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Asynchronous Phase Shifts are Effective for Interferometric Single‐Molecule Localization Microscopy 异步相移是有效的干涉单分子定位显微镜
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-13 DOI: 10.1002/lpor.202500410
Zengxin Huang, Hangfeng Li, Yilin Wang, Wei Wang, Pakorn Kanchanawong
{"title":"Asynchronous Phase Shifts are Effective for Interferometric Single‐Molecule Localization Microscopy","authors":"Zengxin Huang, Hangfeng Li, Yilin Wang, Wei Wang, Pakorn Kanchanawong","doi":"10.1002/lpor.202500410","DOIUrl":"https://doi.org/10.1002/lpor.202500410","url":null,"abstract":"Interferometric techniques offer exceptional axial precision in single‐molecule 3D super‐resolution microscopy but generally rely on complex optical instrumentation to simultaneously measure multiple phase shifts of fluorescence emission. To address this limitation, here two‐step phase‐shifting interferometry (TPSI) is introduced, which utilizes asynchronous phase shifts to achieve ultra‐high interferometric axial precision with a much simpler optical setup. A theoretical framework is presented for the robustness of TPSI against intensity imbalances that arise from the stochastic blinking behaviors of fluorophores. Experimental validation demonstrates that TPSI maintains high axial precision across the entire interferometric depth, achieving 5 nm axial precision for fluorophores when ≈1500 photons are detected. TPSI‐based interferometric single‐molecule localization microscopy thus provides a streamlined and cost‐effective pathway to ultra‐high precision 3D nanoscopy.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"148 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144612794","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Single‐Pass Wavefront Reconstruction via Depth Heterogeneity Self‐Supervised Neural Operator for Turbulence Correction 基于深度非均质自监督神经算子的湍流校正单通波前重建
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-13 DOI: 10.1002/lpor.202500909
Haoyu Zhang, Chaoxu Chen, Fujie Li, Jifan Cai, Li Yao, Fang Dong, Yuan Wei, Yinjun Liu, Xinjie Zhang, Yingjun Zhou, Ziwei Li, Junwen Zhang, Jianyang Shi, Nan Chi
{"title":"Single‐Pass Wavefront Reconstruction via Depth Heterogeneity Self‐Supervised Neural Operator for Turbulence Correction","authors":"Haoyu Zhang, Chaoxu Chen, Fujie Li, Jifan Cai, Li Yao, Fang Dong, Yuan Wei, Yinjun Liu, Xinjie Zhang, Yingjun Zhou, Ziwei Li, Junwen Zhang, Jianyang Shi, Nan Chi","doi":"10.1002/lpor.202500909","DOIUrl":"https://doi.org/10.1002/lpor.202500909","url":null,"abstract":"Turbulence‐induced distortion remains a major bottleneck for high‐fidelity applications such as optical wireless communication and laser‐based remote sensing, as conventional adaptive optics systems struggle to meet the combined demands of bandwidth efficiency, low‐delay and environmental adaptability. Here, a Depth Heterogeneity Self‐supervised Neural Operator (DHSNO) is proposed, a multi‐physics heterogeneous model integrated neural architecture tailored to correct turbulence wavefronts in a single pass without the need for labeled training data. By leveraging dual‐mode intensity detection in a depth‐heterogeneous receiver, DHSNO inherently regularizes the ill‐posed wavefront retrieval problem to deliver robust, high‐accuracy, and low‐latency reconstruction. This capability is validated in both an emulated 50‐meter underwater turbulence channel and a real‐world 5‐meter underwater salinity‐gradient channel, where DHSNO achieves a normalized residual wavefront error below 0.06 with an inference time of 3.6 ms under varying turbulent strengths. Furthermore, this prototype system enabled 12‐Gb/s 4K‐120fps video transmission with near‐perfect fidelity (SSIM > 0.9999) under severe turbulence conditions. These findings not only advance the state‐of‐the‐art in adaptive optics but also provide a scalable framework for next‐generation free‐space and underwater optical systems, underscoring the transformative potential for turbulence correction of integrating physical constraints with data‐driven neural networks.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"67 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144612795","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dual‐Band Electromagnetically Induced Transparency Enabled by Quasi‐Bound States in the Continuum 连续介质中准束缚态实现双波段电磁诱导透明
