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Rising temperatures decrease rare earth element bioavailability and ecological risk in coastal sediments 气温上升降低了沿海沉积物中稀土元素的生物利用度和生态风险
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-07-18 DOI: 10.1007/s10311-025-01864-1
Yang-Guang Gu, Yanpeng Gao, Richard W. Jordan, Shi-Jun Jiang, Hong-Hui Huang
{"title":"Rising temperatures decrease rare earth element bioavailability and ecological risk in coastal sediments","authors":"Yang-Guang Gu,&nbsp;Yanpeng Gao,&nbsp;Richard W. Jordan,&nbsp;Shi-Jun Jiang,&nbsp;Hong-Hui Huang","doi":"10.1007/s10311-025-01864-1","DOIUrl":"10.1007/s10311-025-01864-1","url":null,"abstract":"<div><p>Rare earth elements are sedimentary pollutants of increasing health concern, yet the effect of global warming on their bioavailability and toxicity is unknown. To test this, we applied the diffusive gradients in thin films technique to assess the bioavailability of 15 rare earth elements, including lanthanides and yttrium, in sediments at temperatures ranging from 0 to 40 °C. We modeled the ecotoxicological risk to aquatic organisms using the species sensitivity distribution–probabilistic risk assessment–inclusion–exclusion principle. Results show that the bioavailability of all rare earth elements decreases by 40% to 70% as temperature increases from 0 to 40 °C, indicating reduced mobility and enhanced sediment adsorption. Similarly, the calculated ecotoxicological risk is reduced from 1.75 to 0.08%. This is the first evidence of temperature-driven attenuation of rare earth element risk in sediments, suggesting that global warming should decrease the toxicity of some rare earth elements.</p></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"24 1","pages":"21 - 25"},"PeriodicalIF":20.4,"publicationDate":"2025-07-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146027153","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Benzo[a]pyrene osteotoxicity, neurotoxicity, and epigenetic effects in fishes and mammals: a review 苯并芘在鱼类和哺乳动物中的骨毒性、神经毒性和表观遗传效应综述
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-07-18 DOI: 10.1007/s10311-025-01859-y
Jiezhang Mo, Yinhua Chen, Keng Po Lai, Frauke Seemann, Wenhua Liu
{"title":"Benzo[a]pyrene osteotoxicity, neurotoxicity, and epigenetic effects in fishes and mammals: a review","authors":"Jiezhang Mo,&nbsp;Yinhua Chen,&nbsp;Keng Po Lai,&nbsp;Frauke Seemann,&nbsp;Wenhua Liu","doi":"10.1007/s10311-025-01859-y","DOIUrl":"10.1007/s10311-025-01859-y","url":null,"abstract":"<div><p>Polycyclic aromatic hydrocarbons are well-known pollutants, yet some apects of their osteotoxicity and neurotoxicity have not been reviewed. Here we review benzo[a]pyrene-induced osteotoxicity and neurotoxicity in fish and mammals, with focus on phenotypic changes, cell development, molecular signaling pathways, key gene expression, and epigenetic modifications. Benzo[a]pyrene impairs bone health by suppressing osteoblast formation, promoting bone resorption, and disrupting remodeling, primarily through dysregulation of key transcription factors and signaling pathways. In neural tissues, metabolically-activated benzo[a]pyrene generates reactive oxygen species, triggering oxidative stress, dysregulation of gene expression, mitochondrial dysfunction, altered neurotransmitter levels, and neuronal apoptosis. Benzo[a]pyrene induced multigenerational osteotoxicity in 42% of fish studies, but 0% in rodent studies. It induced multigenerational neurotoxicity in 25% of fish studies and 15% in rodent studies. Epigenetic modifications are a critical mechanism linking benzo[a]pyrene exposure to these multigenerational and transgenerational toxicity in bone and neural systems of both fish and rodents.</p></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 6","pages":"1837 - 1862"},"PeriodicalIF":20.4,"publicationDate":"2025-07-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145374748","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Accelerated carbonation of municipal waste fly ash for carbon sequestration: a review 城市垃圾飞灰加速碳化固碳研究进展
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-07-17 DOI: 10.1007/s10311-025-01866-z
Fikret Muge Alptekin, Alessandra Zanoletti, Laura E. Depero, Elza Bontempi
