Advanced Materials Technologies最新文献

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Dual Enzyme Mimetic Activities of CuBiZr@PAH Nanocomposites for Enzyme Free Colorimetric Detection of Glucose and Uric Acid 双酶模拟活性CuBiZr@PAH纳米复合材料无酶比色法检测葡萄糖和尿酸
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-24 DOI: 10.1002/admt.202500693
Aniqa Sehrish, Romana Manzoor, Jingxian Li, Hongfen Yang, Ren Cai
{"title":"Dual Enzyme Mimetic Activities of CuBiZr@PAH Nanocomposites for Enzyme Free Colorimetric Detection of Glucose and Uric Acid","authors":"Aniqa Sehrish,&nbsp;Romana Manzoor,&nbsp;Jingxian Li,&nbsp;Hongfen Yang,&nbsp;Ren Cai","doi":"10.1002/admt.202500693","DOIUrl":"https://doi.org/10.1002/admt.202500693","url":null,"abstract":"<p>Novel colorimetric sensors are designed for ultrasensitive and highly efficient detection of glucose and uric acid (UA) based on dual enzyme mimetic activities of CuBiZr@PAH nanocomposite (P1). The colorimetric sensor utilizes the glucose oxidase-like (GOx) and peroxidase-like (POD) activities of P1 to detect glucose and UA. When P1 is present in a solution of glucose and 3,3′5,5′-tetramethylbenzidine (TMB), P1 catalyzes two cascade reactions: one between glucose and O<sub>2</sub> and the other between TMB and as-generated hydrogen peroxide (H<sub>2</sub>O<sub>2</sub>). The latter reaction provides visual results of glucose analysis with a LOD of 0.04 m<span>m</span> in the range of 0–40 m<span>m</span> in human serum samples. Furthermore, when P1 is present in a solution of UA, TMB, and H<sub>2</sub>O<sub>2</sub>, P1 catalyzes cascade reactions: one reaction between UA and H<sub>2</sub>O<sub>2</sub> and the other reaction between TMB + H<sub>2</sub>O<sub>2</sub>. UA suppresses the POD-like activity of P1 to detect UA with a LOD of 0.15 µ<span>m</span> in the range of 10 µ<span>m</span>–1.5 m<span>m</span> in urine samples. P1 exhibits dual enzyme mimetic activities for efficient detection of glucose and UA in real samples. The as-designed colorimetric sensors display high selectivity, good stability, excellent specificity, and desirable practicability for detecting glucose and UA in real samples.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230654","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Emerging NH3 MEMS-Sensing Techniques and Application 新兴NH3 mems传感技术及应用
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-22 DOI: 10.1002/admt.202500474
Yang Zhang, Minmin Zhao, Chao Tan, Zhu Zhang, Yi Ouyang, Lei Yang, Qiang Sun, Wei Wang, Zegao Wang, Mingdong Dong
{"title":"Emerging NH3 MEMS-Sensing Techniques and Application","authors":"Yang Zhang,&nbsp;Minmin Zhao,&nbsp;Chao Tan,&nbsp;Zhu Zhang,&nbsp;Yi Ouyang,&nbsp;Lei Yang,&nbsp;Qiang Sun,&nbsp;Wei Wang,&nbsp;Zegao Wang,&nbsp;Mingdong Dong","doi":"10.1002/admt.202500474","DOIUrl":"https://doi.org/10.1002/admt.202500474","url":null,"abstract":"<p>Ammonia, a highly toxic and corrosive gas associated with human health, has important application needs in industry, food, agriculture, and other fields. In the past years, the metal-oxide semiconductor (MOS)-based ammonia sensors have gained much attention and few oxides, nitrides, carbides, and their composites have been employed as the sensing materials, however, these sensors have large volume or requirement of high temperature characteristics, which hinder their application in current electronic system, especially in integrated circuits. Developing Micro-Electro-Mechanical System (MEMS)-based ammonia sensors with high integration and low consumption at room temperature become more and more urgent, but is still a challenge. How to compensate the benefit contributing from the high-ratio-of-surface of MOS-sensor in MEMS-sensor. This review briefly introduces and discusses the on-chip ammonic sensing mechanism and the influence factors. Then, most representative chemical resistance sensors in ammonia sensing, as well as diodes and field-effect transistors sensors related to integrated circuits are summarized. The main coupling strategies used to enhance gas sensitivity in recent years are discussed. Finally, the development prospect of high-performance MEMS-based ammonia sensor is discussed.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230788","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High Photoluminescence Quantum Yield and Tunable Luminescence Lifetimes in the Sub-Second Range of CaS:Eu2+ Phosphors for Tracer Based Sorting 基于示踪剂分选的CaS:Eu2+荧光粉在亚秒范围内的高光致发光量子产率和可调发光寿命
