Nano-Micro Letters最新文献

{"title":"Scalable Ir-Doped NiFe2O4/TiO2 Heterojunction Anode for Decentralized Saline Wastewater Treatment and H2 Production","authors":"Sukhwa Hong,&nbsp;Jiseon Kim,&nbsp;Jaebeom Park,&nbsp;Sunmi Im,&nbsp;Michael R. Hoffmann,&nbsp;Kangwoo Cho","doi":"10.1007/s40820-024-01542-x","DOIUrl":"10.1007/s40820-024-01542-x","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>Ir-doped NiFe₂O₄ (NFI) spinel with TiO₂ heterojunction overlayer brought about outstanding chlorine evolution reaction in circumneutral pH.</p>\u0000 </li>\u0000 <li>\u0000 <p>Electroanalyses including operando X-ray absorption spectroscopy uncovered the active role of TiO₂ for Cl⁻ chemisorption.</p>\u0000 </li>\u0000 <li>\u0000 <p>NFI/TiO₂ anode boosted both NH₄⁺-to-N₂ conversion and H₂ generation in wastewater, and the practical applicability was confirmed with scaled-up anodes and real wastewater.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01542-x.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142492640","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure Sensing","authors":"Qingqing Zhou,&nbsp;Qihang Ding,&nbsp;Zixun Geng,&nbsp;Chencheng Hu,&nbsp;Long Yang,&nbsp;Zitong Kan,&nbsp;Biao Dong,&nbsp;Miae Won,&nbsp;Hongwei Song,&nbsp;Lin Xu,&nbsp;Jong Seung Kim","doi":"10.1007/s40820-024-01548-5","DOIUrl":"10.1007/s40820-024-01548-5","url":null,"abstract":"<div><p>The rising flexible and intelligent electronics greatly facilitate the noninvasive and timely tracking of physiological information in telemedicine healthcare. Meticulously building bionic-sensitive moieties is vital for designing efficient electronic skin with advanced cognitive functionalities to pluralistically capture external stimuli. However, realistic mimesis, both in the skin’s three-dimensional interlocked hierarchical structures and synchronous encoding multistimuli information capacities, remains a challenging yet vital need for simplifying the design of flexible logic circuits. Herein, we construct an artificial epidermal device by in situ growing Cu₃(HHTP)₂ particles onto the hollow spherical Ti₃C₂T_<i>x</i> surface, aiming to concurrently emulate the spinous and granular layers of the skin’s epidermis. The bionic Ti₃C₂T_<i>x</i>@Cu₃(HHTP)₂ exhibits independent NO₂ and pressure response, as well as novel functionalities such as acoustic signature perception and Morse code-encrypted message communication. Ultimately, a wearable alarming system with a mobile application terminal is self-developed by integrating the bimodular senor into flexible printed circuits. This system can assess risk factors related with asthmatic, such as stimulation of external NO₂ gas, abnormal expiratory behavior and exertion degrees of fingers, achieving a recognition accuracy of 97.6% as assisted by a machine learning algorithm. Our work provides a feasible routine to develop intelligent multifunctional healthcare equipment for burgeoning transformative telemedicine diagnosis.</p><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01548-5.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142489622","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Dynamic Regulation of Hydrogen Bonding Networks and Solvation Structures for Synergistic Solar-Thermal Desalination of Seawater and Catalytic Degradation of Organic Pollutants","authors":"Ming-Yuan Yu,&nbsp;Jing Wu,&nbsp;Guang Yin,&nbsp;Fan-Zhen Jiao,&nbsp;Zhong-Zhen Yu,&nbsp;Jin Qu","doi":"10.1007/s40820-024-01544-9","DOIUrl":"10.1007/s40820-024-01544-9","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000<ul>\u0000 <li>\u0000 <p>A flow-bed water purification system with an asymmetric solar-thermal and catalytic membrane is designed for synergistic solar-thermal desalination of seawater/brine and catalytic degradation of organic pollutants.</p>\u0000 </li>\u0000 <li>\u0000 <p>The hydrogen bonding networks can be regulated by the abundant surface –OH groups and the in situ generated ions and radicals during the degradation process for promoting solar-driven steam generation.</p>\u0000 </li>\u0000 <li>\u0000 <p>The de-solvation of solvated Na⁺ and subsequent nucleation/growth of NaCl are effectively inhibited by SO₄²⁻/HSO₅⁻ ions.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01544-9.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142487166","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Solution-Processed Thin Film Transparent Photovoltaics: Present Challenges and Future Development","authors":"Tianle Liu,&nbsp;Munerah M. S. Almutairi,&nbsp;Jie Ma,&nbsp;Aisling Stewart,&nbsp;Zhaohui Xing,&nbsp;Mengxia Liu,&nbsp;Bo Hou,&nbsp;Yuljae Cho","doi":"10.1007/s40820-024-01547-6","DOIUrl":"10.1007/s40820-024-01547-6","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>Recent advancement in solution-processed thin film transparent photovoltaics (TPVs) is summarized, including perovskites, organics, and colloidal quantum dots.