IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.10.020

Lu Song , Ruiyan Guo , Li Pan , Yishakejiang Saimaiti , Shaopeng Wang , Fan Li , Xiuhai Mao , Fei Wang , Qi Li , Dekai Ye , Sisi Jia , Gang Liu , Min Li , Xiaolei Zuo , Chunhai Fan

{"title":"Massively multiplexed optical recording with polychromatic DNA frameworks","authors":"Lu Song , Ruiyan Guo , Li Pan , Yishakejiang Saimaiti , Shaopeng Wang , Fan Li , Xiuhai Mao , Fei Wang , Qi Li , Dekai Ye , Sisi Jia , Gang Liu , Min Li , Xiaolei Zuo , Chunhai Fan","doi":"10.1016/j.matt.2024.10.020","DOIUrl":"10.1016/j.matt.2024.10.020","url":null,"abstract":"<div><div>Rapid data growth highlights the increasing demand for high-density storage solutions. Multiplexed optical recording based on synthetic inorganic nanoparticles represents the next generation of data storage. However, diverse photophysical properties of nanoparticles reduce their reliability and information density. Here, we present a highly programmable polychromatic DNA tetrahedral framework (PDTF) that enables precise control over their optical performances. By programming the size of PDTFs, we reduce the feature size of the recording medium to 3.4 nm, which was 41-fold smaller than that of commercially available Blu-ray technology. PDTF chains with up to 47 million distinct color codes further enhance optical storage with higher information capacity. Additionally, nanopatterning technology integrates the PDTFs into on-chip architectures, achieving an impressive density of 25.9 Gb/cm<sup>2</sup>. Finally, the PDTFs demonstrate excellent re-writability and long-term stability (10,826 years at room temperature), exhibiting promising potential in high-density and secure data storage applications.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101902"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142673718","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Atomic sulfur-bonded titanium carbide nanosheets for flexible piezoresistive sensor in monitoring sleep apnea syndrome 原子硫键合碳化钛纳米片用于监测睡眠呼吸暂停综合征的柔性压阻传感器

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.021

Yan Bai , Longlu Wang , Xiang Zou , Ning Ding , Yuhui Feng , Zhen You , Weiwei Zhao , Weikang Wang , Feifei Lin , Yuzhe Chen , Yijie Zhang , Jianmin Li , Fangyi Guan , Shujuan Liu , Wei Huang , Qiang Zhao

{"title":"Atomic sulfur-bonded titanium carbide nanosheets for flexible piezoresistive sensor in monitoring sleep apnea syndrome","authors":"Yan Bai , Longlu Wang , Xiang Zou , Ning Ding , Yuhui Feng , Zhen You , Weiwei Zhao , Weikang Wang , Feifei Lin , Yuzhe Chen , Yijie Zhang , Jianmin Li , Fangyi Guan , Shujuan Liu , Wei Huang , Qiang Zhao","doi":"10.1016/j.matt.2024.11.021","DOIUrl":"10.1016/j.matt.2024.11.021","url":null,"abstract":"<div><div>Flexible piezoresistive sensors have attracted great attention for the real-time monitoring of sleep apnea syndrome (SAS) through respiratory airflow. Although two-dimensional ultrathin Ti<sub>3</sub>C<sub>2</sub> is regarded as a promising piezoresistive material, its poor structural compressibility and antioxidation limit its practical applications. Here, an innovative atomic sulfur-bonded strategy is proposed to fabricate large-sized, crumpled, and antioxidative Ti<sub>3</sub>C<sub>2</sub>/Na<sub>2</sub>S (TS) flakes for preparing flexible piezoresistive sensors. The fundamental mechanism is rooted in the synergistic effect of lateral boundary assembly of Ti<sub>3</sub>C<sub>2</sub> nanosheets into large flakes (∼7 μm), lattice distortion to induce crumpled structures, and edge passivation by S<sup>2−</sup> ions to mitigate oxidation (105 days). The crumpled microstructure provides abundant voids for enhanced compressibility and contact site variability, resulting in a 5-fold sensitivity improvement over the Ti<sub>3</sub>C<sub>2</sub> sensor and an ultralow detection limit of 0.2 Pa. We demonstrate the practical application of highly sensitive and stable piezoresistive sensors integrated into a respiratory monitoring system for SAS detection.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101927"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142832467","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Multi-band luminescence from a rare earth-based two-dimensional material 基于稀土的二维材料的多波段发光

