Interdisciplinary Materials最新文献_第3页

Construction of dendritic Pt–Pd bimetallic nanotubular heterostructure for advanced oxygen reduction 构建用于高级氧还原的树枝状铂钯双金属纳米管异质结构

IF 24.5

Interdisciplinary Materials Pub Date : 2024-08-23 DOI: 10.1002/idm2.12212

Mingwei Wang, Zhiyi Hu, Jieheng Lv, Zhiwen Yin, Zhewei Xu, Jingfeng Liu, Shihao Feng, Xiaoqian Wang, Jiazhen He, Sicheng Luo, Dafu Zhao, Hang Li, Xuemin Luo, Qi Liu, Damin Liu, Baolian Su, Dongyuan Zhao, Yong Liu

{"title":"Construction of dendritic Pt–Pd bimetallic nanotubular heterostructure for advanced oxygen reduction","authors":"Mingwei Wang, Zhiyi Hu, Jieheng Lv, Zhiwen Yin, Zhewei Xu, Jingfeng Liu, Shihao Feng, Xiaoqian Wang, Jiazhen He, Sicheng Luo, Dafu Zhao, Hang Li, Xuemin Luo, Qi Liu, Damin Liu, Baolian Su, Dongyuan Zhao, Yong Liu","doi":"10.1002/idm2.12212","DOIUrl":"https://doi.org/10.1002/idm2.12212","url":null,"abstract":"Compositions and morphologies of Pt-based electrocatalysts have great impact on the electrocatalytic activity and stability of oxygen reduction reaction (ORR). Herein, we report a novel design of one-dimensional (1D) Pt–Pd dendritic nanotubular heterostructures (DTHs) by controlling the degree of Pt2+-Pt reduction reaction and Pd-Pt galvanic replacement reaction with uniform Pd nanowires as sacrificial templates. The obtained Pt–Pd bimetallic DTHs catalyst exhibited uniform and dense Pt dendritic nanobranches on the surface of 1D hollow Pt–Pd alloy nanotubes, possessing superior catalytic activity for ORR compared to state-of-the-art commercial Pt/C catalysts. Typically, the Pt4Pd DTHs catalyst showed efficient mass activity (MA, 1.05 A mgPt−1) and specific activity (SA, 1.25 mA cmPt−2) at 0.9 V (vs. RHE), and the catalyst exhibited high stability with 90.4% MA retention after 20 000 potential cycles. The Pt–Pd bimetallic DTHs configuration combines the advantages of 1D hollow nanostructures and dense Pt dendritic nanobranches, which results in rich electrochemical active surface sites, fast charge transport, and multiple dendritic anchoring points contact on carbon support, thus boosting its catalytic activity and stability towards electrocatalysis.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"907-918"},"PeriodicalIF":24.5,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12212","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142666115","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Biomolecule-responsive polymers and their bio-applications 生物分子响应聚合物及其生物应用

IF 24.5

Interdisciplinary Materials Pub Date : 2024-08-14 DOI: 10.1002/idm2.12210

Yuting Xiong, Minmin Li, Guangyan Qing

{"title":"Biomolecule-responsive polymers and their bio-applications","authors":"Yuting Xiong, Minmin Li, Guangyan Qing","doi":"10.1002/idm2.12210","DOIUrl":"https://doi.org/10.1002/idm2.12210","url":null,"abstract":"Precise recognition and specific interactions between biomolecules are key prerequisites for ensuring the performance of all actives within living organisms. The convergence of biomolecular recognition systems into synthetic materials could endow the materials with high specificity and biological sensitivity; this, in turn, enables precise drug release, monitoring or detection of important biomolecules, and cell manipulation through targeted capture or release of specific biomolecules. Meanwhile, from the perspective of materials science, the application of conventional polymers in practical biological systems poses several challenges, such as low responsiveness and sensitivity, inadequate targetability, insufficient anti-interference capacities, and unsatisfactory biocompatibility. These problems could be partly attributed to the polymers' weak discrimination abilities toward target biomolecules in the presence of interfering substances with high abundance. In particular, the proposition of “precision medicine” project raises higher demands for the design of biomaterials in terms of their precision and targetability. Therefore, there is an urgent demand for the development of new-generation biomaterials with precise recognition and sensitive responsiveness comparable to biomacromolecules. This promotes a new research direction of biomolecule-responsive polymers and their diverse applications. This review focuses on the origin and construction of biomolecule-responsive polymers, as well as their attractive applications in drug delivery systems, bio-detection, bio-sensing, separation, and enrichment, as well as regulating cell adhesion.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"865-896"},"PeriodicalIF":24.5,"publicationDate":"2024-08-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12210","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142665970","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Upvaluing chlorinated plastic wastes

