Journal of Hazardous Materials最新文献

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Application of ionic wind in sampling of bioaerosols: collection efficiency, ROS/RNS production, and viability assessment 离子风在生物气溶胶采样中的应用:收集效率、ROS/RNS 生成和活力评估
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136612
Milad Massoudifarid, Amin Piri, Massoud Massoudifarid, Jiwoo Jung, Sangwoo Kim, Jungho Hwang
{"title":"Application of ionic wind in sampling of bioaerosols: collection efficiency, ROS/RNS production, and viability assessment","authors":"Milad Massoudifarid, Amin Piri, Massoud Massoudifarid, Jiwoo Jung, Sangwoo Kim, Jungho Hwang","doi":"10.1016/j.jhazmat.2024.136612","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136612","url":null,"abstract":"Studies of bioaerosol particles in airborne particulate matter have revealed their omnipresence. Therefore, spot-on sampling and identification are pivotal for assessing exposure risks. Corona discharge-based sampling has been utilized for the bioaerosol sampling. However, one of the issues regarding corona discharge-based samplers is the production of reactive oxygen species (ROS) and reactive nitrogen species (RNS), which can alter the viability of bioaerosols and damage nucleic acids. Herein, the use of ionic wind as a possible alternative to reduce ROS/RNS damage to microorganisms was studied. An aerosol-to-hydrosol (ATH) ionic wind (IW) sampler was developed and compared with an ATH electrostatic precipitation (ESP) sampler having the exact physical dimensions in terms of collection efficiency, ROS/RNS production, ozone generation, viability of collected biological particles, and damage to the nucleic acids of the particles. Overall, the ESP sampler showed a higher collection efficiency and less damage to the reproducibility of the sampled bioaerosols than the IW sampler. However, polymerase chain reaction analysis of the sampled bioaerosol nucleic acids showed similar results for both devices. The IW sampler has the potential for both bioaerosol sampling and deactivation, as well as for scenarios requiring neutralized sampled particles or particle deposition on any nonmetallic surface.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"5 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142678646","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Study on the characteristics of dust diffusion during a truck travelling in an open-pit coal mine affected by the vertical wind shear 露天煤矿卡车行驶过程中受垂直风切变影响的粉尘扩散特征研究
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136611
Wendong Zhou, Yanwei Cui, Hetang Wang, Li Chen, Ke Xu, Candong Wu, Gehui Ren
{"title":"Study on the characteristics of dust diffusion during a truck travelling in an open-pit coal mine affected by the vertical wind shear","authors":"Wendong Zhou, Yanwei Cui, Hetang Wang, Li Chen, Ke Xu, Candong Wu, Gehui Ren","doi":"10.1016/j.jhazmat.2024.136611","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136611","url":null,"abstract":"Heavy trucks in open-pit mines are significant sources of dust. The diffusion of dust is primarily influenced by wind flow. The surface wind speed exhibits an exponential distribution as height increases. To investigate dust diffusion under the influence of wind shear, a numerical model was developed using real-scale data through computational fluid dynamics. The results indicate that wind shear significantly affects near-ground wind speeds. The ground-level wind speed near the rear of the truck exceeds the dust lift-off speed, reaching over 6<!-- --> <!-- -->m/s. The acceleration of the ambient wind speed leads to extensive areas of turbulence with increased intensity. The location of the vortex zone represents the primary area of negative pressure. A higher ambient wind speed accelerates the dust discharge and generates a greater negative pressure, reaching -68 Pa at a wind speed of 9<!-- --> <!-- -->m/s. The dust concentration behind the truck initially increases before subsequently decreasing. Notably, the local dust concentration at a wind speed of 9<!-- --> <!-- -->m/s is lower than that at a wind speed of 5<!-- --> <!-- -->m/s. The obstruction of airflow by the truck cab can result in elevated dust levels on the driver's side. Furthermore, high dust concentrations along driving paths necessitate appropriate truck spacing to protect operator health.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"6 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142678647","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effects of polystyrene microplastics on the distribution behaviors and mechanisms of metalloid As(Ⅲ) and As(V) on pipe scales in drinking water distribution systems 聚苯乙烯微塑料对金属砷(Ⅲ)和砷(Ⅴ)在饮用水输配系统管道尺度上的分布行为和机制的影响