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.11.023

Rahul Rao , Emmanuel Rowe , Ryan Siebenaller , Jonathan T. Goldstein , Adam Alfieri , Bongjun Choi , Ryan Selhorst , Andrea N. Giordano , Jie Jiang , Christopher E. Stevens , Thuc T. Mai , Tyson C. Back , Ruth Pachter , Joshua R. Hendrickson , Deep Jariwala , Michael A. Susner

{"title":"Multi-band luminescence from a rare earth-based two-dimensional material","authors":"Rahul Rao , Emmanuel Rowe , Ryan Siebenaller , Jonathan T. Goldstein , Adam Alfieri , Bongjun Choi , Ryan Selhorst , Andrea N. Giordano , Jie Jiang , Christopher E. Stevens , Thuc T. Mai , Tyson C. Back , Ruth Pachter , Joshua R. Hendrickson , Deep Jariwala , Michael A. Susner","doi":"10.1016/j.matt.2024.11.023","DOIUrl":"10.1016/j.matt.2024.11.023","url":null,"abstract":"<div><div>Photoluminescence (PL) emission in two-dimensional (2D) materials is of great interest for nanophotonics applications. While excitonic emission has been observed in numerous 2D materials, tunable multi-band luminescence is rare. Here, we present single-crystalline AgErP<sub>2</sub>Se<sub>6</sub>, a 2D material that exhibits bright, multi-band PL emission from Er<sup>3+</sup> ions within the lattice. The emission bands cover a wide range (350–1,550 nm), with ultra-narrow (as low as 0.5 nm at room temperature) emission peaks and room temperature lifetimes up to ∼4 μs. The intensities of the PL emission bands from the single crystals depend strongly on temperature and pressure, enabling sensing over a wide temperature and pressure range. Furthermore, the PL persists in exfoliated flakes down to at least 11 nm thick and demonstrates thickness-dependent Purcell enhancement. This work establishes 2D AgErP<sub>2</sub>Se<sub>6</sub> as a multi-band luminescent emitter and sensor, poised to enable integration into a number of optoelectronic and nanophotonic applications.</div></div>","PeriodicalId":388,"journal":{"name":"Matter","volume":"8 2","pages":"Article 101929"},"PeriodicalIF":17.3,"publicationDate":"2025-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142833036","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Leveraging biomimetic materials for bioelectronics

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2025.101961

Junyi Yin , Shaolei Wang , Xiao Xiao , Farid Manshaii , Kamryn Scott , Jun Chen

引用次数: 0

Modulating hydration states of polymer micropores for ion-selective transport 调节聚合物微孔的水合状态以实现离子选择性传输

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2024.101953

Jing Guo , Yanqiu Zhang , Lu Shao

引用次数: 0

Unlocking the potential hidden in MXene layers through lignin-mediated intercalation

IF 17.3 1区材料科学

Matter Pub Date : 2025-02-05 DOI: 10.1016/j.matt.2025.101960

Qingxiao Zhang , Qinghua Yu , Xiuxia Meng , Naitao Yang , Hui Li

引用次数: 0

Guiding the rational design of biocompatible metal-organic frameworks for drug delivery

IF 18.9 1区材料科学

Matter Pub Date : 2025-01-29 DOI: 10.1016/j.matt.2025.101958

Dhruv Menon, David Fairen-Jimenez

引用次数: 0

Ultratransparent, stretchable, and durable electromagnetic wave absorbers

IF 18.9 1区材料科学

Matter Pub Date : 2025-01-24 DOI: 10.1016/j.matt.2024.101956

Runa Zhang, Bin Yuan, Fei Pan, Hongsheng Liang, Haojie Jiang, Hongtao Guo, Yongchao Rao, Shuhuai Zheng, Lingyang Ruan, Changsheng Wu, Yang Yang, Wei Lu

{"title":"Ultratransparent, stretchable, and durable electromagnetic wave absorbers","authors":"Runa Zhang, Bin Yuan, Fei Pan, Hongsheng Liang, Haojie Jiang, Hongtao Guo, Yongchao Rao, Shuhuai Zheng, Lingyang Ruan, Changsheng Wu, Yang Yang, Wei Lu","doi":"10.1016/j.matt.2024.101956","DOIUrl":"https://doi.org/10.1016/j.matt.2024.101956","url":null,"abstract":"The growing demand for soft robotics, smart displays, and optoelectronics has driven extensive research into expanding the palette of transparent, stretchable, and durable materials and devices. However, existing electromagnetic wave (EMW) absorbers lack one or more of these key attributes. Herein, we present an EMW absorber that combines ultratransparency (94%), high stretchability (824% fracture strain), and remarkable mechanical and environmental durability. This breakthrough is enabled by a phase-separated terpolymer ionogel. Its effective absorption bandwidth (EAB) of 7.85 GHz in the X and Ku bands significantly outperforms that of all other gel-based materials (<6 GHz) and ranks among the best of all absorbers, whether transparent, stretchable, or neither. This ionogel also demonstrates long-term stability alongside other fascinating properties such as hydrophobicity, skin-like modulus, fatigue and puncture resistance, ability to self-clean, and anti-freezing/icing capabilities. These findings add a key element to the palette, paving the way for next-generation transparent, stretchable devices and ionotronics.","PeriodicalId":388,"journal":{"name":"Matter","volume":"34 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143026845","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Stretchable, breathable, wearable batteries using a holey design

