Interdisciplinary Materials最新文献_第10页

Outside Front Cover: Volume 3 Issue 3 封面外页：第 3 卷第 3 期

Interdisciplinary Materials Pub Date : 2024-05-26 DOI: 10.1002/idm2.12179

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Inside Front Cover: Volume 3 Issue 3 封面内页：第 3 卷第 3 期

Interdisciplinary Materials Pub Date : 2024-05-26 DOI: 10.1002/idm2.12195

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Inside Back Cover: Volume 3 Issue 3 封底内页第 3 卷第 3 期

Interdisciplinary Materials Pub Date : 2024-05-26 DOI: 10.1002/idm2.12196

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Polar materials for photocatalytic applications: A critical review 用于光催化应用的极性材料：重要综述

IF 24.5

Interdisciplinary Materials Pub Date : 2024-05-26 DOI: 10.1002/idm2.12176

Xiaoqing Liu, Yu Zhang, Cong Wang, Lei Shen

{"title":"Polar materials for photocatalytic applications: A critical review","authors":"Xiaoqing Liu, Yu Zhang, Cong Wang, Lei Shen","doi":"10.1002/idm2.12176","DOIUrl":"https://doi.org/10.1002/idm2.12176","url":null,"abstract":"The critical challenges of the energy crisis and environmental degradation promote innovative approaches for energy conversion. Semiconductor-based photocatalytic technology, which transforms solar energy into chemical energy, emerges as a promising solution. However, the practical application of this technology faces several challenges, such as the rapid recombination of photogenerated electrons and holes, significantly limiting photocatalytic efficiency. In this review, we provide a detailed discussion, an insightful perspective, and a critical evaluation of recent advances, challenges, and opportunities in the field of photocatalysis using polar materials. We present a comprehensive examination of the photocatalytic mechanisms, activity, and diverse applications of photocatalysts based on polar materials. We also briefly discuss the engineering design of polar photocatalysis in experiments and its scalability in the industry. This review outlines future trends and potential breakthroughs in the photocatalytic field using polar materials, projecting their transformative impact on environmental chemistry and energy engineering.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 4","pages":"530-564"},"PeriodicalIF":24.5,"publicationDate":"2024-05-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12176","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141730241","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Recent progress and perspective on electrocatalysis in neutral media: Mechanisms, materials, and advanced characterizations 中性介质电催化的最新进展和前景：机理、材料和高级表征

IF 24.5

Interdisciplinary Materials Pub Date : 2024-05-23 DOI: 10.1002/idm2.12172

Fayuan Lai, Haochuan Shang, Yuchao Jiao, Xinyi Chen, Tianran Zhang, Xiangfeng Liu

{"title":"Recent progress and perspective on electrocatalysis in neutral media: Mechanisms, materials, and advanced characterizations","authors":"Fayuan Lai, Haochuan Shang, Yuchao Jiao, Xinyi Chen, Tianran Zhang, Xiangfeng Liu","doi":"10.1002/idm2.12172","DOIUrl":"10.1002/idm2.12172","url":null,"abstract":"Electrocatalysis, which involves oxidation and reduction reactions with direct electron transfer, is essential for a variety of clean energy conversion devices. Currently, the vast majority of studies regarding electrocatalysis reactions focus on strong acidic or alkaline media because of the higher catalytic activity. Nevertheless, some inherent drawbacks, including the corrosive environment, expensive proton exchange membranes, and side effects, are still hard to break through. A sustainably promising way to overcome these shortcomings is to deploy neutral/near-neutral electrolytes for electrocatalysis reactions. Unfortunately, insufficient research in this area due to the lack of attention to related issues has slowed down the development process. In this review, we systematically review the catalytic reaction mechanisms, neutral electrolytes, electrocatalysts, and modification strategies carried out in neutral media on the three most common electrocatalytic reactions, that is, hydrogen evolution reaction, oxygen reduction reaction, and oxygen evolution reaction. Furthermore, the advanced characterization tools for guiding catalyst synthesis and mechanistic studies are also summarized. Eventually, we propose some challenges and perspectives on electrocatalysis reactions in neutral media and hope it will attract more research interest and provide guidance in neutral electrocatalysis.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 4","pages":"492-529"},"PeriodicalIF":24.5,"publicationDate":"2024-05-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12172","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141105753","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Convenient folding-hot-pressing fabrication and enhanced piezoelectric properties of high β-phase-content poly(vinylidene fluoride) films 方便折叠-热压制备高 β 相含量聚偏氟乙烯薄膜并增强其压电特性

