Interdisciplinary Materials最新文献_第10页

Emerging advances in fluorescence imaging and phototherapy of arthritis 关节炎荧光成像和光疗的新进展

IF 24.5

Interdisciplinary Materials Pub Date : 2023-12-16 DOI: 10.1002/idm2.12130

Xiaoxuan Wang, Jingying Dai, Cong Shao, Takashi Goto, Honglian Dai

引用次数: 0

Bicontinuous donor and acceptor fibril networks enable 19.2% efficiency pseudo-bulk heterojunction organic solar cells 双连续供体和受体纤维网络可实现 19.2% 效率的伪大体积异质结有机太阳能电池

IF 24.5

Interdisciplinary Materials Pub Date : 2023-12-03 DOI: 10.1002/idm2.12129

Jing Zhou, Donghui Li, Liang Wang, Xinying Zhang, Nan Deng, Chuanhang Guo, Chen Chen, Zirui Gan, Chenhao Liu, Wei Sun, Dan Liu, Wei Li, Zhe Li, Kai Wang, Tao Wang

{"title":"Bicontinuous donor and acceptor fibril networks enable 19.2% efficiency pseudo-bulk heterojunction organic solar cells","authors":"Jing Zhou, Donghui Li, Liang Wang, Xinying Zhang, Nan Deng, Chuanhang Guo, Chen Chen, Zirui Gan, Chenhao Liu, Wei Sun, Dan Liu, Wei Li, Zhe Li, Kai Wang, Tao Wang","doi":"10.1002/idm2.12129","DOIUrl":"10.1002/idm2.12129","url":null,"abstract":"Realizing bicontinuous fibrillar charge transport networks in the photoactive layer has been considered a promising method to achieve high-efficiency organic solar cells (OSCs); however, this has been rarely achieved due to the interference of molecular organization of donor and acceptor components during solution casting. In this contribution, the fibrillization of polymer donor PM6 and small molecular nonfullerene acceptor L8-BO is realized with the assistance of conjugated polymer D18-Cl. Atomic force microscopy and photo-induced force microscopy reveal that PM6 and D18-Cl co-assemble into long and slender fibrils within wide blending ratios due to their high compatibility; in contrast, the fibrillization of L8-BO can be encouraged with the incorporation of 1% D18-Cl. By utilizing a pseudo-bulk heterojunction (p-BHJ) active layer fabricated by layer-by-layer deposition, the optimized PM6+20% D18-Cl/L8-BO+1% D18-Cl OSCs obtain bicontinuous fibril networks, leading to enhanced exciton dissociation and charge transport processes and superior power conversion efficiency of 19.2% (certified 18.91%) compared to 18.8% of the PM6:D18-Cl:L8-BO ternary BHJ OSCs.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 6","pages":"866-875"},"PeriodicalIF":24.5,"publicationDate":"2023-12-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12129","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138604886","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Conductive passivating contact for high fill factor monolithic perovskite/silicon tandem solar cells

IF 24.5

Interdisciplinary Materials Pub Date : 2023-11-29 DOI: 10.1002/idm2.12124

Bingbing Chen, Jin Wang, Ningyu Ren, Pengfei Liu, Xingliang Li, Sanlong Wang, Wei Han, Zhao Zhu, Jingjing Liu, Qian Huang, Ying Zhao, Xiaodan Zhang

