Science of the Total Environment最新文献

{"title":"Analysis of potential human accumulation differences and mechanisms of environmental new flame retardants: Based on in vitro experiments and theoretical calculations","authors":"Junchao Ma ,&nbsp;Chao Qin ,&nbsp;Juan Yan ,&nbsp;Chunyu Wang ,&nbsp;Yu Liu ,&nbsp;Zeming Wang ,&nbsp;Zekai Li ,&nbsp;Yanzheng Gao","doi":"10.1016/j.scitotenv.2025.178542","DOIUrl":"10.1016/j.scitotenv.2025.178542","url":null,"abstract":"<div><div>Hundreds of new flame retardants (NFRs) are widely used, causing environmental pollution and threating human health. In this study, based on the interaction of NFRs and human serum albumin (HSA), we assessed the differences in potential human accumulation of 8 NFRs including 1,2-Dibromo-4-(1,2-dibromoethyl)cyclohexane (TBECH), tetrabromobisphenol A bis(dibromopropyl ether) (TBBPA-DBPE), 2,4,6-tribromophenol (TBP), pentabromophenol (PBP), tri-n-butyl phosphate (TnBP), triphenyl phosphate (TPP), Tri(2-chloroethyl) phosphate (TCEP), and Tri(1,3-dichloro-2-propyl) phosphate (TDCP). All NFRs could bind to HSA and cause slight damage to its structure, suggesting their potential human accumulation ability. Notably, the binding pocket of site 1 was larger than that of site 2, so TBBPA-DBPE with a larger molecular volume exhibited a preference for binding to site 1 and other NFRs with smaller volume bound to site 2. Binding constant (<em>K</em>_A) analysis revealed that TBP and PBP had strongest potential human accumulation ability (<em>K</em>_A: 6.35 × 10⁶–7.84 × 10⁶ L/mol), followed by TnBP, TPP, TCEP, and TDCP (<em>K</em>_A: 3.50 × 10⁴–7.80 × 10⁴ L/mol), while TBBPA-DBPE and TBECH presented the lowest ability (<em>K</em>_A: 5.84 × 10³–8.05 × 10³ L/mol). Theoretical calculations demonstrated that the magnitude of <em>K</em>_A was attributed to the molecular volume and the size and distribution of NFRs' molecular surface electrostatic potential (MSEP). TBP and PBP with smaller molecular volumes exhibited evenly distributed positive and negative MSEP, facilitating their entry into the binding site and interact with HSA. In summary, this study elucidates the influence of pollutants' volume and the size and distribution of MSEP on the binding sites and <em>K</em>_A, providing a crucial theoretical basis for understanding the pollutants' potential human accumulation, which contributes to the screening and monitoring of new environmental pollutants.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178542"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142996675","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Molecular foundations for shear-induced dynamics of natural organic matter","authors":"Kathlyn N. Mealio ,&nbsp;Katherine E. Slamen ,&nbsp;Martha J.M. Wells ,&nbsp;Holly A. Stretz","doi":"10.1016/j.scitotenv.2025.178463","DOIUrl":"10.1016/j.scitotenv.2025.178463","url":null,"abstract":"<div><div>The overall objective of the present work was to quantify how shear, coupled with varying salt concentration, affected the particle size distribution and relaxation/aggregation behavior for various organic sources of nonliving natural organic matter (NNOM) in surface water. NNOM has been implicated as a conditioning agent leading to the formation of biofilms such as algae. NNOM is also a responsible in surface waters for facilitated transport of a variety of anthropogenic pollutants. These are NNOM surface-related phenomena, yet the variable surface area and surface composition of NNOM, which can change dependent on shear rate, is not discussed in the literature. NNOM polymer-like dynamics can interact with stream water velocity differences to determine the process and result of aggregation. The fundamental role of post-shear NNOM molecular structure and dynamic aggregation (self-assembly) is examined here alongside fresh (hydrological) versus mined (terrestrial) NNOM. Shear rate can be seen as a change in the velocities of streamlines in hydrology. In this early work, the response to shear rate for three types of NNOM was measured using a stress-controlled rheometer under varying conditions of ionic strength. Samples were studied for rheological response after a variety of pre-shear conditions, and data then coupled with surface composition data from previously reported fluorescence studies. Interestingly, a size class of 5 μm aggregates disappeared when Aldrich humic acid samples were treated with 0.3 M Ca²⁺. Evidence is also presented that the environmental samples flocculated at shear rates up to 400 s⁻¹, rather than exhibiting particle breakup, with implications for reducing NNOM surface area. Dynamic response of different NNOM sources was not the same, some sources showing evidence of self-assembly. The molecular response to shear may play an important role in understanding the surface area and composition of NNOM responsible for facilitated transport of pollutants and initiation of biofilms.