{"title":"Accelerated carbonation of municipal waste fly ash for carbon sequestration: a review","authors":"Fikret Muge Alptekin,&nbsp;Alessandra Zanoletti,&nbsp;Laura E. Depero,&nbsp;Elza Bontempi","doi":"10.1007/s10311-025-01866-z","DOIUrl":"10.1007/s10311-025-01866-z","url":null,"abstract":"<div><p>The accelerating climate change requires rapid techniques to both sequester carbon dioxide and recycle solid waste. Here we review the accelerated carbonation of fly ash from municipal solid waste with emphasis on carbonation methods, carbon dioxide sequestration capability, influence of carbonation on fly ash properties, fly ash as a cementitious material, non-conventional uses of fly ash, environmental and economic benefits, mixing with other waste materials, pilot and industrial applications, and limitations. We observe that the accelerated carbonation of fly ash allows for carbon dioxide capture of up to 0.24 g CO<sub>2</sub> per gram of ash, reduces heavy metal leaching, facilitates the reuse of stabilized ashes, and generates materials suitable for a wide range of uses. Limitations include possible pH-induced remobilization of toxic metals such as cadmium, chromium, and antimony.</p></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 6","pages":"1661 - 1687"},"PeriodicalIF":20.4,"publicationDate":"2025-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145374974","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Photocatalytic inactivation and disinfection of bioaerosols: a review 生物气溶胶的光催化灭活与消毒研究进展
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-07-05 DOI: 10.1007/s10311-025-01863-2
Amit Kumar, Piyush Verma, Ravinder Kaushik
{"title":"Photocatalytic inactivation and disinfection of bioaerosols: a review","authors":"Amit Kumar,&nbsp;Piyush Verma,&nbsp;Ravinder Kaushik","doi":"10.1007/s10311-025-01863-2","DOIUrl":"10.1007/s10311-025-01863-2","url":null,"abstract":"<div><p>Bioaerosols represent a major health issue because they contain viruses, bacteria, biological fragments or residues and fungal spores. Humans are exposed to nearly 10<sup>4</sup> viable bacteria and 10<sup>4</sup> viable fungi per cubic metre of indoor air. Here, we review bioaerosols with emphasis on their sources, behaviour, detection methods, mitigation, transmission, and photocatalytic disinfection. Disinfection methods include fibrous photocatalytic membranes with interception efficiency comparable to commercial masks and high bactericidal efficiency, Z-scheme and S-scheme heterojunctions-based materials, biofilms loaded with composite catalysts, and photocatalytic filters coupled with air ionizers. Bioaerosols inactivation reaches 99.99% in 4 h under ultraviolet light, and 99.3% in 14.1 s under visible light using advanced heterojunction photocatalysts.</p></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 6","pages":"1777 - 1799"},"PeriodicalIF":20.4,"publicationDate":"2025-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145374857","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The soil microbial carbon pump for carbon sequestration 土壤微生物碳泵用于固碳
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-07-03 DOI: 10.1007/s10311-025-01861-4
Longkai Qiao, Junfei Wang, Shuangshuang Wei, Yilong Ren, Eric Lichtfouse, Jie Han
{"title":"The soil microbial carbon pump for carbon sequestration","authors":"Longkai Qiao,&nbsp;Junfei Wang,&nbsp;Shuangshuang Wei,&nbsp;Yilong Ren,&nbsp;Eric Lichtfouse,&nbsp;Jie Han","doi":"10.1007/s10311-025-01861-4","DOIUrl":"10.1007/s10311-025-01861-4","url":null,"abstract":"","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 5","pages":"1145 - 1151"},"PeriodicalIF":20.4,"publicationDate":"2025-07-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145142155","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Remediation of heavy metal-contaminated soils by washing with green compost humic substances 绿色腐殖质堆肥对重金属污染土壤的修复作用
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-06-23 DOI: 10.1007/s10311-025-01857-0
Ilwan Meignant, Lavinia M. Stancampiano, Mariavittoria Verrillo, Zohreh Barzgar, Antonio G. Caporale, Charlotte Brun, Riccardo Spaccini, Maxime C. Bridoux
