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Co-Upcycling of Waste Electronic Plastics and Algae Biomass into High-Quality Pyrolysis Oil through Self-Catalytic Debromination and Oil Upgrading 废电子塑料和藻类生物质自催化脱溴和油脂升级协同升级制备高品质热解油
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-15 DOI: 10.1021/acsestengg.4c0060010.1021/acsestengg.4c00600
Yuan Kong, Si-Xian Wang, Jia-Wei Huang, Yun Ge, Zhi-Yan Guo, Wen-Wei Li* and Wu-Jun Liu*, 
{"title":"Co-Upcycling of Waste Electronic Plastics and Algae Biomass into High-Quality Pyrolysis Oil through Self-Catalytic Debromination and Oil Upgrading","authors":"Yuan Kong,&nbsp;Si-Xian Wang,&nbsp;Jia-Wei Huang,&nbsp;Yun Ge,&nbsp;Zhi-Yan Guo,&nbsp;Wen-Wei Li* and Wu-Jun Liu*,&nbsp;","doi":"10.1021/acsestengg.4c0060010.1021/acsestengg.4c00600","DOIUrl":"https://doi.org/10.1021/acsestengg.4c00600https://doi.org/10.1021/acsestengg.4c00600","url":null,"abstract":"<p >Upcycling waste plastics into fuel oil and gases offers an important route for waste-to-wealth conversion. However, the valorization of waste electronic plastics (WEP) remains challenging because the brominated flame retardant (BFR) components are easily converted to hazardous brominated organics, which lowers the product quality. Here, we report the copyrolysis of WEP with iron-rich algae biomass waste for high-quality oil production without the need for the external addition of a catalyst for bromine (Br) fixation. Iron-based flocculants are commonly used for collecting algae biomass from an algal-bloomed lake, resulting in iron-rich algae biomass. During its pyrolysis, the iron component was converted into Fe<sub>2</sub>O<sub>3</sub>, which served as an efficient endogenous catalyst to facilitate Br fixation and WEP depolymerization. The oil product of the copyrolysis system (WEP/AB = 1:1, 600 °C) exhibited 80% less Br content, a 30% higher fraction of total aromatic compounds, and a 15% higher oil yield than those of the WEP-alone group. Overall, our work offers a facile self-catalytic debromination strategy for WEP upcycling by simply mixing it with iron-rich algae biomass waste for copyrolysis. Such a “two-birds-one-stone” strategy may also be extended to the upcycling of other halogen-containing organic wastes.</p>","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 5","pages":"1088–1098 1088–1098"},"PeriodicalIF":7.4,"publicationDate":"2025-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143921341","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Environmental Biotechnologies Enabling a Carbon-Neutral Circular Economy 环境生物技术实现碳中和循环经济
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-14 DOI: 10.1021/acsestengg.5c0029110.1021/acsestengg.5c00291
Hee-Deung Park*, George F. Wells, Hyung-Sool Lee and Nancy G. Love, 
{"title":"Environmental Biotechnologies Enabling a Carbon-Neutral Circular Economy","authors":"Hee-Deung Park*,&nbsp;George F. Wells,&nbsp;Hyung-Sool Lee and Nancy G. Love,&nbsp;","doi":"10.1021/acsestengg.5c0029110.1021/acsestengg.5c00291","DOIUrl":"https://doi.org/10.1021/acsestengg.5c00291https://doi.org/10.1021/acsestengg.5c00291","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 5","pages":"1085–1087 1085–1087"},"PeriodicalIF":7.4,"publicationDate":"2025-04-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143921271","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-11
Qiulai He*, Jinfeng Li, Meng Wang, Zhiyi Xie, Peng Bi, Peng Xu, Jingwei Ma*, Baokun Xu and Hongyu Wang, 
{"title":"","authors":"Qiulai He*,&nbsp;Jinfeng Li,&nbsp;Meng Wang,&nbsp;Zhiyi Xie,&nbsp;Peng Bi,&nbsp;Peng Xu,&nbsp;Jingwei Ma*,&nbsp;Baokun Xu and Hongyu Wang,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 4","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00812","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144371450","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-11