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178463"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142996721","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Degradation mechanism of PGNa by the immobilized degrading enzymes from magnetic fermentation residue biochar","authors":"Sinan Zhang ,&nbsp;Zejian Wang ,&nbsp;Sheng Huang ,&nbsp;Jianmin Zhang ,&nbsp;Jiequn Wu ,&nbsp;Shiyong Wu","doi":"10.1016/j.scitotenv.2025.178432","DOIUrl":"10.1016/j.scitotenv.2025.178432","url":null,"abstract":"<div><div>The development of a method to efficiently remove high concentrations of penicillin G sodium (PGNa) from the environment is important for human and animal health and safety. In this study, the degradative enzymes were immobilized by adsorption using biochar from penicillin fermentation waste residue, which could efficiently remove PGNa (900 mg/L) from an aqueous solution, with a removal rate of 99.84 % within 20 min. The successful immobilization of the PGNa-degrading enzymes was verified by scanning electron microscopy, Fourier transform infrared spectroscopy and thermogravimetric analyzer. The adsorption mechanism of SAMB on the enzymes was also analyzed by adsorption kinetics and molecular docking calculations, which were mainly chemisorption and physisorption. By comparing with the free enzymes, the immobilized enzymes were found to have better thermal stability, pH adaptability, reusability, and storage stability. In addition, combined with the LC-MS analysis of the removal products, three removal pathways were postulated, including the reactions of β-lactam ring cleavage, decarboxylation, demethylation, deamidation, and oxidation. Finally, the toxicity of the removal products was evaluated using ECOSAR software, and the results showed that the intermediate products had low toxicity. This study is the first to use penicillin waste residue immobilized degradative enzymes to remove PGNa, and it provides a new low-cost option for remediation of PGNa contamination in the environment. It is important for the efficient degradation of residual PGNa in the environment.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178432"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142997873","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Unraveling the shifts in the belowground microbiota and metabolome of Pinus pinaster trees affected by forest decline","authors":"Ana V. Lasa ,&nbsp;Miriam López-Hinojosa ,&nbsp;Pablo J. Villadas ,&nbsp;Antonio José Fernández-González ,&nbsp;María Teresa Cervera ,&nbsp;Manuel Fernández-López","doi":"10.1016/j.scitotenv.2025.178486","DOIUrl":"10.1016/j.scitotenv.2025.178486","url":null,"abstract":"<div><div><em>Pinus pinaster</em> Aiton (maritime pine) stands are suffering a generalized deterioration due to different decline episodes throughout all its distribution area. It is well known that external disturbances can alter the plant associated microbiota and metabolome, which ultimately can entail the disruption of the normal growth of the hosts. Notwithstanding, very little is known about the shifts in the microbiota and the metabolome in pine trees affected by decline. The aim of our work was to unravel whether bacterial and fungal communities inhabiting the rhizosphere and root endosphere of <em>P. pinaster</em> trees with symptoms of decline and affected by <em>Matsucoccus feytaudi</em> in the National Park of Sierra Nevada (Granada, Spain) showed alterations in the structure, taxonomical profiles and associative patterns. We also aimed at deciphering potential changes in the rhizosphere and root metabolome. Trees infected by <em>M. feytaudi</em> and healthy individual harbored distinct microbial communities at both compositional and associative patterns. Unhealthy trees were enriched selectively in certain plant growth promoting microorganisms such as several ectomycorrhizal fungi (<em>Clavulina</em>) and <em>Streptomyces</em>, while other beneficial microorganisms (<em>Micromonospora</em>) were more abundant in unaffected pines. The rhizosphere of unhealthy trees was richer in secondary metabolites involved in plant defense than healthy pines, while the opposite trend was detected in root samples. The abundance of certain microorganisms was significantly correlated with several antimicrobial metabolites, thus, being all of them worthy of further isolation and study of their role in forest decline.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178486"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142997890","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Unveiling the P-solubilizing potential of bacteria enriched from natural colonies of Red Sea Trichodesmium spp.","authors":"Anna-Neva Visser ,&nbsp;Futing Zhang ,&nbsp;Lior Guttman ,&nbsp;Matan Masasa ,&nbsp;Siyuan Wang ,&nbsp;Coco Koedooder ,&nbsp;Yeala Shaked","doi":"10.1016/j.scitotenv.2025.178446","DOIUrl":"10.1016/j.scitotenv.2025.178446","url":null,"abstract":"<div><div>Phosphorus (P) is pivotal for all organisms, yet its availability is, particularly in the marine habitat, limited. Natural, puff-shaped colonies of <em>Trichodesmium</em>, a genus of diazotrophic cyanobacteria abundant in the Red Sea, have been demonstrated to capture and centre dust particles. While this particle mining strategy is considered to help evade nutrient limitation, details behind the mechanism remain elusive. This study explores P-solubilizing bacteria (PSB) residing within <em>Trichodesmium</em>'s associated microbial community, their potential contribution to the host, and the possible implications for P cycling in marine ecosystems. Bacterial enrichment on YBCII medium resulted in 28 enrichment cultures, primarily comprising bacterial