V. Blideanu , R. Behal , C. Besnard-Vauterin , V. Glagolev , X. Ledoux , J. Mrazek , B. Rapp , E. Simeckova
{"title":"Experimental assessment and analysis of calculations accuracy for the neutron-induced radio-isotopes in copper parts of radiotherapy accelerators","authors":"V. Blideanu , R. Behal , C. Besnard-Vauterin , V. Glagolev , X. Ledoux , J. Mrazek , B. Rapp , E. Simeckova","doi":"10.1016/j.nimb.2024.165553","DOIUrl":"10.1016/j.nimb.2024.165553","url":null,"abstract":"<div><div>Induced radioactivity in particle accelerators is currently not sufficiently addressed, particularly for radiotherapy electron LINACs when the activation occurs via secondary neutrons created in photo-nuclear reactions.</div><div>Methodologies based on Monte-Carlo simulations coupled with activation calculation codes are often used to address this issue. Their accuracy, which is potentially affected by the limited capabilities of the calculation tools to simulate nuclear reactions at the origin of the materials activation, can be deeply analyzed only through comparisons with experimental values but the latter are not widely available.</div><div>New macroscopic data for the activity induced by neutrons in the materials commonly present in medical electron LINACs are presented. Neutron-induced activation has been measured by sample irradiation at SPIRAL2/NFS facility in accurately characterized configurations. Experimental results were compared to the simulations predictions allowing to assess the precision that can be achieved by a fully simulation-based methodology, mainly related to the energy-dependent reaction cross-sections.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165553"},"PeriodicalIF":1.4,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142537431","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Mikko Kivekäs , Kenichiro Mizohata , Jaakko Julin , Markku Kainlauri , Mika Prunnila , Laura Keränen , Matti Putkonen , Tatu Korkiamäki , Mikko Laitinen
{"title":"Elastic recoil and scattering yields measured in low energy heavy ion ERD","authors":"Mikko Kivekäs , Kenichiro Mizohata , Jaakko Julin , Markku Kainlauri , Mika Prunnila , Laura Keränen , Matti Putkonen , Tatu Korkiamäki , Mikko Laitinen","doi":"10.1016/j.nimb.2024.165542","DOIUrl":"10.1016/j.nimb.2024.165542","url":null,"abstract":"<div><div>Experimental yields of low energy recoils and scattered beams in ToF-ERD have been measured and compared against theory. A significant discrepancy between Rutherford or Andersen cross-section predicted yield vs the experimental results is now demonstrated. Scale of the discrepancy is up to 50% compared to yields predicted by theory for low energy Au recoils. MCERD simulations were used to study the carbon foil scattering in the timing detectors to explain the observed discrepancy. Simulations indicate that a major part of the discrepancy occurs due to the scattering of low energy, heavy mass particles in the timing detector foils. The yield discrepancy can be narrowed down by taking into account the reduction of recoil yields caused by the carbon foil scattering. Further studies are in progress to study carbon foil scattering, aiming to further improve the quantitativity of ToF-ERD for the heavy elements.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165542"},"PeriodicalIF":1.4,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142537430","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Validation of crystal surface scattering method for downsizing accelerator mass spectrometry","authors":"Satoshi Jinno , Akihiro Matsubara , Natsuko Fujita , Kenji Kimura","doi":"10.1016/j.nimb.2024.165545","DOIUrl":"10.1016/j.nimb.2024.165545","url":null,"abstract":"<div><div>This study introduces the development of a downsized Accelerator Mass Spectrometry (AMS) system aiming to enhance accessibility and cost-effectiveness in radiocarbon analysis. The “crystal surface stripper method” is introduced as a solution to challenges in AMS downsizing, demonstrating effective ion detection with a smaller angular spread compared to conventional gas stripper methods. The experimental results provide insights into charge conversion capabilities, scattering angle broadening, and energy loss associated with surface scattering.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165545"},"PeriodicalIF":1.4,"publicationDate":"2024-10-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142536120","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"ESR spectroscopic analysis of fructose as a dosimeter for gamma radiation","authors":"Arif Rachmanto , Marrisa Arlinkha Ega Putri , Muhamad Yasin Yunus , Ade Lestari Yunus , Rizka Fitriana , Rahmawati Rahmawati","doi":"10.1016/j.nimb.2024.165551","DOIUrl":"10.1016/j.nimb.2024.165551","url":null,"abstract":"<div><div>In this research, fructose was used as a dosimeter, and ESR examined the influence of radiation dose on the dosimeter’s properties. Microwave power, g-value, and decay of response tests were carried out at doses of 1, 5, and 10 kGy. The results show that fructose possesses linearity at doses of 5 × 10<sup>−2</sup>–30 kGy. The radiation detection sensitivity of fructose is better than sucrose’s but less than alanine’s over the entire dose range. The irradiation dose influences microwave saturation on ESR intensity, occurring at 5 and 10 kGy. The microwave power for irradiated fructose ranges from 1.00 to 2.46 mW. The ESR signal intensity increases with higher radiation doses, primarily due to the formation of more free radicals. Additionally, higher radiation doses lead to faster decay of the fructose dosimeter’s response. The fructose ESR intensity stability compared to alanine and sucrose at 1, 5, and 10 kGy are alanine > sucrose > fructose, alanine > fructose > sucrose, and alanine > fructose ≈ sucrose, respectively.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165551"},"PeriodicalIF":1.4,"publicationDate":"2024-10-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142536122","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
