Carbon EnergyPub Date : 2024-08-23DOI: 10.1002/cey2.601
Chenxiao Chu, Chunting Wang, Weisong Meng, Feipeng Cai, Bo Wang, Nana Wang, Jian Yang, Zhongchao Bai
{"title":"Interfacial chemistry and structural engineering modified carbon fibers for stable sodium metal anodes","authors":"Chenxiao Chu, Chunting Wang, Weisong Meng, Feipeng Cai, Bo Wang, Nana Wang, Jian Yang, Zhongchao Bai","doi":"10.1002/cey2.601","DOIUrl":"10.1002/cey2.601","url":null,"abstract":"<p>Sodium (Na) metal stands out as a highly promising anode material for high-energy-density Na batteries owing to its abundant resources and exceptional theoretical capacity at low redox potential. Nevertheless, the uncontrolled growth of Na dendrites and the accompanying volumetric changes during the plating/stripping process lead to safety concerns and poor electrochemical performances. This study introduces nitrogen and oxygen co-doped carbon nanofiber networks wrapped carbon felt (NO-CNCF), serving as Na deposition skeletons to facilitate a highly reversible Na metal anode. The NO-CNCF framework with uniformly distributed “sodiophilic” functional groups, nanonetwork protuberances, and cross-linked network scaffold structure can avoid charge accumulation and facilitate the dendrite-free Na deposition. Benefiting from these features, the NO-CNCF@Na symmetrical cells demonstrate notable enhancements in cycling stability, achieving 4000 h cycles at 1 mA cm<sup>−2</sup> for 1 mAh cm<sup>−2</sup> and 2400 h cycles at 2 mA cm<sup>−2</sup> for 2 mAh cm<sup>−2</sup> with voltage overpotential of approximately 6 and 10 mV, respectively. Furthermore, the NVP//NO-CNCF@Na full cells achieve stable cycling performance and favorable rate capability. This investigation offers novel insights into fabricating a “sodiophilic” matrix with a multistage structure toward high-performance Na metal batteries.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 12","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.601","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142211822","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Rich electron delocalization structure in carbon nitride inducing radical transfer for high-performance photocatalytic uranyl reduction","authors":"Zhangmeng Liu, Yayao Li, Shuaiqi Yao, Runchao Zhou, Guiting Lin, Yunzhi Fu, Qixin Zhou, Wei Wang, Weijie Chi","doi":"10.1002/cey2.636","DOIUrl":"10.1002/cey2.636","url":null,"abstract":"<p>Investigating the activation of the persulfate process through heterogeneous carbonaceous catalysts to expedite the reduction of uranyl ions (U(VI)) is imperative. The primary hurdle involves understanding the transfer and distribution of photogenerated carriers during the reduction process in this intricate system and deciphering the role of activated groups in promoting reduction efficiency. In this study, we strategically regulate the structure of polymeric carbon nitride to promote the N-doped state, thereby facilitating delocalization electron enrichment. The resulting active sites effectively activate peroxyl disulfate (PDS), generating radicals that expedite the selective reduction of U(VI). This strategic approach mitigates the inherent disadvantage of the short half-life of free radicals in persulfate-based advanced oxidation processes. As a consequence of our endeavors and with the simultaneous presence of PDS and hydrogen peroxide, we achieve an exceptional photoreduction efficiency of 100% within a remarkably short period of 20 min. This breakthrough presents a high-efficiency application with significant potential for addressing the pollution associated with uranyl-containing wastewater. Our findings not only contribute to the fundamental understanding of AOPs but also offer a practical solution with implications for environmental remediation.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 12","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.636","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142211858","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Carbon EnergyPub Date : 2024-08-23DOI: 10.1002/cey2.603
Xinlong Liu, Bingang Xu, Shenzhen Deng, Jing Han, Yongling An, Jingxin Zhao, Qingjun Yang, Yana Xiao, Cuiqin Fang
{"title":"Ion-sieving MXene flakes with quantum dots enable high plating capacity for dendrite-free Zn anodes","authors":"Xinlong Liu, Bingang Xu, Shenzhen Deng, Jing Han, Yongling An, Jingxin Zhao, Qingjun Yang, Yana Xiao, Cuiqin Fang","doi":"10.1002/cey2.603","DOIUrl":"10.1002/cey2.603","url":null,"abstract":"<p>The commercial utilization of Zn metal anodes with high plating capacity is significantly hindered by the uncontrolled growth of dendrites and associated side reactions. Herein, a robust artificial ion-sieving MXene flake (MXF)-coating layer, with abundant polar terminated groups, is constructed to regulate the interfacial Zn<sup>2+</sup> deposition behavior. In particular, the fragmented MXF coupled with in situ generated quantum dots not only has strong Zn