Interdisciplinary Materials最新文献

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Progress and perspectives of in situ polymerization method for lithium-based batteries 锂基电池原位聚合方法的进展与展望
Interdisciplinary Materials Pub Date : 2023-07-24 DOI: 10.1002/idm2.12109
Guanyou Xiao, Hao Xu, Chen Bai, Ming Liu, Yan-Bing He
{"title":"Progress and perspectives of in situ polymerization method for lithium-based batteries","authors":"Guanyou Xiao,&nbsp;Hao Xu,&nbsp;Chen Bai,&nbsp;Ming Liu,&nbsp;Yan-Bing He","doi":"10.1002/idm2.12109","DOIUrl":"https://doi.org/10.1002/idm2.12109","url":null,"abstract":"<p>The application of lithium-based batteries is challenged by the safety issues of leakage and flammability of liquid electrolytes. Polymer electrolytes (PEs) can address issues to promote the practical use of lithium metal batteries. However, the traditional preparation of PEs such as the solution-casting method requires a complicated preparation process, especially resulting in side solvents evaporation issues. The large thickness of traditional PEs reduces the energy density of the battery and increases the transport bottlenecks of lithium-ion. Meanwhile, it is difficult to fill the voids of electrodes to achieve good contact between electrolyte and electrode. In situ polymerization appears as a facile method to prepare PEs possessing excellent interfacial compatibility with electrodes. Thus, thin and uniform electrolytes can be obtained. The interfacial impedance can be reduced, and the lithium-ion transport throughput at the interface can be increased. The typical in situ polymerization process is to implant a precursor solution containing monomers into the cell and then in situ solidify the precursor under specific initiating conditions, and has been widely applied for the preparation of PEs and battery assembly. In this review, we focus on the preparation and application of in situ polymerization method in gel polymer electrolytes, solid polymer electrolytes, and composite polymer electrolytes, in which different kinds of monomers and reactions for in situ polymerization are discussed. In addition, the various compositions and structures of inorganic fillers, and their effects on the electrochemical properties are summarized. Finally, challenges and perspectives for the practical application of in situ polymerization methods in solid-state lithium-based batteries are reviewed.</p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 4","pages":"609-634"},"PeriodicalIF":0.0,"publicationDate":"2023-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12109","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50142808","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
Direct ink writing of metal-based electrocatalysts for Li–S batteries with efficient polysulfide conversion 具有高效多硫化物转化的锂硫电池用金属基电催化剂的直接墨水书写
Interdisciplinary Materials Pub Date : 2023-07-17 DOI: 10.1002/idm2.12110
Ting Meng, Zeyu Geng, Fei Ma, Xiaohan Wang, Haifeng Zhang, Cao Guan
{"title":"Direct ink writing of metal-based electrocatalysts for Li–S batteries with efficient polysulfide conversion","authors":"Ting Meng,&nbsp;Zeyu Geng,&nbsp;Fei Ma,&nbsp;Xiaohan Wang,&nbsp;Haifeng Zhang,&nbsp;Cao Guan","doi":"10.1002/idm2.12110","DOIUrl":"https://doi.org/10.1002/idm2.12110","url":null,"abstract":"<p>Thanks to the significantly higher energy density compared with universal commercialized Li-ion batteries, lithium–sulfur (Li–S) batteries are being investigated for use in prospective energy storage devices. However, the inadequate electrochemical kinetics of reactants and intermediates hinder commercial utilization. This limitation results in substantial capacity degradation and short battery lifespans, thereby impeding the battery's power export. Meanwhile, the capacity attenuation induced by the undesirable shuttle effect further hinders their industrialization. Considerable effort has been invested in developing electrocatalysts to fix lithium polysulfides and boost their conversion effectively. In the conventional process, the planar electrodes are prepared by slurry-casting, which limits the electron and ion transfer paths, especially when the thickness of the electrodes is relatively large. Compared with traditional manufacturing methods, direct ink writing (DIW) technology offers unique advantages in both geometry shaping and rapid prototyping, and even complex three-dimensional structures with high sulfur loading. Hence, this review presents a detailed description of the current developments in terms of Li–S batteries in DIW of metal-based electrocatalysts. A thorough exploration of the behavior chemistry of electrocatalysis is provided, and the adhibition of metal-based catalysts used for Li–S batteries is summarized from the aspect of material usage and performance enhancement. Then, the working principle of DIW technology and the requirements of used inks are presented, with a detailed focus on the latest advancements in DIW of metal-based catalysts in Li–S battery systems. Their challenges and prospects are discussed to guide their future development.</p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 4","pages":"589-608"},"PeriodicalIF":0.0,"publicationDate":"2023-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12110","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50151684","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Building better solid-state batteries with silicon-based anodes 用硅基阳极制造更好的固态电池