{"title":"Remediation of heavy metal-contaminated soils by washing with green compost humic substances","authors":"Ilwan Meignant,&nbsp;Lavinia M. Stancampiano,&nbsp;Mariavittoria Verrillo,&nbsp;Zohreh Barzgar,&nbsp;Antonio G. Caporale,&nbsp;Charlotte Brun,&nbsp;Riccardo Spaccini,&nbsp;Maxime C. Bridoux","doi":"10.1007/s10311-025-01857-0","DOIUrl":"10.1007/s10311-025-01857-0","url":null,"abstract":"<div><p>Remediation of metal-contaminated soils by aqueous washing is actually done using synthetic surfactants, calling for safer alternatives such as biosurfactants. Here we tested coffee-based humic substances extracted from various composts for soil washing of agricultural, industrial and urban soils contaminated by heavy metals. Molecular-level characterization of humic substances was done by <sup>13</sup>C-nuclear magnetic resonance and thermochemolysis gas chromatography-mass spectrometry. Following washing, we measured heavy metals displacement into humic substance suprastructures by inductively coupled plasma mass spectrometry. Humic substance molecular changes were observed by ultrahigh resolution Orbitrap mass spectrometry. Soil toxicity was studied using the Microtox® <i>Aliivibrio fischeri</i> bioluminescence system. Results show that metal removal reached 90% for antimony, 15% for copper, and 13% for zinc. Moreover, toxicity was reduced by up to 62% for industrial soils, 50% for urban soils, and 46% for agricultural soils. The metal removal could be explained by chelation with humic pentacyclic terpenes.</p></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 6","pages":"1453 - 1460"},"PeriodicalIF":20.4,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10311-025-01857-0.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145374854","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Coupled biological and chemical catalysis for jet biofuel production: a review 生物化学耦合催化用于喷气生物燃料生产的研究进展
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-06-12 DOI: 10.1007/s10311-025-01853-4
Arslan Sarwar, My Ha Tran, Tin Hoang Trung Chau, Diep Ngoc Pham, Eun Yeol Lee
{"title":"Coupled biological and chemical catalysis for jet biofuel production: a review","authors":"Arslan Sarwar,&nbsp;My Ha Tran,&nbsp;Tin Hoang Trung Chau,&nbsp;Diep Ngoc Pham,&nbsp;Eun Yeol Lee","doi":"10.1007/s10311-025-01853-4","DOIUrl":"10.1007/s10311-025-01853-4","url":null,"abstract":"<div><p>The use of fossil fuels in the aviation sector is accelerating global warming by emitting carbon dioxide into the atmosphere, calling for carbon neutral jet fuels. Unlike road transport, which is transitioning to electrification, aviation requires high-energy–density fuels, making liquid alternatives essential. Here we review the production of jet biofuels with emphasis on current production technologies, microbial engineering for lipid synthesis, catalytic conversion of lipids, and economic and life cycle assessment aspects. Microbial lipids, including free fatty acids, can be produced from various carbon sources such as sugars, lignocellulose, methane, methanol, and formate. Catalytic upgrading of lipids can be achieved by hydroprocessing, hydrodeoxygenation, hydrocracking, and hydroisomerization. Metabolic engineering strategies to enhance lipid biosynthesis include increasing the precursor supply, repressing β-oxidation, controlling fatty acid chain length, and applying systems-level optimization using flux balancing, biosensor-guided regulation, and evolutionary engineering. These strategies have enabled the production of 98.9 g lipids and 50 g free fatty acids per liter. <i>Pichia pastoris</i> employing methanol as a substrate can produce up to 23 g/L of free fatty acids. Catalytic upgrading via hydrodeoxygenation and hydrocracking achieves conversion efficiencies over 90% and jet fuel selectivity above 70%. Techno-economic and life cycle assessments indicate that microbial oil-based sustainable aviation fuels could be cost-competitive and environmentally favorable.</p></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 6","pages":"1543 - 1568"},"PeriodicalIF":20.4,"publicationDate":"2025-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145374852","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Molar absorption coefficients of water components under vacuum ultraviolet light, implications for pollutant degradation: a review 真空紫外光下水组分的摩尔吸收系数及其对污染物降解的影响
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-06-12 DOI: 10.1007/s10311-025-01851-6
Yuheng Chen, Boqiang Li, Huashe Ou, Madjid Mohseni, Wen-long Wang, Baiyang Chen