</p>\u0000 </li>\u0000 <li>\u0000 <p>Pros and cons of the emerging TPVs are analyzed according to the materials characteristics and the application requirements on the aesthetics and energy generation.</p>\u0000 </li>\u0000 <li>\u0000 <p>Promising TPV applications are discussed with emphasis on agrivoltaics, smart windows and facades.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01547-6.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142487126","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Graphene Aerogel Composites with Self-Organized Nanowires-Packed Honeycomb Structure for Highly Efficient Electromagnetic Wave Absorption","authors":"Xiao You,&nbsp;Huiying Ouyang,&nbsp;Ruixiang Deng,&nbsp;Qiuqi Zhang,&nbsp;Zhenzhong Xing,&nbsp;Xiaowu Chen,&nbsp;Qingliang Shan,&nbsp;Jinshan Yang,&nbsp;Shaoming Dong","doi":"10.1007/s40820-024-01541-y","DOIUrl":"10.1007/s40820-024-01541-y","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>A new strategy for elaborate regulation of microstructure was successfully introduced by the ice template‑assisted 3D printing and chemical vapor deposition strategy, including graphene nanoplate/silicon carbide nanowires hierarchical porous structure and graphene nanoplate/boron nitride composite heterogeneous interface.</p>\u0000 </li>\u0000 <li>\u0000 <p>The composite exhibits excellent electromagnetic wave absorption performance with an <i>RL</i>_min of -37.8 dB and an EAB_max of 9.2 GHz (from 8.8 to 18.0 GHz) at 2.5 mm. And the high-temperature absorption stability makes it a promising absorber candidate under high temperature and oxidizing atmosphere.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01541-y.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142451830","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Integration of Electrical Properties and Polarization Loss Modulation on Atomic Fe–N-RGO for Boosting Electromagnetic Wave Absorption","authors":"Kaili Zhang,&nbsp;Yuefeng Yan,&nbsp;Zhen Wang,&nbsp;Guansheng Ma,&nbsp;Dechang Jia,&nbsp;Xiaoxiao Huang,&nbsp;Yu Zhou","doi":"10.1007/s40820-024-01518-x","DOIUrl":"10.1007/s40820-024-01518-x","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000<ul>\u0000 <li>\u0000 <p>Single-atom Fe–N₄ sites embedded into graphene were successfully synthesized to exert the dielectric properties of graphene.</p>\u0000 </li>\u0000 <li>\u0000 <p>The absorption mechanisms of metal-nitrogen doping reduced graphene oxide mainly include enhanced dipole polarization, interface polarization, conduction loss and defect-induced polarization.\u0000</p>\u0000 </li>\u0000 <li>\u0000 <p>Excellent reflection loss of − 74.05 dB (2.0 mm) and broad effective absorption bandwidth of 7.05 GHz (1.89 mm, with filler loading only 1 wt%) were obtained.\u0000</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01518-x.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142447443","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion Batteries","authors":"Xuanlong He,&nbsp;Jie Peng,&nbsp;Qingyun Lin,&nbsp;Meng Li,&nbsp;Weibin Chen,&nbsp;Pei Liu,&nbsp;Tao Huang,&nbsp;Zhencheng Huang,&nbsp;Yuying Liu,&nbsp;Jiaojiao Deng,&nbsp;Shenghua Ye,&nbsp;Xuming Yang,&nbsp;Xiangzhong Ren,&nbsp;Xiaoping Ouyang,&nbsp;Jianhong Liu,&nbsp;Biwei Xiao,&nbsp;Jiangtao Hu,&nbsp;Qianling Zhang","doi":"10.1007/s40820-024-01546-7","DOIUrl":"10.1007/s40820-024-01546-7","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>NaTFSI/SUL:OTE:FEC facilitates the formation of S, N-rich, dense and robust cathode–electrolyte interphase on NaNMF cathode, which improves the cycling stability under high voltage.</p>\u0000 </li>\u0000 <li>\u0000 <p>By utilizing NaTFSI/SUL:OTE:FEC, the Na||NaNMF batteries achieved an impressive retention of 81.15% after 400 cycles at 2 C with the cutoff voltage of 4.2 V.</p>\u0000 </li>\u0000 <li>\u0000 <p>The study offers a reference for the utilization of sulfolane-based electrolytes in sodium-ion batteries (SIBs), while the nonflammability of the NaTFSI/SUL:OTE:FEC enhances the safety of SIBs.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01546-7.