Interdisciplinary Materials最新文献_第2页

Advances in electrolyte–anode interface engineering of solid-state lithium metal batteries 固态锂金属电池电解质阳极界面工程的进展

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-30 DOI: 10.1002/idm2.12202

Menghong Li, Shubin Yang, Bin Li

{"title":"Advances in electrolyte–anode interface engineering of solid-state lithium metal batteries","authors":"Menghong Li, Shubin Yang, Bin Li","doi":"10.1002/idm2.12202","DOIUrl":"https://doi.org/10.1002/idm2.12202","url":null,"abstract":"Solid-state lithium metal batteries are considered to be the next generation of energy storage systems due to the high energy density brought by the use of metal lithium anode and the safety features brought by the use of solid electrolytes (SEs). Unfortunately, besides the safety features, using SEs brings issues of interfacial contact of lithium anode and electrolytes. Recently, to realize the application of solid-state lithium metal batteries, significant achievements have been made in the interface engineering of solid-state batteries, and various new strategies have been proposed. In this review, from the interface failure perspective of solid-state lithium metal batteries, we summarize failure mechanisms in terms of poor physical contact, weak chemical/electrochemical stability, continuing contact degradation, and uncontrollable lithium deposition. We then focused on the latest strategies for solving interface issues, including advancing in improving the physical solid–solid contact, increasing the electrochemical/chemical stability, restraining continuing contact degradation, and controlling homogeneous lithium deposition. The ultimate and paramount future developing directions of solid-state lithium metal battery interface engineering are proposed.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"805-834"},"PeriodicalIF":24.5,"publicationDate":"2024-07-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12202","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142665154","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Anisotropic thermally conductive films based on two-dimensional nanomaterials 基于二维纳米材料的各向异性导热薄膜

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-21 DOI: 10.1002/idm2.12204

Lei Li, Qunfeng Cheng

{"title":"Anisotropic thermally conductive films based on two-dimensional nanomaterials","authors":"Lei Li, Qunfeng Cheng","doi":"10.1002/idm2.12204","DOIUrl":"10.1002/idm2.12204","url":null,"abstract":"The significant advancement of high-power densification and miniaturization in modern electronic devices has attracted increasing attention to effective thermal management. The primary objective of thermal management is to transfer excess heat from electronics to the outside environment through the use of thermal conductive materials. The anisotropic thermally conductive films (TCFs) based on two-dimensional (2D) nanomaterials exhibit outstanding controlled heat transfer capability, which effectively removes hotspots along the in-plane direction and provides thermal insulation along the cross-plane direction. However, a comprehensive review of anisotropic TCFs is rarely reported. Herein, we first discuss the intrinsic anisotropic thermal conductivity of 2D nanomaterials for preparing TCFs. Then, the preparation methods and anisotropic thermal conductivity of TCFs have been summarized and discussed. Furthermore, we conclude with the practical applications of TCFs for anisotropy thermal management. Finally, a conclusion of the challenges and outlook of TCFs is provided to promote their development in future scientific research.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"847-864"},"PeriodicalIF":24.5,"publicationDate":"2024-07-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12204","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141818759","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Inside Front Cover: Volume 3 Issue 4 封面内页：第 3 卷第 4 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-18 DOI: 10.1002/idm2.12206

引用次数: 0

Inside Back Cover: Volume 3 Issue 4 封底内页第 3 卷第 4 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-18 DOI: 10.1002/idm2.12207

引用次数: 0

Outside Back Cover: Volume 3 Issue 4 封底外页第 3 卷第 4 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-18 DOI: 10.1002/idm2.12208

引用次数: 0

Outside Front Cover: Volume 3 Issue 4 封面外页：第 3 卷第 4 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-18 DOI: 10.1002/idm2.12205

引用次数: 0

Facile synthesis of Pt clusters decorated TiO2 nanoparticles for efficient photocatalytic degradation of antibiotics 简便合成铂团簇装饰的 TiO2 纳米粒子，用于高效光催化降解抗生素

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-17 DOI: 10.1002/idm2.12203

Yin Pan, Weizhen Liang, Zongpeng Wang, Junjie Gong, Yichao Wang, Aijiao Xu, Zhenyuan Teng, Shijie Shen, Lin Gu, Wenwu Zhong, Hongsheng Lu, Baofu Chen

{"title":"Facile synthesis of Pt clusters decorated TiO2 nanoparticles for efficient photocatalytic degradation of antibiotics","authors":"Yin Pan, Weizhen Liang, Zongpeng Wang, Junjie Gong, Yichao Wang, Aijiao Xu, Zhenyuan Teng, Shijie Shen, Lin Gu, Wenwu Zhong, Hongsheng Lu, Baofu Chen","doi":"10.1002/idm2.12203","DOIUrl":"10.1002/idm2.12203","url":null,"abstract":"TiO2 has attracted much attention in the field of photocatalytic degradation of antibiotics due to its good photostability, nontoxicity, and low cost. However, the rapid recombination of photogenerated carriers limits the further improvement of its photocatalytic activity. Here, a facile microwave-assisted hydrothermal method has been developed to prepare Pt clusters decorated TiO2 nanoparticles. Pt clusters ranging in size from 1 to 2 nm are uniformly distributed across the surface of the TiO2 matrix. A pronounced charge transfer phenomenon is discernible between the Pt and TiO2 components. It is revealed that the charge transfer enables faster transfer and separation of photogenerated electrons and holes, which are beneficial for the improvement of photocatalytic degradation of both ofloxacin and levofloxacin. The degradation capability can be attributed to the efficient generation of •OH or •O2− species within the solution. The parallel adsorption model of TiO2 on antibiotic molecules is verified, and the degradation reaction pathway has been elucidated. This work provides a facile method for optimizing the performance of TiO2 photocatalysts, which can be extended to other oxide photocatalysts.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"935-945"},"PeriodicalIF":24.5,"publicationDate":"2024-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12203","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141830492","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Interface strengthening for carbon fiber-reinforced poly(ether-ether-ketone) laminated composites by introducing fluorene-containing branched poly(aryl-ether-ketone) 通过引入含芴支链聚芳醚酮，增强碳纤维增强聚芳醚酮层压复合材料的界面强度