R. Holeňák , E. Ntemou , M. Kokkoris , S. Petrović , D. Primetzhofer
{"title":"Tracing of low-energy protons implanted in different Si crystal orientations by keV recoil detection in transmission geometry","authors":"R. Holeňák , E. Ntemou , M. Kokkoris , S. Petrović , D. Primetzhofer","doi":"10.1016/j.nimb.2024.165546","DOIUrl":"10.1016/j.nimb.2024.165546","url":null,"abstract":"<div><div>The potential of recoil detection in transmission geometry in examining a possible preferential lattice site location of H atoms implanted into thin single crystalline silicon membranes is explored. Low-energy protons were directed onto the membranes along the 〈0<!--> <!-->0<!--> <!-->1〉 Si crystal axis, as well as in random orientation. Position-sensitive and time-resolved detection of recoiling hydrogen species from a pulsed beam of 280 keV <sup>22</sup>Ne<sup>+</sup> primary ions was performed in a time-of-flight medium energy ion scattering system. From the primary beam incidence along different crystal axes, a preferential detection of recoiled hydrogen along the 〈0<!--> <!-->1<!--> <!-->1〉 axis can be revealed, as compared to the 〈0<!--> <!-->0<!--> <!-->1〉 axis. The present approach and possible future developments potentially enabling real-space location of interstitial hydrogen are discussed.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165546"},"PeriodicalIF":1.4,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142536119","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yingying Wang, Yutian Li, Yang Gao, Yiming Chen, Zhanrong Zhou, Xiaofang Shen, Guofeng Jin
{"title":"Study on fragmentation dynamics of NH32+ induced by electron impact","authors":"Yingying Wang, Yutian Li, Yang Gao, Yiming Chen, Zhanrong Zhou, Xiaofang Shen, Guofeng Jin","doi":"10.1016/j.nimb.2024.165547","DOIUrl":"10.1016/j.nimb.2024.165547","url":null,"abstract":"<div><div>In this study, the fragmentation dynamics of ammonia are investigated using the 205-eV electrons impact ionization by a reaction microscope. The two- and three-body dissociation channels of NH<sub>3</sub><sup>2+</sup> ions are identified by the coincidence measurement of fragment ions, and the dication electronic states are determined. In the three-body dissociation channel, including the Dalitz plots and Newton diagrams, the partitioning of the neutral hydrogen’s energy provides a deeper understanding of the fragmentation mechanisms. Using the energy of hydrogen as a filter, the discovery of two electronic states provides a more specific explanation of the mechanism of the direct dissociation process. By employing the kinetic energy (KE) of fragments, the mechanisms of three-body dissociation channels have been further validated. This study provides more detailed information for subsequent research on the dissociation dynamics of ammonia.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165547"},"PeriodicalIF":1.4,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142536121","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Measurements of displacement cross sections of metals for 120-GeV proton beam irradiation","authors":"Yosuke Iwamoto , Hiroki Matsuda , Shin-ichiro Meigo , Katsuya Yonehara , Frederique Pellemoine , Zunping Liu , Kevin Lynch , Makoto Yoshida , Atsushi Yabuuchi , Toshimasa Yoshiie , Shintaro Hashimoto","doi":"10.1016/j.nimb.2024.165543","DOIUrl":"10.1016/j.nimb.2024.165543","url":null,"abstract":"<div><div>The number of displacements per atom (dpa) is widely used as an indicator of irradiation damage of materials in proton accelerator facilities. Experiments have been carried out to validate the dpa of metallic materials for protons with energies below 3 GeV. However, measurements of the displacement cross-sections for high-energy protons above 3 GeV have not been carried out and the calculations have not been validated. To validate the displacement cross section of metals in high-energy region, electrical resistivity changes in wires of aluminum, copper and tungsten at 8 K were measured using protons with energies of 120-GeV. The results show that the Norgett-Robinson-Torrens dpa model of the Particle and Heavy Ion Transport Calculation Code overestimates the experimental data. On the other hand, the calculated results using the athermal recombination corrected dpa model were in agreement with the measured displacement cross sections. In the proton energy region above 1 GeV, the displacement cross section is almost constant, which is due to the fact that the damage energy of the material under 1 GeV proton irradiation is almost the same as under 120 GeV proton irradiation. Damage recovery of defects accumulated in the sample was also measured using isochronal annealing: At 80 K, approximately 60 % and 80 % of the damage remains for copper and tungsten, respectively. These results are the same as those obtained from other experiments on proton and neutron irradiation.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165543"},"PeriodicalIF":1.4,"publicationDate":"2024-10-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142441437","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Frans Munnik , Lars Lorenz , Fabian Härtwig , Stefan Makowski , Matthias Krause