Interdisciplinary Materials Pub Date : 2023-07-17 DOI: 10.1002/idm2.12111
Zhefei Sun, Quanzhi Yin, Haoyu Chen, Miao Li, Shenghui Zhou, Sifan Wen, Jianhai Pan, Qizheng Zheng, Bing Jiang, Haodong Liu, Kangwoon Kim, Jie Li, Xiang Han, Yan-Bing He, Li Zhang, Meicheng Li, Qiaobao Zhang
{"title":"Building better solid-state batteries with silicon-based anodes","authors":"Zhefei Sun,&nbsp;Quanzhi Yin,&nbsp;Haoyu Chen,&nbsp;Miao Li,&nbsp;Shenghui Zhou,&nbsp;Sifan Wen,&nbsp;Jianhai Pan,&nbsp;Qizheng Zheng,&nbsp;Bing Jiang,&nbsp;Haodong Liu,&nbsp;Kangwoon Kim,&nbsp;Jie Li,&nbsp;Xiang Han,&nbsp;Yan-Bing He,&nbsp;Li Zhang,&nbsp;Meicheng Li,&nbsp;Qiaobao Zhang","doi":"10.1002/idm2.12111","DOIUrl":"https://doi.org/10.1002/idm2.12111","url":null,"abstract":"<p>Silicon (Si)-based solid-state batteries (Si-SSBs) are attracting tremendous attention because of their high energy density and unprecedented safety, making them become promising candidates for next-generation energy storage systems. Nevertheless, the commercialization of Si-SSBs is significantly impeded by enormous challenges including large volume variation, severe interfacial problems, elusive fundamental mechanisms, and unsatisfied electrochemical performance. Besides, some unknown electrochemical processes in Si-based anode, solid-state electrolytes (SSEs), and Si-based anode/SSE interfaces are still needed to be explored, while an in-depth understanding of solid–solid interfacial chemistry is insufficient in Si-SSBs. This review aims to summarize the current scientific and technological advances and insights into tackling challenges to promote the deployment of Si-SSBs. First, the differences between various conventional liquid electrolyte-dominated Si-based lithium-ion batteries (LIBs) with Si-SSBs are discussed. Subsequently, the interfacial mechanical contact model, chemical reaction properties, and charge transfer kinetics (mechanical–chemical kinetics) between Si-based anode and three different SSEs (inorganic (oxides) SSEs, organic–inorganic composite SSEs, and inorganic (sulfides) SSEs) are systemically reviewed, respectively. Moreover, the progress for promising inorganic (sulfides) SSE-based Si-SSBs on the aspects of electrode constitution, three-dimensional structured electrodes, and external stack pressure is highlighted, respectively. Finally, future research directions and prospects in the development of Si-SSBs are proposed.</p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 4","pages":"635-663"},"PeriodicalIF":0.0,"publicationDate":"2023-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12111","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50151683","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
Architectural design and electrochemical performance of MOF-based solid-state electrolytes for high-performance secondary batteries 用于高性能二次电池的MOF基固态电解质的结构设计和电化学性能
Interdisciplinary Materials Pub Date : 2023-07-05 DOI: 10.1002/idm2.12108
Biao Yang, Yuxin Shi, Dae Joon Kang, Zhidong Chen, Huan Pang
{"title":"Architectural design and electrochemical performance of MOF-based solid-state electrolytes for high-performance secondary batteries","authors":"Biao Yang,&nbsp;Yuxin Shi,&nbsp;Dae Joon Kang,&nbsp;Zhidong Chen,&nbsp;Huan Pang","doi":"10.1002/idm2.12108","DOIUrl":"https://doi.org/10.1002/idm2.12108","url":null,"abstract":"<p>Nowadays solid-state batteries have become a hot spot in the research of batteries and a significant candidate for commercial batteries for the increasing demands for good safety and excellent energy density. Metal-organic frameworks (MOFs) have been considered as suitable materials for solid-state electrolytes (SSEs) for the merits of regular channels and large specific surface areas, which can provide a promising structural platform for fast-ion conduction. Therefore, numerous kinds of MOF-based SSEs with enhanced electrochemical performance have been successfully synthesized and studied in recent years. In this review, the recent progress (synthesis methods, physical and chemical characteristics) of MOF-based SSEs for secondary batteries have been summarized. Finally, the challenges and opportunities faced by the future development in this field are put forward, hoping to provide some enlightenment for the synthesis of MOF-based SSEs, so as to create more efficient, long-lasting, and safe SSE-based secondary batteries.</p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 4","pages":"475-510"},"PeriodicalIF":0.0,"publicationDate":"2023-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12108","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50130859","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advances in probing single biomolecules: From DNA bases to glycans 探测单个生物分子的研究进展:从DNA碱基到聚糖
