Interdisciplinary Materials最新文献_第3页

Inside Front Cover: Volume 4 Issue 1 封面内页：第 4 卷第 1 期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-01-16 DOI: 10.1002/idm2.12235

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Outside Front Cover: Volume 4 Issue 1 封面外页：第 4 卷第 1 期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-01-16 DOI: 10.1002/idm2.12183

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Inside Back Cover: Volume 4 Issue 1 封底内页第 4 卷第 1 期

IF 24.5

Interdisciplinary Materials Pub Date : 2025-01-16 DOI: 10.1002/idm2.12236

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Exploring the Active Lithium Loss in Anode-Free Lithium Metal Batteries: Mechanisms, Challenges, and Strategies 探索无阳极锂金属电池中的活性锂损失：机制、挑战和策略

IF 24.5

Interdisciplinary Materials Pub Date : 2024-12-30 DOI: 10.1002/idm2.12232

Xuzhi Duan, Jinran Sun, Liang Shi, Shanmu Dong, Guanglei Cui

{"title":"Exploring the Active Lithium Loss in Anode-Free Lithium Metal Batteries: Mechanisms, Challenges, and Strategies","authors":"Xuzhi Duan, Jinran Sun, Liang Shi, Shanmu Dong, Guanglei Cui","doi":"10.1002/idm2.12232","DOIUrl":"https://doi.org/10.1002/idm2.12232","url":null,"abstract":"Anode-free lithium metal batteries (AFLMBs), also known as lithium metal batteries (LMBs) with zero excess lithium, have garnered significant attention due to their substantially higher energy density compared to conventional lithium metal anodes, improved safety characteristics, and lower production costs. However, the current cycling stability of AFLMBs faces formidable challenges primarily caused by significant lithium loss associated with the deposition of lithium metal. Therefore, this review focuses on the crucial aspects of lithium metal nucleation and growth on the anode side. Respectively, aiming to provide an in-depth understanding of the deposition mechanisms, comprehensively summarize the corresponding scientific influencing factors, and analyze specific strategies for addressing these issues through the integration of relevant exemplary cases. Importantly, this review endeavors to offer a profound explication of the scientific essence and intricate mechanisms that underlie the diverse modification strategies. This review possesses the inherent capacity to greatly facilitate the progress and enlightenment of research in this field, offering a valuable resource for the researchers.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 2","pages":"217-234"},"PeriodicalIF":24.5,"publicationDate":"2024-12-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12232","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707653","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Recent Progress in Tactile Sensing and Machine Learning for Texture Perception in Humanoid Robotics 仿人机器人纹理感知触觉与机器学习研究进展

IF 24.5

Interdisciplinary Materials Pub Date : 2024-12-30 DOI: 10.1002/idm2.12233

Longteng Yu, Dabiao Liu

{"title":"Recent Progress in Tactile Sensing and Machine Learning for Texture Perception in Humanoid Robotics","authors":"Longteng Yu, Dabiao Liu","doi":"10.1002/idm2.12233","DOIUrl":"https://doi.org/10.1002/idm2.12233","url":null,"abstract":"Humanoid robots have garnered substantial attention recently in both academia and industry. These robots are becoming increasingly sophisticated and intelligent, as seen in health care, education, customer service, logistics, security, space exploration, and so forth. Central to these technological advancements is tactile perception, a crucial modality through which humanoid robots exchange information with their external environment, thereby facilitating human-like behaviors such as object recognition and dexterous manipulation. Texture perception is particularly vital for these tasks, as the surface morphology of objects significantly influences recognition and manipulation abilities. This review addresses the recent progress in tactile sensing and machine learning for texture perception in humanoid robots. We first examine the design and working principles of tactile sensors employed in texture perception, differentiating between touch-based and sliding-based approaches. Subsequently, we delve into the machine learning algorithms implemented for texture perception using these tactile sensors. Finally, we discuss the challenges and future opportunities in this evolving field. This review aims to provide insights into the state-of-the-art developments and foster advancements in tactile sensing and machine learning for texture perception in humanoid robotics.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 2","pages":"235-248"},"PeriodicalIF":24.5,"publicationDate":"2024-12-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12233","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707654","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Amorphous Metal Metaphosphate for Oxygen Reduction 氧还原用非晶金属偏磷酸盐

IF 24.5

Interdisciplinary Materials Pub Date : 2024-12-01 DOI: 10.1002/idm2.12228

Min Zhou, Jinghui Guo, Ruihu Lu, Jiantao Li, Sungsik Lee, Chunhua Han, Xiaobin Liao, Ping Luo, Yan Zhao, Zhaoyang Wang

{"title":"Amorphous Metal Metaphosphate for Oxygen Reduction","authors":"Min Zhou, Jinghui Guo, Ruihu Lu, Jiantao Li, Sungsik Lee, Chunhua Han, Xiaobin Liao, Ping Luo, Yan Zhao, Zhaoyang Wang","doi":"10.1002/idm2.12228","DOIUrl":"https://doi.org/10.1002/idm2.12228","url":null,"abstract":"Efficient and cost-effective catalysts for oxygen reduction reaction (ORR) are crucial for the commercialization of metal-air batteries. In this study, we utilized theoretical calculations to guide the material synthesis strategy for preparing catalysts. Using density functional theory (DFT) calculations, we systematically explored the ORR performance of metal metaphosphates (A-M(PO3)2, B-M(PO3)2, M = Sc, Ti, V, Cr, Mn, Fe, Co, Ni, Cu, and Zn) with both amorphous and crystalline structures. Amorphous A-Mn(PO3)2 showed optimal adsorption energy and the lowest ORR overpotential of 0.32 eV. Phytic acid was employed as a phosphorus source, and the chelating structure of phytic acid molecules and metal ions was broken through the “metal ion pre-adsorption and spatial confinement strategy” of carbon materials with electron-rich centers. Following high-temperature calcination, we successfully prepared a series of amorphous metal metaphosphate composite catalysts for the first time. In 0.1 M KOH electrolyte, both amorphous Mn(PO3)2-C/C3N4/CQDs (carbon quantum dots) and Mn(PO3)2-C/C3N4/CNTs (carbon nanotubes) exhibited excellent ORR catalytic activity, with half-wave potentials of 0.85 V and 0.80 V, respectively. A linear correlation between theoretical overpotentials and experimental half-wave potentials was discovered through comparison. This work could open a new avenue to the discovery of highly efficient non-precious metal-based catalysts with amorphous structures.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 2","pages":"309-320"},"PeriodicalIF":24.5,"publicationDate":"2024-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12228","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707657","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

