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Counter-Anion-Engineered Solid-State Polymer Electrolytes for Vertically Stacked Artificial Synapses With Configurable Plasticity 具有可配置可塑性的垂直堆叠人工突触的反阴离子工程固态聚合物电解质
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79154
Chiho Youn,Seonkwon Kim,Yeongnam Ko,Jong Chan Shin,Suhyeon Kim,Jihyeon You,Jina Lee,Geon-Soon Jang,Sang-Young Lee,Ki Chul Kim,Minjae Lee,Jeong Ho Cho
{"title":"Counter-Anion-Engineered Solid-State Polymer Electrolytes for Vertically Stacked Artificial Synapses With Configurable Plasticity","authors":"Chiho Youn,Seonkwon Kim,Yeongnam Ko,Jong Chan Shin,Suhyeon Kim,Jihyeon You,Jina Lee,Geon-Soon Jang,Sang-Young Lee,Ki Chul Kim,Minjae Lee,Jeong Ho Cho","doi":"10.1002/adfm.79154","DOIUrl":"https://doi.org/10.1002/adfm.79154","url":null,"abstract":"Counter-anion engineering of solid-state cationic polyurethane electrolytes regulates Li+ transport to realize configurable long-term and short-term synaptic plasticity. Vertically stacked artificial synapses integrate these complementary functions to implement reversible AND/OR logic and multiply–accumulate (MAC) operations, providing a scalable solid-state platform for compact, multifunctional neuromorphic hardware.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"89 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149230348","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Interfacial Evolution, Failure Mechanisms, and Multiscale Stabilization Strategies for Silicon Anodes in Sulfide-Based All-Solid-State Batteries 硫化物基全固态电池中硅阳极的界面演化、失效机制和多尺度稳定策略
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79164
Huikun Liu,Zhixiao Yin,Shuai Wang,Yangzhou Ma,Hailiang Deng,Cuie Wen,Guangsheng Song
{"title":"Interfacial Evolution, Failure Mechanisms, and Multiscale Stabilization Strategies for Silicon Anodes in Sulfide-Based All-Solid-State Batteries","authors":"Huikun Liu,Zhixiao Yin,Shuai Wang,Yangzhou Ma,Hailiang Deng,Cuie Wen,Guangsheng Song","doi":"10.1002/adfm.79164","DOIUrl":"https://doi.org/10.1002/adfm.79164","url":null,"abstract":"Silicon anodes in sulfide-based all-solid-state batteries undergo coupled interfacial reactions, interphase growth, transport heterogeneity, stress evolution, and contact loss. These processes collectively govern degradation under practical operating conditions. Understanding their chemo-mechanical coupling provides a basis for designing stable interfaces, preserving solid–solid contact, and enabling high-capacity, low-pressure operation.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"15 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149225968","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bioinspired Stable Superhydrophobic Hierarchical Luminescence Textiles via Electrospinning and Electrospraying Synergism 基于静电纺丝和静电喷涂协同作用的生物启发的稳定超疏水分层发光纺织品
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79229
Linfei Li,Yaxin Fan,Luming Yang,Yuanzhang Jiang,Shuo Shi,Dong Wang,Yifan Si
{"title":"Bioinspired Stable Superhydrophobic Hierarchical Luminescence Textiles via Electrospinning and Electrospraying Synergism","authors":"Linfei Li,Yaxin Fan,Luming Yang,Yuanzhang Jiang,Shuo Shi,Dong Wang,Yifan Si","doi":"10.1002/adfm.79229","DOIUrl":"https://doi.org/10.1002/adfm.79229","url":null,"abstract":"Inspired by the transparent skin of Aequorea Victoria, a bioinspired superhydrophobic luminescent textile with a hierarchical “skeleton-and-flesh” structure is developed via a periodic electrospinning-electrospraying synergism (EES) strategy for passive, durable optical signaling in extreme environments.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"9 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149230230","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Lone-Pair-Induced Lattice Distortion in Lead-Free Hybrid Perovskites for High-Performance Nanogenerators 高性能纳米发电机用无铅杂化钙钛矿的孤对诱导晶格畸变
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.78818
Majid Haji Bagheri,Asif Abdullah Khan,Md Fahim Al Fattah,Mahmoud Almadhoun,Shamaila Shahzadi,Aixi Pan,Md Soyaeb Hasan,Henry Wu,Arash Aghigh,Bhawna Bhawna,François Légaré,Vivek Maheshwari,Dayan Ban