Interdisciplinary Materials Pub Date : 2023-06-25 DOI: 10.1002/idm2.12106
Baofei Hou, Teng Zhang, Huixia Yang, Xu Han, Liwei Liu, Linfei Li, Cesare Grazioli, Xu Wu, Nan Jiang, Yeliang Wang
{"title":"Advances in probing single biomolecules: From DNA bases to glycans","authors":"Baofei Hou,&nbsp;Teng Zhang,&nbsp;Huixia Yang,&nbsp;Xu Han,&nbsp;Liwei Liu,&nbsp;Linfei Li,&nbsp;Cesare Grazioli,&nbsp;Xu Wu,&nbsp;Nan Jiang,&nbsp;Yeliang Wang","doi":"10.1002/idm2.12106","DOIUrl":"https://doi.org/10.1002/idm2.12106","url":null,"abstract":"<p>Imaging biomolecules in real space is crucial for gaining a comprehensive understanding of the properties and functions of biological systems at the most fundamental level. Among the various imaging techniques available for biomolecules and their assembled nanostructures, scanning probe microscopy (SPM) provides a powerful and nondestructive imaging option. SPM is unique in visualizing intrinsically disordered biomolecules at the nanometer scale (e.g., glycans). This review highlights recent achievements in studying biomolecules using SPM technique, focusing on DNA bases, amino acids, proteins, and glycans. The atomic-level analysis of biomolecules made possible by SPM allows for a more accurate definition of the local structure–property relationship. High-resolution SPM imaging of single biomolecules offers a new way to study basic processes of life at the molecular level.</p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 4","pages":"511-528"},"PeriodicalIF":0.0,"publicationDate":"2023-06-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12106","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50143703","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Electrolyte engineering and material modification for graphite-based lithium-ion batteries operated at low temperature 石墨基低温锂离子电池的电解质工程与材料改性
Interdisciplinary Materials Pub Date : 2023-06-21 DOI: 10.1002/idm2.12105
Yue Yin, Xiaoli Dong
{"title":"Electrolyte engineering and material modification for graphite-based lithium-ion batteries operated at low temperature","authors":"Yue Yin,&nbsp;Xiaoli Dong","doi":"10.1002/idm2.12105","DOIUrl":"https://doi.org/10.1002/idm2.12105","url":null,"abstract":"<p>Graphite offers several advantages as an anode material, including its low cost, high theoretical capacity, extended lifespan, and low Li<sup>+</sup>-intercalation potential. However, the performance of graphite-based lithium-ion batteries (LIBs) is limited at low temperatures due to several critical challenges, such as the decreased ionic conductivity of liquid electrolyte, sluggish Li<sup>+</sup> desolvation process, poor Li<sup>+</sup> diffusivity across the interphase layer and bulk graphite materials. Various approaches have therefore been explored to address these challenges. On the basis of graphite anode and corresponding LIBs, this review herein offers a comprehensive analysis of the latest advances in electrolyte engineering and electrode modification. First, electrolyte engineering is discussed in detail, highlighting the design of new electrolyte formula with broad liquid temperature range, optimized solvation structure, and well-performed inorganic-rich solid electrolyte interface. The advances in material modification have been then depicted with the view of improving the solid bulk diffusion rate to show general strategies with excellent performance at low temperatures. Finally, the corresponding challenges and opportunities have also been outlined to shed light on viable strategies for developing efficient and reliable graphite anode and graphite-based LIBs under low-temperature scenarios.</p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 4","pages":"569-588"},"PeriodicalIF":0.0,"publicationDate":"2023-06-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12105","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50153080","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Inside Front Cover: Volume 2 Issue 3 封面内页:第2卷第3期
Interdisciplinary Materials Pub Date : 2023-05-30 DOI: 10.1002/idm2.12085