families such as <em>Rhodobacteraceae</em>, <em>Alteromonadaceae</em> and <em>Burkholderiaceae</em>. Five enrichment cultures were further grown on hydroxyapatite, revealing their ability to consume and release Nitrogen and P while forming strong physical interactions with the mineral. A drop in pH was observed, indicating acid production as the primary P-solubilizing pathway. Co-cultivation experiments confirmed a positive effect on <em>Trichodesmium erythraeum</em> strain IMS101 growth by the presence of putative PSBs. These results reveal that the enriched bacteria exhibit significant P-solubilizing activity, thus potentially increasing the bioavailability of P in seawater. Thus, PSB could play a vital role in maintaining the P balance in the Red Sea, supporting the growth of <em>Trichodesmium</em> spp. and other marine organisms. Overall, our results contribute to a deeper understanding of the P cycle in the Red Sea and have implications for developing novel strategies for P management in marine ecosystems.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178446"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142997893","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Unveiling the role of saltmarshes as coastal potassium sinks: A perspective from porewater-derived potassium exchange","authors":"Zhengtao Sun ,&nbsp;Xiaogang Chen ,&nbsp;Peiyuan Zhu ,&nbsp;Yan Zhang ,&nbsp;Yijun Ren ,&nbsp;Libo Wang ,&nbsp;Ling Li","doi":"10.1016/j.scitotenv.2025.178535","DOIUrl":"10.1016/j.scitotenv.2025.178535","url":null,"abstract":"<div><div>Saltmarshes serve as repositories for various metal species, primarily due to vegetation removal and mineralization processes. However, the significance of potassium (K), one of the three major nutrients (nitrogen, phosphorus, and K) essential for plant growth, has often been overlooked, particularly in the context of saltmarshes where the mechanisms of K transport via porewater exchange remain poorly understood. To address this knowledge gap, we conducted field observations and laboratory analysis, and developed a ²²²Rn mass balance model to quantify K fluxes via porewater exchange under physical, biological, and anthropogenic drivers. Our findings revealed that saltmarshes function as highly effective K sinks, with porewater exchange rates ranging from 12.2 to 44.5 cm d⁻¹ and related K fluxes spanning −122 to −1260 mmol m⁻² d⁻¹. Interestingly, wet season K fluxes were found to be ∼4.3 times higher than those observed during the dry season. Moreover, we observed that wet season K fluxes peaked during the neap tide, while dry season K fluxes reached their maximum during the spring tide. This suggests that K transport via porewater exchange is influenced by both crab burrow bioturbation and spring-neap exchange mechanisms. In addition, anthropogenic activities, such as biomass burning, also impact K dynamics in addition to physical and biological drivers. Overall, our study highlights the pivotal role of porewater exchange in driving the K cycle within saltmarshes. This exchange mechanism not only facilitates plant growth but also contributes to important mineralogical processes, including cation exchange and reverse weathering, occurring within the saltmarsh ecosystems. By shedding light on the K cycle in saltmarshes, our research contributes to a better understanding of the functioning of coastal wetlands and their implications for the oceanic K budget.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178535"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142997898","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Evaluation of tomato brown rugose fruit virus as a microbial source tracking marker for human sewage in Thailand","authors":"Phongsawat Paisantham ,&nbsp;Supitchaya Theplhar ,&nbsp;Thitima Srathongneam ,&nbsp;Montakarn Sresung ,&nbsp;Skorn Mongkolsuk ,&nbsp;Kwanrawee Sirikanchana","doi":"10.1016/j.scitotenv.2025.178419","DOIUrl":"10.1016/j.scitotenv.2025.178419","url":null,"abstract":"<div><div>Tomato brown rugose fruit virus (ToBRFV) has emerged as a major plant pathogen with the potential to spread through contaminated wastewater, posing risks to agriculture and public health. This study evaluated ToBRFV as a human-specific microbial source tracking (MST) marker in Thailand, comparing its performance to crAssphage. Using qPCR assays, ToBRFV was detected in 62.5 % of building sewage samples (n = 16) and 100.0 % of wastewater treatment plant (WWTP) influent samples (n = 16). Notably, ToBRFV showed minimal cross-detection in non-human fecal samples (35 pooled samples), collected from cows, pigs, chickens, ducks, and goats, with only one detection in a pig fecal-source sample, demonstrating high specificity to human sewage. Concentrations in WWTP influent were significantly higher (mean: 5.19 ± 5.05; range: 3.96–5.62 log₁₀ copies/100 mL) than in building sewage (mean: 4.36 ± 4.40; range: 2.33–4.85 log₁₀ copies/100 mL) (p &lt; 0.001). ToBRFV concentrations were significantly lower than crAssphage in building sewage but higher in WWTP influents. Additionally, ToBRFV and crAssphage exhibited moderate correlations in both building sewage and WWTP influent samples. These results suggest that ToBRFV could serve as a valuable MST marker for identifying human contamination in water bodies, complementing established markers. While ToBRFV's broader utility across diverse geographic regions remains to be fully validated, this study highlights its potential as a reliable indicator of human sewage in environmental surveillance.