Advanced Materials Technologies最新文献

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Microneedles Mediated Delivery of Nanodiamonds for Quantum Sensing of Free Radicals in Skin Tissue 微针介导的纳米金刚石递送用于皮肤组织中自由基的量子传感
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-06-29 DOI: 10.1002/admt.71117
Siyu Fan, Maria Carmona Lobita, Thea Vedelaar, Yue Zhang, Claudia Reyes-San-Martin, Tomás Bauleth-Ramos, Gésinda Geertsema-Doornbusch, Han Gao, Mohammad-Ali Shahbazi, Hélder A. Santos, Romana Schirhagl
{"title":"Microneedles Mediated Delivery of Nanodiamonds for Quantum Sensing of Free Radicals in Skin Tissue","authors":"Siyu Fan,&nbsp;Maria Carmona Lobita,&nbsp;Thea Vedelaar,&nbsp;Yue Zhang,&nbsp;Claudia Reyes-San-Martin,&nbsp;Tomás Bauleth-Ramos,&nbsp;Gésinda Geertsema-Doornbusch,&nbsp;Han Gao,&nbsp;Mohammad-Ali Shahbazi,&nbsp;Hélder A. Santos,&nbsp;Romana Schirhagl","doi":"10.1002/admt.71117","DOIUrl":"https://doi.org/10.1002/admt.71117","url":null,"abstract":"<p>Free radicals in the skin are major contributors to the aging process and the development of cancer, making their detection crucial in both research and clinical diagnosis. Real-time magnetic noise sensing within skin tissues, especially through a quantum sensing technique known as T1 relaxometry, offers a promising approach for monitoring free radical activity. This technique uses fluorescent nanodiamonds (FNDs), whose optical properties change in response to magnetic fluctuations. To effectively deliver FNDs into the epidermis, we developed a dissolving microneedle (DMN) system composed of 10% polyvinylpyrrolidone and 3% hyaluronic acid. The DMNs exhibited strong FND fluorescence intensity concentrated at the microneedle tips (44%), optimizing their deposition within the epidermal layer. Histological analysis confirmed penetration depths of approximately 100–200 µm. To evaluate the sensing performance, T1 relaxometry measurements were conducted using gadolinium chloride solutions at the concentrations of 100 n<span>m</span> and 10 µ<span>m</span> as surrogates for free radicals. Compared to the baseline, the mean T1 values decreased by 35% and 55% for 100 n<span>m</span> and 10 µ<span>m</span> groups, respectively, demonstrating the system's sensitivity. Overall, our results highlight the potential of FND-loaded DMNs as a minimally invasive platform for high-resolution monitoring of oxidative stress and related biological processes in skin tissue.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.71117","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981492","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High-Performance Piezoelectric Nanogenerators Based on Wurtzite BeO Nanowire Arrays 基于纤锌矿BeO纳米线阵列的高性能压电纳米发电机
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-06-30 DOI: 10.1002/admt.71136
Yoonseo Jang, Jihyeon Park, Seoyeah Oh, Jonghyun Bae, Prakash R. Sultane, Christopher W. Bielawski, Jiwon Kim, Jungwoo Oh
{"title":"High-Performance Piezoelectric Nanogenerators Based on Wurtzite BeO Nanowire Arrays","authors":"Yoonseo Jang,&nbsp;Jihyeon Park,&nbsp;Seoyeah Oh,&nbsp;Jonghyun Bae,&nbsp;Prakash R. Sultane,&nbsp;Christopher W. Bielawski,&nbsp;Jiwon Kim,&nbsp;Jungwoo Oh","doi":"10.1002/admt.71136","DOIUrl":"https://doi.org/10.1002/admt.71136","url":null,"abstract":"<p>Wurtzite structured materials have been widely studied for piezoelectric nanogenerators (PENGs) due to their effective piezoelectric response. Among them, beryllium oxide (BeO) has high thermal conductivity (∼370 W/m·K at 300 K) and chemical stability makes it a promising candidate. However, the potential of BeO has been underexplored owing to the challenges in its nanoscale synthesis. In this study, we experimentally demonstrate for the first time the piezoelectric properties of BeO nanowires (NWs) and films. BeO NW arrays were synthesized via atomic layer deposition within anodic aluminum oxide templates. Structural and compositional analyses confirmed BeO NW formation, and piezoresponse force microscopy revealed an effective piezoelectric response with a longitudinal piezoelectric constant (<i>d<sub>33</sub></i>) of 15.8 pm/V for NW, compared to 4.8 pm/V for thin films. Additionally, the BeO NW-based PENG achieved a maximum output voltage of ∼26.1 V and a maximum power density of ∼0.32 µW/cm<sup>2</sup>, which significantly exceed those of thin films (∼12.0 V and ∼0.09 µW/cm<sup>2</sup>, respectively) and are comparable to those of conventional wurtzite material-based systems. These findings establish BeO as an experimentally validated wurtzite-type piezoelectric material and demonstrate its potential for energy harvesting, self-powered sensors, and reliable operation in harsh environments where thermal and chemical stability are essential.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.71136","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981496","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A Direction-Aware Piezo-Transmittance Strain Sensor via Engineered Alignment of Carbon Nanotubes (CNTs) 基于碳纳米管工程对准的定向压电透射应变传感器
