Interdisciplinary Materials最新文献

Outside Back Cover: Volume 4 Issue 4 外封底：第4卷第4期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-07-25 DOI: 10.1002/idm2.70007

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Outside Front Cover: Volume 4 Issue 4 封面：第4卷第4期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-07-25 DOI: 10.1002/idm2.12189

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Materials-Algorithm Co-Optimization for Specific and Quantitative Gas Detection 特定和定量气体检测的材料-算法协同优化

IF 24.5

Interdisciplinary Materials Pub Date : 2025-07-15 DOI: 10.1002/idm2.70001

Long Li, Lanpeng Guo, Binzhou Ying, Xinyi Chen, Wenjian Zhang, Kenan Liu, Shikang Xu, Licheng Zhou, Tiankun Li, Wei Luo, Bingbing Chen, Hua-Yao Li, Huan Liu

{"title":"Materials-Algorithm Co-Optimization for Specific and Quantitative Gas Detection","authors":"Long Li, Lanpeng Guo, Binzhou Ying, Xinyi Chen, Wenjian Zhang, Kenan Liu, Shikang Xu, Licheng Zhou, Tiankun Li, Wei Luo, Bingbing Chen, Hua-Yao Li, Huan Liu","doi":"10.1002/idm2.70001","DOIUrl":"https://doi.org/10.1002/idm2.70001","url":null,"abstract":"Rapid, reliable, and quantitative formaldehyde detection has become increasingly important in the processing industry and environmental protection. As an intelligent electronic instrument, the realization of electronic noses (e-noses) for quantitative gas detection relies on enhanced specificity. Here, we propose a materials-algorithm co-optimization (MACO) method that enables quantitative detection of formaldehyde in e-nose. This approach employs thermokinetic feature engineering to optimize data quality and algorithm selection, thereby reducing dependence on data scale and computing power resources. Specific thermokinetic activation patterns for formaldehyde can be generated through a single materials processing strategy. Through a combination of thermokinetic feature-driven machine learning, we demonstrated an e-nose—comprising only five Co3O4-based gas sensors—capable of discriminating formaldehyde from ethanol. The mathematical model reveals that the physicochemical mechanism of odor coding logic in our e-nose is dictated by the mass action law. A quantitative detection of formaldehyde in 0.1–20 ppm with a precision of 5% full-scale (F.S.) has been demonstrated. We also showcase the adaptability of e-nose for binary mixture analysis. The detection model of the MACO-driven e-nose is simple and interpretable, showing broad prospects to achieve quantitative gas detection rapidly and at a low cost.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"630-639"},"PeriodicalIF":24.5,"publicationDate":"2025-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.70001","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705511","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Evidence of X-Ray Magnetic Circular Dichroism and Low-Field Microwave Absorption in Room-Temperature Organic Ferromagnetic Semiconductor 室温有机铁磁半导体中x射线磁圆二色性和低场微波吸收的证据

IF 24.5

Interdisciplinary Materials Pub Date : 2025-07-10 DOI: 10.1002/idm2.70002

Jiaji Yang, Hanlin Gan, Xiandong He, Yanuo Zhu, Shaohua Tong, Wei Cui, Jiang Zhang, Qinglin Jiang, Yuguang Ma

{"title":"Evidence of X-Ray Magnetic Circular Dichroism and Low-Field Microwave Absorption in Room-Temperature Organic Ferromagnetic Semiconductor","authors":"Jiaji Yang, Hanlin Gan, Xiandong He, Yanuo Zhu, Shaohua Tong, Wei Cui, Jiang Zhang, Qinglin Jiang, Yuguang Ma","doi":"10.1002/idm2.70002","DOIUrl":"https://doi.org/10.1002/idm2.70002","url":null,"abstract":"Room-temperature organic ferromagnetic semiconductors represent a promising frontier in developing next-generation electronic and spintronic devices. However, the origin of magnetic moments in organic ferromagnets and the acquisition of critical evidence for magnetic ordering remain incompletely understood. This study presents compelling evidence for room-temperature ferromagnetism in N,N′-diamino perylene bisimide (2NH2-PBI) radical aggregates through a comprehensive analysis utilizing X-ray magnetic circular dichroism (XMCD), low-field microwave absorption (LFMA) techniques and magnetic characterization. The 2NH2-PBI samples, prepared via hydrothermal reduction, exhibit a significant saturation magnetization of 0.8 emu g−1 (336.3 emu mol−1) at 300 K, with a coercive field of 170 Oe. The XMCD measurements at the carbon K-edge exhibited a pronounced dichroic signal (~8.7%), confirming the origin of ferromagnetism in the π-conjugated electrons of the perylene core. Density functional theory calculations further support this finding by demonstrating that spin density is primarily delocalized on the π-conjugated skeleton, giving a microscopic explanation for the magnetic properties of 2NH2-PBI radicals. Furthermore, LFMA studies provide additional evidence of ferromagnetic ordering, showcasing hysteretic behavior consistent with domain wall dynamics. Our work indicates that imide-based radical molecules with extended π-conjugated structures constitute a class of effective magnetic functional units.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"576-584"},"PeriodicalIF":24.5,"publicationDate":"2025-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.70002","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705573","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

