{"title":"Constructed Mott–Schottky Heterostructure Catalyst to Trigger Interface Disturbance and Manipulate Redox Kinetics in Li-O2 Battery","authors":"Yongji Xia, Le Wang, Guiyang Gao, Tianle Mao, Zhenjia Wang, Xuefeng Jin, Zheyu Hong, Jiajia Han, Dong-Liang Peng, Guanghui Yue","doi":"10.1007/s40820-024-01476-4","DOIUrl":"10.1007/s40820-024-01476-4","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>A carbon free self supported Mott-Schottky heterostructure was constructed as an efficient cathode catalyst for lithium oxygen batteries, achieving homogeneous contact between the two materials for strong interfacial interactions.</p>\u0000 </li>\u0000 <li>\u0000 <p>The heterostructure triggered interfacial perturbations and band structure changes, which accelerated oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) kinetics, resulting in an extremely long cycle life of 800 cycles and an extremely low overpotential of 0.73 V.</p>\u0000 </li>\u0000 <li>\u0000 <p>Combined with advanced characterization techniques and density functional theory calculations, the underlying mechanism behind the boosted ORR/OER activities and the electrocatalytic mechanism were revealed.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11286616/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141787031","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Jianye Li, Hao Wang, Yibing Luo, Zijing Zhou, He Zhang, Huizhi Chen, Kai Tao, Chuan Liu, Lingxing Zeng, Fengwei Huo, Jin Wu
{"title":"Design of AI-Enhanced and Hardware-Supported Multimodal E-Skin for Environmental Object Recognition and Wireless Toxic Gas Alarm","authors":"Jianye Li, Hao Wang, Yibing Luo, Zijing Zhou, He Zhang, Huizhi Chen, Kai Tao, Chuan Liu, Lingxing Zeng, Fengwei Huo, Jin Wu","doi":"10.1007/s40820-024-01466-6","DOIUrl":"10.1007/s40820-024-01466-6","url":null,"abstract":"<div><h2> Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>A novel organohydrogel-based multimodal e-skin with excellent sensing performance for temperature, humidity, pressure, proximity, and NO<sub>2</sub> is proposed for the first time, showing powerful sensing capabilities beyond natural skin.</p>\u0000 </li>\u0000 <li>\u0000 <p>The developed multimodal e-skin exhibited extraordinary sensing performance at room temperature, including fast pressure response time (0.2 s), high temperature sensitivity (9.38% °C<sup>-1</sup>), a wide range of humidity response (22%–98% RH), high NO<sub>2</sub> sensitivity (254% ppm<sup>-1</sup>), a low detection limit (11.1 ppb NO<sub>2</sub>) and the abilities to sense the proximity of objects accurately, which are yet achieved by previous e-skins.</p>\u0000 </li>\u0000 <li>\u0000 <p>The multimodal e-skin was combined with the deep neural network algorithm and wireless alarm circuit to achieve zero-error classification of different objects and rapid response to NO<sub>x</sub> leak incidents, proving the feasibility of the e-skin-assisted rescue robot for post-earthquake rescue.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11286924/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141787032","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yumei Wang, Zhongting Wang, Xiaoyu Xu, Sam Jin An Oh, Jianguo Sun, Feng Zheng, Xiao Lu, Chaohe Xu, Binggong Yan, Guangsheng Huang, Li Lu
{"title":"Ultra-Stable Sodium-Ion Battery Enabled by All-Solid-State Ferroelectric-Engineered Composite Electrolytes","authors":"Yumei Wang, Zhongting Wang, Xiaoyu Xu, Sam Jin An Oh, Jianguo Sun, Feng Zheng, Xiao Lu, Chaohe Xu, Binggong Yan, Guangsheng Huang, Li Lu","doi":"10.1007/s40820-024-01474-6","DOIUrl":"10.1007/s40820-024-01474-6","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000<ul>\u0000 <li>\u0000 <p>The capacity fading mechanism of the conventional Na<sub>3</sub>V<sub>2</sub>(PO<sub>4</sub>)<sub>3</sub>//Na<sub>3</sub>V<sub>2</sub>(PO<sub>4</sub>)<sub>3</sub> (NVP//NVP) cell has been investigated.</p>\u0000 </li>\u0000 <li>\u0000 <p>All-solid-state ferroelectric-engineered composite electrolyte could improve the electrolyte–electrode interfacial stability as well as the interfacial ion conduction of the Na-ion battery using the NVP anode.</p>\u0000 </li>\u0000 <li>\u0000 <p>Outstanding cyclic stability has been achieved in the all-solid-state Na-ion battery using the NVP anode, with a capacity fading rate as low as 0.005% per cycle.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01474-6.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141755271","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Metal–Organic Framework-Based Photodetectors","authors":"Jin-Biao Zhang, Yi-Bo Tian, Zhi-Gang Gu, Jian Zhang","doi":"10.1007/s40820-024-01465-7","DOIUrl":"10.1007/s40820-024-01465-7","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000<ul>\u0000 <li>\u0000 <p>The methods of preparing metal–organic framework (MOF)-based photodetectors and various types of MOFs are introduced.