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-13 DOI: 10.1002/lpor.202500677
Shaojun You, Longxiao Wang, Haoxuan He, Chaobiao Zhou, Lujun Huang
{"title":"Dual‐Band Electromagnetically Induced Transparency Enabled by Quasi‐Bound States in the Continuum","authors":"Shaojun You, Longxiao Wang, Haoxuan He, Chaobiao Zhou, Lujun Huang","doi":"10.1002/lpor.202500677","DOIUrl":"https://doi.org/10.1002/lpor.202500677","url":null,"abstract":"Metasurfaces emerge as exceptional platforms for achieving classical‐analog electromagnetically induced transparency (EIT). In this study, dual‐band EIT is demonstrated by strategically engineering the coupling between a magnetic toroidal dipole (TD) Mie resonance and two quasi‐bound states in the continuum (QBICs) within all‐dielectric metasurfaces. Through deliberate symmetry breaking in the cuboid unit cell—achieved via off‐center holes or U‐shaped configurations—two BICs, predominantly governed by electric TD and magnetic quadrupole modes, are successfully transformed into QBICs with high quality (Q) factors. These QBICs are then coupled to a low‐Q magnetic TD Mie resonance, resulting in the emergence of dual‐band EIT. The corresponding group delays reach up to 9.51 ps (Q = 7,674) and 5.69 ps (Q = 3,631), respectively, and diverge when the Q‐factors approach infinite. Furthermore, the dual‐band EIT with high Q‐factors is experimentally validated by fabricating a series of silicon metasurfaces and characterizing their transmission spectra. Excellent agreement is found between numerical simulation and experimental measurement. Measurement results reveal that both the resonance wavelengths and Q‐factors of the dual‐band EIT are precisely tuned by adjusting the asymmetry parameters. These findings hold significant promise for applications in multi‐wavelength slow light devices and biosensing.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"109 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144612811","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Broken Valley Degeneracy in Epitaxial MoS2 on Plasma‐Engineered AlN 等离子体工程AlN外延MoS2的破谷简并
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-13 DOI: 10.1002/lpor.202500823
Yuxiang Zhang, Weiqing Tang, Haiyang Liu, Mengyu Liu, Anqi Cheng, Shiming Wu, Ying Ye, Min Liu, Zongnan Zhang, Chunmiao Zhang, Yaping Wu, Xu Li, Zhiming Wu, Junyong Kang
{"title":"Broken Valley Degeneracy in Epitaxial MoS2 on Plasma‐Engineered AlN","authors":"Yuxiang Zhang, Weiqing Tang, Haiyang Liu, Mengyu Liu, Anqi Cheng, Shiming Wu, Ying Ye, Min Liu, Zongnan Zhang, Chunmiao Zhang, Yaping Wu, Xu Li, Zhiming Wu, Junyong Kang","doi":"10.1002/lpor.202500823","DOIUrl":"https://doi.org/10.1002/lpor.202500823","url":null,"abstract":"Two‐dimensional transition metal dichalcogenides represent a highly attractive platform for the development of valleytronic devices due to their unique spin‐valley properties. Herein, a plasma‐assisted interfacial engineering is proposed to enhance valley polarization and valley splitting in MoS<jats:sub>2</jats:sub>/AlN heterostructure by modifying the surface configurations of AlN substrates. The experimental results show that after the optimized N<jats:sub>2</jats:sub>‐plasma treatment, the AlN surface becomes smoother with a decreased migration barrier, thereby facilitating the growth of high‐quality MoS<jats:sub>2</jats:sub>. The valley splitting and degree of valley polarization in the optimal sample reach 7.96 meV (the corresponding Landé g factor is 19.6) and 33.8% at −7 T, which are 16.0‐ and 1.0‐fold higher than those in the untreated MoS<jats:sub>2</jats:sub>/AlN heterostructure, respectively. Theoretical simulations indicate that the enhanced spin‐valley properties are predominantly ascribed to the AlN surface magnetism induced by the hybridization of <jats:italic>P<jats:sub>z</jats:sub></jats:italic> and <jats:italic>P<jats:sub>y</jats:sub></jats:italic> orbitals of surface N and O atoms. This work opens a new avenue for manipulating spin‐valley properties in 2D materials via interfacial engineering.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"1 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144612797","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Optical Multimodal Endoscopy 光学多模态内窥镜
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-11 DOI: 10.1002/lpor.202500286