IF 24.5

Interdisciplinary Materials Pub Date : 2024-05-22 DOI: 10.1002/idm2.12175

Jie Shen, Yicheng Zeng, Qiangzhi Li, Jing Zhou, Wen Chen

{"title":"Convenient folding-hot-pressing fabrication and enhanced piezoelectric properties of high β-phase-content poly(vinylidene fluoride) films","authors":"Jie Shen, Yicheng Zeng, Qiangzhi Li, Jing Zhou, Wen Chen","doi":"10.1002/idm2.12175","DOIUrl":"10.1002/idm2.12175","url":null,"abstract":"Poly(vinylidene fluoride) (PVDF) is the most attractive piezoelectric polymer for application in flexible sensors. To attain excellent piezoelectric properties, a substantial amount of spontaneous polar β-phase content is highly desired. Nevertheless, the current reported manufacturing methods to increase β-phase contents are inconvenient and complex, hindering progress in PVDF's application. This work proposes a folding-hot-pressing method to fabricate high β-phase-content PVDF films. Structural characterization indicates that the films have α and β phases and the folding-hot-pressing process transforms the α phase into the β phase. Due to the 97.5% β-phase content and aligned structure, a piezoelectric constant of 20 pC/N is achieved in the three-times folded film. Furthermore, the process method enhances the tensile strength (126.2 MPa) of the films, with a low Young's modulus (0.87 GPa) remaining, making the films applicable for flexible piezoelectric sensors. Additionally, sensors based on the achieved films were assembled and applied for human physiological activity monitoring. This work offers a scalable new melt-processing strategy for developing high-performance PVDF-based piezoelectric composite films for wearable electronic devices.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 5","pages":"715-725"},"PeriodicalIF":24.5,"publicationDate":"2024-05-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12175","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141110358","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Tape-casting electrode architecture permits low-temperature manufacturing of all-solid-state thin-film microbatteries 胶带浇铸电极结构允许低温制造全固态薄膜微型电池

IF 24.5

Interdisciplinary Materials Pub Date : 2024-05-13 DOI: 10.1002/idm2.12174

Bingyuan Ke, Congcong Zhang, Shoulin Cheng, Wangyang Li, Renming Deng, Hong Zhang, Jie Lin, Qingshui Xie, Baihua Qu, Dong-Liang Peng, Xinghui Wang

{"title":"Tape-casting electrode architecture permits low-temperature manufacturing of all-solid-state thin-film microbatteries","authors":"Bingyuan Ke, Congcong Zhang, Shoulin Cheng, Wangyang Li, Renming Deng, Hong Zhang, Jie Lin, Qingshui Xie, Baihua Qu, Dong-Liang Peng, Xinghui Wang","doi":"10.1002/idm2.12174","DOIUrl":"10.1002/idm2.12174","url":null,"abstract":"Along with the constantly evolving functional microsystems toward more diversification, the more rigorous design deliberation of pursuing higher mass-loading of electrode materials and low-temperature fabrication compatibility have imposed unprecedented demand on integrable all-solid-state thin-film microbatteries. While the classic thin-film intercalation cathode prepared by vacuum-based techniques inevitably encountered a post-annealing process, tape-casting technologies hold great merits both in terms of high-mass loading and low-temperature processing. In this work, a novel microbattery configuration is developed by the combination of traditional tape-casting thick electrodes and sputtered inorganic thin-film solid electrolytes (~3 μm lithium phosphorus oxynitride). Enabled by physically pressed or vapor-deposited Li as an anode, solid-state batteries with tape-casted LiFePO4 electrodes exhibit outstanding cyclability and stability. To meet integration requirements, LiFePO4/LiPON/Si microbatteries were successfully fabricated at low temperatures and found to achieve a wide operating temperature range. This novel configuration has good prospects in promoting the thin-film microbattery enabling a paradigm shift and satisfying diversified requirements.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 4","pages":"621-631"},"PeriodicalIF":24.5,"publicationDate":"2024-05-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12174","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140982899","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Chiral twisted molecular carbons: Synthesis, properties, and applications 手性扭曲分子碳：合成、性质和应用

IF 24.5

Interdisciplinary Materials Pub Date : 2024-05-11 DOI: 10.1002/idm2.12173

Yunqin Zhang, Junjie Guan, Leiquan Luo, Xiao Han, Jie Wang, Yongshen Zheng, Jialiang Xu

