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Modulating CO2 Reduction Selectivity over Multi-Metal Electrocatalysts Derived from 0D Alloyed Halide Perovskite Crystals
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-19 DOI: 10.1016/j.nanoen.2025.110684
Ming Zhou, Dianxing Ju, Wupei Dong, Guang-Rui Xu, Xinfa Wei, Huifang Li, Jian Liu
{"title":"Modulating CO2 Reduction Selectivity over Multi-Metal Electrocatalysts Derived from 0D Alloyed Halide Perovskite Crystals","authors":"Ming Zhou, Dianxing Ju, Wupei Dong, Guang-Rui Xu, Xinfa Wei, Huifang Li, Jian Liu","doi":"10.1016/j.nanoen.2025.110684","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110684","url":null,"abstract":"Achieving efficient selectivity and precise control in synthesis of multi-metal catalysts for electroreduction of CO<sub>2</sub> to value-added feedstocks remains a significant challenge. The key to enhancing selectivity lies in improving the adsorption energy of intermediates, which mainly depends on electronic properties of electrocatalysts. By leveraging the electronegativity offset effect, we have integrated multiple metals into 0D hybrid perovskite crystals with precise compositions as promising precursors for multi-metal or high-entropy electrocatalysts. This strategy not only facilitates adjustments to the electronic distribution within matrix materials and enhances intermediate adsorption energies but also enables controllable synthesis of multicomponent catalyst systems. For electrochemical CO<sub>2</sub> reduction demonstration, the prototype multi-metal electrocatalysts CuBi<sub>x</sub>In<sub>1-x</sub> derived from (C<sub>8</sub>H<sub>20</sub>N)<sub>4</sub>In<sub>1−x</sub>Bi<sub>x</sub>CuCl<sub>9</sub> crystals demonstrate tunable selectivity towards HCOO<sup>−</sup> and CO, achieving Faradaic Efficiency (FE) values of 94% at −1.0<!-- --> <!-- -->V vs. RHE for HCOO<sup>−</sup> and 83% at −0.6<!-- --> <!-- -->V vs. RHE for CO, alongside remarkable stability over 70<!-- --> <!-- -->h. This can be contributed to the tunable electronic properties, which enhanced adsorption energies for intermediate and reduced Gibbs free energy associated with formation of formate and CO. The current study introduces an innovative crystal-derived catalyst-on-demand strategy aimed at enhancing efficient energy conversion.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"57 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142989631","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fabrication of alginate-based bio-tribopositive films via amine modification and metal ion coordination for high surface charge density
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-18 DOI: 10.1016/j.nanoen.2025.110677
Hongyu Shen, Lei Wang, Fengmin Zhang, Jianjun Luo, Kai Han, Zhi Zhang, Chi Zhang, Hua Yuan, Zhong Lin Wang, Yaokun Pang
{"title":"Fabrication of alginate-based bio-tribopositive films via amine modification and metal ion coordination for high surface charge density","authors":"Hongyu Shen, Lei Wang, Fengmin Zhang, Jianjun Luo, Kai Han, Zhi Zhang, Chi Zhang, Hua Yuan, Zhong Lin Wang, Yaokun Pang","doi":"10.1016/j.nanoen.2025.110677","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110677","url":null,"abstract":"Developing triboelectric materials with high charge density is crucial for promoting large-scale applications of triboelectric nanogenerators (TENG). However, most of the reported works are only interested in tribonegative materials, while the tribopositive materials are rarely touched. Here, an efficient method was proposed to significantly boost the charge density of sodium alginate (SA)-based tribopositive films by simply grafting polyethyleneimine (PEI) and complexing copper ions. The prepared SA/PEI-Cu (SP-Cu) aerogel films not only have excellent flexibility and good environmental compatibility, but also high output triboelectric performance. Based on the aerogel film with a size of 5×5 cm<sup>2</sup>, the fabricated TENG reveals a high output voltage of 3.5<!-- --> <!-- -->kV, a maximum peak power density of 120<!-- --> <!-- -->W<!-- --> <!-- -->m<sup>-2</sup>, and a remarkable output charge density of 205 μC m<sup>-2</sup>, which is nearly 8.2 times high that of pure SA and breaks the record for all reported biomass tribo-materials under environmental conditions. More than 9000 LEDs and a 24<!