{"title":"Lone-Pair-Induced Lattice Distortion in Lead-Free Hybrid Perovskites for High-Performance Nanogenerators","authors":"Majid Haji Bagheri,Asif Abdullah Khan,Md Fahim Al Fattah,Mahmoud Almadhoun,Shamaila Shahzadi,Aixi Pan,Md Soyaeb Hasan,Henry Wu,Arash Aghigh,Bhawna Bhawna,François Légaré,Vivek Maheshwari,Dayan Ban","doi":"10.1002/adfm.78818","DOIUrl":"https://doi.org/10.1002/adfm.78818","url":null,"abstract":"A lead-free tin-based hybrid perovskite is designed in which stereochemically active lone-pair electrons on tin distort the crystal lattice and break its symmetry. Blended into a flexible polymer, the material converts pressure into electricity at milliwatt-scale power density and continues working far below freezing, powering a commercial wristwatch continuously at minus fifty degrees Celsius for more than 15 min.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"3 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149230245","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Lattice Bromine-Induced Pinning Effect Stabilizes Spinel Co3O4 for Durable Bromine Radical-Mediated Propylene Oxide Electrosynthesis 晶格溴诱导钉钉效应稳定尖晶石Co3O4在持久溴自由基介导的环氧丙烷电合成中的应用
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79251
Shaojian Jiang,Lan Yao,Yafang Luo,Ruidong Yang,Jiabing Geng,Haichuan Liao,Liang Wang,Hongjie Yu,Hongjing Wang
{"title":"Lattice Bromine-Induced Pinning Effect Stabilizes Spinel Co3O4 for Durable Bromine Radical-Mediated Propylene Oxide Electrosynthesis","authors":"Shaojian Jiang,Lan Yao,Yafang Luo,Ruidong Yang,Jiabing Geng,Haichuan Liao,Liang Wang,Hongjie Yu,Hongjing Wang","doi":"10.1002/adfm.79251","DOIUrl":"https://doi.org/10.1002/adfm.79251","url":null,"abstract":"This study developed bromine-doped Co3O4 nanosheet arrays supported on carbon paper (Br-Co3O4/CP) for durable bromine radical-mediated propylene oxide electrosynthesis. The introduction of lattice bromine enhances the Co─O covalent bond of spinel Co3O4 through a pinning effect, suppresses OER side reactions, and improves catalytic stability.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"2 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149230247","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Balanced Cr3+ and RE3+ Luminescence in a Novel Non-Concentration-Quenching Cs2RbCrF6: High-Efficiency Wide-Coverage NIR Phosphors Toward Solvent Extraction Monitoring 新型非浓度猝灭Cs2RbCrF6中Cr3+和RE3+平衡发光：用于溶剂萃取监测的高效宽覆盖近红外荧光粉
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79129
Xixiang Pan,Songbin Liu,Shuyang Liu,Wanfang Zou,Yu Liao,Shuifu Liu,Fengli Yang,Chunpei Yan,Junjun Tan,Jiaqing Peng,Zhihua Xiong,Xinyu Ye
{"title":"Balanced Cr3+ and RE3+ Luminescence in a Novel Non-Concentration-Quenching Cs2RbCrF6: High-Efficiency Wide-Coverage NIR Phosphors Toward Solvent Extraction Monitoring","authors":"Xixiang Pan,Songbin Liu,Shuyang Liu,Wanfang Zou,Yu Liao,Shuifu Liu,Fengli Yang,Chunpei Yan,Junjun Tan,Jiaqing Peng,Zhihua Xiong,Xinyu Ye","doi":"10.1002/adfm.79129","DOIUrl":"https://doi.org/10.1002/adfm.79129","url":null,"abstract":"A novel double-perovskite-structured Cr-rich Cs2RbCrF6 with large interionic separation and non-concentration-quenching was firstly discovered, which enables a favorable balance between broadband Cr3+ NIR-I emission and multiple RE3+ characteristic NIR-II emissions (i.e., Yb3+, Nd3+, Er3+), thereby realizing genuinely wide-coverage NIR luminescence spanning 650-1600 nm.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"75 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149225965","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Pre‑Embedded Intramolecular Donor–Acceptor Engineering in Isoreticular Covalent Organic Frameworks for Efficient Photocatalytic Hydrogen Evolution 等孔共价有机框架中预嵌入的分子内供体-受体工程用于高效光催化析氢
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79158
Xiang-Hao Han,Shun-Feng Li,Ya Lu,Mengyao Su,Jun Lin,Meimei Zhang,Kian Ping Loh,Yubin Fu,Kai Leng
