Progress in Materials Science最新文献_第2页

Dynamic crosslinked elastomers and rubbers 动态交联弹性体和橡胶

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-07-11 DOI: 10.1016/j.pmatsci.2025.101536

Jing Bai , Baochun Guo , Ming Tian , Fei Chen , Liqun Zhang

{"title":"Dynamic crosslinked elastomers and rubbers","authors":"Jing Bai , Baochun Guo , Ming Tian , Fei Chen , Liqun Zhang","doi":"10.1016/j.pmatsci.2025.101536","DOIUrl":"10.1016/j.pmatsci.2025.101536","url":null,"abstract":"<div><div>Classical rubbers and elastomers are normally prepared via a crosslinking process such as vulcanization, which can produce permanent covalently crosslinked structures and endows mechanical robustness, chemical resistance and thermal stability. However, the permanent covalently crosslinked networks make rubbers and elastomers cannot be reprocessed, reshaped or recycled,causing serious pollution and negative impacts on the environment. The design of dynamic covalent crosslinked structures in polymers brings new properties to classical rubber and elastomer materials, in particular in terms of thermal responses, reprocessability and recycling abilities.In recent years, there has been agrowing interest in the design and synthesis of dynamic crosslinked polymers. In this review, the designs, characterizations, and utilizations of dynamic crosslinked elastomers and rubbers are summarized, focusing on the design and synthesis of dynamic crosslinked elastomers and rubbers with sustainability and recyclability, followed by an overview of the applications of dynamic crosslinked elastomers and rubbers. Furthermore, through the tuning and controlling on the dynamic crosslinked structure variedly, some functional behaviors can be realized. To declare and promote the consequence and potential utilization of the dynamic crosslinked elastomers and rubbers, perspectives and suggestions are presented for future research on the design, synthesis, and process strategies of dynamic crosslinked elastomers and rubbers.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"155 ","pages":"Article 101536"},"PeriodicalIF":33.6,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144611471","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Smart responsive materials for antibacterial therapy: Progress, opportunities, and challenges 抗菌治疗用智能反应材料：进展、机遇和挑战

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-07-10 DOI: 10.1016/j.pmatsci.2025.101532

Jieni Fu , Chaofeng Wang , Xiangmei Liu , Shengli Zhu , Yufeng Zheng , Zhaoyang Li , Zhenduo Cui , Yu Zhang , Hui Jiang , Yongping Cao , Paul K Chu , Shuilin Wu

{"title":"Smart responsive materials for antibacterial therapy: Progress, opportunities, and challenges","authors":"Jieni Fu , Chaofeng Wang , Xiangmei Liu , Shengli Zhu , Yufeng Zheng , Zhaoyang Li , Zhenduo Cui , Yu Zhang , Hui Jiang , Yongping Cao , Paul K Chu , Shuilin Wu","doi":"10.1016/j.pmatsci.2025.101532","DOIUrl":"10.1016/j.pmatsci.2025.101532","url":null,"abstract":"<div><div>Bacterial infections threaten global human health, driving the rapid development of antibacterial materials over the past two decades. However, the clinical application is limited due to the rapid presence of antibiotic-resistant bacteria and the brutal penetration of biofilm. ’Smart’ responsive antibacterial materials (SRAMs) that respond to endogenous/exogenous stimuli to release antibacterial factors are appealing therapeutic agents for developing next-generation antibacterial materials. Those materials can evade existing mechanisms associated with acquired drug resistance and could also provide an alternative strategy to treat biofilms due to their spatiotemporal controllability and negligible side effects. SRAMs have emerged as a promising tool to combat bacterial infections that are difficult to treat. To better understand the interaction between SRAMs and biological tissues, this review highlights the mechanisms underlying SRAM-mediated eradication of both planktonic bacteria and biofilms and recent advances in designing SRAMs that respond to internal/external stimuli. Meanwhile, we also summarize the latest progress in the development of SRAMs. Properties of internal- or external-stimuli-responsive smart antibacterial materials are outlined, and we also discuss the potential features required for antibacterial applications of various infectious diseases. Furthermore, it also discussed the current challenges and future prospects, particularly emphasizing clinical translation for these smart antimicrobial platforms.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"155 ","pages":"Article 101532"},"PeriodicalIF":33.6,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144594796","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Computation- and process-based design for advanced structural high-entropy alloy development and analyses: A critical review 先进结构高熵合金开发与分析的基于计算和过程的设计综述