-- --> <!-- -->W fluorescent lamp can be illuminated using this small-size TENG device. In particular, we successfully fabricated a rotating TENG device with a power management module (PMM) for harvesting wind energy to power a wireless environmental sensing system for smart agriculture. This work provides a novel strategy for developing high-performance bio-tribopositive materials, which may promote the practical applications of TENGs.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"205 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142989009","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Corrigendum to “A self-powered vector motion sensor for smart robotics and personalized medical rehabilitation” [Nano Energy 104 (2022) 107936]
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-17 DOI: 10.1016/j.nanoen.2025.110675
Wenyan Qiao, Linglin Zhou, Zhihao Zhao, Di Liu, Shaoxin Li, Jie An, Xinyuan Li, Yikui Gao, Peiyuan Yang, Jiaqi Liu, Zhong Lin Wang, Jie Wang
{"title":"Corrigendum to “A self-powered vector motion sensor for smart robotics and personalized medical rehabilitation” [Nano Energy 104 (2022) 107936]","authors":"Wenyan Qiao, Linglin Zhou, Zhihao Zhao, Di Liu, Shaoxin Li, Jie An, Xinyuan Li, Yikui Gao, Peiyuan Yang, Jiaqi Liu, Zhong Lin Wang, Jie Wang","doi":"10.1016/j.nanoen.2025.110675","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110675","url":null,"abstract":"The authors regret that the article type of the original version is incorrect. The article type should be “Research article”. The authors would like to apologise for any inconvenience caused.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"20 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142989349","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A robust hybrid nanogenerator strategy achieved by regenerative motion transmission toward wind energy harvesting and self-powered sensing
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-16 DOI: 10.1016/j.nanoen.2025.110679
Jiuling Zhu, Kangqi Fan, Weidong Wang, Kangjia Zhai, Li Zhang, Junxiang Zhou, Cheng Li, Yuanbo Li, Jinjian Li, Yan Liu, Zewei Ren, Peihong Wang
{"title":"A robust hybrid nanogenerator strategy achieved by regenerative motion transmission toward wind energy harvesting and self-powered sensing","authors":"Jiuling Zhu, Kangqi Fan, Weidong Wang, Kangjia Zhai, Li Zhang, Junxiang Zhou, Cheng Li, Yuanbo Li, Jinjian Li, Yan Liu, Zewei Ren, Peihong Wang","doi":"10.1016/j.nanoen.2025.110679","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110679","url":null,"abstract":"In rotary-sliding triboelectric-electromagnetic hybrid nanogenerator (RS-TEHG) for wind energy harvesting, the triboelectric nanogenerator (TENG) unit and electromagnetic generator (EMG) unit normally share the same rotor. Hence, the sliding friction between triboelectric layers leads to not only severe material abrasion but also restricted rotor speed and reduced electric outputs of both units. To address this issue, a regenerative motion transmission (RMT) mechanism is proposed herein to implement efficient TEHG (RMT-TEHG) by mechanically connecting TENG and EMG in series. Consisting merely of two cylinders, the RMT mechanism can not only markedly reduce frictional resistance and improve robustness by transforming sliding friction to rolling friction but also work as both a triboelectric pair and a friction pair for driving EMG as well as realizing self-contained sensing of RMT working state, achieving the functionalization of the frictional resistance. With significantly reduced frictional resistance, RMT-TEHG can operate at a low wind speed of 2.5<!-- --> <!-- -->m/s and its TENG unit can maintain 98.9% electric output after 100,000 working cycles; by contrast, RS-TEHG has a high start-up wind speed of 5.1<!-- --> <!-- -->m/s and the TENG unit only retains 60.3% output. As actuated by 4.5<!-- --> <!-- -->m/s wind, RMT-TEHG can deliver 88.4<!-- --> <!-- -->mW electrical power and sustain the continuous operation of a wireless multifunctional environmental sensing system. This work presents a distinctive strategy for constructing robust and efficient hybrid nanogenerators toward wind energy harvesting and self-powered wireless sensing systems.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"8 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142986684","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Self-Powered Electrochemical Protection for Marine Corrosion and Fouling Control: Principles, Advances, and Prospects