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142447444","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Unleashing the Potential of Electroactive Hybrid Biomaterials and Self-Powered Systems for Bone Therapeutics","authors":"Shichang Liu,&nbsp;Farid Manshaii,&nbsp;Jinmiao Chen,&nbsp;Xinfei Wang,&nbsp;Shaolei Wang,&nbsp;Junyi Yin,&nbsp;Ming Yang,&nbsp;Xuxu Chen,&nbsp;Xinhua Yin,&nbsp;Yunlei Zhou","doi":"10.1007/s40820-024-01536-9","DOIUrl":"10.1007/s40820-024-01536-9","url":null,"abstract":"<div><p>The incidence of large bone defects caused by traumatic injury is increasing worldwide, and the tissue regeneration process requires a long recovery time due to limited self-healing capability. Endogenous bioelectrical phenomena have been well recognized as critical biophysical factors in bone remodeling and regeneration. Inspired by bioelectricity, electrical stimulation has been widely considered an external intervention to induce the osteogenic lineage of cells and enhance the synthesis of the extracellular matrix, thereby accelerating bone regeneration. With ongoing advances in biomaterials and energy-harvesting techniques, electroactive biomaterials and self-powered systems have been considered biomimetic approaches to ensure functional recovery by recapitulating the natural electrophysiological microenvironment of healthy bone tissue. In this review, we first introduce the role of bioelectricity and the endogenous electric field in bone tissue and summarize different techniques to electrically stimulate cells and tissue. Next, we highlight the latest progress in exploring electroactive hybrid biomaterials as well as self-powered systems such as triboelectric and piezoelectric-based nanogenerators and photovoltaic cell-based devices and their implementation in bone tissue engineering. Finally, we emphasize the significance of simulating the target tissue’s electrophysiological microenvironment and propose the opportunities and challenges faced by electroactive hybrid biomaterials and self-powered bioelectronics for bone repair strategies.</p><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01536-9.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142440828","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Gradient-Layered MXene/Hollow Lignin Nanospheres Architecture Design for Flexible and Stretchable Supercapacitors","authors":"Haonan Zhang,&nbsp;Cheng Hao,&nbsp;Tongtong Fu,&nbsp;Dian Yu,&nbsp;Jane Howe,&nbsp;Kaiwen Chen,&nbsp;Ning Yan,&nbsp;Hao Ren,&nbsp;Huamin Zhai","doi":"10.1007/s40820-024-01512-3","DOIUrl":"10.1007/s40820-024-01512-3","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>A novel gradient-layered architecture based on single-pore hollow lignin nanospheres (HLNPs)-intercalated MXene layers was created to fabricate highly stretchable (600%) and durable (1000 cycling) supercapacitor electrodes.</p>\u0000 </li>\u0000 <li>\u0000 <p>The architecture reduced the overstacking of MXene, and the micro-chamber structure of HLNPs better utilized lignin’s pseudocapacitive property to improve ion and electron accessibility (specific capacitance reached 1273 mF cm⁻²).</p>\u0000 </li>\u0000 <li>\u0000 <p>HLNPs enhanced mechanical durability and capacitive stability of the integrated wrinkled electrodes during the stretch-release cycling.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01512-3.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142440830","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Ultra-High Sensitivity Anisotropic Piezoelectric Sensors for Structural Health Monitoring and Robotic Perception","authors":"Hao Yin,&nbsp;Yanting Li,&nbsp;Zhiying Tian,&nbsp;Qichao Li,&nbsp;Chenhui Jiang,&nbsp;Enfu Liang,&nbsp;Yiping Guo","doi":"10.1007/s40820-024-01539-6","DOIUrl":"10.1007/s40820-024-01539-6","url":null,"abstract":"<div><p>Monitoring minuscule mechanical signals, both in magnitude and direction, is imperative in many application scenarios, e.g., structural health monitoring and robotic sensing systems. However, the piezoelectric sensor struggles to satisfy the requirements for directional recognition due to the limited piezoelectric coefficient matrix, and achieving sensitivity for detecting micrometer-scale deformations is also challenging. Herein, we develop a vector sensor composed of lead zirconate titanate-electronic grade glass fiber composite filaments with oriented arrangement, capable of detecting minute anisotropic deformations. The as-prepared vector sensor can identify the deformation directions even when subjected to an unprecedented nominal strain of 0.06%, thereby enabling its utility in accurately discerning the 5 μm-height wrinkles in thin films and in monitoring human pulse waves. The ultra-high sensitivity is attributed to the formation of porous ferroelectret and the efficient load transfer efficiency of continuous lead zirconate titanate phase. Additionally, when integrated with machine learning techniques, the sensor’s capability to recognize multi-signals enables it to differentiate between 10 types of fine textures with 100% accuracy. The structural design in piezoelectric devices enables a more comprehensive perception of mechanical stimuli, offering a novel perspective for enhancing recognition accuracy.</p><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"17 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-10-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01539-6.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142438759","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}