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Unveiling the Invisible: Multiscale Molecular Insights through Raman Imaging 揭示不可见：通过拉曼成像的多尺度分子洞察
IF 5.7
Chemical & Biomedical Imaging Pub Date : 2025-07-04 DOI: 10.1021/cbmi.5c00083
Sanjun Fan*,  and , Liang Luo*, 
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引用次数: 0
Spatially Resolving and Regulating Heterogeneity of Electronic Coupling at the Single Silver Nanoentity Level. 单银纳米实体水平上电子耦合的空间分辨与调控异质性。
IF 5.7
Chemical & Biomedical Imaging Pub Date : 2025-06-24 eCollection Date: 2025-09-22 DOI: 10.1021/cbmi.5c00035
Zhihui Wang, Yu-Ling Zou, Bo Jiang, Wei Wang, Hui Wang
{"title":"Spatially Resolving and Regulating Heterogeneity of Electronic Coupling at the Single Silver Nanoentity Level.","authors":"Zhihui Wang, Yu-Ling Zou, Bo Jiang, Wei Wang, Hui Wang","doi":"10.1021/cbmi.5c00035","DOIUrl":"10.1021/cbmi.5c00035","url":null,"abstract":"<p><p>Interfacial electron transfer governs electrochemical heterogeneity at the single-entity level. Herein, we investigated the electronic coupling event during electrodissolution processes of single silver nanoentities on a Au electrode through a synchronized electrochemical-optical tracking platform. By implementing strategic control of interfacial gap distances and electrolyte composition, a marked differentiation of single-particle reaction dynamics can be achieved. The integration of superlocalization methodology reveals position-correlated optical centroid shifts during electrodissolution processes, demonstrating heterogeneous oxidation dynamics arising from spatially nonuniform surface oxide formation. Crucially, SAM-mediated gap regulation enables the precise regulation of interfacial electric field enhancement. Our methodology resolves electronic coupling heterogeneity at subnanowire scale while proving molecular interlayer-dependent modulation of coupling lifetimes. This electrochemical-optical imaging strategy establishes nanoscale spatial mapping of electrochemical dynamics, quantitative correlation between interfacial structure and coupling efficiency, and real-time tracking of transient electronic states. These findings demonstrate the capability of advanced optical imaging methodologies in elucidating structure-activity relationships at nanoscale interfaces, providing mechanistic insights for single-entity electrochemistry and nanoscale energy conversion systems.</p>","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 9","pages":"636-642"},"PeriodicalIF":5.7,"publicationDate":"2025-06-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12458043/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145151922","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemical & Biomedical Imaging Pub Date : 2025-06-23
Yong Tian, Weigeng Huang, Zhijia Sheng, Dingyuan Yan*, Dong Wang* and Ben Zhong Tang*, 
{"title":"","authors":"Yong Tian,&nbsp;Weigeng Huang,&nbsp;Zhijia Sheng,&nbsp;Dingyuan Yan*,&nbsp;Dong Wang* and Ben Zhong Tang*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/cbmi.4c00108","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429116","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemical & Biomedical Imaging Pub Date : 2025-06-23
Maria Niora, Martin Dufva, Liselotte Jauffred* and Kirstine Berg-Sørensen*, 
{"title":"","authors":"Maria Niora,&nbsp;Martin Dufva,&nbsp;Liselotte Jauffred* and Kirstine Berg-Sørensen*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/cbmi.4c00088","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429122","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemical & Biomedical Imaging Pub Date : 2025-06-23
Bret A. Marckx, Hunter Maclennan and Ömer Özgür Capraz*, 
{"title":"","authors":"Bret A. Marckx,&nbsp;Hunter Maclennan and Ömer Özgür Capraz*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/cbmi.5c00003","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429123","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemical & Biomedical Imaging Pub Date : 2025-06-23
{"title":"","authors":"","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/imv003i006_1950127","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429126","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
MRI: A Dynamic Tool in Precision Medicine 核磁共振成像：精准医学的动态工具。
IF 5.7
Chemical & Biomedical Imaging Pub Date : 2025-06-23 DOI: 10.1021/cbmi.5c00080
Zheng Huang,  and , Deju Ye*, 
{"title":"MRI: A Dynamic Tool in Precision Medicine","authors":"Zheng Huang,&nbsp; and ,&nbsp;Deju Ye*,&nbsp;","doi":"10.1021/cbmi.5c00080","DOIUrl":"10.1021/cbmi.5c00080","url":null,"abstract":"","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 7","pages":"398–399"},"PeriodicalIF":5.7,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12308590/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144762328","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemical & Biomedical Imaging Pub Date : 2025-06-23
Kun Wu, Zhicong Chao, Subi Aji, Yu Zhu, Hongxia Zhao, Ying An, Huangxian Ju and Ying Liu*, 
{"title":"","authors":"Kun Wu,&nbsp;Zhicong Chao,&nbsp;Subi Aji,&nbsp;Yu Zhu,&nbsp;Hongxia Zhao,&nbsp;Ying An,&nbsp;Huangxian Ju and Ying Liu*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/cbmi.4c00111","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429127","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemical & Biomedical Imaging Pub Date : 2025-06-23
{"title":"","authors":"","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/imv003i006_1950128","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144343229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemical & Biomedical Imaging Pub Date : 2025-06-23
Xinlan Zhou, Xinzhong Ruan, Xingjiang Li, Weiyuan Xu, Xinhui Xiao, Aiyi Chen, Yinghui Ding, Jilai Zhang, Gengshen Mo, Yong Jian, Xinyang Wu, Fangfu Ye, Zhiqiang Wang*, Yi Li* and Lixiong Dai*, 
{"title":"","authors":"Xinlan Zhou,&nbsp;Xinzhong Ruan,&nbsp;Xingjiang Li,&nbsp;Weiyuan Xu,&nbsp;Xinhui Xiao,&nbsp;Aiyi Chen,&nbsp;Yinghui Ding,&nbsp;Jilai Zhang,&nbsp;Gengshen Mo,&nbsp;Yong Jian,&nbsp;Xinyang Wu,&nbsp;Fangfu Ye,&nbsp;Zhiqiang Wang*,&nbsp;Yi Li* and Lixiong Dai*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":53181,"journal":{"name":"Chemical & Biomedical Imaging","volume":"3 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":0.0,"publicationDate":"2025-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/cbmi.5c00012","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429124","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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