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-16 DOI: 10.1016/j.nanoen.2025.110676
Mingzheng Hua, Ruijie Jiang, Yuqing Lu, Yu Su, Yang Zhao
{"title":"Self-Powered Electrochemical Protection for Marine Corrosion and Fouling Control: Principles, Advances, and Prospects","authors":"Mingzheng Hua, Ruijie Jiang, Yuqing Lu, Yu Su, Yang Zhao","doi":"10.1016/j.nanoen.2025.110676","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110676","url":null,"abstract":"Improving anti-corrosion and anti-fouling performance in marine environments is vital for sustainable development. Traditional electrochemical protection depends on external power sources, leading to high costs and maintenance burdens. In contrast, self-powered electrochemical protection systems, utilizing piezoelectric nanogenerators (PENGs) and triboelectric nanogenerators (TENGs), harness environmental energy to provide cathodic protection and prevent fouling. This approach offers a sustainable and promising alternative for future marine protection. This review explores the principles, advancements, applications and coupling technologies of these self-powered systems. Key applications include anti-corrosion, anti-fouling, and self-powered sensing, while integration with internet technologies, nanotechnologies, and green materials enhances system intelligence, performance, and environmental sustainability. The ecological benefits of these technologies are critically assessed, highlighting their potential as transformative solutions for marine sustainability. Future research should prioritize the development of innovative materials, intelligent system integration, and multifunctional designs to fully realize the potential of self-powered electrochemical protection in marine settings.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"30 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142986861","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Differential-deformation structured pressure sensor for stable measurement of superficial temporal artery pulse
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-16 DOI: 10.1016/j.nanoen.2025.110678
Xue Wang, Jingjing Li, Keyu Meng, Haijun Luo, Feihong Ran, Yufen Wu, Ke Wei, Jin Yang
{"title":"Differential-deformation structured pressure sensor for stable measurement of superficial temporal artery pulse","authors":"Xue Wang, Jingjing Li, Keyu Meng, Haijun Luo, Feihong Ran, Yufen Wu, Ke Wei, Jin Yang","doi":"10.1016/j.nanoen.2025.110678","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110678","url":null,"abstract":"Recent developments have focused on flexible pressure sensors due to their potential for real-time and personalized health monitoring. However, measuring epidermal pressure signals using flexible pressure sensors is frequently plagued by various motion artifacts, which significantly impede the stable monitoring of physiological signs. In this study, we have developed an earphone-mounted flexible pressure sensor (EMFPS), which is composed of polymer materials with differential deformation ability. The EMFPS exhibits a sensitivity of 1.78<!-- --> <!-- -->V/kPa, demonstrating a notable low-frequency response ranging from 1 to 30<!-- --> <!-- -->Hz and good robustness even after 7200 operating cycles. Given these compelling features, the EMFPS mounted on the earphone is capable of detecting tiny superficial temporal artery pressure under various static forces, while simultaneously maintaining stable monitoring of pulsations during walking activities. The EMFPS embodies a simple and comfortable technology for achieving on-the-go personalized health monitoring in daily life.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"37 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142988175","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Acoustic Energy Boosts Air Purification: A Novel Sound-Wave Drive TENG for Filter-less Particulate Capturing 声能促进空气净化:用于无过滤器微粒捕获的新型声波驱动 TENG
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-15 DOI: 10.1016/j.nanoen.2025.110674