Qianqian Song, Weizheng Jin, Ji Qi, Yizhou Tan, Zhong Wen, Liqiang Wang, Chiye Li, Xiaowei Liu, Peng Li, Pinghe Wang, Xu Liu, Ying Gu, Qing Yang
{"title":"Optical Multimodal Endoscopy","authors":"Qianqian Song, Weizheng Jin, Ji Qi, Yizhou Tan, Zhong Wen, Liqiang Wang, Chiye Li, Xiaowei Liu, Peng Li, Pinghe Wang, Xu Liu, Ying Gu, Qing Yang","doi":"10.1002/lpor.202500286","DOIUrl":"https://doi.org/10.1002/lpor.202500286","url":null,"abstract":"Multimodal endoscopy imaging includes two or more imaging modes, for example, optical coherence tomography (OCT), photoacoustic imaging (PAI), microscopy endoscopy, fluorescence imaging (FI), etc. The combination of OCT and PAI obtained comprehensive tissue information with high resolution and a certain imaging depth of a few millimeters, which has the potential to determine the boundary of the tumor and improve the early diagnosis rate. However, they have weak molecular specificity. FI could reveal the changes in the composition and have the ability of targeted recognition. However, the imaging depth and resolution are limited. Super‐resolution imaging could improve the lateral resolution and enable observation of subcellular structures. Multimodal endoscopic imaging could enhance diagnosis and treatment by capturing comprehensive tissue information, monitoring photodynamic therapy efficacy, and revealing targeted changes. It also could accelerate the development of new methods that achieve high resolution, high depth, and high specificity. Here, the progress of research and medical applications of multimodal endoscopy imaging is reviewed. First, the principle and performance of each mode are discussed. Then, representative implementations, research progress, and medical applications of each subsystem and multimodal endoscopy imaging are illustrated. Finally, the current challenges and potential development of multimodal endoscopy imaging are briefly introduced.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"37 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144603007","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Observation of Periodic Perturbation Assisted Stable Bound State in the Continuum 连续体中周期扰动辅助稳定束缚态的观测
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-09 DOI: 10.1002/lpor.202500930
Ziyi Liu, Chen Chen, Jianfei Li, Ying Wang, Zhongxiang Zhou, Jingfeng Yao, Jianlong Liu, Chengxun Yuan
{"title":"Observation of Periodic Perturbation Assisted Stable Bound State in the Continuum","authors":"Ziyi Liu, Chen Chen, Jianfei Li, Ying Wang, Zhongxiang Zhou, Jingfeng Yao, Jianlong Liu, Chengxun Yuan","doi":"10.1002/lpor.202500930","DOIUrl":"https://doi.org/10.1002/lpor.202500930","url":null,"abstract":"Bound states in the continuum (BICs) realized via metasurfaces or photonic crystals typically require strict structural periodicity. Perturbation to such periodicity are often considered detrimental, as they tend to destabilize BICs. However, controlled perturbation can hold significant applications in manipulation and offers new paradigms for high‐dimensional optical control, such as disorder‐assisted real–momentum singular points. In this work, a stable BIC that persists under periodic perturbations is theoretically and experimentally demonstrated, stabilized via edge‐state winding dependent on the layer number. Besides, by tuning the periodicity perturbation, the evolution of discrete BICs is observed from chain BICs (achieved experimentally) to the stable BIC. The findings suggest that BICs need not be strictly confined by structural periodicity, offering a new paradigm for perturbation‐induced BIC research and a flexible approach to their dynamic modulation.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"119 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144593901","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Femtosecond Laser Breaks the Lattice Symmetry and Induces Broadband Second Harmonic Generation in 3D Halide Perovskites 飞秒激光破坏三维卤化物钙钛矿晶格对称并诱导宽带二次谐波产生
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-09 DOI: 10.1002/lpor.202500487
Guan‐Feng Gao, Ze‐Lin Li, Ze‐Kai Chen, Long‐Feng Zhong, Nan Hou, Zhi‐Hao Yan, Jing Wang, Chen‐Hui Li, Fan‐kai Zeng, Xiaozhi Xu, Ieng Wai Un, Yihang Chen, Jiadong Zhou, Lakshminarayana Polavarapu, Xiaowen Hu, Xiao‐Fang Jiang
