Interdisciplinary Materials最新文献_第10页

Synergistic Chemical and Physical Encapsulation Strategies Enable Highly Stable and Lead Leakage-Suppressed Perovskite Solar Cells 协同化学和物理封装策略使高稳定和铅泄漏抑制钙钛矿太阳能电池

IF 24.5

Interdisciplinary Materials Pub Date : 2025-06-02 DOI: 10.1002/idm2.12255

Yumeng Xu, Qingrui Wang, Zhenhua Lin, Siyu Zhang, Xing Guo, Zhaosheng Hu, Juanxiu Xiao, Yue Hao, Liming Ding, Jingjing Chang

{"title":"Synergistic Chemical and Physical Encapsulation Strategies Enable Highly Stable and Lead Leakage-Suppressed Perovskite Solar Cells","authors":"Yumeng Xu, Qingrui Wang, Zhenhua Lin, Siyu Zhang, Xing Guo, Zhaosheng Hu, Juanxiu Xiao, Yue Hao, Liming Ding, Jingjing Chang","doi":"10.1002/idm2.12255","DOIUrl":"https://doi.org/10.1002/idm2.12255","url":null,"abstract":"Although outstanding power conversion efficiency has been achieved in perovskite solar cells (PSCs), poor stability and lead (Pb) toxicity are still the key challenges limiting the commercial application of PSCs. Herein, we adopted both chemical encapsulation and physical encapsulation to address these problems. Via strong chemical interaction between dibutyl phthalate (DBP) and perovskite, the chemical encapsulation strategy results in higher perovskite film quality with reduced trap density, and the device efficiency enhances from 22.07% to 24.36%. Physical encapsulation polymer with high film robustness and self-healing properties could effectively isolate external risks and restore protection after physical damage. Furthermore, both chemical and physical encapsulation materials could trap Pb ions leaking from the perovskite materials by forming coordination interactions. We simulated realistic scenarios in which PSCs encapsulated by different methods suffered water immersion and mechanical damage, and quantitatively measured Pb leakage rates under different conditions. Higher device stability and greater Pb leakage reduction were achieved, confirming the excellent encapsulation effect of the synergy of chemical and physical encapsulation. This study provides an effective strategy to realize safe and environmentally friendly PSCs to promote their commercialization.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"599-609"},"PeriodicalIF":24.5,"publicationDate":"2025-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12255","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705331","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Inside Front Cover: Volume 4 Issue 3 内封面：第4卷第3期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-05-26 DOI: 10.1002/idm2.12257

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Outside Front Cover: Volume 4 Issue 3 外封面：第4卷第3期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-05-26 DOI: 10.1002/idm2.12187

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Inside Back Cover: Volume 4 Issue 3 封底内：第4卷第3期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-05-26 DOI: 10.1002/idm2.12258

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Outside Back Cover: Volume 4 Issue 3 封底外：第4卷第3期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-05-26 DOI: 10.1002/idm2.12259

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Design and Application of Electrocatalyst Based on Machine Learning 基于机器学习的电催化剂设计与应用

IF 24.5

Interdisciplinary Materials Pub Date : 2025-05-15 DOI: 10.1002/idm2.12249

Yulan Gu, Hailong Zhang, Zhen Xu, Rui Ren, Xiangyi Kong, Yafu Wang, Houen Zhu, Dongdong Xue, Yali Zhang, Yuzhu Ma, Dongyuan Zhao, Jiangwei Zhang