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136542
Jiaxin Li, Zhu Peng, Weigao Zhao, Xianxian Chu, Yimei Tian
{"title":"Effects of polystyrene microplastics on the distribution behaviors and mechanisms of metalloid As(Ⅲ) and As(V) on pipe scales in drinking water distribution systems","authors":"Jiaxin Li, Zhu Peng, Weigao Zhao, Xianxian Chu, Yimei Tian","doi":"10.1016/j.jhazmat.2024.136542","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136542","url":null,"abstract":"Pipe scales have long been considered the primary adsorption medium for trace heavy metals in drinking water distribution systems (DWDSs). Microplastics (MPs) potentially affect the distribution of metalloid arsenic (As) pollutants in DWDSs. Herein, the accumulation behaviors of As(Ⅲ) and As(V) on pipe scales and polystyrene microplastics (PSMPs) under different water conditions were studied. Additionally, As(Ⅲ) and As(V) accumulation behaviors on pipe scales coexisting with PSMPs were investigated. Results showed that pipe scales played a key role in the accumulation of As (pipe scales = 1.08–4.80<!-- --> <!-- -->mg/g &gt; PSMPs = 0.02–3.38<!-- --> <!-- -->mg/g). The adsorption amount of As(Ⅲ) on PSMPs was higher than that of As(V). The addition of PSMPs promoted the accumulation of As(Ⅲ) on pipe scales at pH = 3–8 while inhibiting the accumulation of As(V) on pipe scales at pH = 3–10 due to the competitive adsorption. The oxidation of As(III) and the reduction of As(V) occurred during the accumulation of As(Ⅲ) and As(V) on pipe scales. Notably, PSMPs accumulated on pipe scales were beneficial to the oxidation of As(Ⅲ), potentially reducing the As-related risks. Overall, our results provide new insights into the hazards posed by MPs in DWDSs.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"6 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142678648","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dialogue between algorithms and soil: Machine learning unravels the mystery of phthalates pollution in soil 算法与土壤之间的对话:机器学习揭开土壤中邻苯二甲酸盐污染之谜
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136604
Boyou Pan, Jialin Lei, Bogui Pan, Hong Tian, Li Huang
{"title":"Dialogue between algorithms and soil: Machine learning unravels the mystery of phthalates pollution in soil","authors":"Boyou Pan, Jialin Lei, Bogui Pan, Hong Tian, Li Huang","doi":"10.1016/j.jhazmat.2024.136604","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136604","url":null,"abstract":"Soil is a major environmental sink for the emerging organic pollutants phthalates (PAEs), and the determination of key factors influencing PAEs accumulation in soil is crucial for agricultural sustainability and food security. Aiming at the time-consuming and inefficient characteristics of traditional batch experiments and statistical prediction models in comprehensively capturing PAEs dynamics in soil, an intelligent analysis framework based on machine learning was proposed and developed. In this study, thirty features were incorporated, including soil PAEs-concentrations, pollutant emissions, agricultural inputs, soil physicochemical properties, and climatic parameters. Six data-driven machine learning models were established: Random Forest Regression (RFR), Gradient Boosting Regression Tree (GBRT), Extreme Gradient Boosting (XGBoost), Multilayer Perceptron (MLP), Support Vector Regression (SVR), and k-Nearest Neighbors (KNN). Results showed that the MLP model exhibited optimal performance in predicting soil PAEs concentrations (R²=0.8637), followed by SVR (R²=0.8132) and XGBoost (R²=0.8096). Through feature importance analysis, it was determined that hydrometeorological factors, soil moisture conditions, and nutritional characteristics were the key factors controlling PAEs spatial distribution. Furthermore, non-linear effect analysis elucidated significant synergistic interactions among these environmental covariates. The spatiotemporal prediction model revealed continuous declining trends in PAEs pollution levels in eastern coastal regions over the next 5-10 years, while accumulation tendencies were observed in inland provinces particularly in Guizhou. This study demonstrates the effectiveness and advantages of machine learning in predicting soil PAEs-pollution, providing a new perspective for pollutant risk assessment and management in the era of environmental big data.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"71 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142678200","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bryophytes adapt to open-pit coal mine environments by changing their functional traits in response to heavy metal-induced soil environmental changes 草履本植物通过改变其功能特性来适应露天煤矿环境,以应对重金属引起的土壤环境变化
