Advanced Functional Materials最新文献

{"title":"Beyond Volcano Top of Transition Metal‐Based Electrocatalysts Triggered by Spin State Modulation","authors":"Yucheng Lv, Zhi Fang, Linlin Zhou, Puyu Du, Zeyu Gao, Wanting Zhao, Xinmei Hou, Yanghui Lu, Wensheng Yan, Kai Chen, Song Gao, Yanglong Hou","doi":"10.1002/adfm.202520395","DOIUrl":"https://doi.org/10.1002/adfm.202520395","url":null,"abstract":"Although modulating the spin state of transition metal (TM)‐based catalysts has emerged as a strategy to improve the sluggish kinetics of oxygen evolution reaction (OER), the quantitative correlation between spin state and OER activity remains elusive, especially at the experimental level. This hinders the rational design of high‐performance electrocatalysts. Here, ferromagnetic CoSe<jats:sub>2</jats:sub> polycrystalline nanoparticles by hydrothermal and vapor anion exchange methods are synthesized. Zn with various concentrations is doped to regulate the spin quantum number (<jats:italic>S</jats:italic>) of Co. The results show that the saturation magnetization of Co<jats:sub>0.9</jats:sub>Zn<jats:sub>0.1</jats:sub>Se<jats:sub>2</jats:sub>, as a macroscopic feature of <jats:italic>S</jats:italic>, exhibits a remarkable 18‐fold enhancement from 0.74 to 14.2 emu g<jats:sup>−1</jats:sup>. Such enhanced <jats:italic>S</jats:italic> achieves an extraordinary enhancement of OER activity by 448%, surpassing its traditional volcano top. Meanwhile, the OER activity demonstrates a strong linear relationship with <jats:italic>S</jats:italic>, clarifying the effect of total <jats:italic>S</jats:italic> in bulk on the surface active sites. This work systematically quantifies the spin‐catalysis relationship and formulates the guidelines for precision design of spin‐optimized electrocatalysts.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"138 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145311319","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Immunomodulation and Fibroblast Subtype Regulation by a Photoliquefiable Hydrogel Realize Anti‐Scar Skin Regeneration of Refractory Infected Wounds","authors":"Zhenglin Li, Haijuan Zhang, Binbiao Li, Jie Xu, Yanxia Zhang, Junjun Li, Tafadzwa Chaire, Mingying Gao, Jian Wang, Keqing Shi, Zimiao Chen, Ke Tao, Xiaokun Li, Miao Yu, Jian Xiao","doi":"10.1002/adfm.202521060","DOIUrl":"https://doi.org/10.1002/adfm.202521060","url":null,"abstract":"Effective wound repair and preventive strategies against scarring remain challenging especially for chronic refractory wounds, as aberrant healing often encounters with persistent bacterial infection, extensive inflammatory response, impaired angiogenesis, and fibrotic scar formation. Herein, a photoliquefiable hydrogel dressing (denoted as PCS gel) is proposed as promising therapeutic strategy for rapid anti‐scar skin regeneration of refractory wounds. Specifically, the gel exerts robust antibacterial effect via mild thermogenesis for multidrug‐resistant biofilm eradication, and timely regulates tissue redox homeostasis. Upon efficient alleviation of local immoderate inflammation, PCS gel fosters a favorable pro‐regenerative microenvironment by bridging swift transition of the inflammatory stage to the proliferative stage, and thus significantly promotes neoangiogenesis as well as epithelialization. Importantly, the gel simultaneously alters pro‐regenerative fibroblast subpopulations by effective suppression of CD36 receptor during this stage, and hence blocks <jats:italic>JUN</jats:italic> overexpression‐mediated dermal fibrotic scarring. Notably, by thorough testing on both murine infected wound models (including acute wounds, diabetic chronic wounds) and rabbit ear hyperplastic scar wound model, PCS gel aided by thermogenesis facilitates rapid normal skin‐like epithelial closure with no perceptible hyperplastic scars. Therefore, our work emphasizes the promising regenerative strategy of immunomodulation and fibroblast lineage regulation by the PCS gel platform for rapid anti‐scar wound repair.