{"title":"Molar absorption coefficients of water components under vacuum ultraviolet light, implications for pollutant degradation: a review","authors":"Yuheng Chen,&nbsp;Boqiang Li,&nbsp;Huashe Ou,&nbsp;Madjid Mohseni,&nbsp;Wen-long Wang,&nbsp;Baiyang Chen","doi":"10.1007/s10311-025-01851-6","DOIUrl":"10.1007/s10311-025-01851-6","url":null,"abstract":"<div><p>Vacuum ultraviolet light produces reactive species that can degrade aqueous organic pollutants. Here we review the methods for measuring the molar absorption coefficients at 185 nm, the absorption coefficients of water components, and the effect of wavelength, water pH, temperature, and concentration. We present absorption coefficients of water, dissolved gases, ions, organic compounds, oxidants and reductants. We observe that absorption of vacuum ultraviolet photons by trace-level pollutants is negligible. By contrast, absorption of vacuum ultraviolet photons by inorganic compounds such as nitrate and chloride, and by oxidants or reductants, e.g. chlorine and sulfite, are pronounced and often overlooked. Increasing the temperature favors water cleavage but disfavors vacuum ultraviolet absorption by other substances, hence diminishing direct photolysis. Unexpectedly, the molar absorption coefficients of many compounds such as potassium exhibit high variability among published reports.</p></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 6","pages":"1863 - 1876"},"PeriodicalIF":20.4,"publicationDate":"2025-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145374856","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Molecular properties of methylene blue, a common probe in sorption and degradation studies: a review 亚甲基蓝在吸附和降解研究中的分子性质综述
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-06-10 DOI: 10.1007/s10311-025-01856-1
Jean-Claude Bollinger, Eder C. Lima, Lotfi Mouni, Stefano Salvestrini, Hai Nguyen Tran
{"title":"Molecular properties of methylene blue, a common probe in sorption and degradation studies: a review","authors":"Jean-Claude Bollinger,&nbsp;Eder C. Lima,&nbsp;Lotfi Mouni,&nbsp;Stefano Salvestrini,&nbsp;Hai Nguyen Tran","doi":"10.1007/s10311-025-01856-1","DOIUrl":"10.1007/s10311-025-01856-1","url":null,"abstract":"<div><p>Methylene blue is a textile dye widely used as a reference probe in laboratory studies to set optimal removal conditions, yet reported physical properties of methylene blue are often erroneous. Here we review methylene blue properties with emphasis on erroneous or confusing literature data. We present molecular, biological, water solubility, spectroscopic, physicochemical and degradation properties, with focus on medicinal effects, lipophilicity, sorption, X-Ray diffraction, computed molecular structure, specific surface area, ultraviolet–visible, molar absorptivity, solvatochromism, pH, infrared, self-association, acid/base and redox behaviours, photocatalytic degradation, oxidative degradation, and biodegradation. </p></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 5","pages":"1403 - 1424"},"PeriodicalIF":20.4,"publicationDate":"2025-06-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10311-025-01856-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145143104","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Medicinal applications and environmental fate of antimicrobial peptides: a review 抗菌肽的药物应用和环境命运：综述
IF 20.4 2区 环境科学与生态学
Environmental Chemistry Letters Pub Date : 2025-06-09 DOI: 10.1007/s10311-025-01854-3
Owen Daniel, Thomas Thiebault, Elodie Guigon
{"title":"Medicinal applications and environmental fate of antimicrobial peptides: a review","authors":"Owen Daniel,&nbsp;Thomas Thiebault,&nbsp;Elodie Guigon","doi":"10.1007/s10311-025-01854-3","DOIUrl":"10.1007/s10311-025-01854-3","url":null,"abstract":"<div><p>Antimicrobial resistance is a major global issue endangering human, animal, and environmental health, calling for alternative antibiotics. Here, we review antimicrobial peptides with focus on their history, properties, medicinal use, clinical applications, and environmental fate. Antimicrobial peptides include glycopeptides, daptomycin, polymyxins, gramicidin, tyrocidine, and bacitracin. We present their environmental degradation pathways such as hydrolysis, photolysis, biodegradation, and adsorption, and their potential toxicity. Although antimicrobial peptides are increasingly used, their environmental occurrence and transformation products remain poorly known. In particular, emission sources such as wastewater treatment plants are poorly documented, and the influence of antimicrobial peptides on environmental antimicrobial resistance is still largely unknown.</p><h3>Graphical abstract</h3>\u0000<div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":541,"journal":{"name":"Environmental Chemistry Letters","volume":"23 6","pages":"1745 - 1776"},"PeriodicalIF":20.4,"publicationDate":"2025-06-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10311-025-01854-3.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145374855","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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