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136613
Yu Han, Jin Kou, Baichuan Jiang, Junping Li, Changchang Liu, Shaogang Lei, Hongxing Xiao, Chao Feng
{"title":"Bryophytes adapt to open-pit coal mine environments by changing their functional traits in response to heavy metal-induced soil environmental changes","authors":"Yu Han, Jin Kou, Baichuan Jiang, Junping Li, Changchang Liu, Shaogang Lei, Hongxing Xiao, Chao Feng","doi":"10.1016/j.jhazmat.2024.136613","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136613","url":null,"abstract":"Plants have unique adaptability to heavy metal pollution. However, the adaptation strategies of bryophytes are still unclear. In order to better understand the response of bryophytes to different heavy metal and the adaptation mechanisms of different species to heavy metal pollution, we studied soil physicochemical properties, distribution of heavy metal elements, ecological risk assessment and the community structure, functional characteristics of bryophytes in large open-pit coal mines in Inner Mongolia. The results indicate that: 1) The soil in three open-pit mining areas currently does not pose an ecological risk from the heavy metal pollution, but high concentrations of Zn and Hg are found in most parts of the study area; 2) The presence of a single heavy metal drives the distribution of specific taxa of bryophytes. Apart from Hg, Pb, and Zn, all the other heavy metals significantly impact the community structure of bryophytes; 3) With the exception of Pb and Hg, all the other heavy metals have an influence on the functional traits of bryophytes; 4) Different taxa of bryophytes will adapt to changes in soil environments caused by heavy metal pollution by altering their functional traits (blades, leaf cells, or plant size).","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"35 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142678645","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Livestock and poultry manure influence thallium accumulation in chili peppers (Capsicum annuum) under complex toxic elements contamination in soil 家畜和家禽粪便对土壤中复杂有毒元素污染下辣椒(Capsicum annuum)铊积累的影响
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136605
Jianbo Jiang, Jichang Wen, Ruijia Yang, Haixia Yang, Shikai Yang
{"title":"Livestock and poultry manure influence thallium accumulation in chili peppers (Capsicum annuum) under complex toxic elements contamination in soil","authors":"Jianbo Jiang, Jichang Wen, Ruijia Yang, Haixia Yang, Shikai Yang","doi":"10.1016/j.jhazmat.2024.136605","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136605","url":null,"abstract":"Long-term mining activities in the mercury-thallium mining area of Lanmuchang, southwestern China, resulting in contamination of surrounding soils with complex toxic elements such as Tl, As, Sb, Hg, and Cd. While manure aids in pollution control and soil fertilization, its impact on Tl bioavailability in soil remains incompletely understood. This study explored the physiological changes and Tl accumulation in <em>Capsicum annuum</em> under combined pollution stress and application of livestock and poultry manure near the Lanmuchang mining area. The results showed that chicken manure promoted Tl accumulation in <em>Capsicum annuum</em>, whereas pig and cattle manure inhibited it, with pig manure exhibiting the strongest inhibitory effect. Both pig and cattle manure reduced the transpiration rate of <em>Capsicum annuum</em>, which decreased the driving force for Tl transport to the plant's upper parts. Additionally, manure increased organic acid secretion in <em>Capsicum annuum</em> roots and decreased soil Eh. This led to a reduction in Tl<sup>3+</sup> to the more stable Tl<sup>+</sup>, which decreased the content of exchangeable Tl form and its activity. Pig manure significantly reduced Tl content in stems, leaves, and fruits by increasing the area of the Casparian bands in <em>Capsicum annuum</em> roots, which hindered Tl accumulation. In contrast, chicken manure had the opposite effect. The findings of this study provide important theoretical support for scientifically guiding agricultural production safety in areas contaminated with the heavy metal Tl.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"57 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142673557","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Comprehensive elemental and physical characterization of vehicle brake wear emissions from two different brake pads following the Global Technical Regulation methodology 按照《全球技术规范》的方法,对两种不同刹车片产生的汽车制动磨损排放物进行全面的元素和物理特性分析