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"58 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145314576","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Laser Induced Fast Topotactic Phase Transition in Freestanding Oxide Membranes","authors":"Muhammad Shahrukh Saleem, Yanghe Wang, Chenxi Nie, Xiangping Zhang, Yingli Zhang, Honghao Li, Kaizhen liu, Jiahao Song, Mingqiang Cheng, Shuhua Ma, Linkun Wang, Muhammad Zubair Nawaz, Luyong Zhang, Mei‐Huan Zhao, Jinhui Zhong, Guangfu Luo, Changjian Li","doi":"10.1002/adfm.202524555","DOIUrl":"https://doi.org/10.1002/adfm.202524555","url":null,"abstract":"Materials exhibiting topotactic transitions offer unique opportunities for engineering phase‐dependent properties. Topotactic transitions between brownmillerite (BM) and perovskite (PV) oxides are potentially useful for memristive devices, electrochromic, and solid electrolyte applications. However, achieving fast and uniform topotactic phase transition simultaneously is challenging, limiting their applications. Here, fast and well‐controlled laser induced topotactic transitions are shown in freestanding SrCoO<jats:sub>2.5</jats:sub> crystalline membranes, significantly faster than conventional annealing or ionic liquid gating methods. The phase transition is identified by Raman spectroscopy, local conductive atomic force microscopy (CAFM), and confirmed by atomic scale scanning transmission electron microscope (STEM) studies. First‐principles calculations confirm that the strain‐free condition in freestanding oxide membranes is crucial for laser triggered topotactic phase transition. The phase transition induces a 6 times reduction in resistance and multilevel resistance controllable by varying the laser treatment area. The fast, direct laser writing technique works as a simple, scalable method for optically writable memory devices.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"10 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145311315","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Origami Twist‐Inspired Microbuilding Blocks for Multifunctional Shape‐Morphing Micromachines","authors":"Lei Wang, Yunyue Yang, Michael Yu Wang, Tian‐Yun Huang","doi":"10.1002/adfm.202517157","DOIUrl":"https://doi.org/10.1002/adfm.202517157","url":null,"abstract":"The development of intelligent micromachines, crucial for complex tasks in confined spaces, is hindered by limited functionalities due to material constraints and incompatible nanofabrication methods. Drawing inspiration from the efficient motion and deformation of origami structures, a microbuilding block with strong torsional properties is developed. This block serves as a connector between a rigid frame and a soft artificial muscle, fabricated through multistep two‐photon polymerization. When assembled into slender, high‐aspect‐ratio forms, these programmable blocks enable reversible shape changes and sophisticated 3D (three‐dimensional) morphing in response to external stimuli. The design, which integrates rigid and soft materials, enables the rigid surface to be coated with magnetic material, allowing controlled operation under external magnetic fields. When exposed to a rotating magnetic field of 20 mT at 5 Hz, the micromachine assembled from microbuilding blocks reaches a maximum speed of 380 µm s<jats:sup>−1</jats:sup>. In addition, a hybrid fabrication approach is developed that combines 2D (two‐dimensional) lithography with 3D direct laser writing, embedding a microelectronic layer into the shape‐morphing system. The successful cargo delivery in a 3D microchannel shows this method's potential to enhance micromachine intelligence by improving adaptability and enabling closed‐loop control with flexible microelectronics.