{"title":"Stopping of very heavy ions in Mylar","authors":"","doi":"10.1016/j.nimb.2024.165554","DOIUrl":"10.1016/j.nimb.2024.165554","url":null,"abstract":"<div><div>Available experimental data on Mylar stopping powers (<span><math><mrow><mi>S</mi><mi>P</mi></mrow></math></span>s) for heavy ions (HIs) at energies <span><math><mrow><mn>0</mn><mo>.</mo><mn>04</mn><mo>⩽</mo><mi>E</mi><mo>/</mo><mi>A</mi><mo>⩽</mo><mn>15</mn></mrow></math></span> MeV/nucleon have been compared to different semi-empirical model calculations with the aim of probing their possible usage for the estimates of ranges for very heavy ions at <span><math><mrow><mi>E</mi><mo>/</mo><mi>A</mi><mo><</mo><mn>0</mn><mo>.</mo><mn>5</mn></mrow></math></span> MeV/nucleon, which are of practical interest. Significant deviations from the calculated <span><math><mrow><mi>S</mi><mi>P</mi></mrow></math></span> values were found for fission fragments and lighter HIs at <span><math><mrow><mi>E</mi><mo>/</mo><mi>A</mi><mo><</mo><mn>1</mn></mrow></math></span> MeV/nucleon. A new model parameterization for Mylar <span><math><mrow><mi>S</mi><mi>P</mi></mrow></math></span> has been proposed. Range estimates obtained with any <span><math><mrow><mi>S</mi><mi>P</mi></mrow></math></span> model calculation show a critical dependence of their mean values on the approximated electronic stopping powers and the nuclear (collisional) <span><math><mrow><mi>S</mi><mi>P</mi></mrow></math></span> component. The last plays a crucial role at the end of the range and could only be obtained by calculations. Practical applicability of the results of investigation for very heavy evaporation residues (products of complete fusion reactions induced by HIs) implies the use of a thick catcher foil corresponding to the largest ranges derived in the estimates or the range measurements for these products.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-11-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142572080","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Forward and backward emission of secondary ions from biomolecules on single-layer graphene by MeV Cn+ (n = 1–6) impacts","authors":"","doi":"10.1016/j.nimb.2024.165548","DOIUrl":"10.1016/j.nimb.2024.165548","url":null,"abstract":"<div><div>We studied the emission of secondary ions using a cluster ion with MeV energy in transmission secondary ion mass spectrometry. The primary ions used were 0.6 MeV/atom C<em><sub>n</sub></em><sup>+</sup>, where <em>n</em> ranges from 1 to 6. Single-layer graphene was used as a support membrane for depositing a biomolecular target of phenylalanine. Positive secondary ions emitted in both forward and backward directions were measured separately. We found that the yield of forward-emitted secondary ions was higher than that of backward-emitted secondary ions. Our results showed that the yield of secondary ions emitted in both directions increased as the size of incident cluster ions increased. This increase was non-linear and can be attributed to the track overlap effect of incident cluster ions. We also found a scaling parameter consistently describing the incident cluster size dependence of the forward and backward-emitted secondary ion yields.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-11-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142572081","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Gamma irradiation effect on the structural and optical properties of manganese (III) phthalocyanine chloride films: Experimental and theoretical approach for optoelectronic applications","authors":"","doi":"10.1016/j.nimb.2024.165556","DOIUrl":"10.1016/j.nimb.2024.165556","url":null,"abstract":"<div><div>Irradiation using ionizing radiation such as gamma-ray alters the material characteristics of organic semiconductors, especially the optical and electronic properties. The potential changes of manganese phthalocyanine chloride (MnPcCl) films have been investigated after several gamma irradiation doses (50, 150, and 250 kGy). The possible chemical structure and electronic characteristics of MnPcCl dye were analyzed using the density functional theory-based quantum calculations. The X-ray diffraction of various gamma-ray doses confirmed the amorphous nature of MnPcCl. Based on UV–Vis-NIR spectrophotometric measurements, Tauc’s method has been used to deduce the optical bandgap energy of MnPcCl films before and after γ-irradiation. A slight non-linear reduction was observed in the optical bandgap energy, refractive index, and dielectric constant with rising γ-irradiation doses. The reduction in these optical parameters was due to the increase in the defects and the disorder degree created by γ-irradiation. The low effect on the optical parameters of MnPcCl films confirms its optical stability within this high range of γ-irradiation doses. Such investigation highlights the scope for the stability of this organic dye after exposure to γ-irradiation doses for use in optoelectronic/photonic technological devices.