Advanced Materials Technologies最新文献_第8页

Ultrashort Pulsed Laser-Assisted Direct Restoration of Human Enamel Using 3D Printable Biocomposite 超短脉冲激光辅助3D打印生物复合材料直接修复人类牙釉质

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-10 DOI: 10.1002/admt.202401362

Sarathkumar Loganathan, Geeta Sharma, Evangelos Daskalakis, Simon Strafford, Eric Kumi Barimah, Animesh Jha

{"title":"Ultrashort Pulsed Laser-Assisted Direct Restoration of Human Enamel Using 3D Printable Biocomposite","authors":"Sarathkumar Loganathan, Geeta Sharma, Evangelos Daskalakis, Simon Strafford, Eric Kumi Barimah, Animesh Jha","doi":"10.1002/admt.202401362","DOIUrl":"https://doi.org/10.1002/admt.202401362","url":null,"abstract":"Restorative dentistry encounters the prevalence of secondary caries due to the formation of marginal defects during tooth restoration. The present study proposes a dual-wavelength ultrashort-pulsed laser system for the direct restoration of damaged enamel to overcome marginal defects. The 2D finite element (FE) laser-ablative model is developed for studying the laser-tissue interaction. The laser-ablated cavities (rectilinear and circular) are prepared on human enamel using 800 nm, Ti:Sapphire femtosecond (fs) laser (100 fs, 1 kHz, 1 mm s−1) at average laser power of 200 mW. Subsequently, the cavity is filled with 3D printed biocomposite (65 wt.% of 3D-printing resin and 35 wt.% of Ce3+-ion doped hydroxyapatite) and photocured using 405 nm laser. Further, the postprocessing procedure is carried out using fs laser to remove excessive filler materials and improve surface finish at sub-ablation threshold of enamel. The surface morphology, chemical compositions, mechanical and interfacial properties of restored enamel surface are evaluated. The in vitro evaluation study confirmed that the enamel restored with fs laser and 3D printing biocomposite is mechanically and chemically robust for withstanding oral challenges. The proposed method of restoring damaged enamel opens an opportunity for a range of precision restorative dentistry procedures including caries and tooth augmentation.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 9","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202401362","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143904910","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Hybrid Microfluidic Chip Design with Two-Photon Polymerized Protein-Based Hydrogel Microstructures for Single Cell Experiments 单细胞实验用双光子聚合蛋白基水凝胶微流控芯片设计

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-10 DOI: 10.1002/admt.202401571

Dustin Dzikonski, Elena Bekker, Riccardo Zamboni, Dominika Ciechanska, Albrecht Schwab, Cornelia Denz, Jörg Imbrock

{"title":"Hybrid Microfluidic Chip Design with Two-Photon Polymerized Protein-Based Hydrogel Microstructures for Single Cell Experiments","authors":"Dustin Dzikonski, Elena Bekker, Riccardo Zamboni, Dominika Ciechanska, Albrecht Schwab, Cornelia Denz, Jörg Imbrock","doi":"10.1002/admt.202401571","DOIUrl":"https://doi.org/10.1002/admt.202401571","url":null,"abstract":"Although hydrogels are among the most promising materials for a huge variety of biomimicking and tissue engineering applications, conventional materials such as polydimethylsiloxane (PDMS) still outweigh hydrogels in terms of processability for the production of microfluidic devices. Hence, incorporating hydrogel components inside conventional PDMS-based microfluidic chips is a promising approach to take advantage of the many possibilities to utilize hydrogels, while maintaining standard properties of microfluidic devices in terms of mechanical stability. Microfluidic chips produced by standard soft lithography are combined with high-resolution protein-based hydrogel elements fabricated by two-photon polymerization (2PP). Those hybrid chips are used to distinguish mechanical properties of different cell phenotypes by injecting pancreatic cancer cells inside the device and investigate mechanical interactions with the hydrogel microstructures. The Young's modulus of blocks printed at different experimental conditions is determined by atomic force microscopy measurements. To showcase the high 3D resolution of the presented fabrication method, fully 3D fibrous meshes are printed with different configurations inside microchannels. By measuring the velocity and circularity of pancreatic cancer cells that pass through meshes of varying densities, the impact on the cell flow is determined. Furthermore, the hydrogel precursor solution is successfully removed and the meshes are immersed in phosphate buffered saline.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 9","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202401571","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143904911","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Sustainable Sensors Prepared by Environmentally Benign Means for Improving the Environmental Footprint of Wearable Electronics 通过环保手段制备可持续传感器，改善可穿戴电子产品的环境足迹