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-22 DOI: 10.1002/admt.202500353
Arzu Cosgun Ergene, Eduard Madirov, Dmitry Busko, Ian A. Howard, Bryce S. Richards, Andrey Turshatov
{"title":"High Photoluminescence Quantum Yield and Tunable Luminescence Lifetimes in the Sub-Second Range of CaS:Eu2+ Phosphors for Tracer Based Sorting","authors":"Arzu Cosgun Ergene,&nbsp;Eduard Madirov,&nbsp;Dmitry Busko,&nbsp;Ian A. Howard,&nbsp;Bryce S. Richards,&nbsp;Andrey Turshatov","doi":"10.1002/admt.202500353","DOIUrl":"https://doi.org/10.1002/admt.202500353","url":null,"abstract":"<p>The shift toward a circular economy for plastics requires innovative sorting technologies that improve recycling efficiency and material purity. Tracer-based sorting (TBS) is a promising approach that employs luminescent tracers with distinct optical properties for the precise identification of plastics. This study presents the synthesis and characterization of europium-doped calcium sulfide (CaS:Eu<sup>2+</sup>) luminescent materials as potential tracers for TBS. Synthesized via a flux-assisted solid-state reaction, these phosphors achieve photoluminescence quantum yields (PLQYs) of up to 65% with tunable luminescence decay lifetimes ranging from 0.05 to 0.3 seconds. Long-term chemical stability under ambient conditions is confirmed over 18 months. The application of CaS:Eu<sup>2+</sup> in a TBS prototype is demonstrated using a standard CMOS video camera to differentiate materials based on decay times. These results highlight the suitability of CaS:Eu<sup>2+</sup> phosphors as stable, high-performance tracers, offering a viable way to improve plastics recycling processes.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202500353","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230797","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Macroscopic Phase-Change Drug Carrier Ball with Photothermally Controlled Release and Magnetically Controlled Transport Properties 具有光热控释和磁控输运性质的宏观相变药物载体球
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-22 DOI: 10.1002/admt.202500694
Hyunji Lee, Jihyeok Park, Minkyeong Kang, Woochan Kim, Sang Kug Chung, Joohyung Lee
{"title":"Macroscopic Phase-Change Drug Carrier Ball with Photothermally Controlled Release and Magnetically Controlled Transport Properties","authors":"Hyunji Lee,&nbsp;Jihyeok Park,&nbsp;Minkyeong Kang,&nbsp;Woochan Kim,&nbsp;Sang Kug Chung,&nbsp;Joohyung Lee","doi":"10.1002/admt.202500694","DOIUrl":"https://doi.org/10.1002/admt.202500694","url":null,"abstract":"<p>Phase-change materials (PCMs) are widely regarded as effective thermo-responsive gating materials for on-demand drug release. Most previous studies utilizing PCMs for this purpose focus on small colloidal micro- and nanoparticles. In this study, macroscopic phase-change drug carriers are demonstrated in the form of millimeter-sized balls, which offer enhanced visibility. These wax-based phase-change macroballs, composed of paraffin, fatty alcohols, or fatty acids, can be easily fabricated with customizable volumes by depositing melted wax droplets containing functional components–such as drugs, photothermal agents, surfactants, and magnetites–onto omniphobic surfaces, where they spontaneously dewet and solidify upon natural cooling. These macroballs can be rapidly heated and melted upon near-infrared irradiation due to the incorporation of low-melting-point liquid metal (LM) eutectic Ga–In microdroplets as photothermal agents, enabling efficient on-demand drug release. Furthermore, by adsorbing magnetically susceptible Fe₃O₄ nanoparticles onto the LM microdroplets, the transport of the macroballs becomes magnetically controllable, as demonstrated by the use of a permanent magnet or electromagnet. The strategies demonstrated in this study provide a simple and scalable approach to fabricating high-visibility, trackable macroscopic phase-change balls with on-demand photothermal drug release and magnetically controlled transport properties.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202500694","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230807","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Droplet-Based Synthesis of Nanogels for Controlled Drug Delivery via Two Photon Polymerization-3D Printed Microfluidic Device 基于液滴的双光子聚合纳米凝胶合成- 3d打印微流控装置
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-22 DOI: 10.1002/admt.202500108