{"title":"Ion beam microprobe analysis for friction-induced material transfer processes in ta-C/steel and ta-C/brass pairs","authors":"Frans Munnik , Lars Lorenz , Fabian Härtwig , Stefan Makowski , Matthias Krause","doi":"10.1016/j.nimb.2024.165540","DOIUrl":"10.1016/j.nimb.2024.165540","url":null,"abstract":"<div><div>The application of Ion Beam Analysis with a focussed ion beam to the field of tribology, especially solid lubricant coatings that do not need liquid lubricants, is described. As model systems, tetrahedrally-amorphous carbon coatings (ta-C) after friction contact with 100Cr6 steel in high vacuum and with brass in ambient atmosphere were selected. With the appropriate combination of He and H ion beams and techniques like Rutherford Backscattering Spectrometry and Particle Induced X-ray Emission, detailed information was obtained about the laterally- and depth-resolved element composition in the wear tracks and counter body wear scars, leading to insights in the friction induced transformation processes between a solid coating and a counter body, including material loss of the coating and material transfer between the coating and counter body that are correlated with the friction experiments.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165540"},"PeriodicalIF":1.4,"publicationDate":"2024-10-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142425228","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
G. Gutierrez, C. Bernard, P. Billaud, D. Bossu, T. Cloutier, M. Loyer-Prost, H. Martin, E. Meslin, F. Nozais, B. Ridard, G. Sagnes, J.-L. Bechade
{"title":"The JANNuS-Saclay platform: New developments for the understanding of evolutions under irradiation in materials","authors":"G. Gutierrez, C. Bernard, P. Billaud, D. Bossu, T. Cloutier, M. Loyer-Prost, H. Martin, E. Meslin, F. Nozais, B. Ridard, G. Sagnes, J.-L. Bechade","doi":"10.1016/j.nimb.2024.165541","DOIUrl":"10.1016/j.nimb.2024.165541","url":null,"abstract":"<div><div>The JANNuS-Saclay multi-irradiation platform includes a triple beam facility coupled to an in-situ Raman spectrometer, established at CEA Saclay in 2009. In addition to the triple-beam chamber, two single-beam chambers are set up. Sample temperature can be varied from −180 °C to 800 °C, and at −260 °C or at 1200 °C in dedicated devices. The platform is also equipped with a multi-ion Beam Analysis chamber. JANNuS Saclay facility is a powerful tool to understand the changes generated by irradiation in materials, especially in nuclear application fields. This paper presents the recent facility developments since 2020.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165541"},"PeriodicalIF":1.4,"publicationDate":"2024-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142425229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Y. Ishii , R. Yamagata , T. Satoh , S. Matsuyama , T. Kamiya , S. Onoda
{"title":"Preliminary beam formations after the upgrade of the TIARA two microbeam systems","authors":"Y. Ishii , R. Yamagata , T. Satoh , S. Matsuyama , T. Kamiya , S. Onoda","doi":"10.1016/j.nimb.2024.165539","DOIUrl":"10.1016/j.nimb.2024.165539","url":null,"abstract":"<div><div>This paper presents a comprehensive study on the enhancements made to the heavy-ion microbeam (H-MB) and light-ion microbeam (L-MB) systems at the Takasaki Institute for Advanced Quantum Science, part of the National Institutes for Quantum Science and Technology (QST), and their implications for future research in ion microbeam technology. Our work addresses the critical need for submicron beam sizes in advanced ion microbeam applications, a challenge previously unmet due to limitations in the original system designs and aging components. The manuscript details the extensive upgrades undertaken for both the H-MB and L-MB systems, including the implementation of new quadruple magnets, refined demagnification strategies, and advanced control systems, culminating in the successful formation of submicron ion beams. The meticulous alignment procedures for both the H-MB and L-MB have enabled precise ion beam focusing. The current beam sizes have been measured at 1.0 × 1.1 µm<sup>2</sup> with a beam current of approximately 10 pA for the H-MB, and 500 × 600 nm<sup>2</sup> with a beam current of approximately 50 pA for the L-MB at a 3 MeV H<sup>+</sup> beam.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":"557 ","pages":"Article 165539"},"PeriodicalIF":1.4,"publicationDate":"2024-10-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142425227","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}