affinity to homogenize electric fields but also generates numerous zincophilic sites to reduce nucleation energy, thus securing a uniform dendrite-free surface. Additionally, the porous coating layer with polar groups allows the downward diffusion of Zn<sup>2+</sup> to achieve bottom-up deposition and repels the excessive free water and anions to prevent parasitic reactions. The ion-sieving effect of MXF is firmly verified in symmetric cells with high areal capacity of 10–40 mAh cm<sup>−2</sup> (1.0 mA cm<sup>−2</sup>) and depth of discharge of 15%–60%. Therefore, the functional MXF-coated anode manifests long-term cycling with 2700 h of stable plating/stripping in Zn||Zn cell. Such rational design of MXF protective layer breaks new ground in developing high plating capacity zinc anodes for practical applications.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 10","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.603","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142211845","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Carbon EnergyPub Date : 2024-08-23DOI: 10.1002/cey2.578
Hun Kim, Jae-Min Kim, Ha-Neul Choi, Kyeong-Jun Min, Shivam Kansara, Jang-Yeon Hwang, Jung Ho Kim, Hun-Gi Jung, Yang-Kook Sun
{"title":"Improving reaction uniformity of high-loading lithium-sulfur pouch batteries","authors":"Hun Kim, Jae-Min Kim, Ha-Neul Choi, Kyeong-Jun Min, Shivam Kansara, Jang-Yeon Hwang, Jung Ho Kim, Hun-Gi Jung, Yang-Kook Sun","doi":"10.1002/cey2.578","DOIUrl":"10.1002/cey2.578","url":null,"abstract":"<p>Lithium-sulfur batteries (LSBs) have garnered attention from both academia and industry because they can achieve high energy densities (>400 Wh kg<sup>–1</sup>), which are difficult to achieve in commercially available lithium-ion batteries. As a preparation step for practically utilizing LSBs, there is a problem, wherein battery cycle life rapidly reduces as the loading level of the sulfur cathode increases and the electrode area expands. In this study, a separator coated with boehmite on both sides of polyethylene (hereinafter denoted as boehmite separator) is incorporated into a high-loading Li-S pouch battery to suppress sudden capacity drops and achieve a longer cycle life. We explore a phenomenon by which inequality is generated in regions where an electrochemical reaction occurs in the sulfur cathode during the discharging and charging of a high-capacity Li-S pouch battery. The boehmite separator inhibits the accumulation of sulfur-related species on the surface of the sulfur cathode to induce an even reaction across the entire cathode and suppresses the degradation of the Li metal anode, allowing the pouch battery with an areal capacity of 8 mAh cm<sup>–2</sup> to operate stably for 300 cycles. These results demonstrate the importance of customizing separators for the practical use of LSBs.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 11","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.578","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142211836","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Carbon EnergyPub Date : 2024-08-23DOI: 10.1002/cey2.611
Li-Feng Zhou, Jia-Yang Li, Jian Peng, Li-Ying Liu, Hang Zhang, Yi-Song Wang, Yameng Fan, Jia-Zhao Wang, Tao Du
{"title":"Advanced characterization techniques for phosphate cathodes in aqueous rechargeable zinc-based batteries","authors":"Li-Feng Zhou, Jia-Yang Li, Jian Peng, Li-Ying Liu, Hang Zhang, Yi-Song Wang, Yameng Fan, Jia-Zhao Wang, Tao Du","doi":"10.1002/cey2.611","DOIUrl":"10.1002/cey2.611","url":null,"abstract":"<p>Aqueous zinc-based batteries are emerging as highly promising alternatives to commercially successful lithium-ion batteries, particularly for large-scale energy storage in power stations. Phosphate cathodes have garnered significant research interest owing to their adjustable operation potential, electrochemical stability, high theoretical capacity, and environmental robustness. However, their application is impeded by various challenges, and research progress is hindered by unclear mechanisms. In this review, the various categories of phosphate materials as zinc-based battery cathodes are first summarized according to their structure and their corresponding electrochemical performance. Then, the current advances to reveal the Zn<sup>2+</sup> storage mechanisms in phosphate cathodes by using advanced characterization techniques are discussed. Finally, some critical perspectives on the characterization techniques used in zinc-based batteries and the application potential of phosphates are provided. This review aims to guide researchers toward advanced characterization technologies that can address key challenges, thereby accelerating the practical application of phosphate cathodes in zinc-based batteries for large-scale energy storage.