On-Chip Construction of Hierarchically Macro-/Mesoporous Cerium Oxide/Pt Gas Sensitive Film for Ultrasensitive Detection of Trace Oxygen 级联宏/介孔氧化铈/铂气敏膜超灵敏检测痕量氧的片上构建

IF 24.5

Interdisciplinary Materials Pub Date : 2025-07-01 DOI: 10.1002/idm2.12254

Yu Deng, Keyu Chen, Wenhe Xie, Xin-Yu Huang, Fengluan Jiang, Lingxiao Xue, Ziling Zhang, Qin Yue, Limin Wu, Wei Luo, Yonghui Deng

{"title":"On-Chip Construction of Hierarchically Macro-/Mesoporous Cerium Oxide/Pt Gas Sensitive Film for Ultrasensitive Detection of Trace Oxygen","authors":"Yu Deng, Keyu Chen, Wenhe Xie, Xin-Yu Huang, Fengluan Jiang, Lingxiao Xue, Ziling Zhang, Qin Yue, Limin Wu, Wei Luo, Yonghui Deng","doi":"10.1002/idm2.12254","DOIUrl":"https://doi.org/10.1002/idm2.12254","url":null,"abstract":"Hierarchically porous structure is extremely favorable for many applications, including heterogeneous catalysis, chemical sensing, and energy conversion and storage. In these applications, controllable synthesis and assembly of transition metal oxide materials with tailored hierarchically porous structure and chemical microenvironments are highly desired but challenging. Herein, uniform mesoporous cerium oxide (mCeO2) microspheres functionalized with Pt nanoparticles (NPs) were designed via efficient nanoemulsion approach and used to construct hierarchical macro-/mesoporous CeO2/Pt film on micro-electromechanical system (MEMS) chips. The resultant functional chip-based devices have controllable porous structure and rich highly accessible active Pt–CeO2 interfaces, and thus they exhibit outstanding performance as oxygen sensors with an unprecedented low limit of detection (LOD, 7.16 ppm), high sensitivity at a relatively low working temperature (250°C). Finite element analysis, density functional theory calculations, and in situ characterizations reveal that, such an excellent performance is mainly due to the favorable mass transfer and gas–solid interface interaction, the oxygen spillover effect enabled by the nanosized Pt, and the enhanced catalytic reaction causing the dramatic change of electronic resistance of the sensing layer in oxygen atmosphere. Finally, a smart gas sensing module capable of real-time precise detection of oxygen was fabricated, demonstrating the possibility for commercial application.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"585-598"},"PeriodicalIF":24.5,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12254","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705326","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Efficient Inverted Perovskite Solar Cells Enabled by Sequential Passivation Using Two-Dimensional Perovskites 利用二维钙钛矿序贯钝化实现高效倒置钙钛矿太阳能电池

IF 24.5

Interdisciplinary Materials Pub Date : 2025-07-01 DOI: 10.1002/idm2.12256

Bingcan Ke, Jing Li, Zewei Zhu, Siqi Zhang, Ruixuan Jiang, Chengkai Jin, Chang Hu, Qi Zhang, Jie Su, Sai Bai, Fuzhi Huang, Yi-Bing Cheng, Tongle Bu

