Jicheng Liu, Yani Wu, Chunli Zheng*, Mingjiao Tian, Zeyu Jiang*, Reem Albilali and Chi He*,
{"title":"多组分VOC净化工程功能催化剂研究进展","authors":"Jicheng Liu, Yani Wu, Chunli Zheng*, Mingjiao Tian, Zeyu Jiang*, Reem Albilali and Chi He*, ","doi":"10.1021/acsestengg.5c0015910.1021/acsestengg.5c00159","DOIUrl":null,"url":null,"abstract":"<p >Volatile organic compounds (VOCs) have caused serious harm to human health and the ecological environment. As a promising strategy, the catalytic oxidation of VOCs into harmless products such as H<sub>2</sub>O and CO<sub>2</sub> has been widely employed. Although many catalysts have been developed for VOC decomposition, the design and synthesis of functional catalysts toward multicomponent VOC purification in industrial exhaust gas under reality remains a great challenge. In the actual vent, the composition of multicomponent VOCs is complex and impurities such as NO<sub><i>x</i></sub>, SO<sub>2</sub>, and H<sub>2</sub>O are also present. Traditional catalysts often suffer from poor stability, deactivation by impurities, and inefficient oxidation of complex VOC mixtures in industrial settings. Addressing these challenges requires a deeper understanding of the fundamental mechanisms and advanced catalyst design strategies. Therefore, elucidating the mechanism of multicomponent VOC oxidation and revealing the influential behavior of impurities are urgently required to guide researchers on how to synthesize effective and stable catalysts proactively for multicomponent VOC purification under reality. Accordingly, this review systematically summarizes the recent advances in the engineering of highly active and durable catalysts for the oxidation of multicomponent VOCs. The experimental and theoretical studies revealing the mixing effects occurring in the catalytic oxidation process of multicomponent VOCs are also highlighted. Further development of and research on catalysts to be adopted in multipollutant controlling are proposed. This review can help researchers to better understand the catalytic elimination of multicomponent VOCs and provide a great foundation for future design and practical industrial application of VOC oxidation catalysts.</p>","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"1316–1337 1316–1337"},"PeriodicalIF":7.4000,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Recent Advances in Engineering Functional Catalysts toward Multicomponent VOC Purification under Reality\",\"authors\":\"Jicheng Liu, Yani Wu, Chunli Zheng*, Mingjiao Tian, Zeyu Jiang*, Reem Albilali and Chi He*, \",\"doi\":\"10.1021/acsestengg.5c0015910.1021/acsestengg.5c00159\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Volatile organic compounds (VOCs) have caused serious harm to human health and the ecological environment. As a promising strategy, the catalytic oxidation of VOCs into harmless products such as H<sub>2</sub>O and CO<sub>2</sub> has been widely employed. Although many catalysts have been developed for VOC decomposition, the design and synthesis of functional catalysts toward multicomponent VOC purification in industrial exhaust gas under reality remains a great challenge. In the actual vent, the composition of multicomponent VOCs is complex and impurities such as NO<sub><i>x</i></sub>, SO<sub>2</sub>, and H<sub>2</sub>O are also present. Traditional catalysts often suffer from poor stability, deactivation by impurities, and inefficient oxidation of complex VOC mixtures in industrial settings. Addressing these challenges requires a deeper understanding of the fundamental mechanisms and advanced catalyst design strategies. Therefore, elucidating the mechanism of multicomponent VOC oxidation and revealing the influential behavior of impurities are urgently required to guide researchers on how to synthesize effective and stable catalysts proactively for multicomponent VOC purification under reality. Accordingly, this review systematically summarizes the recent advances in the engineering of highly active and durable catalysts for the oxidation of multicomponent VOCs. The experimental and theoretical studies revealing the mixing effects occurring in the catalytic oxidation process of multicomponent VOCs are also highlighted. Further development of and research on catalysts to be adopted in multipollutant controlling are proposed. This review can help researchers to better understand the catalytic elimination of multicomponent VOCs and provide a great foundation for future design and practical industrial application of VOC oxidation catalysts.</p>\",\"PeriodicalId\":7008,\"journal\":{\"name\":\"ACS ES&T engineering\",\"volume\":\"5 6\",\"pages\":\"1316–1337 1316–1337\"},\"PeriodicalIF\":7.4000,\"publicationDate\":\"2025-05-16\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS ES&T engineering\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsestengg.5c00159\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS ES&T engineering","FirstCategoryId":"1085","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsestengg.5c00159","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
Recent Advances in Engineering Functional Catalysts toward Multicomponent VOC Purification under Reality
Volatile organic compounds (VOCs) have caused serious harm to human health and the ecological environment. As a promising strategy, the catalytic oxidation of VOCs into harmless products such as H2O and CO2 has been widely employed. Although many catalysts have been developed for VOC decomposition, the design and synthesis of functional catalysts toward multicomponent VOC purification in industrial exhaust gas under reality remains a great challenge. In the actual vent, the composition of multicomponent VOCs is complex and impurities such as NOx, SO2, and H2O are also present. Traditional catalysts often suffer from poor stability, deactivation by impurities, and inefficient oxidation of complex VOC mixtures in industrial settings. Addressing these challenges requires a deeper understanding of the fundamental mechanisms and advanced catalyst design strategies. Therefore, elucidating the mechanism of multicomponent VOC oxidation and revealing the influential behavior of impurities are urgently required to guide researchers on how to synthesize effective and stable catalysts proactively for multicomponent VOC purification under reality. Accordingly, this review systematically summarizes the recent advances in the engineering of highly active and durable catalysts for the oxidation of multicomponent VOCs. The experimental and theoretical studies revealing the mixing effects occurring in the catalytic oxidation process of multicomponent VOCs are also highlighted. Further development of and research on catalysts to be adopted in multipollutant controlling are proposed. This review can help researchers to better understand the catalytic elimination of multicomponent VOCs and provide a great foundation for future design and practical industrial application of VOC oxidation catalysts.
期刊介绍:
ACS ES&T Engineering publishes impactful research and review articles across all realms of environmental technology and engineering, employing a rigorous peer-review process. As a specialized journal, it aims to provide an international platform for research and innovation, inviting contributions on materials technologies, processes, data analytics, and engineering systems that can effectively manage, protect, and remediate air, water, and soil quality, as well as treat wastes and recover resources.
The journal encourages research that supports informed decision-making within complex engineered systems and is grounded in mechanistic science and analytics, describing intricate environmental engineering systems. It considers papers presenting novel advancements, spanning from laboratory discovery to field-based application. However, case or demonstration studies lacking significant scientific advancements and technological innovations are not within its scope.
Contributions containing experimental and/or theoretical methods, rooted in engineering principles and integrated with knowledge from other disciplines, are welcomed.