{"title":"Conductive passivating contact for high fill factor monolithic perovskite/silicon tandem solar cells","authors":"Bingbing Chen, Jin Wang, Ningyu Ren, Pengfei Liu, Xingliang Li, Sanlong Wang, Wei Han, Zhao Zhu, Jingjing Liu, Qian Huang, Ying Zhao, Xiaodan Zhang","doi":"10.1002/idm2.12124","DOIUrl":"https://doi.org/10.1002/idm2.12124","url":null,"abstract":"Perovskite/silicon tandem solar cells (PK/Si TSCs) blaze the way in pushing power conversion efficiency (PCE) beyond the single-junction Shockley–Queisser limit. Meanwhile, localized defects in perovskite subcells result in a lower fill factor (FF), which limits further improvement of PCE in PK/Si TSCs. Herein, we report a conductive passivation contact layer by posttreatment of bis(2-hydroxyethyl)dimethylammonium chloride (BDAC) zwitterion molecule on the perovskite surface. It can passivate the positive and negative localized defects, inhibit the formation of Pb0, and spontaneously convert the perovskite surface to be a more n-type conductive contact layer for charge separation. These combined enhancements enabled a PCE of 21.4% with an enhanced VOC of 80 mV and an FF of 82.84% for the inverted single-junction device prepared by the two-step method. Moreover, BDAC passivation achieved a PCE of 28.67% with an FF of 80.02% for PK/Si TSCs. In addition, the scaling-up device with an active area of 11.879 cm2 delivers a PCE of 24.46%, and a minimodule with power conversion over 2 W is designed and fabricated.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 6","pages":"855-865"},"PeriodicalIF":24.5,"publicationDate":"2023-11-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12124","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143253719","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Outside Front Cover: Volume 2 Issue 5 封面外：第2卷第5期

Interdisciplinary Materials Pub Date : 2023-10-31 DOI: 10.1002/idm2.12125

引用次数: 0

Three-dimensional multicellular biomaterial platforms for biomedical application 用于生物医学应用的三维多细胞生物材料平台

Interdisciplinary Materials Pub Date : 2023-10-31 DOI: 10.1002/idm2.12122

Jianxin Hao, Chen Qin, Chengtie Wu

{"title":"Three-dimensional multicellular biomaterial platforms for biomedical application","authors":"Jianxin Hao, Chen Qin, Chengtie Wu","doi":"10.1002/idm2.12122","DOIUrl":"https://doi.org/10.1002/idm2.12122","url":null,"abstract":"The three-dimensional (3D) multicellular platforms prepared by cells or biomaterials have been widely applied in biomedical fields for the regeneration of complex tissues, the exploration of cell crosstalk, and the establishment of tissue physiological and pathological models. Compared with the traditional 2D culture methods, the 3D multicellular platforms are easier to adjust the components and structures of extracellular matrix (ECM) because of the synthesis of ECM by cells and the use of biomaterials. Moreover, the 3D multicellular platforms also can customize the cell distribution and precisely design micro and macro structures of the systems. Based on these typical advantages of 3D multicellular platforms and their increasingly important position in the biomedical field, this review summarizes the present 3D multicellular platforms. Herein, current 3D multicellular platforms are divided into two major types: scaffold-free and scaffold-based 3D multicellular platforms. The specific characteristics and applications of different types of 3D multicellular platforms are thoroughly introduced to help readers understand how different models affect and regulate cell behaviors and inspire researchers on how to select and design suitable 3D multicellular platforms according to different application scenarios.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 5","pages":"714-734"},"PeriodicalIF":0.0,"publicationDate":"2023-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71924617","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Inside Front Cover: Volume 2 Issue 5 封面内页：第2卷第5期

Interdisciplinary Materials Pub Date : 2023-10-31 DOI: 10.1002/idm2.12126

引用次数: 0

Dual-mode smart flipping materials and devices for thermal management 用于热管理的双模智能翻转材料和设备

Interdisciplinary Materials Pub Date : 2023-10-31 DOI: 10.1002/idm2.12123

Gaoyang Kong, Jianing Xu, Wei Xie, Ya Sun, Yile Fan, Haoyu Wang, Hiroki Kondo, Han Zhou