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-17 DOI: 10.1002/idm2.12200

Zheng Liu, Xuerong Fan, Xinghan Lu, Xuetao Shi, Junliang Zhang, Hua Guo, Mukun He, Junwei Gu

{"title":"Interface strengthening for carbon fiber-reinforced poly(ether-ether-ketone) laminated composites by introducing fluorene-containing branched poly(aryl-ether-ketone)","authors":"Zheng Liu, Xuerong Fan, Xinghan Lu, Xuetao Shi, Junliang Zhang, Hua Guo, Mukun He, Junwei Gu","doi":"10.1002/idm2.12200","DOIUrl":"10.1002/idm2.12200","url":null,"abstract":"Fluorene-containing branched poly(aryl-ether-ketone) (BFPAEK) with terminal hydroxyl groups is synthesized by random copolycondensation reaction; then, the CF@BFPAEK/PEEK laminated composite is prepared by the “powder impregnation-high temperature compression molding” method with poly(ether-ether-ketone) (PEEK) as the matrix and BFPAEK-modified carbon fiber (CF@BFPAEK) as the reinforcement. When the content of branched units in BFPAEK is 10% and the coating amount of BFPAEK on the carbon fiber (CF) surface is 3 wt%, the CF@BFPAEK/PEEK laminated composite has outstanding mechanical properties, with an interlaminar shear strength (ILSS) of 57.3 MPa and flexural strength of 589.4 MPa, which are 80.2% and 44.3% higher than those of the pure CF/PEEK laminated composite (31.8 and 408.4 MPa), respectively. After 288 h of hydrothermal aging and high/low-temperature alternating aging, the corresponding retention rate of ILSS and flexural strength are respectively 87.9% and 84.7%, higher than those of pure CF/PEEK laminated composites (74.5% and 70.4%). The thermal conductivity coefficient and temperature for 5% weight loss of CF@BFPAEK/PEEK laminated composite are 1.85 W m−1 K−1 and 538.0°C, respectively.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"919-934"},"PeriodicalIF":24.5,"publicationDate":"2024-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12200","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141830074","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Atypical artificial cells: Novel biomimetic materials for combating cancer 非典型人工细胞：用于抗癌的新型仿生材料

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-17 DOI: 10.1002/idm2.12199

Zhao-yang Ren, Qian-qian Wan, Yi-na Zhu, Ling Li, Kai-yan Wang, Fei Zhao, Kai Jiao, Michelle Tang, Franklin Tay, Mei-chen Wan, Li-na Niu

引用次数: 0

Oxygenated carbon nitride-based high-energy-density lithium-metal batteries 含氧氮化碳基高能量密度锂金属电池

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-10 DOI: 10.1002/idm2.12201

Mengnan Shen, Ying Wei, Man Ge, Shengdong Yu, Ronghui Dou, Liuhua Chen, Feng Wang, Yunhui Huang, Henghui Xu

{"title":"Oxygenated carbon nitride-based high-energy-density lithium-metal batteries","authors":"Mengnan Shen, Ying Wei, Man Ge, Shengdong Yu, Ronghui Dou, Liuhua Chen, Feng Wang, Yunhui Huang, Henghui Xu","doi":"10.1002/idm2.12201","DOIUrl":"10.1002/idm2.12201","url":null,"abstract":"Lithium (Li)-metal batteries with polymer electrolytes are promising for high-energy-density and safe energy storage applications. However, current polymer electrolytes suffer either low ionic conductivity or inadequate ability to suppress Li dendrite growth at high current densities. This study addresses both issues by incorporating two-dimensional oxygenated carbon nitride (2D OCN) into a polyvinylidene fluoride (PVDF)-based composite polymer electrolyte and modifying the Li anode with OCN. The OCN nanosheets incorporated PVDF electrolyte exhibits a high ionic conductivity (1.6 × 10−4 S cm−1 at 25°C) and Li+ transference number (0.62), wide electrochemical window (5.3), and excellent fire resistance. Furthermore, the OCN-modified Li anode in situ generates a protective layer of Li3N during cycling, preventing undesirable reactions with PVDF electrolyte and effectively suppressing Li dendrite growth. Symmetric cells using the upgraded PVDF polymer electrolyte and modified Li anode demonstrate long cycling stability over 2500 h at 0.1 mA cm−2. Full cells with a high-voltage LiNi0.8Co0.1Mn0.1O2 cathode exhibit high energy density and long-term cycling stability, even at a high loading of 8.2 mg cm−2. Incorporating 2D OCN nanosheets into the PVDF-based electrolyte and Li-metal anode provides an effective strategy for achieving safe and high-energy-density Li-metal batteries.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 5","pages":"791-800"},"PeriodicalIF":24.5,"publicationDate":"2024-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12201","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141662431","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0