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-10 DOI: 10.1002/admt.202401600

Cephas Amoah, Usmaan Mahmood, W. G. Skene

{"title":"Sustainable Sensors Prepared by Environmentally Benign Means for Improving the Environmental Footprint of Wearable Electronics","authors":"Cephas Amoah, Usmaan Mahmood, W. G. Skene","doi":"10.1002/admt.202401600","DOIUrl":"https://doi.org/10.1002/admt.202401600","url":null,"abstract":"Sustainable electronic devices offer the virtue of energy efficiency. However, their fabrication is often reliant on environmentally deleterious methods and materials that overshadow the environmental benefits the devices provide. Toward improving the overall environmental footprint of devices, stretchable and conductive substrates for enabling wearable electronics are fabricated predominately from both sustainable and biodegradable materials (chitosan and sorbitol) along with an environmental benign solvent: water. Indeed, the >95 wt.% of the stretchable and bendable sensor consists of sustainable and biodegradable materials. By blending a collectively self-doped and water-soluble conductive homopolymer during processing, stretchable films with a transverse resistance as low as 0.08 MΩ are obtained. Both the conductivity and mechanical properties of the films including elongation at break and Young's modulus are contingent on the chitosan molecular weight. The elongation at break of the films prepared from high molecular weight chitosan is upward of 200%, with the optical transmission of 60% above 500 nm, and minimal conductive hysteresis with stretching. Both the mechanical compliance and conductivity of the sustainable films are ideal for enabling wearing electronics. This is demonstrated by their use as strain sensors for tracking both human movement and phonation detection.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 9","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202401600","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143904999","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

High-Performance 3D Printed Mechanically Interlocked Soft–Hard Interfaces of Hydrogels and Polylactide 高性能3D打印水凝胶和聚乳酸的机械互锁软硬界面

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-09 DOI: 10.1002/admt.202401081

L.B. Kunkels, M. Cruz Saldívar, N.E. Putra, C. Pitta Kruize, S. Panahkhahi, M.A. Leeflang, L.E. Fratila-Apachitei, A.A. Zadpoor, M.J. Mirzaali

{"title":"High-Performance 3D Printed Mechanically Interlocked Soft–Hard Interfaces of Hydrogels and Polylactide","authors":"L.B. Kunkels, M. Cruz Saldívar, N.E. Putra, C. Pitta Kruize, S. Panahkhahi, M.A. Leeflang, L.E. Fratila-Apachitei, A.A. Zadpoor, M.J. Mirzaali","doi":"10.1002/admt.202401081","DOIUrl":"https://doi.org/10.1002/admt.202401081","url":null,"abstract":"High-performance soft–hard interfaces are inherently difficult to fabricate due to the dissimilar mechanical properties of both materials, especially when connecting extremely soft biomaterials, such as hydrogels, to much harder biomaterials, such as rigid polymers. Nevertheless, there is significant clinical demand for synthetic soft–hard interfaces. Here, soft–hard interface geometries are proposed, designed with the aid of computational analyses and fabricated as 3D-printed hydrogel-to-polylactide (PLA) structures. Two primary interlocking geometries (i.e., anti-trapezoidal (AT) and double-hook (DH)) are used to study the envelope of 2.5D geometric interlocking designs, fabricated through hybrid 3D printing, combining pneumatic extrusion with fused deposition modeling. Finite-element analysis, uniaxial tensile tests, and digital image correlation (DIC) are used to characterize the geometries and identify parameters that significantly influence their mechanical performance. These findings reveal significant differences between geometric designs, where DH geometries performed significantly better than AT geometries, exhibiting a 190% increase in the maximum force, Fmax, and a 340% increase in the fracture toughness, W. Compared to the control groups (i.e., flat, inset, and 90° interfaces), Fmax and W values increased by 500%–990% and 350%–1200%, respectively. The findings of this study can serve as a guideline for the design and fabrication of efficient soft–hard interfaces with performances close to predicted values.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 9","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-01-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202401081","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143905062","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Supercapacitive Multimode Sensing with Tunable Graphene Sheet Film Electrodes (Adv. Mater. Technol. 1/2025) 可调谐石墨烯薄膜电极的超电容多模传感。抛光工艺。1/2025)