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"1 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145311317","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"The Coupling of Rh‐Ru Dual Sites with Interfacial Oxygen Endows MoSe2 with Efficient Ammonia Electrosynthesis","authors":"Zhaoyan Luo, Lijiao Shi, Yinnan Qian, Zijie Yang, Jiale Li, Lei Zhang, Qianling Zhang, Chuanxin He, Xiangzhong Ren","doi":"10.1002/adfm.202513568","DOIUrl":"https://doi.org/10.1002/adfm.202513568","url":null,"abstract":"The electrochemical nitritereduction reaction (NO<jats:sub>2</jats:sub>RR) to ammonia (NH<jats:sub>3</jats:sub>) is an intricate multielectron coupled proton transfer process, involving the adsorption and deoxygenation of NO<jats:sub>2</jats:sub><jats:sup>−</jats:sup> to form intermediates (*NO), followed by the protonation of *NO to generate NH<jats:sub>3</jats:sub>. Tandem catalysis is a promising approach for enhancing the NO<jats:sub>2</jats:sub>RR and suppressing side effects; however, it is still challenged by the lack of well‐designed catalysts to drive this catalytic process. Herein, a catalyst is introduced, featuring Rh−Ru atomic‐pair dual sites that couple with interfacial oxygen‐containing species confined within a MoSe<jats:sub>2</jats:sub> lattice (RhRu‐MoSe<jats:sub>2‐x</jats:sub>O<jats:sub>y</jats:sub>), enabling the unprecedented selective conversion of NO<jats:sub>2</jats:sub><jats:sup>−</jats:sup> to NH<jats:sub>3</jats:sub> under a low potential. Systematic experimental and computational studies reveal that the construction of Rh‐Ru sites married with adjacent oxygen‐containing groups can achieve the synchronous dispatch of water activation and hydrogenation of NO<jats:sub>2</jats:sub>. Moreover, the nitrite reduction on RhRu‐MoSe<jats:sub>2‐x</jats:sub>O<jats:sub>y</jats:sub> preferably proceeds via the NHO* pathway (NO*→NHO*), effectively circumventing the high energy barrier associated with the O‐side pathway (NO*→NOH*). Consequently, such a tandem system holds superior performance for robust NH<jats:sub>3</jats:sub> electrosynthesis at a relatively low potential, achieving a high NH<jats:sub>3</jats:sub> Faradaic efficiency of 93.0% at −0.2 V (vs RHE) and an exceptional NH<jats:sub>3</jats:sub> production rate of 9.2725 mmol h<jats:sup>−1</jats:sup> mg<jats:sub>cat</jats:sub><jats:sup>−1</jats:sup> at –0.4 V. Furthermore, the resulting catalysts attain ultra‐low overpotentials in a membrane electrode assembly (MEA) electrolyzer, featuring cell voltages of 2.1 V at current densities of 400 mA cm<jats:sup>−2</jats:sup> and stable operation under industrial conditions for 200 min.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"3 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145314577","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Highly Sensitive Surface Acoustic Wave Magnetic Field Sensor Based on a Strongly Coupled Magnon‐Phonon System","authors":"Chong Chen, Mingyuan Ma, Weiqi Du, Zheng Sun, Deqi Tao, Lei Han, Sulei Fu, Feng Pan, Cheng Song","doi":"10.1002/adfm.202518999","DOIUrl":"https://doi.org/10.1002/adfm.202518999","url":null,"abstract":"Strong coupling between quasiparticles enables breakthroughs in quantum technologies. Surface acoustic waves (SAWs), carrying coherent gigahertz‐frequency phonons, provide a platform to achieve strong coupling between SAW phonons and quasiparticles like magnons. SAWs devices also utilize the delta‐<jats:italic>E</jats:italic> or delta‐<jats:italic>G</jats:italic> effect for magnetic field sensing, achieving an ultra‐low limit of detection (LoD) down to tens of picotesla. Concomitant disadvantages include unidirectional response, millimeter size, complex structure, and fabrication still remain. The strong magnon‐phonon coupling has great potential to overcome these challenges for weak magnetic detection. Here, an ultra‐compact and highly sensitive SAW magnetic field sensor based on a strongly coupled magnon‐phonon system is demonstrated, featuring a thin FeGaB film embedded in an acoustic cavity. In the strong coupling regime, the SAW frequency exhibits anti‐crossing and responds dramatically to external magnetic fields, enabling high sensitivities. Notably, within the anti‐crossing region, a frequency sensitivity of 600 kHz/Oe and a phase sensitivity of 44 °/Oe are achieved. Combined with phase noise evaluation, the LoD is determined to be 126 pT/Hz<jats:sup>0.5</jats:sup> @ 10 Hz and 27 pT/Hz<jats:sup>0.5</jats:sup> @ 100 Hz. Besides its fundamental significance for hybrid quasiparticles, this work proposes a brand‐new sensing mechanism for developing miniaturized, highly sensitive, and low‐LoD SAW magnetic field sensors.