Vladimir Matining, Camillo Colli, Emanuela Jacchetti, Giulia Nicoletti, Laura Rosanò, Manuela Teresa Raimondi, Bianca Maria Colosimo, Emanuele Mauri, Davide Moscatelli
{"title":"Droplet-Based Synthesis of Nanogels for Controlled Drug Delivery via Two Photon Polymerization-3D Printed Microfluidic Device","authors":"Vladimir Matining,&nbsp;Camillo Colli,&nbsp;Emanuela Jacchetti,&nbsp;Giulia Nicoletti,&nbsp;Laura Rosanò,&nbsp;Manuela Teresa Raimondi,&nbsp;Bianca Maria Colosimo,&nbsp;Emanuele Mauri,&nbsp;Davide Moscatelli","doi":"10.1002/admt.202500108","DOIUrl":"https://doi.org/10.1002/admt.202500108","url":null,"abstract":"<p>Nanogels (NGs) show great potential for innovative therapies due to their capability of reproposing the hydrogels features at the nanoscale. However, conventional batch syntheses exhibit shortcomings that bind the control over the reaction parameters and batch-to-batch reproducibility. Droplet-based microfluidics represents a valuable strategy to overcome these constraints, enabling precise manipulation of fluids/molecules to design nanoscaffolds. Standard microfluidic fabrication methods, such as soft lithography, hot-embossing or molding, require multistep process, and the successful fabrication depends on several factors, including the operator expertise. This work proposes two-photon polymerization (TPP) 3D printing as a straightforward method to produce a microfluidic device for droplet-based synthesis of NGs. The microfluidic platform enables controlled generation of microdroplets (150–80 µm, with size variation up to 47%), which work as microreactors, allowing modulation of NG dimensions (320–175 nm) and properties, while preserving an extremely low polydispersity (&lt;0.1). NGs composed of polyallylamine and hyaluronic acid are synthesized and evaluated in vitro for cisplatin delivery in ovarian cancer cells. Compared to free drug administration, NG-mediated delivery enhances the therapeutic effect by ≈30% after 72 h. This highlights the potential of the nanomaterial in tumoral scenarios and proves the functionality of the TPP-printed microfluidic device in NG droplet-based synthesis.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202500108","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230787","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A Reconfigurable Soft Actuator with Tunable Deformation and Stiffness 一种变形和刚度可调的可重构软执行器
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-22 DOI: 10.1002/admt.202500772
Zhiwen Song, Cunxiang Wei, Zichao Wang, Bozhen Liu, Xuegang Zhang, Yongxin Song
{"title":"A Reconfigurable Soft Actuator with Tunable Deformation and Stiffness","authors":"Zhiwen Song,&nbsp;Cunxiang Wei,&nbsp;Zichao Wang,&nbsp;Bozhen Liu,&nbsp;Xuegang Zhang,&nbsp;Yongxin Song","doi":"10.1002/admt.202500772","DOIUrl":"https://doi.org/10.1002/admt.202500772","url":null,"abstract":"<p>Currently, it is challenging for a soft actuator to simultaneously achieve tunable deformation and maintain high load capacity. To address this issue, this paper presents a reconfigurable soft actuator with tunable deformation and stiffness (RATDS). The soft actuator consists of a skeleton and a thermoplastic polyurethane (TPU) skin. The skeleton is composed of two shapes of cavity units with particles filled and a polyethylene terephthalate (PET) sheet. It can realize various deformations with different assembly models of the cavity units under vacuum pressure. Stiffness variation is achieved by increasing vacuum pressure, causing the cavities to shrink and leading to particle jamming. The convenient manufacturing and assembly methods are demonstrated. The finite element analysis (FEA) simulations and experiments show that the actuator's deformation can transition from 2D bending to 3D twisting and multi-direction deformation with different assembly models, respectively. Durability experiments confirm its functionality even after 5000 cycles. The actuator exhibits fast response time (0.35 s) excellent stiffness enhancement (from 0.019 N mm<sup>−1</sup> (0 kPa) to 0.219 N mm<sup>−1</sup>(−40 kPa)) and good tip force (averaging 3.85 N). Furthermore, it shows good grasping capabilities (maximum loads 2110 g (three-finger gripper) and 700 g (single-finger gripper)) and crawling capability (10.7 mm s<sup>−1</sup>).</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230806","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Flow Analysis in Pathological Microvascular Models by Ultrasound Localization Microscopy 病理微血管模型的超声定位显微镜血流分析