IF 18.9 1区材料科学

Matter Pub Date : 2025-01-24 DOI: 10.1016/j.matt.2025.101959

Lin Xu, Qiongyu Chen, Sumedha Vishalini Pichchamuttu, Lianping Wu, Elijah Pate, Christine Wu, Tangyuan Li, Xueying Zheng, Chong Yang, Kexia Jin, Ping Liu, Teng Li, Liangbing Hu

{"title":"Stretchable, breathable, wearable batteries using a holey design","authors":"Lin Xu, Qiongyu Chen, Sumedha Vishalini Pichchamuttu, Lianping Wu, Elijah Pate, Christine Wu, Tangyuan Li, Xueying Zheng, Chong Yang, Kexia Jin, Ping Liu, Teng Li, Liangbing Hu","doi":"10.1016/j.matt.2025.101959","DOIUrl":"https://doi.org/10.1016/j.matt.2025.101959","url":null,"abstract":"The rigid and non-breathable nature of conventional batteries has remained a significant limitation on wearable electronics, particularly in applications involving dynamic physical activities. Herein, we present a \"holey\" battery design, which is both breathable and deformable while maintaining high energy density and ease of fabrication. Guided by the finite element method (FEM), this design incorporates a strategic array of holes within a standard pouch cell framework that significantly enhances the battery’s breathability (twice as much as conventional cotton) and stretchability—maintaining robust electrochemical performance under 10% stretching deformation. Importantly, this architecture allows for a high areal energy density, achieving 7.2 mW h/cm<sup>2</sup> in a single-layer pouch, which is scalable to 14.4 mW h/cm<sup>2</sup> using double electrode layers. The battery is resilient under physical stress, including 10% diagonal stretching (>90% capacity) and 180° folding (>95% capacity), with quick recovery upon release, marking a significant advance in the field of e-textiles.","PeriodicalId":388,"journal":{"name":"Matter","volume":"71 4 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143027061","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Controlling stack pressure inhomogeneity in anode-free solid-state batteries using elastomeric interlayers 利用弹性中间层控制无阳极固态电池的堆压不均匀性

IF 18.9 1区材料科学

Matter Pub Date : 2025-01-23 DOI: 10.1016/j.matt.2024.101955

Micah A. Thorpe, Mengyao Zhang, Daniel W. Liao, Stephanie Elizabeth Sandoval, Younggyu Kim, Matthew T. McDowell, M.D. Thouless, Neil P. Dasgupta

{"title":"Controlling stack pressure inhomogeneity in anode-free solid-state batteries using elastomeric interlayers","authors":"Micah A. Thorpe, Mengyao Zhang, Daniel W. Liao, Stephanie Elizabeth Sandoval, Younggyu Kim, Matthew T. McDowell, M.D. Thouless, Neil P. Dasgupta","doi":"10.1016/j.matt.2024.101955","DOIUrl":"https://doi.org/10.1016/j.matt.2024.101955","url":null,"abstract":"“Anode-free” solid-state batteries (SSBs) can enable high energy densities through <em>in situ</em> formation of a lithium (Li)-metal anode. This work investigates the effects of inhomogeneous stack pressure on Li plating and stripping at the interface between a Li<sub>6</sub>PS<sub>5</sub>Cl solid electrolyte and copper current collector. Elastomeric interlayers are shown to promote a uniform pressure distribution, which can compensate for interfacial roughness and/or misalignment of the external plates used to apply stack pressure. Owing to the improved pressure uniformity, the Li plating coverage increases from 49% to 70% after charging to 2 mAh/cm<sup>2</sup>, and Coulombic efficiency increases from 89% to 94%. The interfacial stress distribution is quantified using finite-element simulations under different interlayer conditions. This work demonstrates that stack pressure should not be defined as a singular quantity but as a parameter that varies in space and time as cycling evolves. This highlights the importance of packaging and component design for SSBs.","PeriodicalId":388,"journal":{"name":"Matter","volume":"18 1","pages":""},"PeriodicalIF":18.9,"publicationDate":"2025-01-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143020943","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

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