Advanced Materials Technologies最新文献_第5页

Masthead: (Adv. Mater. Technol. 20/2024) 刊头：（Adv. Mater. Technol.）

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-21 DOI: 10.1002/admt.202470094

引用次数: 0

Ambipolar Charge Injection and Bright Light Emission in Hybrid Oxide/Polymer Transistors Doped with Poly(9-Vinylcarbazole) Based Polyelectrolytes (Adv. Mater. Technol. 20/2024) 掺杂聚（9-乙烯基咔唑）基聚电解质的混合氧化物/聚合物晶体管中的双极电荷注入和亮光发射（Adv. Mater. Technol.）

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-21 DOI: 10.1002/admt.202470092

Yu Jung Park, Hee Kyung Hwang, Yejoo Park, Ju-Hyeon Lee, Jin Hee Lee, Bright Walker, Han-Ki Kim, Jung Hwa Seo

{"title":"Ambipolar Charge Injection and Bright Light Emission in Hybrid Oxide/Polymer Transistors Doped with Poly(9-Vinylcarbazole) Based Polyelectrolytes (Adv. Mater. Technol. 20/2024)","authors":"Yu Jung Park, Hee Kyung Hwang, Yejoo Park, Ju-Hyeon Lee, Jin Hee Lee, Bright Walker, Han-Ki Kim, Jung Hwa Seo","doi":"10.1002/admt.202470092","DOIUrl":"https://doi.org/10.1002/admt.202470092","url":null,"abstract":"Light-Emitting Electrochemical TransistorsThe cover image illustrates the integration of polyelectrolytes in light-emitting electrochemical transistors (LECTs), showcasing their multifunctional capabilities in electrochemistry and optoelectronics. In article number 2302207, Bright Walker, Han-Ki Kim, Jung Hwa Seo, and co-workers present LECTs that feature a streamlined device architecture enabled by electrochemical doping using poly(9-vinylcarbazole) doped with lithium ions (Li+) and copper (II) ions (Cu2+). The synergistic effects of these hybrid polyelectrolytes markedly enhance electron-hole recombination efficiency, resulting in bright and efficient electroluminescence.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture>\u0000 </div>\u0000 </figure>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"9 20","pages":""},"PeriodicalIF":6.4,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202470092","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142524741","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

An Artificial Tactile Perception System with Spatio-Temporal Recognition Capability (Adv. Mater. Technol. 20/2024) 具有时空识别能力的人工触觉感知系统（Adv. Mater. Technol.）

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-21 DOI: 10.1002/admt.202470096

Li Yuan, Tingting Zhao, Hao Zhang, Hai Liu, Yu Zong, Xingwei Ding, Jianhua Zhang

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High-Efficient Microfluidic Single-Cell Trapping and Arraying with Absolute Sequential Capture and High Success Rate of Perfect Capture

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-17 DOI: 10.1002/admt.202401018

Tingting Xuanyuan, Meilin Sun, Jinwei Zhang, Xufang Liu, Danyang Yu, Zeping Liu, Wenming Liu

{"title":"High-Efficient Microfluidic Single-Cell Trapping and Arraying with Absolute Sequential Capture and High Success Rate of Perfect Capture","authors":"Tingting Xuanyuan, Meilin Sun, Jinwei Zhang, Xufang Liu, Danyang Yu, Zeping Liu, Wenming Liu","doi":"10.1002/admt.202401018","DOIUrl":"https://doi.org/10.1002/admt.202401018","url":null,"abstract":"Methodological improvement to single-cell manipulation is critical for exploring the fundamentals of cellular life and unraveling biological complexity. Although micro-manipulation technologies capable of precise cell localization have been widely established, scaling existing platforms for highly efficient single-cell immobilization without sacrificing cell viability and sample quantity has proven challenging. Here, a highly efficient single-cell trapping and arraying approach is introduced by advancing the performance of a microfluidic mechanical trapping chip. The chip can achieve representative single-cell capture with over 99% efficiency and at least a 75% success rate of perfect capture, a precisely controlled single-cell array, absolute sequential cell captures without cell loss, and the maintenance of high cell viability during the whole manipulation process. This approach enables diverse single-cell trapping, large-scale arraying manipulations, and dynamic cellular and molecular analysis, and offers a path toward the development of high-performance single-cell systems.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 3","pages":""},"PeriodicalIF":6.4,"publicationDate":"2024-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143116265","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Engineering of the High-Power Laser-Induced Synthesis of Ni-Based Metal-Organic Framework: Investigation of its Optical Properties, Computational Methodology, Electrocatalytic Performances, and Glucose-Sensing Ability