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-20 DOI: 10.1002/admt.202402208
Yarin Gershman, Grigori Shapiro, Tamar Mano, Tali Ilovitsh
{"title":"Flow Analysis in Pathological Microvascular Models by Ultrasound Localization Microscopy","authors":"Yarin Gershman,&nbsp;Grigori Shapiro,&nbsp;Tamar Mano,&nbsp;Tali Ilovitsh","doi":"10.1002/admt.202402208","DOIUrl":"https://doi.org/10.1002/admt.202402208","url":null,"abstract":"<p>This study presents a new class of ultrasound-compatible gelatin-based phantoms designed to mimic microvascular pathologies, such as vessel narrowing and blockages, in small arteries and arterioles. These phantoms enable detailed investigation of blood flow dynamics under pathological conditions. Using ultrasound localization microscopy (ULM), microbubble (MB) contrast agents are tracked to generate high-resolution velocity maps for assessing flow alterations within microvascular structures. MB velocities ranging from 0.01 to 25 mm s<sup>−1</sup> are quantified in phantoms with 60% and 80% constriction, demonstrating strong agreement with computational fluid dynamics (CFD) simulations. Phantoms with main channels of 500 µm and bifurcations narrowing to 200 and 100 µm are used to study the effects of geometric narrowing on flow dynamics. The redevelopment length of flow depended on narrowing severity and velocity, ranging from 0.2 to 0.85 mm for velocities of 3.3 to 33.3 mm s<sup>−1</sup>. A four-outlet phantom replicated complex vascular structures to explore obstruction-induced flow alterations. This platform serves as a versatile tool for studying clinically relevant microvascular conditions, providing valuable insights into disease mechanisms and therapeutic strategies. By bridging imaging and translational research, this study highlights the potential of ULM and biomaterial-based phantoms to advance diagnostics and treatment of small vessel diseases.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202402208","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230573","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advanced Time Series Data Processing Using Various Memristor-Integrated Devices 先进的时间序列数据处理使用各种忆阻器集成器件
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-20 DOI: 10.1002/admt.202500838
Sung Keun Shim, Joon-Kyu Han, Janguk Han, Soo Hyung Lee, Dong Hoon Shin, Sunwoo Cheong, Sungho Kim, Hanyong Jeong, Yoon Ho Jang, Cheol Seong Hwang
{"title":"Advanced Time Series Data Processing Using Various Memristor-Integrated Devices","authors":"Sung Keun Shim,&nbsp;Joon-Kyu Han,&nbsp;Janguk Han,&nbsp;Soo Hyung Lee,&nbsp;Dong Hoon Shin,&nbsp;Sunwoo Cheong,&nbsp;Sungho Kim,&nbsp;Hanyong Jeong,&nbsp;Yoon Ho Jang,&nbsp;Cheol Seong Hwang","doi":"10.1002/admt.202500838","DOIUrl":"10.1002/admt.202500838","url":null,"abstract":"<p>Modern edge devices, from wearable health monitors to robot-mounted sensors, generate continuous streams of time-series data that require fast and energy-efficient processing. Memristors, which combine memory and computation in a compact device, offer a promising solution for real-time hardware-based temporal data analysis. This perspective reviews how memristors are used in time-series processors, focusing on two main approaches: conventional reservoir computing (RC) architectures and newly emerging temporal kernels (TKs). While RC systems often rely on volatile memristors and network structures to extract features from time-varying signals, TKs enhance flexibility by combining memristors with circuit elements like resistors, capacitors, or semiconductor devices. This feature allows precise tuning of signal delays, thresholds, and nonlinear behaviors. Several representative TK designs and variations are introduced, each with strengths in capturing different temporal features. These are well suited for edge applications where quick and selective signal processing is essential. Future efforts must focus on optimizing kernel behavior and integrating TKs directly with sensors to move toward practical use. This direction can enable real-time tasks such as on-device health monitoring, biometric authentication, and adaptive sensing, positioning memristive TKs as a core technology for next-generation intelligent edge systems.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 15","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202500838","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144782914","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Biomimetic Hierarchical Fabric with Thermochromic-Superhydrophobic Dual-Functionality for Adaptive Radiative Cooling and Self-Cleaning 具有热致变色-超疏水双功能的自适应辐射冷却和自清洁仿生分层织物