{"title":"Inside Front Cover: Volume 2 Issue 3","authors":"","doi":"10.1002/idm2.12085","DOIUrl":"https://doi.org/10.1002/idm2.12085","url":null,"abstract":"<p><b>Inside Front Cover</b>: The sodium-ion storage is characterized by redox reactions occurring with the V<sup>5+</sup>/V<sup>4+</sup> to V<sup>3+</sup> at the surface of VN particles. Such pseudocapacitive sodium-ion storage is able to overcome the limitations associated with sluggish diffusion-control process, which combines the high energy densities from faradaic reactions and the high-power density that results from capacitor-like kinetics.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure>\u0000 </p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 3","pages":"ii"},"PeriodicalIF":0.0,"publicationDate":"2023-05-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12085","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50148324","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Front Cover: Volume 2 Issue 3 封面外:第2卷第3期
Interdisciplinary Materials Pub Date : 2023-05-30 DOI: 10.1002/idm2.12084
{"title":"Outside Front Cover: Volume 2 Issue 3","authors":"","doi":"10.1002/idm2.12084","DOIUrl":"https://doi.org/10.1002/idm2.12084","url":null,"abstract":"<p><b>Outside Front Cover</b>: Advanced high-performance MOF-based photothermal composite PCMs are prepared by simultaneously integrating photon absorber guest and thermal storage guest into MOF host. The quilt made of photothermal composite PCMs can efficiently absorb solar energy in the daytime and store it in the form of heat energy, making people warm and comfortable when sleeping at night even in the cold winter.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 3","pages":"i"},"PeriodicalIF":0.0,"publicationDate":"2023-05-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12084","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50148331","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Back Cover: Volume 2 Issue 3 外封底:第2卷第3期
Interdisciplinary Materials Pub Date : 2023-05-30 DOI: 10.1002/idm2.12107
{"title":"Outside Back Cover: Volume 2 Issue 3","authors":"","doi":"10.1002/idm2.12107","DOIUrl":"https://doi.org/10.1002/idm2.12107","url":null,"abstract":"<p><b>Outside Back Cover</b>: Regulation voltage of LiNiPO<sub>4</sub> by DFT calculation to move towards practical application. The electrochemical performance of the designed materials was evaluated by X. He et al. in doi: 10.1002/idm2.12088 from multiple dimensions such as volume change, band gap, formation energy, elasticity and anisotropy. The Cr or Fe doped LiNiPO<sub>4</sub> are considered to have leading performance and can be used for applicable high-voltage lithium-ion batteries.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure>\u0000 </p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 3","pages":"iii"},"PeriodicalIF":0.0,"publicationDate":"2023-05-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12107","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50148443","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Polypyrrole-boosted photothermal energy storage in MOF-based phase change materials 聚吡咯增强MOF相变材料的光热储能
Interdisciplinary Materials Pub Date : 2023-05-22 DOI: 10.1002/idm2.12092
Panpan Liu, Mengke Huang, Xiao Chen, Yan Gao, Yang Li, Cheng Dong, Ge Wang
{"title":"Polypyrrole-boosted photothermal energy storage in MOF-based phase change materials","authors":"Panpan Liu,&nbsp;Mengke Huang,&nbsp;Xiao Chen,&nbsp;Yan Gao,&nbsp;Yang Li,&nbsp;Cheng Dong,&nbsp;Ge Wang","doi":"10.1002/idm2.12092","DOIUrl":"https://doi.org/10.1002/idm2.12092","url":null,"abstract":"<p>Infiltrating phase change materials (PCMs) into nanoporous metal–organic frameworks (MOFs) is accepted as a cutting-edge thermal energy storage concept. However, weak photon capture capability of pristine MOF-based composite PCMs is a stumbling block in solar energy utilization. Towards this goal, we prepared advanced high-performance pristine MOF-based photothermal composite PCMs by simultaneously integrating photon absorber guest (polypyrrole [PPy]) and thermal storage guest (1-octadecanol [ODA]) into an MOF host (Cr-MIL-101-NH<sub>2</sub>). The coated PPy layer on the surface of ODA@MOF not only serves as a photon harvester, but also serves as a phonon enhancer. Resultantly, ODA@MOF/PPy composite PCMs exhibit intense and broadband light absorption characteristic in the ultraviolet–visible–near-infrared region, and higher heat transfer ability than ODA@MOF. Importantly, the photothermal conversion and storage efficiency of ODA@MOF/PPy-6% is up to 88.3%. Additionally, our developed MOF-based photothermal composite PCMs also exhibit long-standing antileakage stability, energy storage stability, and photothermal conversion stability. The proposed coating strategy and in-depth understanding mechanism are expected to facilitate the development of high-efficiency MOF-based photothermal composite PCMs in solar energy utilization.</p>","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 3","pages":"423-433"},"PeriodicalIF":0.0,"publicationDate":"2023-05-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12092","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50141350","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
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