{"title":"Efficient Inverted Perovskite Solar Cells Enabled by Sequential Passivation Using Two-Dimensional Perovskites","authors":"Bingcan Ke, Jing Li, Zewei Zhu, Siqi Zhang, Ruixuan Jiang, Chengkai Jin, Chang Hu, Qi Zhang, Jie Su, Sai Bai, Fuzhi Huang, Yi-Bing Cheng, Tongle Bu","doi":"10.1002/idm2.12256","DOIUrl":"https://doi.org/10.1002/idm2.12256","url":null,"abstract":"Refining the process in which two-dimensional (2D) perovskites passivate three-dimensional (3D) perovskites is vital for improving the performance of perovskite solar cells (PSCs), yet is frequently overlooked. Herein, a novel sequential passivation process that initially employs phenethylamine iodide (PEAI) on the 3D perovskite surface, followed by treatment with 4-trifluoromethylphenylethylamine iodide (CF3PEAI) is presented. A comprehensive comparison of the intrinsic molecular structures and their impact on the perovskites reveals that the small-sized, low-polarized PEA molecule induces minimal lattice strain and a negative shift of the vacuum energy level of perovskite surface, whereas the large-sized, high-polarized CF3PEA molecule leads to larger lattice strain and a positive shift of the vacuum energy level. By leveraging the opposing properties of these molecules through our tailored sequential passivation strategy, optimal passivation effects and efficient interface charge transfer are obtained, outperforming the posttreatment with mixed ligands and greatly surpassing posttreatment with a single ligand. Consequently, a champion efficiency of 26.27% is achieved for the inverted PSCs, along with outstanding operational stability featuring a T80 lifetime exceeding 1000 h under continuous light illumination at the maximum power point tracking.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"620-629"},"PeriodicalIF":24.5,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12256","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705328","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Creating Biomimetic Bouligand Architectures for Biomedical and Healthcare Applications 为生物医学和医疗保健应用创建仿生Bouligand建筑

IF 24.5

Interdisciplinary Materials Pub Date : 2025-07-01 DOI: 10.1002/idm2.12260

Hongye Yang, Xinyu Zhang, Shilei Wang, Yize Wang, Rui Xiong, Cui Huang

{"title":"Creating Biomimetic Bouligand Architectures for Biomedical and Healthcare Applications","authors":"Hongye Yang, Xinyu Zhang, Shilei Wang, Yize Wang, Rui Xiong, Cui Huang","doi":"10.1002/idm2.12260","DOIUrl":"https://doi.org/10.1002/idm2.12260","url":null,"abstract":"The hierarchical Bouligand structure, ubiquitous in organisms and endowing natural creatures with exceptional performance attributes, stands as a prime example of nature's evolutionary prowess. Following the example of nature, the construction of biomimetic Bouligand structures will significantly propel advancements and innovations within the domain of biomedical and healthcare applications. In this review, we summarize cutting-edge research progress of biomimetic Bouligand architectures. Firstly, the natural Bouligand structures in animals, plants, and humans are introduced. On this basis, the relationship between properties and Bouligand structure is briefly discussed, including toughening mechanism, optical characteristics, and biological properties. Subsequently, the review details the construction strategies of the biomimetic Bouligand architectures, covering a variety of methods such as self-assembly, biomimetic mineralization, shear brushing, electrostatic spinning, and 3D printing. Finally, the utilization of biomimetic Bouligand architectures in biomedical and healthcare fields, especially for bone regeneration, tooth repair, body protection, and biosensor transmission, is discussed in detail. Despite the significant theoretical advantages of Bouligand structure, its feasibility in biomedical and healthcare applications still remains in its infancy. We eagerly anticipate the future development of biomimetic Bouligand architectures with superior performance, tailored to clinical scenarios and health needs, thereby fulfilling the grand vision of “inspiration from nature and giving back to life.”","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"539-567"},"PeriodicalIF":24.5,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12260","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705329","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Ultrathin Nanocomposite Membrane With Robust Anti-Wettability for Stable Membrane Distillation 用于稳定膜蒸馏的超强抗润湿性超薄纳米复合膜

IF 24.5

Interdisciplinary Materials Pub Date : 2025-07-01 DOI: 10.1002/idm2.12253

Zhongao Chen, Yongxuan Wang, Xiao Chen, Cheng Huang, Shiqing Xu, Quanwei Xu, Shuaifei Zhao, Wojciech Kujawski, Pengchao Zhang