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-07-09 DOI: 10.1016/j.pmatsci.2025.101534

Zaigham Saeed Toor , Renhao Wu , Muhammad Raihan Hashmi , Jeong Ah Lee , Xiaoqing Li , Harada Yuji , Haiming Zhang , Hyoung Seop Kim

{"title":"Computation- and process-based design for advanced structural high-entropy alloy development and analyses: A critical review","authors":"Zaigham Saeed Toor , Renhao Wu , Muhammad Raihan Hashmi , Jeong Ah Lee , Xiaoqing Li , Harada Yuji , Haiming Zhang , Hyoung Seop Kim","doi":"10.1016/j.pmatsci.2025.101534","DOIUrl":"10.1016/j.pmatsci.2025.101534","url":null,"abstract":"<div><div>Over the past decades, high-entropy alloys (HEAs) have been rapidly designed, developed, prepared, and tested to achieve superior performance across a multitude of applications. Computational materials science driven design techniques, including molecular dynamics, density functional theory, calculation of phase diagrams, phase-field modeling, crystal plasticity modelling, and artificial intelligence, combined with additive manufacturing and severe plastic deformation, present unprecedented opportunities to tailor microstructural features with remarkable flexibility and feasibility. This integration significantly enhances material properties. This review paper focuses on the computation-driven and processing-guided designs for structural HEAs (SHEAs), focusing on the relationship among materials, processing, microstructures, and properties. A succinct introduction to the computational design of SHEAs is first presented. Following this, we delve into the complex interplay between computational microstructures at various scales and the mechanical properties of SHEAs, revealing the underlying mechanisms. Additionally, we explore the distinctive features, advantages, and practical applications of these promising materials have been further explored. In conclusion, we address the prevailing challenges and anticipate future prospects in this burgeoning field.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"155 ","pages":"Article 101534"},"PeriodicalIF":33.6,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144594738","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Smart micro/nanorobots for drug delivery in the brain 用于大脑药物输送的智能微/纳米机器人

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-07-06 DOI: 10.1016/j.pmatsci.2025.101533

Di Shi , Xiang Wang , Yulin Deng , Huaijuan Zhou , Yilong Wang , Paul K. Chu , Jinhua Li

{"title":"Smart micro/nanorobots for drug delivery in the brain","authors":"Di Shi , Xiang Wang , Yulin Deng , Huaijuan Zhou , Yilong Wang , Paul K. Chu , Jinhua Li","doi":"10.1016/j.pmatsci.2025.101533","DOIUrl":"10.1016/j.pmatsci.2025.101533","url":null,"abstract":"<div><div>Pharmacotherapy is the core approach for treating various brain diseases. However, the intricate anatomical structure and the blood–brain barrier (BBB) of the brain present challenges for intracerebral drug delivery and therapeutic efficacy. Although systemic administration and surgical interventions can alleviate symptoms, they are limited by low therapeutic effects and potential adverse side effects. Moreover, due to their complex pathogenesis, insidious development, and deep-seated lesions, brain diseases are difficult to diagnose accurately. To address these challenges, there is an urgent need to develop intelligent nanocarriers that can efficiently load drugs and penetrate the BBB for precise therapy of brain diseases. In this connection, micro/nanorobots (MNRs) are multifunctional drug carriers at the micro-nano scale, which possess exceptional penetration and targeting capabilities. Employing externally powered propulsion or chemical self-propulsion, MNRs can navigate in the brain and cross the BBB. This review comprehensively summarizes the recent advances and future outlook of smart MNR drug delivery systems for brain disease treatment. It covers broad topics from nanocarriers to active smart MNRs. Furthermore, it elucidates the therapeutic mechanisms of these smart MNR drug delivery systems in brain diseases based on pathogenesis and pathology. Our aim is to provide a reference for designing and developing novel smart MNRs for drug delivery in the brain, paving the way for their clinical applications in treating brain diseases.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"155 ","pages":"Article 101533"},"PeriodicalIF":33.6,"publicationDate":"2025-07-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144568882","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Stimuli-responsive shape-morphing soft actuators: metrics, materials, mechanism, design and applications 刺激响应变形软致动器：指标，材料，机制，设计和应用

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-07-05 DOI: 10.1016/j.pmatsci.2025.101531