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-16 DOI: 10.1002/admt.202401245

Saliha Mutlu, Bülend Ortaç, Ali Karatutlu, Taylan Gorkan, Engin Durgun, Dilek Söyler, Saniye Söylemez, Nergis Arsu, Sevil Savaskan Yılmaz

{"title":"Engineering of the High-Power Laser-Induced Synthesis of Ni-Based Metal-Organic Framework: Investigation of its Optical Properties, Computational Methodology, Electrocatalytic Performances, and Glucose-Sensing Ability","authors":"Saliha Mutlu, Bülend Ortaç, Ali Karatutlu, Taylan Gorkan, Engin Durgun, Dilek Söyler, Saniye Söylemez, Nergis Arsu, Sevil Savaskan Yılmaz","doi":"10.1002/admt.202401245","DOIUrl":"https://doi.org/10.1002/admt.202401245","url":null,"abstract":"Metal-organic frameworks (MOFs) are porous materials with numerous chemical and structural possibilities. Due to their ease of modification, well-organized structure, and diverse guest molecule chemistry, MOFs are ideal platforms for uncovering improved functional material design characteristics. Quantitative analysis of glucose is crucial, especially in some food products, for quality control as well as evaluation of the glucose levels helps diagnose and treat diabetes. Recent glucose sensing devices have relied heavily on MOFs and other nanomaterials to enable user-friendly and safe non-invasive sensing methods. Nevertheless, the conventional synthesis methods involve multi-day reactions, cooling, and depressurization processes. This study demonstrates the unprecedented high-power laser-induced rapid synthesis (LIRS) of Ni-based MOF nanospheres with interconnected nano-rods and noncentrosymmetric primitive triclinic crystalline structure, highlighting their multifunctional usage in sensing and gas sorption applications. Ab initio simulations show excellent agreement with the experimental physical and gas sorption properties. Furthermore, the Ni-MOF-based biosensor accurately measures glucose real-life beverage samples, yielding promising glucose detection biosensor results with a low limit of the detection (LOD) of 13.96 µM and high sensitivity of 120.606 µA mM−1 cm−2.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 3","pages":""},"PeriodicalIF":6.4,"publicationDate":"2024-10-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202401245","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143115999","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Efficient Large Area Semi-Transparent Dye-Sensitized Solar Cells (DSSCs) Printed with DMD400 Technology 用DMD400技术印刷的高效大面积半透明染料敏化太阳能电池（DSSCs）

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-12 DOI: 10.1002/admt.202400637

Mahfoudh Raïssi, Himal Muwanwella, Falak Naz, Anaïs Bianchi, Didier Rousseau, Muhammad Tariq Sajjad