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 10","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.611","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142227923","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Surface sulfidation constructing gradient heterojunctions for high-efficiency (approaching 18%) HTL-free carbon-based inorganic perovskite solar cells","authors":"Xiaonan Huo, Jinqing Lv, Kexiang Wang, Weiwei Sun, Weifeng Liu, Ran Yin, Yansheng Sun, Yukun Gao, Tingting You, Penggang Yin","doi":"10.1002/cey2.586","DOIUrl":"10.1002/cey2.586","url":null,"abstract":"<p>Due to the advantages of cost-effectiveness and tunable band gap, hole transport layer (HTL)-free CsPbI<sub><i>X</i></sub>Br<sub>3−<i>X</i></sub> carbon-based inorganic perovskite solar cells (C-IPSCs) are emerging candidates for both single junction and tandem solar cells. Because of the direct contact between the carbon electrode and the perovskite surface, energy barriers and defects at the interface limit the enhancement of power conversion efficiency (PCE). In this work, we first reported a preparation method of CsPbI<sub>2.75</sub>Br<sub>0.25</sub> HTL-free C-IPSCs and developed an effective surface sulfidation regulation (SSR) strategy to promote hole extraction and inhibit non-radiative recombination of inorganic perovskite by 2-(thiocyanomethylthio)benzothiazole (TCMTB) surface modification. The introduced S<sup>2−</sup> anions form strong binding with uncoordinated Pb ions, inhibit the perovskite degradation reaction, and effectively passivate the surface defects. In addition, PbS formed by the SSR strategy constructed a gradient heterojunction, which promoted the arrangement energy levels and enhanced hole extraction. An additional back-surface field is induced at the interface of perovskite by energy band bending, which increases the open-circuit voltage (V<sub>OC</sub>). As a result, the SSR-based CsPbI<sub>2.75</sub>Br<sub>0.25</sub> HTL-free C-IPSCs showed a PCE of 17.88% with a fill factor of 81.56% and V<sub>OC</sub> of 1.19 V, which was among the highest reported values of CsPbI<sub>2.75</sub>Br<sub>0.25</sub> HTL-free C-IPSCs.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 12","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.586","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142211857","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Low-temperature performance of Na-ion batteries","authors":"Meng Li, Haoxiang Zhuo, Qihang Jing, Yang Gu, Zhou Liao, Kuan Wang, Jiangtao Hu, Dongsheng Geng, Xueliang Sun, Biwei Xiao","doi":"10.1002/cey2.546","DOIUrl":"10.1002/cey2.546","url":null,"abstract":"<p>Sodium-ion batteries (NIBs) have become an ideal alternative to lithium-ion batteries in the field of electrochemical energy storage due to their abundant raw materials and cost-effectiveness. With the progress of human society, the requirements for energy storage systems in extreme environments, such as deep-sea exploration, aerospace missions, and tunnel operations, have become more stringent. The comprehensive performance of NIBs at low temperatures (LTs) has also become an important consideration. Under LT conditions, challenges such as increased viscosity of electrolyte, abnormal growth of solid electrolyte interface, and poor contact between collector and electrode materials emerge. The aforementioned issues hinder the diffusion kinetics of sodium ions (Na<sup>+</sup>) at the electrode/electrolyte interface and cause rapid degradation of battery performance. Consequently, the optimization of electrolyte composition and cathode/anode materials becomes an effective approach to improve LT performance. This review discusses the conduction behavior and limiting factors of Na<sup>+</sup> in both solid electrodes and liquid electrolytes at LT. Furthermore, it systematically reviews the recent research progress of LT NIBs from three aspects: cathode materials, anode materials, and electrolyte components. This review aims to provide a valuable reference for developing high-performance LT NIBs.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 10","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.546","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142211859","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Carbon EnergyPub Date : 2024-08-13DOI: 10.1002/cey2.580
Yuhang Zhang, Ya Han, Fengjun Deng, Tingyu Zhao, Ze Liu, Dongxu Wang, Jinlong Luo, Yingjian Yu
