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Frontispiece: Surface Chemistry of WC Powder Electrocatalysts Probed In Situ with NAP-XPS 前言：用NAP-XPS原位探测WC粉末电催化剂的表面化学
Angewandte Chemie Pub Date : 2025-06-23 DOI: 10.1002/ange.202582602
{"title":"Frontispiece: Surface Chemistry of WC Powder Electrocatalysts Probed In Situ with NAP-XPS","authors":"","doi":"10.1002/ange.202582602","DOIUrl":"https://doi.org/10.1002/ange.202582602","url":null,"abstract":"<p>Changes in electrode surface chemistry under electrochemical conditions critically influence electrocatalytic performance. In their Communication (e202500965), Julia Kunze-Liebhäuser et al. employed in-situ electrochemical X-ray photoelectron spectroscopy to monitor the surface state of tungsten carbide (WC) powder electrodes during the hydrogen evolution reaction (HER) and at oxidative potentials. Upon electrochemical polarization, the ubiquitous oxide layer dissolves, which causes exposure of the catalytically active carbide surface under HER conditions.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 26","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202582602","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144339680","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Front Cover: AI.zymes – A Modular Platform for Evolutionary Enzyme Design (Angew. Chem. 27/2025) 封面：AI。zymes -进化酶设计的模块化平台。化学27/2025)
Angewandte Chemie Pub Date : 2025-06-23 DOI: 10.1002/ange.202512748
Lucas P. Merlicek, Jannik Neumann, Abbie Lear, Vivian Degiorgi, Moor M. de Waal, Tudor-Stefan Cotet, Prof. Adrian J. Mulholland, Dr. H. Adrian Bunzel
{"title":"Front Cover: AI.zymes – A Modular Platform for Evolutionary Enzyme Design (Angew. Chem. 27/2025)","authors":"Lucas P. Merlicek,&nbsp;Jannik Neumann,&nbsp;Abbie Lear,&nbsp;Vivian Degiorgi,&nbsp;Moor M. de Waal,&nbsp;Tudor-Stefan Cotet,&nbsp;Prof. Adrian J. Mulholland,&nbsp;Dr. H. Adrian Bunzel","doi":"10.1002/ange.202512748","DOIUrl":"https://doi.org/10.1002/ange.202512748","url":null,"abstract":"<p>Enzymes are powerful catalysts. Unfortunately, computational enzyme design remains challenging. In their Research Article, H. Adrian Bunzel and co-workers develop AI.zymes (e202507031), a modular platform integrating state-of-the-art computational tools through evolutionary design. AI.zymes boost enzymes by optimizing biocatalytic features such as transition-state binding, protein stability, and electrostatic catalysis. Its modular architecture will facilitate the integration of emerging design algorithms and enable addressing diverse design challenges.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 27","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202512748","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144514795","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Correction to “Carbodicarbene-Stibenium Ion-Mediated Functionalization of C(sp3)−H and C(sp)−H Bonds” 对“碳羰基-锑离子介导的C(sp3)−H和C(sp)−H键功能化”的修正
Angewandte Chemie Pub Date : 2025-06-18 DOI: 10.1002/ange.202512489
{"title":"Correction to “Carbodicarbene-Stibenium Ion-Mediated Functionalization of C(sp3)−H and C(sp)−H Bonds”","authors":"","doi":"10.1002/ange.202512489","DOIUrl":"https://doi.org/10.1002/ange.202512489","url":null,"abstract":"<p><i>Angew. Chem. Int. Ed</i>. <b>2025</b>, <i>64</i>, e202415070, http://10.1002/ange.202415070</p><p>This correction adds an important reference to the position where Refs. [5e] and [8] are cited in <i>Angew. Chem. Int. Ed</i>. <b>2025</b>, <i>64</i>, e202415070; https://doi.org/10.1002/ange.202415070. Krempner and coworkers show that the C–H bonds of terminal alkynes can be activated via coordination with an antimony center via base catalysis (<i>Angew. Chem. Int. Ed</i>. <b>2024</b>, <i>63</i>, e202407822; https://doi.org/10.1002/ange.202407822).</p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 28","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202512489","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144573199","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Correction to “Strongly Coupled Cobalt Diselenide Monolayers for Selective Electrocatalytic Oxygen Reduction to H2O2 under Acidic Conditions” 修正“在酸性条件下选择性电催化氧还原为H2O2的强偶联二硒化钴单分子层”