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178419"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142997984","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"It's getting hot in here: Spatial impact of humidity on heat wave severity in the U.S.","authors":"Anuska Narayanan ,&nbsp;Mostafa Rezaali ,&nbsp;Erin L. Bunting ,&nbsp;David Keellings","doi":"10.1016/j.scitotenv.2025.178397","DOIUrl":"10.1016/j.scitotenv.2025.178397","url":null,"abstract":"","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178397"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142998003","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A review of effects of electromagnetic fields on ageing and ageing dependent bioeffects of electromagnetic fields","authors":"Xiaoxia Wei ,&nbsp;Yun Huang ,&nbsp;Chuan Sun","doi":"10.1016/j.scitotenv.2025.178491","DOIUrl":"10.1016/j.scitotenv.2025.178491","url":null,"abstract":"<div><div>Thanks to the progress of science and technology, human life expectancy has dramatically increased in the past few decades, but accompanied by rapid ageing of population, resulting in increased burden on society. At the same time, the living environment, especially the electromagnetic environment, has also greatly changed due to science and technology advances. The effect of artificial electromagnetic fields (EMFs) emitted from power lines, mobile phones, wireless equipment, and other devices on ageing and ageing-related diseases are receiving increasing attention. However, the information on the relationship between EMFs and ageing and ageing related susceptibility to EMFs is fragmentary, a review is needed. Only few studies directly investigate the effect of EMFs on ageing, and we reviewed the impact of EMFs on lifespan and cellular senescence to pry whether EMFs have an effect on ageing, and reviewed the age-dependent bioeffects and health impacts of EMFs to see whether ageing would affect biological susceptibility to EMFs. The results indicated that EMFs may have an effect on longevity and cellular senescence, but the results were inconsistent which may depend on EMF types (frequency, intensity, wave shape, etc.), species, and cell lines. Ageing has an impact on the biological or health effects of EMFs; however, the results differ depending on the EMF type and the endpoint or health outcome. Age-dependent changes in free radical metabolism, ion homeostasis, gene expression, enzyme activity, and tissue biophysical properties may be the reason; however, the underlying mechanisms are not fully elucidated.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178491"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142998089","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Addressing drivers and data gaps in Spain's non-compliance of drinking water quality standards","authors":"Delia M. Andries ,&nbsp;Alberto Garrido ,&nbsp;Lucia De Stefano","doi":"10.1016/j.scitotenv.2025.178412","DOIUrl":"10.1016/j.scitotenv.2025.178412","url":null,"abstract":"<div><div>In 2021 Spain passed a new law regarding the quality of drinking water, increasing the transparency and introducing a risk assessment approach to the catchment area, which ascribe to the shift in recent years in how drinking water management is understood in the European Union legislation. Good data quality is important to ensure the correct implementation of policies. We used the drinking quality data uploaded to Spain's National Drinking Water Information System to gauge the state of the drinking water reporting in Spain, the differences between rural urban and rural areas in both quality and reporting and identify which variables at catchment level influence the probability of a municipality incurring in drinking water quality non-compliance. Random forest modeling was used to assess the drivers of non-compliance, including environmental (e.g., land cover, lithology, climate, state of the water supply source) and demographic (e.g., tap water expenditure, population density) data.</div><div>We found that rural municipalities are more vulnerable both because of a lack of reporting but also because they have higher non-compliance rates for arsenic, microbiological and contaminants and nitrogen compounds (e.g. nitrate). We also found different spatial patterns of non-compliance according to each group of contaminants (e.g., microbiological violations are widespread in the northern half of Spain). The random forest model suggests that agriculture and confined livestock farming are behind nitrogen and microbiological non-compliances. Climate drivers have also emerged for all the groups of contaminants, which underscores the importance of studying drinking water quality non-compliance on a case-by-case basis in order to properly adapt to local realities and enhance compliance across Spain.</div></div>","PeriodicalId":422,"journal":{"name":"Science of the Total Environment","volume":"963 ","pages":"Article 178412"},"PeriodicalIF":8.2,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142998092","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}