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Frontispiz: Liquid Metal Nanobiohybrids for High-Performance Solar-Driven Methanogenesis via Multi-Interface Engineering 基于多界面工程的高性能太阳能驱动甲烷生成的液态金属纳米生物杂化体
Angewandte Chemie Pub Date : 2025-04-07 DOI: 10.1002/ange.202581561
Wenzhi Gu, Jing Hu, Lei Li, Mingqiu Hong, Dong Zhang, Jiajing Chen, Prof. Jie Ye, Prof. Shungui Zhou
{"title":"Frontispiz: Liquid Metal Nanobiohybrids for High-Performance Solar-Driven Methanogenesis via Multi-Interface Engineering","authors":"Wenzhi Gu,&nbsp;Jing Hu,&nbsp;Lei Li,&nbsp;Mingqiu Hong,&nbsp;Dong Zhang,&nbsp;Jiajing Chen,&nbsp;Prof. Jie Ye,&nbsp;Prof. Shungui Zhou","doi":"10.1002/ange.202581561","DOIUrl":"https://doi.org/10.1002/ange.202581561","url":null,"abstract":"<p>Liquid metal nanobiohybrids facilitated high-performance solar-driven methanogenesis via multi-interface engineering, as reported by Shungui Zhou, Jie Ye and co-workers in their Research Article (e202423336). This study introduces an informative concept for nanobiohybrid design, opening a new avenue for the sustainable and scalable conversion of CO<sub>2</sub> to biofuels under ambient conditions.\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure>\u0000 </p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 15","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202581561","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143793735","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Frontispiz: Selbstorganisation von ZIF-8-Nanopartikeln zu “Brick-and-Mortar”-Membranen für die Wasserstofftrennung durch ein Zink-Koordinations-Polymer 前页：锌配位聚合物将 ZIF-8 纳米颗粒自组装成 "砖墙 "膜，用于氢气分离
Angewandte Chemie Pub Date : 2025-04-03 DOI: 10.1002/ange.202581462
Dr. Xinxin Li, Prof. Chengli Jiao, Dr. Xiaoqian Zhang, Xiaoya Xu, Prof. Saeed Gul, Fangyi Liang, Prof. Jürgen Caro, Prof. Heqing Jiang
{"title":"Frontispiz: Selbstorganisation von ZIF-8-Nanopartikeln zu “Brick-and-Mortar”-Membranen für die Wasserstofftrennung durch ein Zink-Koordinations-Polymer","authors":"Dr. Xinxin Li,&nbsp;Prof. Chengli Jiao,&nbsp;Dr. Xiaoqian Zhang,&nbsp;Xiaoya Xu,&nbsp;Prof. Saeed Gul,&nbsp;Fangyi Liang,&nbsp;Prof. Jürgen Caro,&nbsp;Prof. Heqing Jiang","doi":"10.1002/ange.202581462","DOIUrl":"https://doi.org/10.1002/ange.202581462","url":null,"abstract":"<p>A nacre-inspired composite membrane with “brick-and-mortar” structure is reported by Jürgen Caro, Heqing Jiang et al. in their Communication (e202416919). Dominant “brick” microporous zeolitic imidazolate framework nanoparticles allow fast H<sub>2</sub> transport, while the “mortar” coordination polymer interlayer combined with an adhesive interface reduces the intercrystalline transport and provides a highly H<sub>2</sub> selective transport pathway, resulting in an exceptional H<sub>2</sub>/CO<sub>2</sub> separation performance.\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure>\u0000 </p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 14","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202581462","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143762227","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Frontispiz: Fluorescent Artificial Receptor for Dopamine based on Molecular Recognition-driven Dynamic Covalent Chemistry in a Lipid Nanoreactor 在脂质纳米反应器中基于分子识别驱动的动态共价化学的多巴胺荧光人工受体
Angewandte Chemie Pub Date : 2025-04-03 DOI: 10.1002/ange.202581461
Bohdan Kozibroda, Jean-Marie Lehn, Andrey S. Klymchenko