Jonathan Burkhardt*, Thomas F. Speth, Stanley Gorzelnik, Alexander S. Gorzalski, Orlando Coronell, Ahmed Rachid El-Khattabi and Mohamed Ateia*, 
{"title":"","authors":"Jonathan Burkhardt*,&nbsp;Thomas F. Speth,&nbsp;Stanley Gorzelnik,&nbsp;Alexander S. Gorzalski,&nbsp;Orlando Coronell,&nbsp;Ahmed Rachid El-Khattabi and Mohamed Ateia*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 4","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.5c00036","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144345748","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-11
Shuai Chen, Fan Yang, Sha Liang*, Mingxuan Wen, Zhengkang Zou, Shushan Yuan, Huabo Duan, Wenbo Yu, Jingping Hu and Jiakuan Yang, 
{"title":"","authors":"Shuai Chen,&nbsp;Fan Yang,&nbsp;Sha Liang*,&nbsp;Mingxuan Wen,&nbsp;Zhengkang Zou,&nbsp;Shushan Yuan,&nbsp;Huabo Duan,&nbsp;Wenbo Yu,&nbsp;Jingping Hu and Jiakuan Yang,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 4","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00727","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144371482","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-11
Jian Lu, Huan He, Tianyang Zhang, Qi Fu, Renjie Pan, Chao Zeng*, Yanbo Zhou and Bin Xu*, 
{"title":"","authors":"Jian Lu,&nbsp;Huan He,&nbsp;Tianyang Zhang,&nbsp;Qi Fu,&nbsp;Renjie Pan,&nbsp;Chao Zeng*,&nbsp;Yanbo Zhou and Bin Xu*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 4","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00782","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144345753","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-11
Danielle Abigail Clyde, Khai Yang Tan, Wen Jie Yiang, Wen Siong Poh, Jessin Tiu, Jiexiang Wang, Jun-tao Li, Nay Ming Huang, Binghui Chen and Chuan Yi Foo*, 
{"title":"","authors":"Danielle Abigail Clyde,&nbsp;Khai Yang Tan,&nbsp;Wen Jie Yiang,&nbsp;Wen Siong Poh,&nbsp;Jessin Tiu,&nbsp;Jiexiang Wang,&nbsp;Jun-tao Li,&nbsp;Nay Ming Huang,&nbsp;Binghui Chen and Chuan Yi Foo*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 4","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00744","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144345754","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-11
Qin Dong, Timothy E. Mattes* and Gregory H. LeFevre*, 
{"title":"","authors":"Qin Dong,&nbsp;Timothy E. Mattes* and Gregory H. LeFevre*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 4","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00718","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144372031","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
ACS ES&T Engineering’s 2024 Excellence in Review Awards ACS ES&T Engineering获得2024年卓越评审奖
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-11 DOI: 10.1021/acsestengg.5c0022510.1021/acsestengg.5c00225
Wonyong Choi*, Jingyun Fang, Manish Kumar, Jaehong Kim, Robert Nerenberg, Brian Chaplin and Fan Dong, 
{"title":"ACS ES&T Engineering’s 2024 Excellence in Review Awards","authors":"Wonyong Choi*,&nbsp;Jingyun Fang,&nbsp;Manish Kumar,&nbsp;Jaehong Kim,&nbsp;Robert Nerenberg,&nbsp;Brian Chaplin and Fan Dong,&nbsp;","doi":"10.1021/acsestengg.5c0022510.1021/acsestengg.5c00225","DOIUrl":"https://doi.org/10.1021/acsestengg.5c00225https://doi.org/10.1021/acsestengg.5c00225","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 4","pages":"829 829"},"PeriodicalIF":7.4,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143814590","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 7.4
ACS ES&T engineering Pub Date : 2025-04-11
Daichi Takami, Taku Kishimura, Yasutaka Kuwahara* and Hiromi Yamashita*, 
{"title":"","authors":"Daichi Takami,&nbsp;Taku Kishimura,&nbsp;Yasutaka Kuwahara* and Hiromi Yamashita*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 4","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00707","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144345744","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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