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-07-07 DOI: 10.1002/admt.71130
Byeongmin Kang, Kwangjun Kim, Jimin Gu, Junseong Ahn, Yongrok Jeong, Ji-Hwan Ha, Sohee Jeon, Soonhyoung Hwang, Byung-Ho Kang, Jihyeon Ahn, Jong-An Choi, Minwook Kim, Yeonguk Jung, Jun-Ho Jeong, Jong G. Ok, Inkyu Park
{"title":"A Direction-Aware Piezo-Transmittance Strain Sensor via Engineered Alignment of Carbon Nanotubes (CNTs)","authors":"Byeongmin Kang,&nbsp;Kwangjun Kim,&nbsp;Jimin Gu,&nbsp;Junseong Ahn,&nbsp;Yongrok Jeong,&nbsp;Ji-Hwan Ha,&nbsp;Sohee Jeon,&nbsp;Soonhyoung Hwang,&nbsp;Byung-Ho Kang,&nbsp;Jihyeon Ahn,&nbsp;Jong-An Choi,&nbsp;Minwook Kim,&nbsp;Yeonguk Jung,&nbsp;Jun-Ho Jeong,&nbsp;Jong G. Ok,&nbsp;Inkyu Park","doi":"10.1002/admt.71130","DOIUrl":"https://doi.org/10.1002/admt.71130","url":null,"abstract":"<p>Stretchable and flexible strain sensors are essential components for next-generation wearable devices and human–machine interfaces. Among various approaches, piezo-transmittance-based strain sensors offer fast response and environmental stability. However, achieving both high sensitivity and precise directional decoupling remains a significant challenge. While sensors relying on random microcracks exhibit high gauge factors, their stochastic nature hinders axis-specific sensing. On the other hand, engineered macroscopic structures like metamaterials provide structural predictability, yet they often suffer from reduced sensitivity and notable mechanical crosstalk between orthogonal axes. In this study, a direction-aware piezo-transmittance strain sensor was developed by engineering a controlled linear gap-opening mechanism in an aligned carbon nanotubes (CNTs)/polydimethylsiloxane (PDMS) composite. The uniform gap-opening structure overcomes the limitations of traditional crack-based sensors, achieving enhanced directionality, high sensitivity (gauge factor ≈ 283), low detection limit (0.03%), and excellent sensor-to-sensor uniformity (relative standard deviation &lt; 12%). The sensor exhibits reliable performance over 17,621 strain cycles and enables precise multi-directional strain sensing through sensor arrays that quantitatively decouple orthogonal strain components. Finally, the developed sensor was integrated into wearable platforms, including attachment to joints and incorporation into stretchable exercise bands, demonstrating its potential for real-time human motion monitoring and for integration into wearable fitness and rehabilitation devices.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.71130","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981411","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Artificial Synaptic Device Based on Self-Aligned c-In2O3 TFTs With an Ultrathin MgO Interlayer 基于超薄MgO夹层自对准c-In2O3 tft的人工突触器件
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-07-05 DOI: 10.1002/admt.71145
Samiran Roy, Jewel Kumer Saha, Jin Jang
{"title":"Artificial Synaptic Device Based on Self-Aligned c-In2O3 TFTs With an Ultrathin MgO Interlayer","authors":"Samiran Roy,&nbsp;Jewel Kumer Saha,&nbsp;Jin Jang","doi":"10.1002/admt.71145","DOIUrl":"https://doi.org/10.1002/admt.71145","url":null,"abstract":"<p>In this work, we report a synaptic thin film transistor (TFT) based on crystalline indium oxide (c-In<sub>2</sub>O<sub>3</sub>), employing a plasma-enhanced chemical vapor deposition (PECVD) SiO<sub>2</sub> gate insulator (GI) and an ultrathin magnesium oxide (MgO) interlayer. Owing to high electron density c-In<sub>2</sub>O<sub>3</sub>, the TFT with SiO<sub>2</sub> GI exhibits conducting behavior. In contrast, the c-In<sub>2</sub>O<sub>3</sub>/MgO TFT demonstrates well-defined anticlockwise hysteresis with a large memory window of 17 V, a high I<sub>ON</sub>/I<sub>OFF</sub> ratio of 10<sup>8</sup>, and threshold voltage of 0 V. The interlayer passivates oxygen vacancies in c-In<sub>2</sub>O<sub>3</sub>, thereby reducing the carrier concentration. Meanwhile, mobile protons (H<sup>+</sup>) in the GI can contribute to the hysteresis through proton-related interfacial polarization, consistent with the capacitance response. The device successfully emulates key biological synaptic functions, including excitatory and inhibitory postsynaptic current (EPSC/IPSC), paired-pulse facilitation (PPF), short-term plasticity (STP), and long-term plasticity (LTP). Note that stable synaptic weight modulation is achieved over repeated potentiation and depression cycles. The results indicate the effectiveness of the MgO interlayer for achieving CCW hysteresis and reliable synaptic operation in coplanar In<sub>2</sub>O<sub>3</sub>-based TFTs, compatible with SiO<sub>2</sub> GI.