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-20 DOI: 10.1002/admt.202500540
Jing Tan, Ningbo Cheng, Na Meng, Xianfeng Wang, Jianyong Yu, Bin Ding
{"title":"Biomimetic Hierarchical Fabric with Thermochromic-Superhydrophobic Dual-Functionality for Adaptive Radiative Cooling and Self-Cleaning","authors":"Jing Tan,&nbsp;Ningbo Cheng,&nbsp;Na Meng,&nbsp;Xianfeng Wang,&nbsp;Jianyong Yu,&nbsp;Bin Ding","doi":"10.1002/admt.202500540","DOIUrl":"https://doi.org/10.1002/admt.202500540","url":null,"abstract":"<p>Passive radiative cooling textiles confront the trilemma of balancing chromatic aesthetics, self-adaptive radiative cooling, and environmental durability. Herein, inspired by hierarchical structures of taro-leaf, biomimetic thermochromic radiative cooling fabric (TRCF) is developed through an innovative evaporation/vapor-induced phase separation (E-VIPS) technique. This phase separation strategy integrates poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP), polyurethane (PU), and thermochromic microcapsules (TCMC) into multi-scale porous networks featuring rough surface topography and optical structure. The resultant fabric demonstrates temperature-modulated visible reflectance enhancement (ΔR = 6.56–14.67%). Notably, the prepared yellow, red, and blue TRCF exhibit high solar reflectance of 95.5%, 90.9%, and 89.9%, with strong infrared emissivity of 91.4%, 90.6%, and 92.4%. Actual outdoor cooling tests show that the yellow, red, and blue TRCF achieve sub-ambient cooling performance with temperature reductions of approximately 7.8 °C, 5.5 °C, and 2.2 °C, respectively, relative to the substrate. In addition, the biomimetic microstructure's rough structure endows the material with exceptional superhydrophobicity for durability, while retaining self-cleaning functionality after 30 cycles of abrasion. This work pioneers a pathway toward adaptive, multifunctional textiles for sustainable outdoor thermal management.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230822","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Pick-and-Place Grippers with Tunable Adhesion from Capped Soft Hollow Pillar Structure 拾取和放置夹持器可调附着力从封顶软空心支柱结构
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-06-19 DOI: 10.1002/admt.202500216
Yanbing Tang, Farshad Goodarzi, Guangchao Wan, Wanliang Shan
{"title":"Pick-and-Place Grippers with Tunable Adhesion from Capped Soft Hollow Pillar Structure","authors":"Yanbing Tang,&nbsp;Farshad Goodarzi,&nbsp;Guangchao Wan,&nbsp;Wanliang Shan","doi":"10.1002/admt.202500216","DOIUrl":"10.1002/admt.202500216","url":null,"abstract":"<p>Dynamically tunable dry adhesion has numerous applications in biological systems and industrial processes. Soft hollow pillars (SHPs) have demonstrated to have exceptional adhesion tunability under pneumatic actuation through sidewall buckling or bulging mechanisms. However, the adhesion strength of SHPs is significantly lower than that of solid elastomeric pillars, which can limit their practical use. In this study, mushroom-shaped SHPs with a mushroom cap, or capped SHPs (C-SHPs), are introduced to enhance the adhesion performance of soft grippers based on hollow pillar structures. Experiments and finite element modeling demonstrate that the cap significantly improves adhesion strength (1.8 to 2.9×) and adhesion tunability (∼1000×) by optimizing stress distribution and altering the crack initiation process at the contact interface. The effect of the cap size on the adhesion strength of C-SHPs under various pressures is systematically investigated. Miniaturized SHPs and C-SHPs are fabricated for pick-and-place manipulation of lightweight objects. An untethered device containing a C-SHP is designed and assembled to highlight the energy-efficient operation of C-SHPs, with a ∼139 mJ energy consumption per pick-and-place cycle, showcasing their potential for applications in precision handling tasks. This work establishes C-SHPs as a robust and adaptable solution for tunable dry adhesion systems.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 18","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-06-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202500216","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145101924","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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