{"title":"Frontispiz: Fluorescent Artificial Receptor for Dopamine based on Molecular Recognition-driven Dynamic Covalent Chemistry in a Lipid Nanoreactor","authors":"Bohdan Kozibroda,&nbsp;Jean-Marie Lehn,&nbsp;Andrey S. Klymchenko","doi":"10.1002/ange.202581461","DOIUrl":"https://doi.org/10.1002/ange.202581461","url":null,"abstract":"<p>In their Research Article (e202419905), Andrey S. Klymchenko et al. introduce a dynamic artificial receptor for neurotransmitter dopamine that synergically combines molecular recognition with dynamic imine bond formation of a fluorescent dye inside a lipid nanoreactor, triggering its emission color change. This nanoprobe enables dopamine detection with remarkable selectivity without interference of competing biogenic amines and biological fluids, such as blood serum, plasma, urine and cell lysate.\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure>\u0000 </p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 14","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202581461","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143762226","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Front Cover: Catalyst Improved Stereoselectivity and Regioselectivity Control to Access Completely Alternating Poly(lactic-co-glycolic acid) with Enhanced Properties (Angew. Chem. 17/2025) 外封面：催化剂改善立体选择性和区域选择性控制，以获得具有增强性能的完全交替聚（乳酸-羟基乙酸）。化学17/2025)
Angewandte Chemie Pub Date : 2025-04-02 DOI: 10.1002/ange.202506759
Xuanhua Guo, Hassan Ahmed, Guangqiang Xu, Qinggang Wang
{"title":"Outside Front Cover: Catalyst Improved Stereoselectivity and Regioselectivity Control to Access Completely Alternating Poly(lactic-co-glycolic acid) with Enhanced Properties (Angew. Chem. 17/2025)","authors":"Xuanhua Guo,&nbsp;Hassan Ahmed,&nbsp;Guangqiang Xu,&nbsp;Qinggang Wang","doi":"10.1002/ange.202506759","DOIUrl":"https://doi.org/10.1002/ange.202506759","url":null,"abstract":"<p>An improved stereoselective and regioselective ring-opening polymerization enables the formation of completely alternating poly(lactic-co-glycolic acid) (PLGA), as reported by Guangqiang Xu, Qinggang Wang et al. in their Communcation (e202417075). This breakthrough PLGA exhibits a record-high melting temperature (143.1°C), forms a stereocomplex (211.8°C) and demonstrates linear hydrolytic degradation with controlled drug release behavior, positioning it as an ideal carrier for long-acting therapeutic delivery.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 17","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202506759","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143861562","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Back Cover: Straightforward Formation of Borirenes from Boroles and Dialkynes (Angew. Chem. 18/2025) 外封底：硼炔和双炔直接形成硼炔(新。化学18/2025)
Angewandte Chemie Pub Date : 2025-03-30 DOI: 10.1002/ange.202506308
Pedro H. R. Oliveira, Marieli O. Rodrigues, Caren D. G. da Silva, Josina Bohlen, Merle Arrowsmith, Arumugam Jayaraman, Lukas Lubczyk, Felipe Fantuzzi, Eufrânio N. da Silva Júnior, Holger Braunschweig
{"title":"Outside Back Cover: Straightforward Formation of Borirenes from Boroles and Dialkynes (Angew. Chem. 18/2025)","authors":"Pedro H. R. Oliveira,&nbsp;Marieli O. Rodrigues,&nbsp;Caren D. G. da Silva,&nbsp;Josina Bohlen,&nbsp;Merle Arrowsmith,&nbsp;Arumugam Jayaraman,&nbsp;Lukas Lubczyk,&nbsp;Felipe Fantuzzi,&nbsp;Eufrânio N. da Silva Júnior,&nbsp;Holger Braunschweig","doi":"10.1002/ange.202506308","DOIUrl":"https://doi.org/10.1002/ange.202506308","url":null,"abstract":"<p>In their Research Article (e202423391), Felipe Fantuzzi, Eufrânio N. da Silva Júnior, Holger Braunschweig et al. report a selective one-step synthesis of perarylated borirenes from boroles and 1,3-diynes. The study includes substrate scope, X-ray, and DFT analyses. The cover illustrates this process with a phenyl balloon carrying a borirene ring arising above a sky filled with borole precursors, highlighting the novelty and aromaticity of the three-membered boron-bearing rings (Cover design: Danilo Londoño).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 18","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-03-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202506308","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143880053","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Back Cover: Giant Bulk Photovoltaic Effect in a Chiral Polar Crystal based on Helical One-dimensional Lead Halide Perovskites (Angew. Chem. 16/2025) 封底外页：基于螺旋一维卤化铅包晶石的手性极性晶体中的巨型块状光伏效应（Angew.）