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.71145","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981459","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Scaling Direct Ink Writing: A Multiscale Materials–Process–System Framework 缩放直接墨水书写:多尺度材料-过程-系统框架
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-07-09 DOI: 10.1002/admt.71147
Jochen Mueller
{"title":"Scaling Direct Ink Writing: A Multiscale Materials–Process–System Framework","authors":"Jochen Mueller","doi":"10.1002/admt.71147","DOIUrl":"https://doi.org/10.1002/admt.71147","url":null,"abstract":"<div>\u0000 \u0000 <p>Direct ink writing (DIW) enables unparalleled materials diversity and multimaterial integration, yet its scalability remains fundamentally constrained. Achievable part-size-to-feature-size ratios rarely exceed three orders of magnitude, highlighting a persistent gap between laboratory-scale resolution and manufacturing-scale throughput. This review shows that this limitation is not incidental, but arises from tightly coupled, multiscale constraints that preclude monotonic scaling of DIW processes. We develop a unified framework that identifies six interacting sources of limitation, spanning nozzle geometry, flow-rate and deposition dynamics, ink rheology, interlayer bonding, filament and structural mechanics, and system-level control and environmental effects. We treat material classes as boundary conditions for scalability and formulate scaling relationships that connect throughput, recovery kinetics, bonding windows, filament stability, and attainable part-size-to-feature-size ratios. These relations distinguish scaling barriers that are fundamentally materials-limited from those addressable through architectural or control innovations, and clarify how post-deposition transformation and constraint ultimately bound manufacturability at scale.</p>\u0000 </div>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981484","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
An Imaging-Guided, Patient-Specific Guiding Aid (RWNGuide) for Safe and Reproducible Inner Ear Drug Delivery 一种安全、可重复的内耳给药成像引导、患者特异性引导辅助装置(RWNGuide)
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-06-30 DOI: 10.1002/admt.71096
Yanjing Luo, Shanshan Jiang, Yimian Luo, Adele Moatti, Farnaz Matin-Mann
{"title":"An Imaging-Guided, Patient-Specific Guiding Aid (RWNGuide) for Safe and Reproducible Inner Ear Drug Delivery","authors":"Yanjing Luo,&nbsp;Shanshan Jiang,&nbsp;Yimian Luo,&nbsp;Adele Moatti,&nbsp;Farnaz Matin-Mann","doi":"10.1002/admt.71096","DOIUrl":"https://doi.org/10.1002/admt.71096","url":null,"abstract":"<p>Local drug delivery to the inner ear offers a promising approach for sensorineural hearing loss but remains challenging. Current techniques, direct round window injections, remain invasive, whereas trans-tympanic injection is imprecisions and surgeon-dependent, often failing to localize therapeutics within the round window niche (RWN). A patient-specific external ear guiding aid, RWNGuide, is developed as a precision guide for standardized, reproducible delivery to the RWN. Cone-beam computed tomography datasets from 23 patients are reconstructed to characterize the external ear channel (EEC) and RWN morphology. Computational modeling and trajectory optimization guide RWNGuide design, conforming to the EEC while maintaining coaxial alignment with the RWN. Devices are fabricated using Polyjet 3D printing and evaluated in human cadaveric temporal bones. Inserting fit, channel alignment, handling, and delivery accuracy are assessed and compared against conventional injection methods. RWNGuide demonstrates secure positioning, accurate channel orientation toward the RWN, and reproducible delivery without injury to adjacent middle ear structures. Quantitative surface analysis confirms sub-millimeter fit accuracy. Compared with trans-tympanic and direct RWN injections, RWNGuide improves delivery accuracy and safety, with longer procedural time due to intraoperative verification. This image-based, patient-specific device reduces procedural variability and enhances precision, supporting a scalable strategy for image-guided inner ear delivery.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.71096","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981497","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hierarchical-Structured Thermochromic Microcapsules With Second‑Scale Response and High‑Contrast for Low‑Temperature Visual Indicators 层次结构的热致变色微胶囊与第二尺度响应和低温视觉指标的高对比度