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136609
Carsten Neukirchen, Mohammad Reza Saraji-Bozorgzad, Michael Mäder, Ajit Paul Mudan, Philipp Czasch, Johannes Becker, Sebastiano Di Bucchianico, Christian Trapp, Ralf Zimmermann, Thomas Adam
{"title":"Comprehensive elemental and physical characterization of vehicle brake wear emissions from two different brake pads following the Global Technical Regulation methodology","authors":"Carsten Neukirchen, Mohammad Reza Saraji-Bozorgzad, Michael Mäder, Ajit Paul Mudan, Philipp Czasch, Johannes Becker, Sebastiano Di Bucchianico, Christian Trapp, Ralf Zimmermann, Thomas Adam","doi":"10.1016/j.jhazmat.2024.136609","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136609","url":null,"abstract":"Non-exhaust emissions have gained increasing attention during the last years, with the upcoming EURO 7 regulation defining maximum PM<sub>10</sub> emission factors for tire and brake emissions for the first time. This study, therefore, focusses on broadening the knowledge on chemical composition and physical characteristics of brake dust to define emission factors for heavy metal and organic pollutants. Particles from two pads were analyzed utilizing the Worldwide Harmonised Light Vehicle Test Procedure (WLTP) brake cycle. Geometric mean diameters for both pads were found with a bimodal distribution in the ultrafine range. PM<sub>10</sub> emission factors of 15.1 ± 0.1<!-- --> <!-- -->mg/km and 16.3 ± 0.4<!-- --> <!-- -->mg/km were measured, which is 2.15 and 2.32 times higher than upcoming maximum permitted emission factor of 7<!-- --> <!-- -->mg/km. On average 54.9% and 58.1% of PM10 was emitted as iron, with a wide variety of Fe concentrations between 43 – 75% by mass found in individual particles. Other heavy metals, such as Cu, Cr, Mn and Zn, were also found and a high contribution of wear from the brake disc was noticeable, based on the elemental composition. Fe emission factors calculated from the WLTP brake cycle were 8-9 times higher than previously reported values in literature, while Cu levels were significantly lower based on recent trends in brake pad formulations. Four different PAH were detected even at the relatively low temperatures that are common for the WLTP brake test cycle.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"1 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142678199","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A core-shell structured crystalline@amorphous MnO2 with enhanced plasma catalytic degradation performance for Volatile Organic Sulfur Compounds and degradation mechanism exploration 增强等离子体催化降解挥发性有机硫化合物性能的核壳结构晶体@非晶态二氧化锰及其降解机理探索
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136597
Wenji Feng, Chong Wang, Mengyu Liu, Haiqiang Wang, Zhongbiao Wu
{"title":"A core-shell structured crystalline@amorphous MnO2 with enhanced plasma catalytic degradation performance for Volatile Organic Sulfur Compounds and degradation mechanism exploration","authors":"Wenji Feng, Chong Wang, Mengyu Liu, Haiqiang Wang, Zhongbiao Wu","doi":"10.1016/j.jhazmat.2024.136597","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136597","url":null,"abstract":"A crystalline@amorphous MnO<sub>2</sub> (HT@RT) plasma catalyst was successfully constructed in this study to address the problem of odor pollution, especially from volatile organic sulfur compounds (VOSCs) with low olfactory thresholds. Complete conversion of dimethyl sulfide (DMS) at 140<!-- --> <!