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-08 DOI: 10.1002/admt.202570006

Chunfeng Yin, Peimei Dong, Zengcai Zhao, Yaping Lu, Yuzhu Jin, Qiaolan Fan, Weitao Su, Yu Zhang, Xudong Liu, Zhenyu Xue, Dihua Wu, Yangxin Zhou

引用次数: 0

3D-Printed Highly Porous Functional Materials for the Efficient Removal of Adenovirus (Adv. Mater. Technol. 1/2025) 高效去除腺病毒的3d打印高孔功能材料抛光工艺。1/2025)

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-08 DOI: 10.1002/admt.202570003

Benedikt Keitel, Sandra Dietl, Tom Philipp, Gregor Neusser, Christine Kranz, Harald Sobek, Boris Mizaikoff, Mehmet Dinc

引用次数: 0

Advancing Brain Organoid Electrophysiology: Minimally Invasive Technologies for Comprehensive Characterization 推进脑类器官电生理：综合表征的微创技术

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-08 DOI: 10.1002/admt.202401585

Mujeeb Yousuf, Jean-Christophe (Chris) Rochet, Pushpapraj Singh, Muhammad Mustafa Hussain

{"title":"Advancing Brain Organoid Electrophysiology: Minimally Invasive Technologies for Comprehensive Characterization","authors":"Mujeeb Yousuf, Jean-Christophe (Chris) Rochet, Pushpapraj Singh, Muhammad Mustafa Hussain","doi":"10.1002/admt.202401585","DOIUrl":"https://doi.org/10.1002/admt.202401585","url":null,"abstract":"Human brain organoids, which originate from pluripotent stem cells, serve as valuable tools for a wide range of research endeavors, replicating brain function. Their capacity to replicate cellular interactions, morphology, and division provides invaluable insights into brain development, disease modeling, and drug screening. However, conventional morphological analysis methods are often invasive and lack real-time monitoring capabilities, posing limitations to achieving a comprehensive understanding. Therefore, advancing the comprehension of brain organoid electrophysiology necessitates the development of minimally invasive measurement technologies with long-term, high-resolution capabilities. This review highlights the significance of human brain organoids and emphasizes the need for electrophysiological characterization. It delves into conventional assessment methods, particularly focusing on 3D microelectrode arrays, electrode insertion mechanisms, and the importance of flexible electrode arrays to facilitate minimally invasive recordings. Additionally, various sensors tailored to monitor organoid properties are introduced, enriching the understanding of their chemical, thermal, and mechanical dynamics.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 7","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-01-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202401585","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143770385","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Tendon-Driven Stiffness-Tunable Soft Actuator via Thermoelectric-based Bidirectional Temperature Control (Adv. Mater. Technol. 1/2025) 基于热电双向温度控制的肌腱驱动刚度可调软执行器。抛光工艺。1/2025)

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-08 DOI: 10.1002/admt.202570004

Yunlong Gao, Shikun Lin, Chuanwei Liang, Siqi Qiu, Chengyun Long, Yingjun Wang, Yunquan Li, Yuan-Fang Zhang

引用次数: 0

Design of Modular, 3D-Printed Millifluidic Mixers to Enable Sequential NanoPrecipitation (SNaP) for the Tunable Synthesis of Drug-Loaded Nanoparticles and Microparticles (Adv. Mater. Technol. 1/2025) 模块化的设计，3d打印的微流体混合器，使顺序纳米沉淀（SNaP）可调合成药物负载的纳米颗粒和微粒（Adv. Mater.）。抛光工艺。1/2025)

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-08 DOI: 10.1002/admt.202570002

Thomas Y. Belinky, Nouha El Amri, Parker K. Lewis, Allie Karakosta LeMay, Rachel E. Pollard, Nathalie M. Pinkerton

引用次数: 0

Accurate and Robust Wide-Range Luminescent Microthermometer Based on ALD-Encapsulated Ga2O3:Cr DBR Microcavities (Adv. Mater. Technol. 1/2025) 基于ald封装Ga2O3:Cr DBR微腔的精确、鲁棒宽量程发光微温度计抛光工艺。1/2025)

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2025-01-08 DOI: 10.1002/admt.202570001

Manuel Alonso-Orts, Ruben J. T. Neelissen, Daniel Carrasco, Marco Schowalter, Andreas Rosenauer, Emilio Nogales, Bianchi Méndez, Martin Eickhoff

引用次数: 0