Angewandte Chemie Pub Date : 2025-03-27 DOI: 10.1002/ange.202506098
Ayumi Ishii, Ryohei Sone, Tomohide Yamada, Mizuki Noto, Hikari Suzuki, Daiki Nakamura, Kei Murata, Takuya Shiga, Kazuyuki Ishii, Masayuki Nihei
{"title":"Outside Back Cover: Giant Bulk Photovoltaic Effect in a Chiral Polar Crystal based on Helical One-dimensional Lead Halide Perovskites (Angew. Chem. 16/2025)","authors":"Ayumi Ishii,&nbsp;Ryohei Sone,&nbsp;Tomohide Yamada,&nbsp;Mizuki Noto,&nbsp;Hikari Suzuki,&nbsp;Daiki Nakamura,&nbsp;Kei Murata,&nbsp;Takuya Shiga,&nbsp;Kazuyuki Ishii,&nbsp;Masayuki Nihei","doi":"10.1002/ange.202506098","DOIUrl":"https://doi.org/10.1002/ange.202506098","url":null,"abstract":"<p>In their Research Article (e202424391), Ayumi Ishii and co-workers present a giant bulk photovoltaic effect (BPVE) in chiral polar crystals of helical 1D lead halide perovskites using chiral naphthylethylamine cations. The crystals, with a C2 space group, exhibit strong circular dichroism and an exceptional BPVE, achieving an open-circuit voltage of 15 V—five times their band gap. These findings highlight the potential of chiral polar semiconductors for high-efficiency photovoltaic applications.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 16","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202506098","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143836409","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inside Back Cover: Single-Step Synthesis of Dimethyl Ether from Syngas over Nanoparticle-Derived Bifunctional Pd/CeO2/Al2O3 Catalysts (Angew. Chem. 16/2025) 内页后盖：在纳米颗粒衍生的双功能Pd/CeO2/Al2O3催化剂上从合成气一步合成二甲醚(Angew。化学16/2025)
Angewandte Chemie Pub Date : 2025-03-27 DOI: 10.1002/ange.202505854
Bing Wang, Zairan Yu, Shuang Chen, Nicola Da Roit, Dieter Schild, Michael Zimmermann, Yuemin Wang, Silke Behrens
{"title":"Inside Back Cover: Single-Step Synthesis of Dimethyl Ether from Syngas over Nanoparticle-Derived Bifunctional Pd/CeO2/Al2O3 Catalysts (Angew. Chem. 16/2025)","authors":"Bing Wang,&nbsp;Zairan Yu,&nbsp;Shuang Chen,&nbsp;Nicola Da Roit,&nbsp;Dieter Schild,&nbsp;Michael Zimmermann,&nbsp;Yuemin Wang,&nbsp;Silke Behrens","doi":"10.1002/ange.202505854","DOIUrl":"https://doi.org/10.1002/ange.202505854","url":null,"abstract":"<p>The single-step syngas-to-dimethyl ether process offers both economic and technical advantages over the current two-step industrial synthesis. A highly active bifunctional Pd/CeO<sub>2</sub>/γ-Al<sub>2</sub>O<sub>3</sub> catalyst is reported by Yuemin Wang, Silke Behrens et al. in their Research Article (e202423273). Pd clusters/particles confined on the nanoparticulate ceria matrix feature abundant interfacial Pd<sup>2+</sup> sites and adjacent O vacancies, accounting for the superior performance in both activity and stability.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 16","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202505854","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143836408","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Back Cover: Boosting C─O Bond Cleavage and Reverse Water-Gas Shift Activity via Enriched in-plane Sulfur Vacancies in Single-Layer Molybdenum Disulfide (Angew. Chem. 17/2025) 外封底：单层二硫化钼平面内硫空位富集促进C─O键解理和逆水气转换活性[j]。化学17/2025)
Angewandte Chemie Pub Date : 2025-03-27 DOI: 10.1002/ange.202506409
Zhiyuan Zheng, Xin Shang, Weijue Wang, Xiaofeng Yang, Xiong Su, Yanqiang Huang