{"title":"Design and Application of Electrocatalyst Based on Machine Learning","authors":"Yulan Gu, Hailong Zhang, Zhen Xu, Rui Ren, Xiangyi Kong, Yafu Wang, Houen Zhu, Dongdong Xue, Yali Zhang, Yuzhu Ma, Dongyuan Zhao, Jiangwei Zhang","doi":"10.1002/idm2.12249","DOIUrl":"https://doi.org/10.1002/idm2.12249","url":null,"abstract":"Data-driven artificial intelligence provides strong technical support for addressing global energy and environmental issues. The powerful data processing and analysis capabilities of machine learning (ML) can quickly predict electrocatalytic performance, improving the efficiency of catalyst design and addressing the time-consuming and inefficient nature of traditional catalyst design. By integrating ML with theoretical calculations and experiments, catalytic reaction processes can be precisely regulated. This not only accelerates the discovery of new catalysts but also drives the development of more efficient and environmentally friendly sustainable energy technologies. In this article, we discuss new approaches to discovering novel catalysts driven by ML, focusing on catalytic activity prediction, reaction energy barrier optimization, and the design of innovative catalytic materials. We systematically analysis the application of ML in the field of electrocatalysis and explore the future prospects of ML in this domain. We provide a comprehensive and in-depth analysis of the application of ML in the field of electrocatalysis and explore its potential for future development.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 3","pages":"456-479"},"PeriodicalIF":24.5,"publicationDate":"2025-05-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12249","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144135729","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Developing Advanced Mg-Based Solid-State Materials for Gas Separation and Purification: A Review 气体分离与净化用先进镁基固态材料的研究进展

IF 24.5

Interdisciplinary Materials Pub Date : 2025-05-12 DOI: 10.1002/idm2.12250

Ning Zhang, Xi Lin, Zhigang Hu, Wenjiang Ding, Jianxin Zou

{"title":"Developing Advanced Mg-Based Solid-State Materials for Gas Separation and Purification: A Review","authors":"Ning Zhang, Xi Lin, Zhigang Hu, Wenjiang Ding, Jianxin Zou","doi":"10.1002/idm2.12250","DOIUrl":"https://doi.org/10.1002/idm2.12250","url":null,"abstract":"Magnesium (Mg) is globally abundant in resources, and Mg-based compounds—such as magnesium based hydrides, hydroxides, oxides, and magnesium metal-organic frameworks (Mg MOFs)—have shown significant application prospects in gas separation. This is largely due to the electronic characteristics of Mg or Mg2⁺ ions, which facilitate the capture of hydrogen (H2) and acidic gases such as carbon dioxide (CO2) and sulfur dioxide (SO2) from other gases. Consequently, exploring the use of Mg-based materials in gas separation and purification applications could not only advance the scientific understanding of solid-gas interaction mechanisms but also provide cost-effective solutions for gas separation technology at an industrial level. This review summarizes the recent practices and explorations of Mg-based solid-state materials in various gas separation and purification methods, including physical adsorption-based separation, chemical absorption-based separation, and membrane-based separation. For each separation method, the relevant Mg-based materials are discussed in detail, and key findings from existing research are presented and analyzed. Additionally, inspired by the straightforward design of air-stable hydrogen storage materials, this review specifically addresses anti-passivation strategies for Mg-based hydrides, which are crucial for their applications in hydrogen gas separation and purification. Finally, this review highlights key issues and fields for future research and development in Mg-based gas separation materials.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 3","pages":"480-501"},"PeriodicalIF":24.5,"publicationDate":"2025-05-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12250","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144135652","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Engineered Living Energy Materials 工程生物能源材料

IF 24.5

Interdisciplinary Materials Pub Date : 2025-04-29 DOI: 10.1002/idm2.12245

Xinyi Yuan, Haiyi Xu, Xingwu Liu, Jicong Zhang, Jing Li, Qianyi Liang, Bolin An, Giuseppe Maria Paternò, Minyue Zhang, Yuqing Tang, Chen Zhang, Dake Xu, Chao Zhong, Ke Li, Xinyu Wang