Yiting Zhang, Siu-Kai Lai, Chen Wang, Kin-Fai Ho, Chun H. Wang
{"title":"Acoustic Energy Boosts Air Purification: A Novel Sound-Wave Drive TENG for Filter-less Particulate Capturing","authors":"Yiting Zhang, Siu-Kai Lai, Chen Wang, Kin-Fai Ho, Chun H. Wang","doi":"10.1016/j.nanoen.2025.110674","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110674","url":null,"abstract":"Maintaining good indoor air quality is crucial for human health, as poor air quality in enclosed spaces can elevate the risk of infection and cause premature deaths. This study introduces a novel low-cost, filter-less method for capturing ultrafine particulates to improve air purification efficiency in air ductworks. The new technology employs sound waves to cluster particulates and simultaneously activate triboelectric nanogenerators (TENGs) to operate as electrostatic precipitators, creating a synergistic approach where two techniques complement and enhance each other. The sound waves, created within a U-shaped acoustic resonating chamber using loudspeakers, cluster the particulates and excite the TENG to generate high electrical fields between its electrodes. This high electrical field captures the clustered particulates by electrostatic precipitation. Experimental tests are utilized in this work. The peak electrical output of the electrospun nanofiber-based TENG was recorded at approximately 60<!-- --> <!-- -->V (peak-to-peak value) in the presence of sound fields. In addition, we fabricated a scaled-down ventilation model to examine the efficiency of particle filtration. Experimental results show that this technique significantly improves the removal efficiency, particularly for ultrafine particulates (0.3–1.0<!-- --> <!-- -->µm). The maximum removal efficiency for PM<sub>2.5</sub> can reach 97.5%, comparable to that of HEPA filters. The findings of this work demonstrate the effectiveness and controllability of this novel filter-less air purification method.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"92 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142981278","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Skillful Promotion of Charge Separation via Defect-Mediated Built-in Electric Field and LSPR Effect for Enhanced Photocatalytic Activity 通过缺陷介导的内置电场和 LSPR 效应巧妙促进电荷分离,从而提高光催化活性
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-15 DOI: 10.1016/j.nanoen.2025.110672
Hui Guo, Wenxuan Chen, Xiu-Qing Qiao, Chen Li, Bojing Sun, Dongfang Hou, Meidi Wang, Xueqian Wu, Tao Wu, Ruan Chi, Dong-Sheng Li
{"title":"Skillful Promotion of Charge Separation via Defect-Mediated Built-in Electric Field and LSPR Effect for Enhanced Photocatalytic Activity","authors":"Hui Guo, Wenxuan Chen, Xiu-Qing Qiao, Chen Li, Bojing Sun, Dongfang Hou, Meidi Wang, Xueqian Wu, Tao Wu, Ruan Chi, Dong-Sheng Li","doi":"10.1016/j.nanoen.2025.110672","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110672","url":null,"abstract":"Emerging S-scheme heterostructures offer distinct advantages in controlling charge transfer and maintaining redox capabilities. However, charge separation efficiency remains suboptimal, primarily due to the weak driving force for charge transfer. In this study, a novel plasmonic S-scheme MoO<sub>3-x</sub>/CdS heterojunction was built to promote charge separation and enhance H<sub>2</sub> evolution, embodying the concept of “Two Birds with One Stone.”. The rich oxygen vacancy in MoO<sub>3-x</sub> serves as the one to this dual enhancement. First, the oxygen vacancy intensifies the internal electric field (IEF), thereby accelerating charge transfer kinetics. Second, it enhances the localized surface plasmonic resonance (LSPR) effect, boosting catalytic activity at high reaction temperatures. This strategy successfully achieves efficient charge separation through an LSPR-assisted S-scheme charge-transfer pathway, enabling long-lived electrons in the conduction band of CdS to contribute to H<sub>2</sub> evolution. As a result, the optimized MoO<sub>3-x</sub>/CdS heterojunction demonstrates optimal H<sub>2</sub> evolution rates of 19.85 and 54.04<!-- --> <!-- -->mmol·g<sup>−1</sup>·h<sup>−1</sup> under visible light and full-spectrum irradiation, respectively. The concept of exploiting defect synergy to tune the IEF and photothermal effects in S-scheme heterostructures presents a promising strategy for the rational design of high-performance photocatalysts.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"22 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142986685","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Triboelectric nanogenerators in harsh conditions: A critical review