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142572079","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Reevaluation of neutron energy spectrum in Heavy-Water neutron irradiation facility of Kyoto University research Reactor using multifoil activation method","authors":"","doi":"10.1016/j.nimb.2024.165555","DOIUrl":"10.1016/j.nimb.2024.165555","url":null,"abstract":"<div><div>The Heavy-Water Thermal Neutron Facility at Kyoto University Research Reactor (KUR) has been operational for boron neutron capture therapy (BNCT) since May 1974. Following a facility construction update in 1996, the facility name was changed to the Heavy-Water Neutron Irradiation Facility (HWNIF), and the neutron energy spectra were evaluated using the multifoil activation method. In May 2010, the KUR transitioned its operations from high-enrichment fuel to low-enrichment fuel. However, the neutron energy spectrum in the KUR-HWNIF has not been reevaluated with high accuracy since then. This paper reports the reevaluation of the neutron energy spectrum for the standard epithermal-neutron irradiation mode using the multifoil activation method. Based on the reevaluated results, the epithermal- and fast-neutron fluxes increased by approximately 34 % and 19 %, respectively. The neutron absorption dose rate at evaluation point was approximately 17 % lower than the previous one; however, it remained acceptable from the perspective of BNCT biological irradiation.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142572078","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"A Comprehensive study of the exposure and energy absorption buildup factors in some polymer composites for point isotropic Source, including the effect of bremsstrahlung","authors":"","doi":"10.1016/j.nimb.2024.165552","DOIUrl":"10.1016/j.nimb.2024.165552","url":null,"abstract":"<div><div>The exposure (EBF) and energy absorption buildup factors (EABF) of different polymer composites (SiW, PHEMA-WO<sub>3</sub>, CaWO<sub>4</sub>, EWO<sub>3</sub>, BaTiO<sub>3</sub>, PbCl<sub>2</sub>) has been investigated for photon isotropic source with the energy range of 0.015–15 MeV and the penetration depth of 1–10 mean free path(mfp). Furthermore, the contribution of bremsstrahlung effect on selected polymer composites EBF has been discussed. Simulations were performed by MCNPX Monte Carlo code. Model validation was carried out by comparing theoretical uncollided flux and EBF of water with similar published data. The results indicate that EBF and EABF values are dependent on the incident photon energy and the depth of penetration. The maximum and minimum values of EBF and EABF are related to BaTiO<sub>3</sub> and SiW, respectively. Moreover, it is observed that considering bremsstrahlung increases values, especially at energies greater than 3 MeV.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142572077","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Measurement of flux-weighted average cross-section in the photo-neutron reactions of Nb at the bremsstrahlung end-point energies of 20 MeV and 67 MeV","authors":"","doi":"10.1016/j.nimb.2024.165557","DOIUrl":"10.1016/j.nimb.2024.165557","url":null,"abstract":"<div><div>The photo-neutron flux-weighted average cross-sections for <sup>93</sup>Nb(γ,xn) reactions at the bremsstrahlung end-point energies of 20 MeV and 67 MeV have been measured by the activation technique using the electron linear accelerator LUE-75 located at the A.I. Alikhanyan National Science Laboratory (AANL). Furthermore, the isomeric cross-section ratio has been determined for the <sup>89m,g</sup>Nb isomeric pair. TALYS 1.96 and EMPIRE 3.2 nuclear codes were used to calculate the <sup>93</sup>Nb(γ,xn) reaction cross-sections and isomeric ratio as functions of bremsstrahlung end-point energy. The energy distribution of bremsstrahlung photons has been calculated by GEANT4. The measured experimental data has been compared with currently available literature data as well as with the values based on theoretical calculations.