{"title":"Dual-mode smart flipping materials and devices for thermal management","authors":"Gaoyang Kong, Jianing Xu, Wei Xie, Ya Sun, Yile Fan, Haoyu Wang, Hiroki Kondo, Han Zhou","doi":"10.1002/idm2.12123","DOIUrl":"https://doi.org/10.1002/idm2.12123","url":null,"abstract":"Thermal management is of great significance for human activities. Attaining thermal comfort not only requires thermal control of building's macroenvironment, but also additionally personal thermal regulation. Radiative cooling technologies are anticipated to effectively lower building energy utilization and provide optimal thermal comfort for individuals in hot weather. Nevertheless, these static and single-purpose characteristics lack the ability to adjust to rapidly changing weather conditions, often leading to excessive cooling. To overcome this challenge, the emergence of dual-mode smart flipping technologies has provided a pathway for dynamically adjusting the heating or cooling of objects in response to fluctuations in ambient temperature. First, the underlying principles of dual-mode smart flipping are shown. Then the evolving materials and approaches of smart flipping are given an introduction to adapt to different environments under external stimuli, such as mechanical flipping, temperature, humidity, and so forth. Afterward, we present the recent applications of dual-mode smart flipping materials and devices in personal thermal management, thermoelectric generation, energy-saving buildings, and smart windows. Finally, the challenges and outlook of dual-mode smart flipping are presented and future directions are identified.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 5","pages":"735-760"},"PeriodicalIF":0.0,"publicationDate":"2023-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71924616","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Outside Back Cover: Volume 2 Issue 5 外封底：第2卷第5期

Interdisciplinary Materials Pub Date : 2023-10-31 DOI: 10.1002/idm2.12128

引用次数: 0

Inside Back Cover: Volume 2 Issue 5 封底：第2卷第5期

Interdisciplinary Materials Pub Date : 2023-10-31 DOI: 10.1002/idm2.12127

引用次数: 0

Fluorinated boron nitride nanosheet enhanced ultrathin and conductive polymer electrolyte for high-rate solid-state lithium metal batteries 氟化氮化硼纳米片增强超薄导电聚合物电解质用于高速率固态锂金属电池

Interdisciplinary Materials Pub Date : 2023-10-31 DOI: 10.1002/idm2.12121

Linjun Wang, Haodong Shi, Yingpeng Xie, Zhong-Shuai Wu

{"title":"Fluorinated boron nitride nanosheet enhanced ultrathin and conductive polymer electrolyte for high-rate solid-state lithium metal batteries","authors":"Linjun Wang, Haodong Shi, Yingpeng Xie, Zhong-Shuai Wu","doi":"10.1002/idm2.12121","DOIUrl":"https://doi.org/10.1002/idm2.12121","url":null,"abstract":"Polyethylene oxide (PEO)-based polymer solid electrolytes (PSE) have been pursued for the next-generation extremely safe and high-energy-density lithium metal batteries due to their exceptional flexibility, manufacturability, and lightweight nature. However, the practical application of PEO-PSE has been hindered by low ionic conductivity, limited lithium-ion transfer number (tLi+), and inferior stability with lithium metal. Herein, an ultrathin composite solid-state electrolyte (CSSE) film with a thickness of 20 μm, incorporating uniformly dispersed two-dimensional fluorinated boron nitride (F-BN) nanosheet fillers (F-BN CSSE) is fabricated via a solution-casting process. The integration of F-BN effectively reduces the crystallinity of the PEO polymer matrix, creating additional channels that facilitate lithium-ion transport. Moreover, the presence of F-BN promotes an inorganic phase-dominated electrolyte interface film dominated by LiF, Li2O, and Li3N on the lithium anode surface, greatly enhancing the stability of the electrode-electrolyte interface. Consequently, the F-BN CSSE exhibits a high ionic conductivity of 0.11 mS cm−1 at 30°C, high tLi+ of 0.56, and large electrochemical window of 4.78 V, and demonstrates stable lithium plating/striping behavior with a voltage of 20 mV for 640 h, effectively mitigating the formation of lithium dendrites. When coupled with LiFePO4, the as-assembled LiFePO4|F-BN CSSE|Li solid-state battery achieves a high capacity of 142 mAh g−1 with an impressive retention rate of 82.4% after 500 cycles at 5 C. Furthermore, even at an ultrahigh rate of 50 C, a capacity of 37 mAh g−1 is achieved. This study provides a novel and reliable strategy for the design of advanced solid-state electrolytes for high-rate and long-life lithium metal batteries.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"2 5","pages":"789-799"},"PeriodicalIF":0.0,"publicationDate":"2023-10-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71924624","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0