Angewandte Chemie Pub Date : 2025-06-18 DOI: 10.1002/ange.202512608
{"title":"Correction to “Strongly Coupled Cobalt Diselenide Monolayers for Selective Electrocatalytic Oxygen Reduction to H2O2 under Acidic Conditions”","authors":"","doi":"10.1002/ange.202512608","DOIUrl":"https://doi.org/10.1002/ange.202512608","url":null,"abstract":"<p><i>Angew. Chem. Int. Ed</i>. <b>2021</b>, <i>60</i>, 26922–26931, https://doi.org/10.1002/ange.202111075</p><p>Figure S8d in the Supporting Information of this Research Article contains an error. The SEM image was mistakenly used from an unrelated sample. The corrected version of Figure S8 is shown below. The correction does not affect the scientific conclusions demonstrated in the published article.</p><p>The original Supporting Information was replaced with a corrected version of the Supporting Information. The authors apologize for these errors, which do not affect the data analysis and conclusions of the original Research Article.</p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 29","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202512608","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144624867","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Theodor Förster: Leben und FRET von 1933 bis 1951. Ein Blick aus den Archiven 西奥多·福斯特：1933年至1951年的生活和FRET。从档案馆看
Angewandte Chemie Pub Date : 2025-06-17 DOI: 10.1002/ange.202416843
Dr. Frank Eckart, Hans-Gerd Löhmannsröben, Niko Hildebrandt
{"title":"Theodor Förster: Leben und FRET von 1933 bis 1951. Ein Blick aus den Archiven","authors":"Dr. Frank Eckart,&nbsp;Hans-Gerd Löhmannsröben,&nbsp;Niko Hildebrandt","doi":"10.1002/ange.202416843","DOIUrl":"https://doi.org/10.1002/ange.202416843","url":null,"abstract":"","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 28","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144573894","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Min Zhou 最小值周
Angewandte Chemie Pub Date : 2025-06-17 DOI: 10.1002/ange.202512066
Min Zhou
{"title":"Min Zhou","authors":"Min Zhou","doi":"10.1002/ange.202512066","DOIUrl":"https://doi.org/10.1002/ange.202512066","url":null,"abstract":"<p>“<i>One book I can whole-heartedly recommend is</i> In a Flight of Starlings: The Wonder of Complex Systems <i>by Giorgio Parisi (2021 Nobel Prize in Physics)… My favorite name principle is Zachariasen's rule</i>…”</p><p>Find out more about Min Zhou in her Introducing… Profile.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 29","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202512066","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144624677","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Frontispiece: Stabilizing Lattice Oxygen to Enable Durable MnO2 Electrocatalyst for Simultaneous Acidic Hydrogen Production and Biomass Valorization 前文：稳定晶格氧，使持久的二氧化锰电催化剂同时用于酸性制氢和生物质增值
Angewandte Chemie Pub Date : 2025-06-16 DOI: 10.1002/ange.202582501
{"title":"Frontispiece: Stabilizing Lattice Oxygen to Enable Durable MnO2 Electrocatalyst for Simultaneous Acidic Hydrogen Production and Biomass Valorization","authors":"","doi":"10.1002/ange.202582501","DOIUrl":"https://doi.org/10.1002/ange.202582501","url":null,"abstract":"<p>The cover image illustrates the advancement of earth-abundant electrocatalysts for proton exchange membrane water electrolysis. The soil represents the manganese oxide anode, which is shielded from degradation during water oxidation by plant biomass. Meanwhile, biomass-derived sugars are transformed into valuable formic acid, offering a sustainable route for hydrogen production, as reported by Mingfei Shao, Hua Zhou et al. in their Research Article (e202502847).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 25","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202582501","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144299740","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inside Front Cover: Identification of an Activity Selector for the Nitroso-Forming Activity in Bacterial Type-III Copper Enzymes (Angew. Chem. 26/2025) 内页封面：细菌iii型铜酶中亚硝基形成活性选择器的鉴定（新）。化学26/2025)
Angewandte Chemie Pub Date : 2025-06-12 DOI: 10.1002/ange.202512251
Hoa Le Xuan, Felix Panis, Annette Rompel