{"title":"Efficient Large Area Semi-Transparent Dye-Sensitized Solar Cells (DSSCs) Printed with DMD400 Technology","authors":"Mahfoudh Raïssi, Himal Muwanwella, Falak Naz, Anaïs Bianchi, Didier Rousseau, Muhammad Tariq Sajjad","doi":"10.1002/admt.202400637","DOIUrl":"https://doi.org/10.1002/admt.202400637","url":null,"abstract":"This work presents the development of fully printed, large-area, semi-transparent Dye-Sensitized Solar Cells (DSSCs) using TiO2 nanoparticles treated with TiCl4, a “D35” push-pull dye sensitizer, and I3−/I− redox mediator. Cells with areas of 4 and 200 cm2 were printed using hexagonal, stripe, and standard designs, employing digital materials deposition (DMD) technology. The porous films printed via DMD, confirmed by scanning electron microscopy (SEM), improved solar cells performance by enhancing the Open Circuit Voltage (Voc) and fill factor (FF). The hexagonal design, in particular, facilitated better electrolyte impregnation in the TiO2 mesoporous structure, boosting current density. This design yielded a power conversion efficiency (PCE) of 7.05% for 4 cm2 DSSCs, surpassing the stripe (5.50%) and standard (5.48%) designs. Its higher performance can be attributed to lower interfacial charge recombination rates and improvedcharge transfer and collection efficiency. Photophysical measurements indicated faster charge transfer rates in hexagonal cells (≈ 1.3 × 109s−1) compared to the stripe (9.8 × 108 s−1) and standard (9.5 × 108 s−1) designs. Hence, our work highlights the potential of hexagonal design to improve both efficiency and transparency while reducing material consumption, offering a promising approach for manufacturing semi-transparent solar cells.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"9 23","pages":""},"PeriodicalIF":6.4,"publicationDate":"2024-10-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202400637","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142762817","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Multi-Layer LDPE Pouch Robots Enabled by Inkjet-Printed Masking Layers

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-10 DOI: 10.1002/admt.202401052

Yifan You, Chen Dai, Ezequiel Goldschmidt, Ronald S. Fearing

{"title":"Multi-Layer LDPE Pouch Robots Enabled by Inkjet-Printed Masking Layers","authors":"Yifan You, Chen Dai, Ezequiel Goldschmidt, Ronald S. Fearing","doi":"10.1002/admt.202401052","DOIUrl":"https://doi.org/10.1002/admt.202401052","url":null,"abstract":"Inflatable pouches are attractive as actuators and structural links in soft robots due to their low deflated profile and high deformation ratio. However, current pouch robot fabrication methods have relatively large minimum feature sizes and multi-layer fabrication challenges, limiting the integration of mechanisms with many independent degrees of freedom (DoF). A new monolithic prototype fabrication method utilizes inkjet printing of a masking ink layer, which prevents film bonding and thus defines inflatable regions. Multi-layer inflatable pouches of any planar geometry can be created using thermal fusing, with inter-layer connections and a minimum feature resolution of 0.3 mm. The multi-layer fabrication process enables the integration of pouches for bending actuation and structure, pneumatic channels, and external port connections. This high level of integration enables the fabrication of pouch robots with many independent DoFs. Specific examples using four layers of 38 micrometer thick Low-density polyethylene (LDPE) include 1) a 38 mm-wide 4-fingered robot hand with 8 independent DoFs which rotates a cube within its palm and 2) a 138 mm-long planar continuum manipulator with 10 independent DoFs for pick-and-place of a cylinder. These example designs demonstrate the capability of ink-patterned masking to achieve new levels of functionality for thin-film pouch robots.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 3","pages":""},"PeriodicalIF":6.4,"publicationDate":"2024-10-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143113909","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Analog-Digital Hybridity of Resistive Switching in Ion-Irradiated BiFeO3 Memristor for Synergistic Neuromorphic Functionality and Artificial Learning

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-09 DOI: 10.1002/admt.202400557

Suman Roy, Mousam Charan Sahu, Anjan Kumar Jena, Sameer Kumar Mallik, Roshan Padhan, Jyoti Ranjan Mohanty, Satyaprakash Sahoo