{"title":"Outside Back Cover: Boosting C─O Bond Cleavage and Reverse Water-Gas Shift Activity via Enriched in-plane Sulfur Vacancies in Single-Layer Molybdenum Disulfide (Angew. Chem. 17/2025)","authors":"Zhiyuan Zheng,&nbsp;Xin Shang,&nbsp;Weijue Wang,&nbsp;Xiaofeng Yang,&nbsp;Xiong Su,&nbsp;Yanqiang Huang","doi":"10.1002/ange.202506409","DOIUrl":"https://doi.org/10.1002/ange.202506409","url":null,"abstract":"<p>A precise strategy for tuning defective structures in two-dimensional catalysts was developed by Yanqiang Huang, Xiong Su, Xin Shang et al. in their Research Article (e202422953). By employing a soft–hard dual-template approach, single-layer MoS<sub>2</sub> with enriched in-plane sulfur vacancies was synthesized. These vacancies significantly promote C─O bond cleavage, resulting in remarkable catalytic performance in the reverse water–gas shift reaction.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 17","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202506409","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143861951","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inside Front Cover: Data-Driven Accelerated Discovery Coupled with Precise Synthesis of Single-Atom Catalysts for Robust and Efficient Water Purification (Angew. Chem. 18/2025) 内部封面：数据驱动的加速发现与精确合成的单原子催化剂相结合，用于稳健和高效的水净化。化学18/2025)
Angewandte Chemie Pub Date : 2025-03-27 DOI: 10.1002/ange.202506096
Keng-Qiang Zhong, Fu-Yun Yu, Di Zhang, Zheng-Hao Li, Dong-Hua Xie, Ting-Ting Li, Yun Zhang, Li Yuan, Hao Li, Zhen-Yu Wu, Guo-Ping Sheng
{"title":"Inside Front Cover: Data-Driven Accelerated Discovery Coupled with Precise Synthesis of Single-Atom Catalysts for Robust and Efficient Water Purification (Angew. Chem. 18/2025)","authors":"Keng-Qiang Zhong,&nbsp;Fu-Yun Yu,&nbsp;Di Zhang,&nbsp;Zheng-Hao Li,&nbsp;Dong-Hua Xie,&nbsp;Ting-Ting Li,&nbsp;Yun Zhang,&nbsp;Li Yuan,&nbsp;Hao Li,&nbsp;Zhen-Yu Wu,&nbsp;Guo-Ping Sheng","doi":"10.1002/ange.202506096","DOIUrl":"https://doi.org/10.1002/ange.202506096","url":null,"abstract":"<p>A data-driven prediction coupled with precise synthesis strategy is proposed to accelerate the development of advanced catalysts. This strategy enables rapid screening of catalytic sites, followed by precise structural modulation for optimistic activity. A well-designed Fe single-atom catalyst exhibits ultra-high decontamination and excellent stability for water purification, as reported by Guo-Ping Sheng, Zhen-Yu Wu, Hao Li, Zheng-Hao Li et al. in their Research Article (e202500004).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 18","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202506096","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143880054","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inside Back Cover: Elucidating the Role of Electric Fields in Fe Oxidation via an Environmental Atom Probe (Angew. Chem. 18/2025) 内页封底：通过环境原子探针阐明电场在铁氧化中的作用。化学18/2025)
Angewandte Chemie Pub Date : 2025-03-27 DOI: 10.1002/ange.202506093
Sten V. Lambeets, Naseeha Cardwell, Isaac Onyango, Mark G. Wirth, Eric Vo, Yong Wang, Pierre Gaspard, Cornelius F. Ivory, Daniel E. Perea, Hierry Visart de Bocarmé, Jean-Sabin McEwen
{"title":"Inside Back Cover: Elucidating the Role of Electric Fields in Fe Oxidation via an Environmental Atom Probe (Angew. Chem. 18/2025)","authors":"Sten V. Lambeets,&nbsp;Naseeha Cardwell,&nbsp;Isaac Onyango,&nbsp;Mark G. Wirth,&nbsp;Eric Vo,&nbsp;Yong Wang,&nbsp;Pierre Gaspard,&nbsp;Cornelius F. Ivory,&nbsp;Daniel E. Perea,&nbsp;Hierry Visart de Bocarmé,&nbsp;Jean-Sabin McEwen","doi":"10.1002/ange.202506093","DOIUrl":"https://doi.org/10.1002/ange.202506093","url":null,"abstract":"<p>Environmental atom probe tomography and multi-scale modeling reveal electric field effects in iron oxidation, as demonstrated by Sten V. Lambeets, Jean-Sabin McEwen et al. in their Research Article (e202423434). The inhomogeneous field on an iron tip (grey/black spheres) creates an uneven oxygen distribution. The field gradient, shown as an intensity grid, is strongest near the tip. Surface composition is probed upon exposure to oxygen (red spheres) by collecting emitted iron oxide cations, which are then compared to field-based oxidation calculations.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 18","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202506093","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143880055","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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