{"title":"Chiral twisted molecular carbons: Synthesis, properties, and applications","authors":"Yunqin Zhang, Junjie Guan, Leiquan Luo, Xiao Han, Jie Wang, Yongshen Zheng, Jialiang Xu","doi":"10.1002/idm2.12173","DOIUrl":"10.1002/idm2.12173","url":null,"abstract":"In recent years, the precisely controlled synthesis of chiral twisted molecular carbons has emerged as a forefront topic in the research of carbon materials. Molecular carbons refer to carbon nanomaterials synthesized with precision at the atomic level. Through rational design, rigid and stable chiral twisted structures can be synthesized. The exploration in the field of chiral twisted molecular carbons is key to fully understanding the various twisted configurations of carbon materials and delving into the relationship between structure design and functionality. This review explores chiral twisted configurations of carbon nanomaterials such as nanographene, carbon nanobelts, carbon nanosheets, graphdiyne, etc. It emphasizes the role of photocyclization, Scholl reaction, and Diels–Alder reactions in achieving precise chiral control and discusses a range of innovative design strategies. These strategies have led to the development of various twisted structures, such as helical, propeller, and Möbius strip configurations. The introduction of chirality, combined with the inherent exceptional optical properties of nanocarbon materials, has facilitated the creation of materials with superior chiroptical performances. This advancement is driving applications in fields such as optoelectronics and chiral optics.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 4","pages":"453-479"},"PeriodicalIF":24.5,"publicationDate":"2024-05-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12173","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140988125","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Single-element amorphous metals 单元素非晶金属

IF 24.5

Interdisciplinary Materials Pub Date : 2024-05-10 DOI: 10.1002/idm2.12171

Xiao Han, Geng Wu, Dong Sheng He, Xun Hong

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Three-dimensional-printed Ni-based scaffold design accelerates bubble escape for ampere-level alkaline hydrogen evolution reaction 基于镍的三维打印支架设计可加速安培级碱性氢进化反应中的气泡逸出

IF 24.5

Interdisciplinary Materials Pub Date : 2024-04-29 DOI: 10.1002/idm2.12169

Jingxuan Chen, Gangwen Fu, Yu Tian, Xingchuan Li, Mengqi Luo, Xiaoyu Wei, Ting Zhang, Tian Gao, Cheng Chen, Somboon Chaemchuen, Xi Xu, Xing Sun, Tongle Bu, Francis Verpoort, John Wang, Zongkui Kou

{"title":"Three-dimensional-printed Ni-based scaffold design accelerates bubble escape for ampere-level alkaline hydrogen evolution reaction","authors":"Jingxuan Chen, Gangwen Fu, Yu Tian, Xingchuan Li, Mengqi Luo, Xiaoyu Wei, Ting Zhang, Tian Gao, Cheng Chen, Somboon Chaemchuen, Xi Xu, Xing Sun, Tongle Bu, Francis Verpoort, John Wang, Zongkui Kou","doi":"10.1002/idm2.12169","DOIUrl":"https://doi.org/10.1002/idm2.12169","url":null,"abstract":"Alkaline hydrogen evolution reaction (HER) for scalable hydrogen production largely hinges on addressing the sluggish bubble-involved kinetics on the traditional Ni-based electrode, especially for ampere-level current densities and beyond. Herein, 3D-printed Ni-based sulfide (3DPNS) electrodes with varying scaffolds are designed and fabricated. In situ observations at microscopic levels demonstrate that the bubble escape velocity increases with the number of hole sides (HS) in the scaffolds. Subsequently, we conduct multiphysics field simulations to illustrate that as the hole shapes transition from square, pentagon, and hexagon to circle, where a noticeable reduction in the bubble-attached HS length and the pressure balance time around the bubbles results in a decrease in bubble size and an acceleration in the rate of bubble escape. Ultimately, the 3DPNS electrode with circular hole configurations exhibits the most favorable HER performance with an overpotential of 297 mV at the current density of up to 1000 mA cm−2 for 120 h. The present study highlights a scalable and effective electrode scaffold design that promotes low-cost and low-energy green hydrogen production through the ampere-level alkaline HER.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 4","pages":"595-606"},"PeriodicalIF":24.5,"publicationDate":"2024-04-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12169","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141730354","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0