IF 24.5

Interdisciplinary Materials Pub Date : 2024-08-14 DOI: 10.1002/idm2.12211

Shuyi Zhang, Hao Han, Muhan Cao, Yeping Xie, Jinxing Chen

引用次数: 0

Ductile inorganic semiconductors for deformable electronics 用于可变形电子器件的延展性无机半导体

IF 24.5

Interdisciplinary Materials Pub Date : 2024-08-02 DOI: 10.1002/idm2.12209

Xiaocui Li, Fu-Rong Chen, Yang Lu

{"title":"Ductile inorganic semiconductors for deformable electronics","authors":"Xiaocui Li, Fu-Rong Chen, Yang Lu","doi":"10.1002/idm2.12209","DOIUrl":"https://doi.org/10.1002/idm2.12209","url":null,"abstract":"Traditionally, it is relatively easy to process metal materials and polymers (plastics), while ceramic and inorganic semiconductor materials are hard to process, due to their intrinsic brittleness caused by directional covalent bonds or the strong electrostatic interactions among ionic species. The brittleness of semiconductor materials, which may degrade their functional performance and cause catastrophic failures, has excluded them from many application scenarios. The exploration on room-temperature ductile semiconductors has been a long pursuit of mankind for fabricating deformable and more robust electronics. Guided by this goal, researchers have already found that the plasticity of brittle semiconductors can be enhanced by size effects, which include fewer pre-existing micro-cracks and increased dislocation activity, charge characteristics, and defect density. It has also been explored that a few quasi-layered/van der Waals semiconductors can have exceptional room-temperature metal-like plasticity, enabled by the relatively weak interlayer bonding and easy interlayer gliding. More recently, intrinsic exceptional plasticity has been found in a group of all-inorganic perovskites (CsPbX3, X = Cl, Br and I), which can be morphed into distinct morphologies through multislip at room temperature, without affecting their functional properties and bandgap energy. Based on the above research status, in this review, we will discuss and present the relevant works on the plasticity found in inorganic semiconductors and the proposed deformation mechanisms. The potential applications and bottlenecks of plastic semiconductors in manufacturing next-generation deformable electronic/optoelectronic devices and energy systems will also be discussed.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"835-846"},"PeriodicalIF":24.5,"publicationDate":"2024-08-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12209","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142664624","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Advances in electrolyte–anode interface engineering of solid-state lithium metal batteries 固态锂金属电池电解质阳极界面工程的进展

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-30 DOI: 10.1002/idm2.12202

Menghong Li, Shubin Yang, Bin Li

{"title":"Advances in electrolyte–anode interface engineering of solid-state lithium metal batteries","authors":"Menghong Li, Shubin Yang, Bin Li","doi":"10.1002/idm2.12202","DOIUrl":"https://doi.org/10.1002/idm2.12202","url":null,"abstract":"Solid-state lithium metal batteries are considered to be the next generation of energy storage systems due to the high energy density brought by the use of metal lithium anode and the safety features brought by the use of solid electrolytes (SEs). Unfortunately, besides the safety features, using SEs brings issues of interfacial contact of lithium anode and electrolytes. Recently, to realize the application of solid-state lithium metal batteries, significant achievements have been made in the interface engineering of solid-state batteries, and various new strategies have been proposed. In this review, from the interface failure perspective of solid-state lithium metal batteries, we summarize failure mechanisms in terms of poor physical contact, weak chemical/electrochemical stability, continuing contact degradation, and uncontrollable lithium deposition. We then focused on the latest strategies for solving interface issues, including advancing in improving the physical solid–solid contact, increasing the electrochemical/chemical stability, restraining continuing contact degradation, and controlling homogeneous lithium deposition. The ultimate and paramount future developing directions of solid-state lithium metal battery interface engineering are proposed.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"805-834"},"PeriodicalIF":24.5,"publicationDate":"2024-07-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12202","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142665154","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Anisotropic thermally conductive films based on two-dimensional nanomaterials 基于二维纳米材料的各向异性导热薄膜

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-21 DOI: 10.1002/idm2.12204

Lei Li, Qunfeng Cheng

{"title":"Anisotropic thermally conductive films based on two-dimensional nanomaterials","authors":"Lei Li, Qunfeng Cheng","doi":"10.1002/idm2.12204","DOIUrl":"10.1002/idm2.12204","url":null,"abstract":"The significant advancement of high-power densification and miniaturization in modern electronic devices has attracted increasing attention to effective thermal management. The primary objective of thermal management is to transfer excess heat from electronics to the outside environment through the use of thermal conductive materials. The anisotropic thermally conductive films (TCFs) based on two-dimensional (2D) nanomaterials exhibit outstanding controlled heat transfer capability, which effectively removes hotspots along the in-plane direction and provides thermal insulation along the cross-plane direction. However, a comprehensive review of anisotropic TCFs is rarely reported. Herein, we first discuss the intrinsic anisotropic thermal conductivity of 2D nanomaterials for preparing TCFs. Then, the preparation methods and anisotropic thermal conductivity of TCFs have been summarized and discussed. Furthermore, we conclude with the practical applications of TCFs for anisotropy thermal management. Finally, a conclusion of the challenges and outlook of TCFs is provided to promote their development in future scientific research.","PeriodicalId":100685,"journal":{"name":"Interdisciplinary Materials","volume":"3 6","pages":"847-864"},"PeriodicalIF":24.5,"publicationDate":"2024-07-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/idm2.12204","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141818759","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Inside Front Cover: Volume 3 Issue 4 封面内页：第 3 卷第 4 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-18 DOI: 10.1002/idm2.12206

引用次数: 0

Inside Back Cover: Volume 3 Issue 4 封底内页第 3 卷第 4 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-18 DOI: 10.1002/idm2.12207

引用次数: 0

Outside Back Cover: Volume 3 Issue 4 封底外页第 3 卷第 4 期

IF 24.5

Interdisciplinary Materials Pub Date : 2024-07-18 DOI: 10.1002/idm2.12208