{"title":"Enhancement of the performance of Ge–air batteries under high temperatures using conductive MOF-modified Ge anodes","authors":"Yuhang Zhang, Ya Han, Fengjun Deng, Tingyu Zhao, Ze Liu, Dongxu Wang, Jinlong Luo, Yingjian Yu","doi":"10.1002/cey2.580","DOIUrl":"10.1002/cey2.580","url":null,"abstract":"<p>Germanium (Ge)–air batteries have gained significant attention from researchers owing to their high power density and excellent safety. However, self-corrosion and surface passivation issues of Ge anode limit the development of high-performance Ge–air batteries. In this study, conductive metal-organic framework (MOF) Ni<sub>3</sub>(HITP)<sub>2</sub> material was synthesized by the gas–liquid interface approach. The Ni<sub>3</sub>(HITP)<sub>2</sub> material was deposited on the surface of the Ge anode to prevent corrosion and passivation reactions inside the battery. At 16°C, the discharge time of Ge anodes protected with MOFs was extended to 59 h at 195 μA cm<sup>−2</sup>, which was twice that of bare Ge anodes. The positive effect of MOFs on Ge–air batteries at high temperatures was observed for the first time. The Ge@Ni<sub>3</sub>(HITP)<sub>2</sub> anodes discharged over 600 h at 65.0 μA cm<sup>−2</sup>. The experimental results confirmed that the two-dimensional conductive MOF material effectively suppressed the self-corrosion and passivation on Ge anodes. This work provides new ideas for improving the performance of batteries in extreme environments and a new strategy for anode protection in air batteries.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 11","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.580","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142211860","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Novel cable-like tin@carbon whiskers derived from the Ti2SnC MAX phase for ultra-wideband electromagnetic wave absorption","authors":"Feiyue Hu, Pei Ding, Fushuo Wu, Peigen Zhang, Wei Zheng, Wenwen Sun, Rui Zhang, Longzhu Cai, Bingbing Fan, ZhengMing Sun","doi":"10.1002/cey2.638","DOIUrl":"10.1002/cey2.638","url":null,"abstract":"<p>One-dimensional (1D) metals are well known for their exceptional conductivity and their ease of formation of interconnected networks that facilitate electron migration, making them promising candidates for electromagnetic (EM) attenuation. However, the impedance mismatch from high conductivity and their singular mode of energy loss hinder effective EM wave dissipation. Construction of cable structures not only optimizes impedance matching but also introduces a multitude of heterojunctions, increasing attenuation modes and potentially enhancing EM wave absorption (EMA) performance. Herein, we showcase the scalable synthesis of tin (Sn) whiskers from a Ti<sub>2</sub>SnC MAX phase precursor, followed by creation of a 1D tin@carbon (Sn@C) cable structure through polymerization of PDA on their surface and annealing in argon. The EMA capabilities of Sn@C significantly surpass those of uncoated Sn whiskers, with an effective absorption bandwidth reaching 7.4 GHz. Remarkably, its maximum radar cross section reduction value of 27.85 dB m<sup>2</sup> indicates its exceptional stealth capabilities. The enhanced EMA performance is first attributed to optimized impedance matching, and furthermore, the Sn@C cable structures have rich SnO<sub>2</sub>/C and Sn/SnO<sub>2</sub> heterointerfaces and the associated defects, which increase interfacial and defect-induced polarization losses, as visually demonstrated by off-axis electron holography. The development of the Sn@C cable structure represents a notable advancement in broadening the scope of materials with potential applications in stealth technology, and this study also contributes to the understanding of how heterojunctions can improve EMA performance.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 12","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.638","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142211861","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Carbon EnergyPub Date : 2024-08-02DOI: 10.1002/cey2.595
Hainan Sun, Xiaomin Xu, Gao Chen, Zongping Shao
{"title":"Perovskite oxides as electrocatalysts for water electrolysis: From crystalline to amorphous","authors":"Hainan Sun, Xiaomin Xu, Gao Chen, Zongping Shao","doi":"10.1002/cey2.595","DOIUrl":"10.1002/cey2.595","url":null,"abstract":"<p>Crystalline perovskite oxides are regarded as promising electrocatalysts for water electrolysis, particularly for anodic oxygen evolution reactions, owing to their low cost and high intrinsic activity. Perovskite oxides with noncrystalline or amorphous characteristics also exhibit promising electrocatalytic performance toward electrochemical water splitting. In this review, a fundamental understanding of the characteristics and advantages of crystalline, noncrystalline, and amorphous perovskite oxides is presented. Subsequently, recent progress in the development of advanced electrocatalysts for water electrolysis by engineering and breaking the crystallinity of perovskite oxides is reviewed, with a special focus on the underlying structure–activity relationships. Finally, the remaining challenges and unsolved issues are presented, and an outlook is briefly proposed for the future exploration of next-generation water-splitting electrocatalysts based on perovskite oxides.</p>","PeriodicalId":33706,"journal":{"name":"Carbon Energy","volume":"6 11","pages":""},"PeriodicalIF":19.5,"publicationDate":"2024-08-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cey2.595","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141885327","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}