{"title":"Femtosecond Laser Breaks the Lattice Symmetry and Induces Broadband Second Harmonic Generation in 3D Halide Perovskites","authors":"Guan‐Feng Gao, Ze‐Lin Li, Ze‐Kai Chen, Long‐Feng Zhong, Nan Hou, Zhi‐Hao Yan, Jing Wang, Chen‐Hui Li, Fan‐kai Zeng, Xiaozhi Xu, Ieng Wai Un, Yihang Chen, Jiadong Zhou, Lakshminarayana Polavarapu, Xiaowen Hu, Xiao‐Fang Jiang","doi":"10.1002/lpor.202500487","DOIUrl":"https://doi.org/10.1002/lpor.202500487","url":null,"abstract":"3D halide perovskites have shown exceptional promise not only in photovoltaic and optoelectronic applications but also in nonlinear optics such as second harmonic generation (SHG). However, their efficiency in SHG is limited by the centrosymmetric nature of their crystal structures, and thus achieving SHG from 3D perovskites by breaking their inversion symmetry remains a formidable challenge. In this work, the precision and versatility of the femtosecond (fs) pulse laser writing technique are leveraged to fabricate microstructures of hybrid and inorganic perovskites with non‐centrosymmetric. These microstructures exhibit a strong SHG signal across a broad wavelength range (790–1210 nm), while the pristine 3D perovskites do not show any SHG. The enhanced SHG response is attributed to the laser‐induced modifications of the A‐site cations (MA, Cs) and halide defects in the pristine 3D perovskites, which disrupt the inversion symmetry. Furthermore, the potential of using non‐centrosymmetric microstructures of perovskites for ultrafast pulse characterization via the Frequency‐Resolved Optical Gating technique is demonstrated. These findings highlight the precise control of non‐centrosymmetric states using fs lasers, paving the way for the design and utilization of perovskites in advanced nonlinear optical and photonic applications.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"47 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144593845","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ultrasensitive Vector Displacement Measurement Based on Pancharatnam‐Berry Phase Optical Element 基于Pancharatnam - Berry相位光学元件的超灵敏矢量位移测量
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-09 DOI: 10.1002/lpor.202500741
Yingjie Shang, Siyuan Qiao, Yinghui Guo, Qi Zhang, Mingbo Pu, Xiaoyin Li, Hengshuo Guo, Fei Zhang, Mingfeng Xu, Xiangang Luo
{"title":"Ultrasensitive Vector Displacement Measurement Based on Pancharatnam‐Berry Phase Optical Element","authors":"Yingjie Shang, Siyuan Qiao, Yinghui Guo, Qi Zhang, Mingbo Pu, Xiaoyin Li, Hengshuo Guo, Fei Zhang, Mingfeng Xu, Xiangang Luo","doi":"10.1002/lpor.202500741","DOIUrl":"https://doi.org/10.1002/lpor.202500741","url":null,"abstract":"Precise transverse displacement metrology is essential for super‐resolution microscopy, precision engineering, and semiconductor manufacturing. Conventional methods encounter challenges related to miniaturization, complexity, and sensitivity to transverse motion. Metasurface‐based methods achieve nanometric resolution but are hindered by fabrication complexity, limited dynamic range, and ambiguity in absolute displacement measurement. An ultrasensitive vector displacement sensor utilizing liquid crystal optical elements (LCOE) under vector beam illumination is presented. By mapping the transverse displacement to the polarization change of a radial vector beam, the displacement length can be directly inferred using Malus' law, and the displacement direction can be easily determined from the rotation of the vector beam speckle. Remarkably, uncertainties of 47 and 55 pm are achieved over centimeter‐scale ranges, with step sizes of 10 and 5 nm, respectively. This method combines nanometric resolution, an extended dynamic range, and compactness, providing innovative metrological principles for next‐generation precision measurement applications. The integration of LCOEs and vector beams enables absolute displacement measurement without the need for complex nanofabrication, overcoming critical limitations of current technologies.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"690 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144593897","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advanced Mid‐Infrared Laser Spectroscopy for Ultra‐Low Concentration Protein Detection 用于超低浓度蛋白质检测的先进中红外激光光谱
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-09 DOI: 10.1002/lpor.202500718
Zihao Liu, Jing Ni, Zhouzhuo Tang, Qi Jie Wang, Xia Yu