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142555058","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Phase and composition analysis of erbium deuteride thin films prepared by magnetron reactive sputtering for proton source target","authors":"","doi":"10.1016/j.nimb.2024.165558","DOIUrl":"10.1016/j.nimb.2024.165558","url":null,"abstract":"<div><div>This study explores the synthesis and characterization of erbium deuteride (ErD<sub>x</sub>) thin films using magnetron reactive sputtering (MRS) under varying deuterium gas flow rates. The findings reveal that the stoichiometric ratio of deuterium to erbium (D/Er) can be effectively controlled by adjusting the D<sub>2</sub> flow rate, transitioning compositions from ErD<sub>2</sub> to ErD<sub>3</sub>. All films exhibited a cubic structure, with deuterium atoms occupying both tetrahedral and octahedral sites. Compared to the traditional two-step method, MRS-prepared films showed lower oxidation levels and higher preparation efficiency. Proton-source quality evaluation (PQE) confirmed the suitability of these films as high-quality targets. Additionally, this study introduces a rapid IBA method applicable during PQE, offering a non-destructive and cost-effective means to determine the composition within films.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142555057","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Study of 3089 keV gamma-ray emission from the reaction of 12C(d, pγ1-0)13C for analytical applications","authors":"","doi":"10.1016/j.nimb.2024.165549","DOIUrl":"10.1016/j.nimb.2024.165549","url":null,"abstract":"<div><div>In this work, the differential cross-sections of the <sup>12</sup>C(d, pγ<sub>1-0</sub>)<sup>13</sup>C reaction channel at an angle of 90° have been measured in the 585–1993 keV range using thin targets. The validity the present differential cross sections is checked by a benchmarking experiment. The obtained results are compared with the existing ones from literature. The total uncertainty of cross-sections is estimated to be 9 %.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142537429","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Experimental assessment and analysis of calculations accuracy for the neutron-induced radio-isotopes in copper parts of radiotherapy accelerators","authors":"","doi":"10.1016/j.nimb.2024.165553","DOIUrl":"10.1016/j.nimb.2024.165553","url":null,"abstract":"<div><div>Induced radioactivity in particle accelerators is currently not sufficiently addressed, particularly for radiotherapy electron LINACs when the activation occurs via secondary neutrons created in photo-nuclear reactions.</div><div>Methodologies based on Monte-Carlo simulations coupled with activation calculation codes are often used to address this issue. Their accuracy, which is potentially affected by the limited capabilities of the calculation tools to simulate nuclear reactions at the origin of the materials activation, can be deeply analyzed only through comparisons with experimental values but the latter are not widely available.</div><div>New macroscopic data for the activity induced by neutrons in the materials commonly present in medical electron LINACs are presented. Neutron-induced activation has been measured by sample irradiation at SPIRAL2/NFS facility in accurately characterized configurations. Experimental results were compared to the simulations predictions allowing to assess the precision that can be achieved by a fully simulation-based methodology, mainly related to the energy-dependent reaction cross-sections.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142537431","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Elastic recoil and scattering yields measured in low energy heavy ion ERD","authors":"","doi":"10.1016/j.nimb.2024.165542","DOIUrl":"10.1016/j.nimb.2024.165542","url":null,"abstract":"<div><div>Experimental yields of low energy recoils and scattered beams in ToF-ERD have been measured and compared against theory. A significant discrepancy between Rutherford or Andersen cross-section predicted yield vs the experimental results is now demonstrated. Scale of the discrepancy is up to 50% compared to yields predicted by theory for low energy Au recoils. MCERD simulations were used to study the carbon foil scattering in the timing detectors to explain the observed discrepancy. Simulations indicate that a major part of the discrepancy occurs due to the scattering of low energy, heavy mass particles in the timing detector foils. The yield discrepancy can be narrowed down by taking into account the reduction of recoil yields caused by the carbon foil scattering. Further studies are in progress to study carbon foil scattering, aiming to further improve the quantitativity of ToF-ERD for the heavy elements.</div></div>","PeriodicalId":19380,"journal":{"name":"Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms","volume":null,"pages":null},"PeriodicalIF":1.4,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142537430","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}