{"title":"Ultrathin Nanocomposite Membrane With Robust Anti-Wettability for Stable Membrane Distillation","authors":"Zhongao Chen, Yongxuan Wang, Xiao Chen, Cheng Huang, Shiqing Xu, Quanwei Xu, Shuaifei Zhao, Wojciech Kujawski, Pengchao Zhang","doi":"10.1002/idm2.12253","DOIUrl":"https://doi.org/10.1002/idm2.12253","url":null,"abstract":"Hydrophobic porous membrane is the key to the desalination performance of membrane distillation (MD). However, traditional MD membranes suffer from poor hydrophobicity of pore surfaces, leading to pore wetting and causing the loss of desalination stability. In this study, we present an ultrathin polyvinylidene fluoride (PVDF) nanocomposite membrane with robust anti-wetting properties and high permeability for stable MD desalination. The improved anti-wetting properties are achieved by enhancing the hydrophobicity of membrane pore surfaces via introducing hydrophobic silica nanoparticles to build nanostructures on the pore surfaces. The hydrophobic nanostructured pore surfaces induce the formation of the nano-Cassie state upon contact with water, thereby enhancing the specific liquid entry pressure of water (LEPw) with 788% compared to commercial PVDF membranes. The resulted porous structure and 10 μm membrane thickness (i.e., 20 times thinner than commercial PVDF membranes) enable the stable desalination flux of 20.30 kg m−2 h−1 and high salt rejection of > 99.9% with 60°C seawater. Our ultrathin nanocomposite membranes provide a promising solution for long-term MD seawater desalination.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"610-619"},"PeriodicalIF":24.5,"publicationDate":"2025-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12253","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705327","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Synergistic Chemical and Physical Encapsulation Strategies Enable Highly Stable and Lead Leakage-Suppressed Perovskite Solar Cells 协同化学和物理封装策略使高稳定和铅泄漏抑制钙钛矿太阳能电池

IF 24.5

Interdisciplinary Materials Pub Date : 2025-06-02 DOI: 10.1002/idm2.12255

Yumeng Xu, Qingrui Wang, Zhenhua Lin, Siyu Zhang, Xing Guo, Zhaosheng Hu, Juanxiu Xiao, Yue Hao, Liming Ding, Jingjing Chang

{"title":"Synergistic Chemical and Physical Encapsulation Strategies Enable Highly Stable and Lead Leakage-Suppressed Perovskite Solar Cells","authors":"Yumeng Xu, Qingrui Wang, Zhenhua Lin, Siyu Zhang, Xing Guo, Zhaosheng Hu, Juanxiu Xiao, Yue Hao, Liming Ding, Jingjing Chang","doi":"10.1002/idm2.12255","DOIUrl":"https://doi.org/10.1002/idm2.12255","url":null,"abstract":"Although outstanding power conversion efficiency has been achieved in perovskite solar cells (PSCs), poor stability and lead (Pb) toxicity are still the key challenges limiting the commercial application of PSCs. Herein, we adopted both chemical encapsulation and physical encapsulation to address these problems. Via strong chemical interaction between dibutyl phthalate (DBP) and perovskite, the chemical encapsulation strategy results in higher perovskite film quality with reduced trap density, and the device efficiency enhances from 22.07% to 24.36%. Physical encapsulation polymer with high film robustness and self-healing properties could effectively isolate external risks and restore protection after physical damage. Furthermore, both chemical and physical encapsulation materials could trap Pb ions leaking from the perovskite materials by forming coordination interactions. We simulated realistic scenarios in which PSCs encapsulated by different methods suffered water immersion and mechanical damage, and quantitatively measured Pb leakage rates under different conditions. Higher device stability and greater Pb leakage reduction were achieved, confirming the excellent encapsulation effect of the synergy of chemical and physical encapsulation. This study provides an effective strategy to realize safe and environmentally friendly PSCs to promote their commercialization.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"599-609"},"PeriodicalIF":24.5,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12255","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705331","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Inside Front Cover: Volume 4 Issue 3 内封面：第4卷第3期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-05-26 DOI: 10.1002/idm2.12257

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