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"13 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145311320","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Solid-State Norbornadiene Photothermal Films for Efficient Solar Energy Storage","authors":"Wenbo Tian, Yu Han, Fei Song, Jialin Fu, Ke Wang, Dongxing Song","doi":"10.1002/adfm.202507162","DOIUrl":"https://doi.org/10.1002/adfm.202507162","url":null,"abstract":"A solid-state photothermal (PT) energy storage film based on norbornadiene (NBD) molecules has been developed, which converts solar energy into chemical energy through photoisomerization reactions and releases it as thermal energy upon heating. The optical absorption, energy storage properties, tensile strength, and thermal conductivity of the four NBD molecules are evaluated. Among them, the NBD4 film demonstrates the highest thermal storage capacity, reaching up to 202 J g⁻¹. In addition, the influence mechanism of different substituents and polystyrene (PS) concentrations on NBD is analyzed from a microscopic perspective. When integrated with photovoltaic (PV) cells, the solid-state PT energy storage films absorb UV light, lowering the PV cell temperature ≈5 °C while simultaneously storing UV photons as chemical energy. This results in ≈3% increase in overall system efficiency. After irradiation, the NBD film is additionally integrated with the thermoelectric generator (TEG). The stored energy is converted into electrical energy, enhancing thermoelectric conversion efficiency. The solid-state film proposed in this study effectively addresses the issues of poor thermal stability and leakage associated with liquid-based systems while remaining fully compatible with existing PV modules, thereby enhancing solar energy storage and heat release efficiency.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"64 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145305795","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Unlocking Advanced UV NLO Crystals in Rare-Earth Metal Borate Fluorides via [B3O6]-Mediated Structural Modulation","authors":"Qianzhen Zhang, Ran An, Abudukadi Tudi, Jiongquan Chen, Xiaoqin Ma, Xifa Long, Zhihua Yang, Shilie Pan, Yun Yang","doi":"10.1002/adfm.202520516","DOIUrl":"https://doi.org/10.1002/adfm.202520516","url":null,"abstract":"Developing new short-wavelength nonlinear optical (NLO) crystals has always been a significant and challenging area of research. Herein, guided by the cooperative optimization strategy, three new rare-earth metal borate fluorides, K₂GdB₃O₆F₂, Rb₂LuB₃O₆F₂, and Cs₂LuB₃O₆F₂, are rationally designed and fabricated by synergically assembling advantageous functional groups. Among them, a structural evolution from centrosymmetric K₂GdB₃O₆F₂ to non-centrosymmetric Rb₂LuB₃O₆F₂ and Cs₂LuB₃O₆F₂ reveals that the [B₃O₆] group contributes to the control of structural symmetry, owing to its sensitivity to the coordination of rare earth metal polyhedra. Notably, all the three title compounds exhibit short cutoff edges less than 200 nm, with Cs₂LuB₃O₆F₂ displaying a large experimental frequency doubling effect of 1.5 × KH₂PO₄. The type-I shortest phase-matching wavelengths for Rb₂LuB₃O₆F₂ and Cs₂LuB₃O₆F₂ are evaluated to be 210 and 202 nm, respectively, indicating their potential for direct output of 213 coherent lights through a fifth harmonic generation process of Nd: YAG laser. This study provides new insights into the rational design and development of short-wavelength NLO materials by exploring the sensitivity of the [B₃O₆] groups to the surrounding coordination environment, thereby fostering innovation in the field of NLO materials.