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-07-05 DOI: 10.1002/admt.71139
Fanghua Pan, Yuwei Hao, Shouzheng Jiao, Changcheng Han, Zhengyu Chen, Lu Han, Ruping Liu, Yuanyuan Liu, Yang Zhou, Zhicheng Sun
{"title":"Hierarchical-Structured Thermochromic Microcapsules With Second‑Scale Response and High‑Contrast for Low‑Temperature Visual Indicators","authors":"Fanghua Pan,&nbsp;Yuwei Hao,&nbsp;Shouzheng Jiao,&nbsp;Changcheng Han,&nbsp;Zhengyu Chen,&nbsp;Lu Han,&nbsp;Ruping Liu,&nbsp;Yuanyuan Liu,&nbsp;Yang Zhou,&nbsp;Zhicheng Sun","doi":"10.1002/admt.71139","DOIUrl":"https://doi.org/10.1002/admt.71139","url":null,"abstract":"<div>\u0000 \u0000 <p>Reliable temperature monitoring in cold chain logistics and food storage necessitates rapid detection of temperature excursions to ensure safety and quality. However, most existing approaches depend on powered sensors and complex data systems, limiting their suitability as passive, intuitive, and large area indicators for low temperature anomalies. Herein, raspberry-like low-temperature thermochromic microcapsules (RLTMs) were developed via a two-step interfacial polymerization approach as passive, large area visual indicators for low temperature monitoring. Structural analysis confirmed a hierarchical architecture with strong SiO<sub>2</sub> confinement, lowering the phase change onset from 12.1°C to −6°C and enabling graded thermal transitions. The RLTMs exhibited rapid, reversible color switching from −10°C to 37°C, achieving a visually distinct color difference (ΔE &gt; 50) within 2 s at −10°C and full transition within 10 s. This high sensitivity originated from multi scale surface curvature that enhances diffuse scattering while minimizing glare. After 50 thermal cycles, the microcapsules retained fast response (&lt;5 s) and high chromatic contrast, demonstrating excellent cycling stability. With a uniform size of 46.33 ± 5 µm, they can be directly screen printed as durable visual labels for food packaging and cold chain monitoring applications.</p>\u0000 </div>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981458","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Mask-Integrated Triboelectric Nanogenerator With Electrical Discharge Output and Sustained Wearability via Ultralight Silver-Coated Balls 通过超轻镀银球实现放电输出和持续耐磨性的掩膜集成摩擦电纳米发电机
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-06-30 DOI: 10.1002/admt.71138
Myunghwan Song, Sujung Kang, Seungjae Lee, Jaeung Choi, Minseok Kim, Jinkee Hong, Youngho Jin, Sangmin Lee
{"title":"Mask-Integrated Triboelectric Nanogenerator With Electrical Discharge Output and Sustained Wearability via Ultralight Silver-Coated Balls","authors":"Myunghwan Song,&nbsp;Sujung Kang,&nbsp;Seungjae Lee,&nbsp;Jaeung Choi,&nbsp;Minseok Kim,&nbsp;Jinkee Hong,&nbsp;Youngho Jin,&nbsp;Sangmin Lee","doi":"10.1002/admt.71138","DOIUrl":"https://doi.org/10.1002/admt.71138","url":null,"abstract":"<div>\u0000 \u0000 <p>Human breathing generates continuous low-frequency airflow in daily life, which can serve as a naturally available mechanical energy source for wearable energy harvesting without requiring additional user action. Breathing-driven airflow has attracted attention as an input source for mask-integrated self-powered wearable systems. However, breathing-induced airflow is typically low in intensity (3–6 m/s) and frequency (12–20 breaths/min). Even small structural additions to mask-based wearables can increase their weight and volume, thereby reducing their wearability. To address these challenges, we developed a mask-integrated ultralight triboelectric nanogenerator with silver-coated balls and a discharge-based power-generation structure. By coating the expanded polystyrene balls with silver paste, the device maintained metal-to-metal contact while minimizing weight. Under breathing-driven operation, the optimized device produced 22.4 V and 12.8 mA and remained electrically stable over 1 million operating cycles. These results indicate its potential as a compact, lightweight, and comfortable energy harvester for breathing-based wearable devices.</p>\u0000 </div>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981495","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
