceptional structural quality, it demonstrates high-performance photodetectors utilizing a doping-free Al2O3/Si core-shell architecture. The conformal Al2O3 coating induces an inversion layer that functions analogously to a p-n junction while simultaneously providing surface passivation, enabling efficient carrier separation without conventional thermal doping. The photodetector exhibits superior responsivity (0.45 A W−1) and stable switching characteristics even under zero-bias conditions. This room-temperature nanofabrication strategy, combining unprecedented etching rates with superior structural control, provides a promising platform for industrial-scale manufacturing of high-performance nanodevices.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"58 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745725","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Optimized Crystallization of CsPbI2Br Films through the Incorporation of H2O for High-Efficiency All-Inorganic Perovskite/Organic Tandem Solar Cell

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202502966

Kun Lang, Jia Xu, Huifang Han, Huijing Liu, Yao Fu, Xueqi Zhang, Zhengxu Sun, Qianzheng Shi, Zhan'ao Tan, Jianxi Yao

{"title":"Optimized Crystallization of CsPbI2Br Films through the Incorporation of H2O for High-Efficiency All-Inorganic Perovskite/Organic Tandem Solar Cell","authors":"Kun Lang, Jia Xu, Huifang Han, Huijing Liu, Yao Fu, Xueqi Zhang, Zhengxu Sun, Qianzheng Shi, Zhan'ao Tan, Jianxi Yao","doi":"10.1002/adfm.202502966","DOIUrl":"https://doi.org/10.1002/adfm.202502966","url":null,"abstract":"Among all-inorganic perovskites, CsPbI2Br possesses excellent photovoltaic performance, intrinsic thermal stability and suitable bandgap and superior phase-stability, demonstrating large application potential for single-junction perovskite solar cells (PSCs) and perovskite/organic tandem solar cells (TSCs). However, a critical challenge persists in the effective control of the crystallization process of the CsPbI2Br film, as inadequate crystallization can result in a substantial decrease in the photoelectric efficiency of solar cells. Herein, a simple approach utilizing a small amount of H2O additive is introduced to optimize the crystallization process of CsPbI2Br film. Specifically, the introduction of water facilitates the formation of numerous CsPbI2Br seed crystals within the precursor solution, promoting subsequent Ostwald ripening process of the perovskite film. Additionally, the presence of water enhances the desorption of DMSO from CsPbI2Br, further improving overall crystallization. As a result, a CsPbI2Br-basedPSC exhibits a high power conversion efficiency (PCE) of 16.7% and an open-circuit voltage (VOC) of 1.36 V. By integrating these CsPbI2Br-based front sub-cells with narrow-bandgap PM6:Y6-based rear sub-cells, a high PCE of 23.21% and VOC of 2.17 V is achieved, illustrating the potential of TSCs for high-efficiency tandem solar cells. Furthermore, the unencapsulated TSCs display superior stability under ambient air conditions and operation.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"183 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745521","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Chloride-Mediated Electron Buffering on Ni-Fe Anodes for Ampere-Level Alkaline Seawater Electrolysis

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202504872

Qian Niu, Fei-Yue Gao, Xiaogang Sun, Yao Zheng, Shi-Zhang Qiao

{"title":"Chloride-Mediated Electron Buffering on Ni-Fe Anodes for Ampere-Level Alkaline Seawater Electrolysis","authors":"Qian Niu, Fei-Yue Gao, Xiaogang Sun, Yao Zheng, Shi-Zhang Qiao","doi":"10.1002/adfm.202504872","DOIUrl":"https://doi.org/10.1002/adfm.202504872","url":null,"abstract":"In water electrolysis, the long-term stability of anodes is compromised by their degradation under oxidative conditions. This issue becomes more pronounced in seawater electrolysis, where the natural chloride ion (Cl−) induces the chlorine evolution reaction (ClER) to produce corrosive byproducts. Herein, a series of small organic molecules (SOMs), featuring an aromatic carbon ring with para-positioned carbonyl groups, are integrated with the conventional nickel-iron (Ni-Fe) based anode. This integration triggers a unique electron buffering effect to address anode degradation in natural seawater-based electrolytes. It is found that preferential adsorption of Cl− onto SOMs prevents its direct interaction with metal active sites. Furthermore, SOM-Cl serving as an electron buffering group significantly reduces the dissolution of Fe sites under the highly oxidative environment. As a result, the SOM-Cl-engineered anode enhances oxygen evolution activity by ≈1.7 times in seawater compared to pure water. In addition, the rationally designed anode works stably for over 200 h at a high current density of 1.3 A cm−2 in an alkaline seawater electrolyzer (ASE).","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"122 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745523","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Rapid Synthesis and Recycling of Carbonized Wood Catalyst Decorated with Co Nanoparticles for High-Efficiency Degradation of Rhodamine B 用 Co 纳米粒子装饰的碳化木催化剂的快速合成与循环利用，实现罗丹明 B 的高效降解

IF 19 1区材料科学

Advanced Functional Materials Pub Date : 2025-04-01 DOI: 10.1002/adfm.202420933

Pengyu Xing, Yaoxing Wang, Xueqin Fan, Xueqi Li, Peiru Wang, Quankuo Zhang, Qiuyu Du, Yanjun Xie, Ran Yin, Wentao Gan

{"title":"Rapid Synthesis and Recycling of Carbonized Wood Catalyst Decorated with Co Nanoparticles for High-Efficiency Degradation of Rhodamine B","authors":"Pengyu Xing, Yaoxing Wang, Xueqin Fan, Xueqi Li, Peiru Wang, Quankuo Zhang, Qiuyu Du, Yanjun Xie, Ran Yin, Wentao Gan","doi":"10.1002/adfm.202420933","DOIUrl":"https://doi.org/10.1002/adfm.202420933","url":null,"abstract":"Developing catalysts for purifying organic pollutants in wastewater is significant for environmental remediation. Herein, a high-temperature (1000 K) thermal shock (HTS) method is employed to rapidly synthesize a self-supporting catalyst consisting of cobalt (Co) nanoparticles (NPs) and carbonized wood (CW) within 2 s. Thanks to the porous structure of wood and uniformly distributed Co NPs, the wood catalyst exhibits excellent catalytic activity, achieving over 99% removal of 25 mg L−1 Rhodamine B (RhB) within 10 min using the activated peroxymonosulfate advanced oxidation processes, while the leaching rate of Co ions is less than 1 mg L−1. As a proof of concept, a continuous filter is constructed based on the CW catalysts for efficient RhB degradation in flowing water. With a flow rate of 20 mL min−1, it maintains the removal of over 90% of RhB from wastewater for a duration of 2 h. Benefiting from the rapid synthesis of HTS method, a “deactivation-regeneration” strategy is proposed that extends the recycling cycles of wood catalysts to 20 times, surpassing most reported Co-based catalysts. Derived from renewable wood materials, this catalyst offers advantages of high efficiency, low cost, simple synthesis, and durability, showing great potential for application in various fields including water treatment, electrocatalytic conversion, and energy storage.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"19 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143745522","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0