{"title":"Pre‑Embedded Intramolecular Donor–Acceptor Engineering in Isoreticular Covalent Organic Frameworks for Efficient Photocatalytic Hydrogen Evolution","authors":"Xiang-Hao Han,Shun-Feng Li,Ya Lu,Mengyao Su,Jun Lin,Meimei Zhang,Kian Ping Loh,Yubin Fu,Kai Leng","doi":"10.1002/adfm.79158","DOIUrl":"https://doi.org/10.1002/adfm.79158","url":null,"abstract":"Unlike conventional intermolecular donor–acceptor covalent organic frameworks (COFs) assembled from independent donor and acceptor monomers, pre-embedded intramolecular donor–acceptor engineering covalently locks donor and acceptor units within a single building block. The resulting framework facilitates exciton conversion, utilization of photogenerated charge, and electron transfer to the platium (Pt) cocatalyst, enabling a 150-fold enhancement in photocatalytic hydrogen evolution.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"8 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149225985","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Molecular Bridges for 2D Nanomaterials 二维纳米材料的分子桥
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79162
Yudhajit Bhattacharjee,Kevin Synnatschke,Andreas Fery,Hendrik Schlicke
{"title":"Molecular Bridges for 2D Nanomaterials","authors":"Yudhajit Bhattacharjee,Kevin Synnatschke,Andreas Fery,Hendrik Schlicke","doi":"10.1002/adfm.79162","DOIUrl":"https://doi.org/10.1002/adfm.79162","url":null,"abstract":"Molecular cross-linking provides a versatile strategy to engineer interfaces in 2D materials. By tuning the linker backbone, binding mode, and interflake spacing, molecular bridges can regulate charge transport, mechanical integrity, chemical functionality, and processing. This Perspective connects established concepts in the field of nanoparticles with emerging MXene and broader 2D material architectures for programmable interfacial design across applications.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"15 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149230234","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Vinylene-Linked Covalent Organic Framework-Directed Facet Orientation Reconstruction in Inverted Perovskite Solar Cells 乙烯链共价有机框架-定向面取向重构倒置钙钛矿太阳能电池
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79131
Liang Ma,Heng Zhang,Zhiqiang Zhang,Wenjie Zhang,Ziyang Chang,Dan Huang,Changlin Yao,Hai Zhong,Qi Zhang,Zhengyan He,Shufang Zhang
{"title":"Vinylene-Linked Covalent Organic Framework-Directed Facet Orientation Reconstruction in Inverted Perovskite Solar Cells","authors":"Liang Ma,Heng Zhang,Zhiqiang Zhang,Wenjie Zhang,Ziyang Chang,Dan Huang,Changlin Yao,Hai Zhong,Qi Zhang,Zhengyan He,Shufang Zhang","doi":"10.1002/adfm.79131","DOIUrl":"https://doi.org/10.1002/adfm.79131","url":null,"abstract":"Vinylene-linked TBD-COF directs perovskite facet orientation toward enhanced (012) domains, reducing lattice strain and recombination for efficient and stable inverted perovskite solar cells.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"13 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149225974","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Low-Flicker-Noise MoS2 Transistors Enabled by High-κ Rare-Earth Oxychlorides for Mixed-Signal Electronics 高κ稀土氧氯化物使能混合信号电子学中的低闪烁噪声MoS2晶体管
IF 19 1区 材料科学
Advanced Functional Materials Pub Date : 2026-10-21 DOI: 10.1002/adfm.79151
Chanho Lee,Changwoo Pyo,Seungchan Lee,Juho Son,Yoongi Cho,Jiho Shin,Sungmoon Park,Sungjin Kim,Changmin An,Heein Yoon,Myungsoo Kim
{"title":"Low-Flicker-Noise MoS2 Transistors Enabled by High-κ Rare-Earth Oxychlorides for Mixed-Signal Electronics","authors":"Chanho Lee,Changwoo Pyo,Seungchan Lee,Juho Son,Yoongi Cho,Jiho Shin,Sungmoon Park,Sungjin Kim,Changmin An,Heein Yoon,Myungsoo Kim","doi":"10.1002/adfm.79151","DOIUrl":"https://doi.org/10.1002/adfm.79151","url":null,"abstract":"Single-crystalline LaOCl and GdOCl form atomically abrupt, Cl-terminated interfaces with MoS2, enabling near-ideal switching and suppressed flicker noise. Carrier-number-fluctuation analysis yields effective noise-derived interface trap densities of 1.15–1.94 × 1010 cm−2 eV−1, approaching hexagonal boron nitride levels with high-κ coupling. Circuit sensitivity analysis indicates reduced oscillator and phase-locked-loop jitter and up to a 1.45-bit improvement in analog-to-digital converter effective resolution.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"43 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149225977","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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