Linchao Sun , Zhong Li , Yan Zhang , Yao Lu , Shiguo Zhang

{"title":"Stimuli-responsive shape-morphing soft actuators: metrics, materials, mechanism, design and applications","authors":"Linchao Sun , Zhong Li , Yan Zhang , Yao Lu , Shiguo Zhang","doi":"10.1016/j.pmatsci.2025.101531","DOIUrl":"10.1016/j.pmatsci.2025.101531","url":null,"abstract":"<div><div>The rapid development of flexible wearable devices and the integration of artificial intelligence (AI) in robotics have driven the evolution of soft actuators, positioning soft shape-morphing actuators at the forefront of cutting-edge research in soft robotics, intelligent devices, and bio-inspired engineering. Stimuli-responsive soft actuators are intelligent devices constructed from flexible materials capable of precise and controllable deformation in response to external stimuli, attracting growing scientific and technological interest. This review systematically delineates and evaluates critical performance metrics essential for evaluating actuator functionality. It offers a comprehensive analysis of the predominant stimuli-responsive actuating materials, elucidating their actuation mechanisms while critically examining their inherent advantages, limitations, and emerging research trajectories. Fundamental design principles are meticulously articulated to guide the development of next-generation shape-morphing actuators. Furthermore, this review extensively surveys diverse practical applications, underscoring the versatility and broad technological impact of stimuli-responsive soft actuators across multiple domains. Finally, key challenges in the current state-of-the-art and prospective research pathways are thoroughly discussed, aiming to foster the development and widespread adoption of soft actuators in both academic research and industrial applications.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"155 ","pages":"Article 101531"},"PeriodicalIF":33.6,"publicationDate":"2025-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144566676","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Bioinspired multifunctional antifogging surfaces: Progress, AI design and challenges 仿生多功能防雾表面：进展、人工智能设计和挑战

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-07-02 DOI: 10.1016/j.pmatsci.2025.101530

Hanpeng Gao , Zetian Xing , Siyu Chang , Fangyi Zhao , Honglin Zhang , Zong Meng , Zhiwu Han , Yan Liu

{"title":"Bioinspired multifunctional antifogging surfaces: Progress, AI design and challenges","authors":"Hanpeng Gao , Zetian Xing , Siyu Chang , Fangyi Zhao , Honglin Zhang , Zong Meng , Zhiwu Han , Yan Liu","doi":"10.1016/j.pmatsci.2025.101530","DOIUrl":"10.1016/j.pmatsci.2025.101530","url":null,"abstract":"<div><div>Over the past few decades, various antifogging strategies and preparation methods have been proposed. Unfortunately, a surface with a single antifogging function cannot achieve a wide range of practical applications. For example, medical endoscopes require antifogging and antibacterial capabilities to improve diagnostic accuracy and safety. Inspired by the near-perfect multifunctional properties of natural creatures, antifogging materials with specific functions have drawn more and more attention owing to their promising and wide applications. However, the design of bioinspired antifogging surfaces with broad applicability still presents some challenges, such as the integration of multifunctional properties, and the optimization of preparation routes. In this review, beginning with the fogging mechanism and wettability theory, the latest antifogging surface materials and pattern designs are analyzed in detail and critically evaluated. The natural biomaterials with multifunctional characteristics are summarized, and the integration mechanism and design difficulties of the four multifunctional characteristics are then emphatically analyzed. Based on artificial intelligence (AI) assisted design optimization, we introduce the neural network into the bionic multifunction antifogging path realization for the first time and summarize the antifogging prototype and antifogging multifunction database. Finally, the challenges and future trends of bioinspired multifunction antifogging surfaces (MF-AFS) are presented.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"155 ","pages":"Article 101530"},"PeriodicalIF":33.6,"publicationDate":"2025-07-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144533707","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Flame-retardant strategies for lignocellulose: recent progress and prospect 木质纤维素阻燃策略：最新进展与展望

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-06-28 DOI: 10.1016/j.pmatsci.2025.101529

Huayu Liu , Yeling Zhu , Yuhang Ye , Isabella Therrien , Felix Wiesner , Feng Jiang

引用次数: 0

Triptycene-based porous organic network polymers: From synthesis to applications 三苯基多孔有机网状聚合物：从合成到应用

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-06-26 DOI: 10.1016/j.pmatsci.2025.101528

Akhtar Alam, Atikur Hassan, Neeladri Das

引用次数: 0

Dynamic bioinks for tissue/organ bioprinting: Principle, challenge, and perspective 用于组织/器官生物打印的动态生物墨水：原理、挑战和前景