{"title":"Engineered Living Energy Materials","authors":"Xinyi Yuan, Haiyi Xu, Xingwu Liu, Jicong Zhang, Jing Li, Qianyi Liang, Bolin An, Giuseppe Maria Paternò, Minyue Zhang, Yuqing Tang, Chen Zhang, Dake Xu, Chao Zhong, Ke Li, Xinyu Wang","doi":"10.1002/idm2.12245","DOIUrl":"https://doi.org/10.1002/idm2.12245","url":null,"abstract":"To foster sustainable development, a pivotal trend lies in harnessing sustainable energy supplies that propel modern economic and societal progress. Recent advancements in living materials for energy applications have sparked a groundbreaking research area: engineered living energy materials (ELEMs), which seamlessly integrate biological and artificial systems for efficient energy conversion and storage. To consolidate and propel this research area, herein, we summarize and delve into the evolution of ELEMs. Firstly, we provide an overview of the structural features and energy conversion mechanisms employed by bio-modules spanning proteins, organelles, and entire organisms. They can be directly used as components for constructing ELEMs or provide inspirations for the design of such entities. Then, we comprehensively review the latest research strides in ELEMs based on their distinct energy conversion modes. Finally, we discuss the challenges confronting ELEMs and envision their future trajectories. The progress of ELEMs holds immense potential to catalyze interdisciplinary research endeavors encompassing medicine, environmental science, and energy technologies.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 3","pages":"412-455"},"PeriodicalIF":24.5,"publicationDate":"2025-04-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12245","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144135774","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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Nature Inspires New High-Performance Metal Composites 大自然激发出新的高性能金属复合材料

IF 24.5

Interdisciplinary Materials Pub Date : 2025-04-29 DOI: 10.1002/idm2.12251

Yanyan Liu, Zengqian Liu, Zhenyu Liu, Wenhao Zhou, Sen Yu, Bolv Xiao, Zongyi Ma, Zhefeng Zhang, Robert O. Ritchie

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All Inorganic Halide Perovskite Superlattices With All Visible Spectral Collective Coherent Emissions 所有无机卤化物钙钛矿超晶格与所有可见光谱集体相干发射

IF 24.5

Interdisciplinary Materials Pub Date : 2025-04-17 DOI: 10.1002/idm2.12248

Xiaoqian Wang, Zisheng Tang, Wanli Liu, Jiazhen He, Yuqing Li, Dafu Zhao, Cheng Wang, Ti Wang, Kang Song, Bao-Lian Su, Dongyuan Zhao, Yong Liu

{"title":"All Inorganic Halide Perovskite Superlattices With All Visible Spectral Collective Coherent Emissions","authors":"Xiaoqian Wang, Zisheng Tang, Wanli Liu, Jiazhen He, Yuqing Li, Dafu Zhao, Cheng Wang, Ti Wang, Kang Song, Bao-Lian Su, Dongyuan Zhao, Yong Liu","doi":"10.1002/idm2.12248","DOIUrl":"https://doi.org/10.1002/idm2.12248","url":null,"abstract":"Self-assembled inorganic halide perovskite superlattices (HPSLs) have attracted extensive attention for their well-ordered structure and unique collective photonic properties, which differ from those of individual nanocrystals (NCs). However, the manipulation of ordered HPSLs with all-halogen and alloyed halogen components, as well as the regulation of their coherent spontaneous emission across the visible spectrum, remains underexplored. In this study, we employ a combination of anion-exchange reactions and a slow solvent evaporation strategy to self-assemble monodisperse, uniform all inorganic perovskite NCs into a series of well-defined, long-range ordered, and densely packed CsPbX3 (X = Cl, Br, I, and mixed halide systems such as Cl/Br, Br/I, and Cl/Br/I) superlattices, achieving coherent photoluminescence (PL) emission across the entire visible spectrum (400–700 nm). Notably, the collective coherent emission of all HPSLs exhibits dynamic redshifts and accelerated collective radiative decay due to strong electronic coupling between NCs at cryogenic temperatures (7 K). This study not only systematically investigates all-halide compositional HPSLs but also paves the way for quantum light source applications across the visible spectrum.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 4","pages":"568-575"},"PeriodicalIF":24.5,"publicationDate":"2025-04-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12248","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705581","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0