</p>\u0000 </li>\u0000 <li>\u0000 <p>The applications of MOF photodetectors in the detection of X-ray, ultraviolet, and infrared radiation, biosensing, and circularly polarized light detection are summarized.</p>\u0000 </li>\u0000 <li>\u0000 <p>Challenges in developing practical MOF photodetector and concepts to solve those critical challenges are discussed.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01465-7.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141755270","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Xinzhe Xue, Longsheng Feng, Qiu Ren, Cassidy Tran, Samuel Eisenberg, Anica Pinongcos, Logan Valdovinos, Cathleen Hsieh, Tae Wook Heo, Marcus A. Worsley, Cheng Zhu, Yat Li
{"title":"Interpenetrated Structures for Enhancing Ion Diffusion Kinetics in Electrochemical Energy Storage Devices","authors":"Xinzhe Xue, Longsheng Feng, Qiu Ren, Cassidy Tran, Samuel Eisenberg, Anica Pinongcos, Logan Valdovinos, Cathleen Hsieh, Tae Wook Heo, Marcus A. Worsley, Cheng Zhu, Yat Li","doi":"10.1007/s40820-024-01472-8","DOIUrl":"10.1007/s40820-024-01472-8","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>A new and compact device configuration was created with two interpenetrated, individually addressable electrodes, allowing precise control over the geometric features and interactions between the electrodes.</p>\u0000 </li>\u0000 <li>\u0000 <p>The interpenetrated electrode design improves ion diffusion kinetics in electrochemical energy storage devices by shortening the ion diffusion length and reducing ion concentration inhomogeneity.</p>\u0000 </li>\u0000 <li>\u0000 <p>The device with interpenetrated electrodes outperformed the traditional separate electrode configuration, enhancing both volumetric energy density and capacity retention rate.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-024-01472-8.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141755334","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Hongzheng Wu, Shenghao Luo, Hubing Wang, Li Li, Yaobing Fang, Fan Zhang, Xuenong Gao, Zhengguo Zhang, Wenhui Yuan
{"title":"A Review of Anode Materials for Dual-Ion Batteries","authors":"Hongzheng Wu, Shenghao Luo, Hubing Wang, Li Li, Yaobing Fang, Fan Zhang, Xuenong Gao, Zhengguo Zhang, Wenhui Yuan","doi":"10.1007/s40820-024-01470-w","DOIUrl":"10.1007/s40820-024-01470-w","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000<ul>\u0000 <li>\u0000 <p>The development history and working mechanism of dual-ion batteries are reviewed, with an emphasis on the latest advancement in anode materials.</p>\u0000 </li>\u0000 <li>\u0000 <p>A comprehensive and detailed summary of the synthesis strategies, structural optimization, performance characterization, and reaction principles of four types of anode materials for dual-ion batteries is presented.</p>\u0000 </li>\u0000 <li>\u0000 <p>The current challenges of anode materials are highlighted, and the optimization strategies of advanced anode materials and battery systems are discussed, providing future research directions for the design of commercial dual-ion batteries.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11269562/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141750815","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Delivering Microrobots in the Musculoskeletal System","authors":"Mumin Cao, Renwang Sheng, Yimin Sun, Ying Cao, Hao Wang, Ming Zhang, Yunmeng Pu, Yucheng Gao, Yuanwei Zhang, Panpan Lu, Gaojun Teng, Qianqian Wang, Yunfeng Rui","doi":"10.1007/s40820-024-01464-8","DOIUrl":"10.1007/s40820-024-01464-8","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000<ul>\u0000 <li>\u0000 <p>A systematic review of recent advances of microrobots applied in the musculoskeletal system with an emphasis on design strategies of microrobotic systems for tissue regeneration.</p>\u0000 </li>\u0000 <li>\u0000 <p>The fabrication, motion and control, and image-guided delivery of microrobots in the musculoskeletal system are reviewed based on the up-to-date works.</p>\u0000 </li>\u0000 <li>\u0000 <p>Prospects and challenges for future clinical translation of microrobots in the musculoskeletal system and regenerative medicine are discussed.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11263536/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141733163","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yexin Pan, Ruohan Yu, Yalong Jiang, Haosong Zhong, Qiaoyaxiao Yuan, Connie Kong Wai Lee, Rongliang Yang, Siyu Chen, Yi Chen, Wing Yan Poon, Mitch Guijun Li