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-06-20 DOI: 10.1016/j.pmatsci.2025.101527

Duo Ma , Juan Liu , William Weijia Lu , Wenguang Liu , Changshun Ruan

{"title":"Dynamic bioinks for tissue/organ bioprinting: Principle, challenge, and perspective","authors":"Duo Ma , Juan Liu , William Weijia Lu , Wenguang Liu , Changshun Ruan","doi":"10.1016/j.pmatsci.2025.101527","DOIUrl":"10.1016/j.pmatsci.2025.101527","url":null,"abstract":"<div><div>Bioprinting that can quickly generate custom-shaped organ-like constructs opens up a new horizon for tissue engineering and regenerative medicine. The importance of bioinks cannot be overemphasized in advancing bioprinting development. Superior to conventional static bioink, dynamic bioink, mimicking the natural extracellular matrix, possesses reversible dynamic molecular networks that provide cellular activity and growth and thus enhance the maturation of bioprinted organ-like constructs, which has gained lots of attention and developed rapidly in the past decade. This paper completely summarizes the progress of dynamic bioink in bioprinting. First, we outline the molecular design principle of dynamic bioinks, involving two main patterns: supramolecular force and reversible chemical bonding. Then, key factors of dynamic bioinks in advancing bioprinting, including printability, structural stability, and modulation of cell behavior, are highlighted. Finally, the review further discusses the challenges and perspectives in fabricating tissues and organs with dynamic bioinks, aiming to offer an illuminating insight into bioprinting.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"155 ","pages":"Article 101527"},"PeriodicalIF":33.6,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144335086","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Single atom horizons for shaping the future of catalysis and sustainability: the next frontiers in energy conversion and storage 塑造催化和可持续性未来的单原子视野：能量转换和存储的下一个前沿

IF 33.6 1区材料科学

Progress in Materials Science Pub Date : 2025-06-19 DOI: 10.1016/j.pmatsci.2025.101525

Ghulam Yasin , Mohammad Tabish , Saira Ajmal , Qiongfang Zhuo , Muhammad Asim Mushtaq , Ali Saad , Mohammed Mujahid Alam , Huaihe Song

{"title":"Single atom horizons for shaping the future of catalysis and sustainability: the next frontiers in energy conversion and storage","authors":"Ghulam Yasin , Mohammad Tabish , Saira Ajmal , Qiongfang Zhuo , Muhammad Asim Mushtaq , Ali Saad , Mohammed Mujahid Alam , Huaihe Song","doi":"10.1016/j.pmatsci.2025.101525","DOIUrl":"10.1016/j.pmatsci.2025.101525","url":null,"abstract":"<div><div>Single-atom catalysts have recently emerged as a revolutionary frontier in catalysis, energy production, and storage. Due to their compositional diversity, structural tunability, and modulated distinctive electronic properties, SACs pave significant promises for viable avenues toward a more sustainable future. Here, the discussion begins with the emergence of SACs, their synthesis techniques to regulate atomic dispersion, atomically-resolved advanced characterizations, probing different supports, and engineering strategies to boost stability and reactivity. This review as a key reference in this field comprises the mechanistic understanding of SACs in electrocatalysis, photocatalysis, and thermocatalysis for energy and environmental applications. We also discussed their transformative potential in H<sub>2</sub> and O<sub>2</sub> evolution reactions for water splitting, the reduction of O<sub>2</sub>, carbon dioxide, N<sub>2</sub>, and nitrate for electrocatalysis and photocatalysis, and their remarkable role in energy storage technologies, including metal-O<sub>2</sub>, lithium-sulfur, and metal-CO<sub>2</sub> batteries. Additionally, we assess their efficiency in environmental remediation by removing harmful nitrogen oxides, various hydrogenation processes, catalytic oxidation, and CO<sub>2</sub> hydrogenation, which sets this review apart from others. Despite the considerable progress, challenges persist in the scalability and commercial implementation of SACs. This comprehensive review significantly delivers valuable insights into the current advancement of SACs, highlighting their substantial potential and suggesting future research avenues that would enable next-generation technologies for energy conversion, storage, environmental sustainability, and various other functional applications.</div></div>","PeriodicalId":411,"journal":{"name":"Progress in Materials Science","volume":"155 ","pages":"Article 101525"},"PeriodicalIF":33.6,"publicationDate":"2025-06-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144329139","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0