-- -->J/L was achieved, and the ozone concentration in the exhaust gas was maintained below 5 ppm. Deeper mineralization of DMS was achieved in the HT@RT sample than in the individual HT and RT samples. A comprehensive analysis of multiple characterization techniques revealed that the HT@RT sample exhibited excellent DMS adsorption capacity, appropriate electric field responsiveness, high oxygen vacancy content, and abundant reactive oxygen species, which play key roles in the degradation of DMS. In addition, the DMS degradation process was investigated using in situ plasma diffuse reflectance infrared Fourier transform (DRIFT) spectroscopy. Combined with the results of gas chromatography-mass spectrometry, degradation pathways for DMS were proposed. The HT@RT sample combined the advantages of both amorphous and crystalline materials, significantly enhancing the activity and stability of the catalyst. Therefore, the crystalline@amorphous structured catalysts constructed in this study not only offer new insights for improving the performance of plasma catalysis but also provide an effective solution for eliminating odorous gases.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"99 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142673556","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Simultaneous removal of ammonia, copper ions and sulfamethoxazole from aquaculture wastewater with low carbon to nitrogen ratio enhanced by manganese redox driven by a two-stage synergistic bioreactor: Optimization and potential mechanism 两级协同生物反应器在锰氧化还原作用驱动下同时去除低碳氮比水产养殖废水中的氨氮、铜离子和磺胺甲噁唑:优化与潜在机制
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136586
Meng Cao, Yihan Bai, Yue Wang, Junfeng Su, Jingting Feng
{"title":"Simultaneous removal of ammonia, copper ions and sulfamethoxazole from aquaculture wastewater with low carbon to nitrogen ratio enhanced by manganese redox driven by a two-stage synergistic bioreactor: Optimization and potential mechanism","authors":"Meng Cao, Yihan Bai, Yue Wang, Junfeng Su, Jingting Feng","doi":"10.1016/j.jhazmat.2024.136586","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136586","url":null,"abstract":"The problem of low carbon-nitrogen ratio (C/N) in wastewater is a major challenge for biological treatment, especially the complex pollution of ammonia nitrogen (NH<sub>4</sub><sup>+</sup>-N), sulfamethoxazole (SMX), and copper ions (Cu(II)). Herein, a strain of <em>Pseudoxanthomonas</em> sp. MA23 with manganese (Mn) reduction-coupled ammonia oxidation properties was isolated. Subsequently, kaolin and bentonite were used as the main raw materials, and a mixture of coconut shell biochar (CSBC) and different Mn ores were added to make ceramsite carriers to load the target strain MA23. To achieve complete N removal and Mn redox process, <em>Dechloromonas</em> sp. YZ8 with Mn redox and denitrification performance was introduced, and a second-stage bioreactor was constructed with volcanic rock as the biocarrier. The results showed that the bioreactor was most effective when the hydraulic retention time (HRT) was 20.0 and 2.0<!-- --> <!-- -->h, C/N was 1.5, and pH was 6.5. The response of the bioreactors was investigated by inflowing different concentrations of Cu(II) and SMX. Appropriate Cu(II) concentrations promoted the electron transfer in the system, and Cu(II) and SMX were together removed by biological action and chemisorption. Furthermore, genes involved in N metabolism were enriched in the bioreactors and the microorganisms responded to environmental changes by up or down-regulating relevant metabolic genes. The synergistic system proposed in this study provided a promising attempt to simultaneously address NH<sub>4</sub><sup>+</sup>-N-Cu(II)-SMX pollution in low C/N wastewater.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"20 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142673595","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Corrigendum to “Global air quality enhancement pathways to health benefits and environmental justice” [J Hazard Mater 480 (2024) 136460] 全球空气质量改善途径对健康的益处和环境正义 "的更正[J Hazard Mater 480 (2024) 136460]
IF 13.6 1区 环境科学与生态学
Journal of Hazardous Materials Pub Date : 2024-11-20 DOI: 10.1016/j.jhazmat.2024.136589
Yong Xu, Shang-Chen Zhou, Yu-Xi Feng, Bin Zou, Chao He
{"title":"Corrigendum to “Global air quality enhancement pathways to health benefits and environmental justice” [J Hazard Mater 480 (2024) 136460]","authors":"Yong Xu, Shang-Chen Zhou, Yu-Xi Feng, Bin Zou, Chao He","doi":"10.1016/j.jhazmat.2024.136589","DOIUrl":"https://doi.org/10.1016/j.jhazmat.2024.136589","url":null,"abstract":"The authors regret for the following errors in the original article:","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"35 1","pages":""},"PeriodicalIF":13.6,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142673644","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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