{"title":"Heterogeneous CuxO Nano-Skeletons from Waste Electronics for Enhanced Glucose Detection","authors":"Yexin Pan, Ruohan Yu, Yalong Jiang, Haosong Zhong, Qiaoyaxiao Yuan, Connie Kong Wai Lee, Rongliang Yang, Siyu Chen, Yi Chen, Wing Yan Poon, Mitch Guijun Li","doi":"10.1007/s40820-024-01467-5","DOIUrl":"10.1007/s40820-024-01467-5","url":null,"abstract":"<div><p>Electronic waste (e-waste) and diabetes are global challenges to modern societies. However, solving these two challenges together has been challenging until now. Herein, we propose a laser-induced transfer method to fabricate portable glucose sensors by recycling copper from e-waste. We bring up a laser-induced full-automatic fabrication method for synthesizing continuous heterogeneous Cu<sub><i>x</i></sub>O (h-Cu<sub><i>x</i></sub>O) nano-skeletons electrode for glucose sensing, offering rapid (< 1 min), clean, air-compatible, and continuous fabrication, applicable to a wide range of Cu-containing substrates. Leveraging this approach, h-Cu<sub><i>x</i></sub>O nano-skeletons, with an inner core predominantly composed of Cu<sub>2</sub>O with lower oxygen content, juxtaposed with an outer layer rich in amorphous Cu<sub><i>x</i></sub>O (a-Cu<sub><i>x</i></sub>O) with higher oxygen content, are derived from discarded printed circuit boards. When employed in glucose detection, the h-Cu<sub><i>x</i></sub>O nano-skeletons undergo a structural evolution process, transitioning into rigid Cu<sub>2</sub>O@CuO nano-skeletons prompted by electrochemical activation. This transformation yields exceptional glucose-sensing performance (sensitivity: 9.893 mA mM<sup>−1</sup> cm<sup>−2</sup>; detection limit: 0.34 μM), outperforming most previously reported glucose sensors. Density functional theory analysis elucidates that the heterogeneous structure facilitates gluconolactone desorption. This glucose detection device has also been downsized to optimize its scalability and portability for convenient integration into people’s everyday lives. </p><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11258110/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141632272","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Defect Engineering and Carbon Supporting to Achieve Ni-Doped CoP3 with High Catalytic Activities for Overall Water Splitting","authors":"Daowei Zha, Ruoxing Wang, Shijun Tian, Zhong-Jie Jiang, Zejun Xu, Chu Qin, Xiaoning Tian, Zhongqing Jiang","doi":"10.1007/s40820-024-01471-9","DOIUrl":"10.1007/s40820-024-01471-9","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 <ul>\u0000 <li>\u0000 <p>Plasma-assisted phosphorization has been used to prepare defect-rich metal phosphides.</p>\u0000 </li>\u0000 <li>\u0000 <p>The p-NiCoP/NCF@CC shows high activities and excellent stability for the hydrogen evolution reaction and the oxygen evolution reaction.</p>\u0000 </li>\u0000 <li>\u0000 <p>The p-NiCoP/NCF@CC shows great potential for overall water splitting.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11258119/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141632271","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yuwen Wei, Priyanuj Bhuyan, Suk Jin Kwon, Sihyun Kim, Yejin Bae, Mukesh Singh, Duy Thanh Tran, Minjeong Ha, Kwang-Un Jeong, Xing Ma, Byeongjin Park, Sungjune Park
{"title":"Liquid Metal Grid Patterned Thin Film Devices Toward Absorption-Dominant and Strain-Tunable Electromagnetic Interference Shielding","authors":"Yuwen Wei, Priyanuj Bhuyan, Suk Jin Kwon, Sihyun Kim, Yejin Bae, Mukesh Singh, Duy Thanh Tran, Minjeong Ha, Kwang-Un Jeong, Xing Ma, Byeongjin Park, Sungjune Park","doi":"10.1007/s40820-024-01457-7","DOIUrl":"10.1007/s40820-024-01457-7","url":null,"abstract":"<div><div>\u0000 \u0000<ul>\u0000 <li>\u0000 <p>Multiple internal reflection-based absorption-dominant stretchable electromagnetic shielding thin film by incorporating liquid metal grid structure is developed.</p>\u0000 </li>\u0000 <li>\u0000 <p>The device demonstrates high electromagnetic shielding effectiveness (SE) (SE<sub>T</sub> of up to 75 dB) with low reflectance (SE<sub>R</sub> of 1.5 dB at the resonant frequency).</p>\u0000 </li>\u0000 <li>\u0000 <p>The shielding properties of the device can be tuned by adjusting the liquid metal patterned grid spaces upon strain.</p>\u0000 </li>\u0000 </ul>\u0000 </div></div>","PeriodicalId":714,"journal":{"name":"Nano-Micro Letters","volume":"16 1","pages":""},"PeriodicalIF":26.6,"publicationDate":"2024-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11255180/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141625590","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}