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"30 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145305798","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Emergent Magnetic Structures at the 2D Limit of the Altermagnet MnTe","authors":"Marc G. Cuxart, Roberto Robles, Beatriz Muñiz Cano, Pierluigi Gargiani, Clara Rebanal, Iolanda Di Bernardo, Alireza Amiri, Fabián Calleja, Manuela Garnica, Miguel A. Valbuena, Amadeo L. Vázquez de Parga","doi":"10.1002/adfm.202516924","DOIUrl":"https://doi.org/10.1002/adfm.202516924","url":null,"abstract":"MnTe has recently emerged as a canonical altermagnet, a newly identified class of magnetism characterized by compensated antiferromagnetic order coexisting with spin-split electronic bands, traditionally considered exclusive to ferromagnets. However, the extent to which altermagnetism persists as altermagnets are thinned to the 2D limit remains largely unexplored. Here, the magnetic behavior of two-dimensional (2D) MnTe is investigated, specifically atomically-thin monolayers (MLs) and bilayers (BLs) grown on graphene/Ir(111) substrate, by combining experimental scanning tunneling microscopy, X-ray photoelectron microscopy, X-ray absorption spectroscopy, and X-ray magnetic circular dichroism with density functional theory calculations. It is found that while ML and BL MnTe adopt atomic structures with symmetries incompatible with altermagnetism, they exhibit intriguing magnetic phases: the BL forms a highly-robust layered antiferromagnet with in-plane spin anisotropy, whereas the ML presents characteristics compatible with spin-glass behavior below its freezing temperature, a phenomenon not previously observed in an atomically thin material. These findings highlight how reduced dimensionality can promote the emergence of unusual magnetic structures distinct from those of their 3D counterparts, providing new insights into low-dimensional magnetism.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"64 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145305806","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Deciphering Key Features Determining Electrochemical Stability and Conductivity of Halide Solid-State Electrolytes","authors":"Weiqi Hou, Deyuan Li, Guangwen Zhang, Fangbing Li, Huilin Ge, Ao Du, Zhenshen Li, Quan-Hong Yang, Kai Song, Chunpeng Yang","doi":"10.1002/adfm.202524886","DOIUrl":"https://doi.org/10.1002/adfm.202524886","url":null,"abstract":"Halide solid-state electrolytes (HSSEs) are promising electrolytes for all-solid-state batteries (ASSBs), benefiting from their high ionic conductivity and compatibility with high-voltage cathodes. However, HSSEs exhibit poor interfacial stability against anodes (such as lithium (Li) metal and Li alloys), and interlayers are commonly introduced to circumvent the interfacial instability, which would reduce the overall energy density. Meanwhile, the underlying factors governing the stability of HSSEs against anodes remain poorly understood. Herein, key predictors of stability against anodes and ionic conductivity are identified using a series of Li_aZrCl_bO_cBr_dF_e (LZOXs) solid-state electrolytes through multi-anion substitution and chemistry-informed machine learning. As a result, the optimal composition, Li₂ZrCl_4.4O_0.4Br_0.4F_0.4 (LZOX) enables 1500 h of stable cycling in LiAl symmetric cells and achieves 200 cycles at 0.5 C and 600 cycles at 2 C in LiCoO₂ ASSBs without anode interlayers, effectively doubling the cycling life. More importantly, chemistry-informed machine learning deciphers key features—especially electronegativity for interfacial stability and cationic polarization for ionic conductivity—in the design of HSSEs, offering a strategy to develop HSSEs with enhanced compatibility toward high-performance ASSBs.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"101 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2025-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145306034","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}