{"title":"Inside Front Cover: Identification of an Activity Selector for the Nitroso-Forming Activity in Bacterial Type-III Copper Enzymes (Angew. Chem. 26/2025)","authors":"Hoa Le Xuan,&nbsp;Felix Panis,&nbsp;Annette Rompel","doi":"10.1002/ange.202512251","DOIUrl":"https://doi.org/10.1002/ange.202512251","url":null,"abstract":"<p>Enzyme specificity defines function: aminophenol oxidase uniquely converts aminophenols into nitrosophenols, whereas tyrosinase transforms them into quinone imines. This distinction is governed by a key amino acid near the copper(A) active site. In their Research Article (e202501560), Annette Rompel et al. demonstrated that a single amino acid exchange—swapping asparagine in SgGriF with isoleucine in SzTYR—can effectively invert the enzymes’ functions.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 26","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202512251","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144339397","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Back Cover: A Single-Molecule Liposome Assay for Membrane Permeabilisation (Angew. Chem. 26/2025) 外封底：膜透性的单分子脂质体测定(Angew。化学26/2025)
Angewandte Chemie Pub Date : 2025-06-12 DOI: 10.1002/ange.202512274
Krzysztof M. Bąk, Daniel C. Edwards, Dylan George, Bhanu Singh, Ryan Ferguson, Tianxiao Zhao, Kristin Piché, Ariel Louwrier, Scott L. Cockroft, Mathew H. Horrocks
{"title":"Outside Back Cover: A Single-Molecule Liposome Assay for Membrane Permeabilisation (Angew. Chem. 26/2025)","authors":"Krzysztof M. Bąk,&nbsp;Daniel C. Edwards,&nbsp;Dylan George,&nbsp;Bhanu Singh,&nbsp;Ryan Ferguson,&nbsp;Tianxiao Zhao,&nbsp;Kristin Piché,&nbsp;Ariel Louwrier,&nbsp;Scott L. Cockroft,&nbsp;Mathew H. Horrocks","doi":"10.1002/ange.202512274","DOIUrl":"https://doi.org/10.1002/ange.202512274","url":null,"abstract":"<p>A single-molecule liposome assay for membrane permeabilization using confocal microscopy paired with a fast-flow microfluidics device is reported by Scott L. Cockroft, Mathew H. Horrocks et al. in their Research Article (e202503678). Liposomes, encapsulating calcium-sensitive dye, pass through the channel aligned with the microscope. Membrane-permeabilizing agents allow calcium influx, sensitizing the dye which is detected as the liposome passes through the confocal volume. As successive liposomes pass through the volume, signals acquired indicate the permeabilising properties of the analyte.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 26","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202512274","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144339398","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Back Cover: Enhancing Cold Adaptation of Bidomain Amylases by High-Throughput Computational Engineering (Angew. Chem. 29/2025) 外封底：利用高通量计算工程增强biddomain淀粉酶的冷适应性[j]。化学29/2025)
Angewandte Chemie Pub Date : 2025-06-11 DOI: 10.1002/ange.202512250
Ning Ding, Yaoyukun Jiang, Robbie Ge, Qianzhen Shao, Wook Shin, Xinchun Ran, Zhongyue J. Yang
{"title":"Outside Back Cover: Enhancing Cold Adaptation of Bidomain Amylases by High-Throughput Computational Engineering (Angew. Chem. 29/2025)","authors":"Ning Ding,&nbsp;Yaoyukun Jiang,&nbsp;Robbie Ge,&nbsp;Qianzhen Shao,&nbsp;Wook Shin,&nbsp;Xinchun Ran,&nbsp;Zhongyue J. Yang","doi":"10.1002/ange.202512250","DOIUrl":"https://doi.org/10.1002/ange.202512250","url":null,"abstract":"<p>The cover art symbolizes the transformation of the mesophilic amylase psA (red) into its cold-adapted variant psA121 (cyan) through computational linker engineering. The central swirling motif reflects a shift in temperature adaptation, driven by increased interdomain separation between the catalytic domain and the carbohydrate-binding module. This visual captures how a simple change in linker sequence enables enhanced enzymatic activity at low temperatures by modifying the conformational dynamics of bidomain enzyme amylase, as described by Zhongyue J. Yang et al. in their Research Article (e202505991).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 29","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-06-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202512250","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144624434","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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