A Stretchable, Attachable, and Transparent Polyionic Ecological Skin for Robust Self-Powered Interactive Sensing 一种可拉伸、可附着、透明的多离子生态皮肤，用于鲁棒自供电交互传感

IF 24.5

Interdisciplinary Materials Pub Date : 2024-11-29 DOI: 10.1002/idm2.12229

Zhiqing Bai, Yunlong Xu, Yuan Fan, Qichong Zhang

{"title":"A Stretchable, Attachable, and Transparent Polyionic Ecological Skin for Robust Self-Powered Interactive Sensing","authors":"Zhiqing Bai, Yunlong Xu, Yuan Fan, Qichong Zhang","doi":"10.1002/idm2.12229","DOIUrl":"https://doi.org/10.1002/idm2.12229","url":null,"abstract":"Bioinspired energy-autonomous interactive electronics are prevalent. However, self-powered artificial skins are often challenging to be combined with excellent mechanical properties, optical transparency, autonomous attachability, and biocompatibility. Herein, a robust ecological polyionic skin (polyionic eco-skin) based on triboelectric mechanism consisting of ethyl cellulose/waterborne polyurethane/Cu nanoparticles (EWC) green electroactive sensitive material and polyethylene oxide/waterborne polyurethane/phytic acid (PWP) polyionic current collector is proposed. The polyionic eco-skin features sufficient stretchability (90%) and low Young's modulus (0.8 MPa) close to that of human soft tissue, high transparency (> 84% of transmission) in the visible light range, and broad static/dynamic adhesiveness, which endows it with strong adaptive implementation capacity in flexible curved electronics. More importantly, the self-powered polyionic eco-skin exhibits enhanced force-electric conversion performance by coordinating the effect of nanoparticle-polymer interfacial polarization and porous structure of sensitive material. Integrating multiple characteristics enables the polyionic eco-skin to effectively convert biomechanical energy into electrical energy, supporting self-powered functionality for itself and related circuits. Moreover, the eco-skin can be utilized to construct an interactive system and realize the remote noncontact manipulation of targets. The polyionic eco-skin holds tremendous application potential in self-powered security systems, human–machine interaction interfaces, and bionic robots, which is expected to inject new vitality into a human–cyber–physical intelligence integration.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 2","pages":"321-332"},"PeriodicalIF":24.5,"publicationDate":"2024-11-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12229","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707649","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Optimizing Hydrazine Activation on Dual-Site Co-Zn Catalysts for Direct Hydrazine-Hydrogen Peroxide Fuel Cells 二元Co-Zn催化剂在肼-过氧化氢直接燃料电池上的活化优化

IF 24.5

Interdisciplinary Materials Pub Date : 2024-11-18 DOI: 10.1002/idm2.12227

Qian Liu, Junwei Han, Yue Yang, Zerui Chen, Hao Bin Wu

{"title":"Optimizing Hydrazine Activation on Dual-Site Co-Zn Catalysts for Direct Hydrazine-Hydrogen Peroxide Fuel Cells","authors":"Qian Liu, Junwei Han, Yue Yang, Zerui Chen, Hao Bin Wu","doi":"10.1002/idm2.12227","DOIUrl":"https://doi.org/10.1002/idm2.12227","url":null,"abstract":"Direct hydrazine-hydrogen peroxide fuel cells (DHzHPFCs) offer unique advantages for air-independent applications, but their commercialization is impeded by the lack of high-performance and low-cost catalysts. This study reports a novel dual-site Co-Zn catalyst designed to enhance the hydrazine oxidation reaction (HzOR) activity. Density functional theory calculations suggested that incorporating Zn into Co catalysts can weaken the binding strength of the crucial N2H3* intermediate, which limits the rate-determining N2H3* desorption step. The synthesized p-Co9Zn1 catalyst exhibited a remarkably low reaction potential of −0.15 V versus RHE at 10 mA cm−2, outperforming monometallic Co catalysts. Experimental and computational analyses revealed dual active sites at the Co/ZnO interface, which facilitate N2H3* desorption and subsequent N2H2* formation. A liquid N2H4-H2O2 fuel cell with p-Co9Zn1 catalyst achieved a high open circuit voltage of 1.916 V and a maximum power density of 195 mW cm−2, demonstrating the potential application of the dual-site Co-Zn catalyst. This rational design strategy of tuning the N2H3* binding energy through bimetallic interactions provides a pathway for developing efficient and economical non-precious metal electrocatalysts for DHzHPFCs.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"4 2","pages":"300-308"},"PeriodicalIF":24.5,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12227","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143707663","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Outside Back Cover: Volume 3 Issue 6 封底外页：第 3 卷第 6 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-11-15 DOI: 10.1002/idm2.12231

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Outside Front Cover: Volume 3 Issue 6 封面外页：第 3 卷第 6 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-11-15 DOI: 10.1002/idm2.12230

引用次数: 0