{"title":"Advanced Mid‐Infrared Laser Spectroscopy for Ultra‐Low Concentration Protein Detection","authors":"Zihao Liu, Jing Ni, Zhouzhuo Tang, Qi Jie Wang, Xia Yu","doi":"10.1002/lpor.202500718","DOIUrl":"https://doi.org/10.1002/lpor.202500718","url":null,"abstract":"Mid‐infrared absorption spectroscopy stands as a pivotal technique for protein analysis, offering noninvasive, label‐free detection and the capability of real‐time monitoring, and can reflect conformational changes through spectral characteristics. Despite its significance, the prevailing mid‐infrared absorption spectroscopy systems for protein analysis are hampered by instrument complexity, high costs, and limited sensitivity, which impede their widespread application. Here, a high‐sensitivity protein mid‐infrared laser spectroscopy sensor using a quartz hollow waveguide as a microfluidic reaction vessel is proposed. On the ultra‐long reaction path provided by quartz hollow waveguides, gold core–shell nanoparticles are modified to induce surface‐enhanced infrared absorption (SEIRA) effect, and further biotin functionalization to obtain streptavidin capture capability. Notably, the gold core–shell particles are optimized based on the time‐coupled mode theory (TCMT) to better match the hollow waveguide transmission structure. The results demonstrate that the detection limits of streptavidin in the amide I and amide II bands are 35.68 and 38.69 ng mL<jats:sup>−1</jats:sup>, respectively. The proposed surface enhanced hollow waveguide realizes the simultaneous detection of the lowest detection limit of the protein amide I and amide II bands by infrared spectroscopy, which provides a powerful platform for protein analysis.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"10 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144594057","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Multimode Long‐Persistent Luminescence and Photochromism From Lead‐Doped CsCdCl3 Metal Halide Toward Advanced Multiple Anti‐Counterfeiting and Information Storage 铅掺杂CsCdCl3金属卤化物在先进多重防伪和信息存储方面的多模长持久发光和光致变色性能
IF 11 1区 物理与天体物理
Laser & Photonics Reviews Pub Date : 2025-07-07 DOI: 10.1002/lpor.202500959
Zutao Fan, Yayin Liu, Jinhong Chen, Jie Zhang, Chengxue Deng, Yu Wang
{"title":"Multimode Long‐Persistent Luminescence and Photochromism From Lead‐Doped CsCdCl3 Metal Halide Toward Advanced Multiple Anti‐Counterfeiting and Information Storage","authors":"Zutao Fan, Yayin Liu, Jinhong Chen, Jie Zhang, Chengxue Deng, Yu Wang","doi":"10.1002/lpor.202500959","DOIUrl":"https://doi.org/10.1002/lpor.202500959","url":null,"abstract":"Doping in single‐component metal halide perovskites to adjust defect levels plays a crucial role in self‐trapped exciton (STE) emission, which is critical for tunable multi‐mode luminescence and photochromism (PC). The introduction of cations (Pb<jats:sup>2+</jats:sup>) into the hexagonal CsCdCl<jats:sub>3</jats:sub> perovskite results in the disruption of the local symmetry of the matrix framework, establishing new trap states and trap centers, which in turn facilitate the creation of multimode persistent luminescence (PersL) materials. Temperature‐dependent fluorescence and thermoluminescence (TL) spectra reveal that Pb<jats:sup>2+</jats:sup> influences the redistribution of defects, providing new emission pathways and enabling efficient tuning of the room‐temperature emission. In addition, chlorine vacancies (V<jats:sub>Cl</jats:sub>) in CsCdCl<jats:sub>3</jats:sub>:Pb facilitates the capture of electrons to form F‐centers, resulting in remarkable PC. First‐principles theory simulations demonstrate the introduction of Pb<jats:sup>2+</jats:sup> ions alter the original energy band structure and charge distribution, confirming their tendency to induce defect formation at different symmetry sites. This effective method of modifying the optical properties of CsCdCl<jats:sub>3</jats:sub> microcrystals through Pb<jats:sup>2+</jats:sup> doping integrates multimode tunable UV/X‐ray induced PersL and rewritable PC, offering promising material candidates for more reliable and efficient anti‐counterfeiting and information storage applications.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"21 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144577858","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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