NaI-Mediated Dispersion of Cuprous Halide Clusters via Ball-Milling for Efficient White Light-Emitting Diodes 高效白光发光二极管中砷化亚铜团簇的球磨扩散
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-07-06 DOI: 10.1002/admt.71082
Ying Chu, Liang Chen, Chen Yu, Yuan Xie, Jia Jia, Aifei Wang, Tianshi Qin
{"title":"NaI-Mediated Dispersion of Cuprous Halide Clusters via Ball-Milling for Efficient White Light-Emitting Diodes","authors":"Ying Chu,&nbsp;Liang Chen,&nbsp;Chen Yu,&nbsp;Yuan Xie,&nbsp;Jia Jia,&nbsp;Aifei Wang,&nbsp;Tianshi Qin","doi":"10.1002/admt.71082","DOIUrl":"https://doi.org/10.1002/admt.71082","url":null,"abstract":"<div>\u0000 \u0000 <p>Cuprous (Cu(I)) halide clusters have garnered significant attention for light-emitting devices (LEDs) due to their high photoluminescence quantum yields and broadband emission, both originating from self-trapped excitons. However, their practical implementation is impeded by poor solution processability and challenges in fabricating high-quality films. Herein, we report a facile, scalable mechanochemical synthesis of highly luminescent Cu(I) halide clusters via direct ball milling under ambient conditions. Notably, the incorporation of sodium iodide enhances the dispersibility and solution processability of these clusters without deteriorating their emission properties, enabling the preparation of stable colloidal dispersions and the one-step solution deposition of smooth, uniform films. The resultant electroluminescent devices achieve a peak external quantum efficiency of 5.9% and exhibit uniform yellow emission over a large area of 5 × 5 cm<sup>2</sup>. Through judicious selection of charge-transport layers, we further demonstrate broadband white electroluminescence with voltage-tunable color temperature. Our strategy provides a practical pathway to efficient, scalable, and low-toxicity Cu(I) halide cluster LEDs, while offering key design principles for developing high-performance solution-processable emissive materials in next-generation solid-state lighting.</p>\u0000 </div>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981356","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Porous Silicon-Based Biosensors for Food Safety and Quality Monitoring: A Comprehensive Review 多孔硅基生物传感器在食品安全和质量监测中的应用综述
IF 6 3区 材料科学
Advanced Materials Technologies Pub Date : 2026-09-18 Epub Date: 2026-07-06 DOI: 10.1002/admt.71149
D. Nanda Kumar, Giorgi Shtenberg, Rangappa S. Keri
{"title":"Porous Silicon-Based Biosensors for Food Safety and Quality Monitoring: A Comprehensive Review","authors":"D. Nanda Kumar,&nbsp;Giorgi Shtenberg,&nbsp;Rangappa S. Keri","doi":"10.1002/admt.71149","DOIUrl":"https://doi.org/10.1002/admt.71149","url":null,"abstract":"<div>\u0000 \u0000 <p>Porous silicon (PSi) has attracted significant attention as a functional material for biosensing due to its tunable porosity, large surface area, and compatibility with various surface chemistries. This review highlights recent advances in PSi-based biosensors for food safety monitoring, covering the detection of bacteria, viruses, enzymes, mycotoxins, pesticides, heavy metals, and volatile organic compounds. Developments in optical and electrochemical transduction strategies, including reflectance interferometry, photoluminescence, impedance, and surface-enhanced Raman scattering, are discussed with emphasis on improving sensitivity and selectivity. Functionalization with aptamers, antibodies, peptides, and nanomaterials like Ag, TiO<sub>2</sub>, and ZnO has enabled rapid, label-free, and multiplexed detection of food contaminants at trace levels. In addition, hybrid and microstructured architectures, including Fabry–Pérot interferometers and photonic microcavities, have enhanced real-time signal response and analytical reproducibility. The integration of PSi with plasmonic nanostructures and portable platforms further supports its application in on-site monitoring. Future efforts should focus on improving stability, reproducibility, sensor miniaturization, and multiplex capability in complex food matrices. Combining PSi biosensors with artificial intelligence-assisted analysis and Internet of Things-enabled systems may further accelerate a sustainable, cost-effective, and scalable pathway for the development of intelligent and automated food safety diagnostics.</p>\u0000 </div>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"11 18","pages":""},"PeriodicalIF":6.0,"publicationDate":"2026-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148981352","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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