{"title":"Analog-Digital Hybridity of Resistive Switching in Ion-Irradiated BiFeO3 Memristor for Synergistic Neuromorphic Functionality and Artificial Learning","authors":"Suman Roy, Mousam Charan Sahu, Anjan Kumar Jena, Sameer Kumar Mallik, Roshan Padhan, Jyoti Ranjan Mohanty, Satyaprakash Sahoo","doi":"10.1002/admt.202400557","DOIUrl":"https://doi.org/10.1002/admt.202400557","url":null,"abstract":"Memristors-based neuromorphic devices represent emerging computing architectures to perform complex tasks by outpacing the traditional Von-Neumann architectures in terms of speed, and energy efficiency. In this work, the resistive switching (RS) behavior of sol-gel grown and ion-irradiated BFO films is investigated under electrical stimulus. The Ag/BFO/FTO memristors emulate a combination of digital and analog RS behavior within a single device. The possible mechanism of analog digital hybridity is addressed by considering the formation of the conducting filament by oxygen vacancies, Ag+ ions and Schottky barrier height modulation. The ion-irradiated BFO samples are analyzed using the Raman, XRD, and XPS studies. To uphold bioinspired synaptic actions, crucial synaptic functionalities like pair-pulse facilitation and long-term potentiation/depression are effectively achieved. More intricate synaptic behaviors are also demonstrated such as spike-time-dependent plasticity and Pavlovian classical conditioning, which represent the prominent attributes of both learning and forgetting behavior. Additionally, high pattern recognition accuracy (96.1%) is achieved in an artificial neural network simulation by using the synaptic weights of the memristors. This synergistic effect of digital and analog RS in ion-irradiated BFO can be beneficial for the emulation of complex learning behavior as well as its incorporation into low-power neuromorphic computing.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 2","pages":""},"PeriodicalIF":6.4,"publicationDate":"2024-10-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143113954","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Stretchable Wearable Wireless Bioelectronics Using All Printed Pressure Sensors and Strain Gauges

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-09 DOI: 10.1002/admt.202400998

Nathan Zavanelli, Yoon Jae Lee, Myungchul Kim, Allison Bateman, Matthew Guess, Hyeonseok Kim, Dinesh K. Patel, Woon-Hong Yeo

{"title":"Stretchable Wearable Wireless Bioelectronics Using All Printed Pressure Sensors and Strain Gauges","authors":"Nathan Zavanelli, Yoon Jae Lee, Myungchul Kim, Allison Bateman, Matthew Guess, Hyeonseok Kim, Dinesh K. Patel, Woon-Hong Yeo","doi":"10.1002/admt.202400998","DOIUrl":"https://doi.org/10.1002/admt.202400998","url":null,"abstract":"The sense of touch and perception of hand motion form an essential part of the somatic sensory system. Although piezoelectric sensors demonstrate high sensitivity and linearity, they are traditionally not employed for electronic skins because of their limited stretchability. Here, a printed, skin-conformal, electronic system consisting of stretchable piezoelectric pressure sensors and carbon nanotube strain gauges capable of identifying tactile sensations and joint movements on the hand is introduced. The pressure sensor demonstrates both high sensitivity (19.9 mV kPa−1) and linearity (0.1–1000 kPa) while being reliably stretchable to above 15%. To complement the pressure sensing functionality, a strain gauge is fabricated in a rapid stamp printing process and designed to demonstrate excellent mechanical reliability with up to 70% strain and high sensitivity (36.5-gauge factor). These sensors can seamlessly conform to numerous anatomical regions and cover wide areas of the skin, making them ideal for deployment in an electronic skin. Finally, the sensors are integrated with a flexible microelectronic device to demonstrate their functionality in human touch and prosthetic hand applications.","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 3","pages":""},"PeriodicalIF":6.4,"publicationDate":"2024-10-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202400998","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143113507","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

3D-Printed Hydrogel Filter for Biocatalytic CO2 Capture (Adv. Mater. Technol. 19/2024) 用于生物催化二氧化碳捕获的三维打印水凝胶过滤器（Adv. Mater. Technol.）

IF 6.4 3区材料科学

Advanced Materials Technologies Pub Date : 2024-10-07 DOI: 10.1002/admt.202470087

Sen Zhang, Jialong Shen, Peiqi Zhang, Thomas B. H. Schroeder, Jiahui Chen, Casey Carnevale, Sonja Salmon, Xiaomeng Fang

引用次数: 0