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-14 DOI: 10.1016/j.nanoen.2025.110661
C. Callaty, C. Rodrigues, J. Ventura
{"title":"Triboelectric nanogenerators in harsh conditions: A critical review","authors":"C. Callaty, C. Rodrigues, J. Ventura","doi":"10.1016/j.nanoen.2025.110661","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110661","url":null,"abstract":"The rapid rise in energy consumption and an accelerating climatic crisis has resulted in a surge in the study of clean energy sources. Triboelectric nanogenerators (TENGs) are energy harvesters that convert mechanical into electrical energy in a highly efficient manner. They are low cost, light, flexible, require limited maintenance and are environmentally friendly, being therefore very attractive for a large range of applications, such as wearables, self-power sensors or maritime deployment. However, harsh environmental conditions still hinder their performance. High humidity disperse the accumulated charge, while high temperatures facilitate electron emission and decrease surface charge density. Air components in the atmosphere can lead to changes in the charge tendency of tribomaterials, while pressure can hinder or enhance electrostatic breakdown conditions. Here, we thoroughly review the available literature on how TENGs outputs depend on environmental factors and how to tune material properties to preserve or even enhance TENG performance under harsh conditions. These are crucial aspects to obtain reliable and robust devices and to broaden TENG application spectrum towards commercialization.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"84 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142981279","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Efficient multi-physical crosslinked nanocomposite hydrogel for a conformal strain and self-powered tactile sensor
IF 17.6 1区 材料科学
Nano Energy Pub Date : 2025-01-14 DOI: 10.1016/j.nanoen.2025.110669
Xiangyu Zeng, Lijing Teng, Xinping Wang, Tao Lu, Weng Leng, Xujie Wu, Dan Li, Yeshuang Zhong, Xiaomin Sun, Simian Zhu, Yu Dong, Puchuan Tan, Zhu Zeng, Zuquan Hu, Zhou Li, Qiang Zheng
{"title":"Efficient multi-physical crosslinked nanocomposite hydrogel for a conformal strain and self-powered tactile sensor","authors":"Xiangyu Zeng, Lijing Teng, Xinping Wang, Tao Lu, Weng Leng, Xujie Wu, Dan Li, Yeshuang Zhong, Xiaomin Sun, Simian Zhu, Yu Dong, Puchuan Tan, Zhu Zeng, Zuquan Hu, Zhou Li, Qiang Zheng","doi":"10.1016/j.nanoen.2025.110669","DOIUrl":"https://doi.org/10.1016/j.nanoen.2025.110669","url":null,"abstract":"Conductive hydrogels offer significant promise for conformal electronic skin and self-powered systems. However, developing hydrogels with multifunctionality, including stretchability, self-healing, tissue adhesion, and biocompatibility, remains a significant challenge. In this study, multiple physically crosslinked nanocomposite hydrogels were developed through the in situ doping of poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) in a Laponite® (LAP) crosslinked oligo ethylene glycol (OEG) methyl ether methacrylate copolymer. Through combined covalent and non-covalent interactions, coupled with metal ion doping, the developed conductive nanocomposite hydrogel achieved excellent stretchability (~450%), high self-healing efficiency (~95%), robust tissue force (∼0.5<!-- --> <!-- -->N/cm<sup>2</sup>), and good biocompatibility. These features made it highly suitable for applications as a skin conformal strain sensor for human motion monitoring. In addition, it could be used as a flexible electrode in triboelectric nanogenerators, enabling tactile sensing for human–machine interactions and demonstrating its potential in self-powered electronics.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"16 1","pages":""},"PeriodicalIF":17.6,"publicationDate":"2025-01-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142981280","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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