Current Opinion in Chemical Engineering最新文献

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Techniques for kinetic parameter estimation in free radical polymerization models
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-03-12 DOI: 10.1016/j.coche.2025.101117
Lauren A Gibson, Kimberley B McAuley
{"title":"Techniques for kinetic parameter estimation in free radical polymerization models","authors":"Lauren A Gibson,&nbsp;Kimberley B McAuley","doi":"10.1016/j.coche.2025.101117","DOIUrl":"10.1016/j.coche.2025.101117","url":null,"abstract":"<div><div>Free radical polymerization (FRP) systems can have many reactions, leading to many kinetic parameters. The most common method to obtain values for kinetic parameters is weighted-least squares estimation, which uses multiple types of measured responses. Error-in-variables model estimation is used when there is significant uncertainty in the model inputs. When FRP models have many unknown parameters, it is difficult to estimate them all uniquely, so modelers often resort to model simplification or subset selection methods for parameter estimation. The aim of this review is to describe the most common techniques that modelers use for kinetic parameter estimation in FRP models.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101117"},"PeriodicalIF":8.0,"publicationDate":"2025-03-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143600530","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Recent trends in optimization models for industrial decarbonization
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-03-11 DOI: 10.1016/j.coche.2025.101118
Raymond R Tan , Maria Victoria Migo-Sumagang , Kathleen B Aviso
{"title":"Recent trends in optimization models for industrial decarbonization","authors":"Raymond R Tan ,&nbsp;Maria Victoria Migo-Sumagang ,&nbsp;Kathleen B Aviso","doi":"10.1016/j.coche.2025.101118","DOIUrl":"10.1016/j.coche.2025.101118","url":null,"abstract":"<div><div>The global call for deep decarbonization poses the critical challenge of cutting greenhouse gas emissions from industrial operations. Decarbonization can be achieved with a mix of strategies and technologies, but decision-support models are needed to help optimize their emissions reduction portfolios. This review surveys the development and use of models to support industrial decarbonization decisions and proposes a research roadmap for the future. Four key modeling challenges are identified: epistemic uncertainties inherent in new technologies, feedback loops between techno-economic performance and technology selection, the interplay between multiple decision-makers, and embedding within a broader decarbonization context.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101118"},"PeriodicalIF":8.0,"publicationDate":"2025-03-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143591531","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nanoplastic mitigation technologies: challenges and sustainability considerations
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-03-08 DOI: 10.1016/j.coche.2025.101107
Nisha Singh , Nitin Khandelwal , Ryota Nakajima , Amina K Stoddart , Graham A Gagnon
{"title":"Nanoplastic mitigation technologies: challenges and sustainability considerations","authors":"Nisha Singh ,&nbsp;Nitin Khandelwal ,&nbsp;Ryota Nakajima ,&nbsp;Amina K Stoddart ,&nbsp;Graham A Gagnon","doi":"10.1016/j.coche.2025.101107","DOIUrl":"10.1016/j.coche.2025.101107","url":null,"abstract":"<div><div>The rise of plastic pollution has led to widespread environmental contamination by their tiny fragments, posing alarming environmental threats and health risks. Nanoplastics, NPs (&lt;1000 nm) are particularly concerning due to their enhanced reactivity, potential to cross biological barriers and complex interactions with environmental matrices. Laboratory studies rely heavily on synthetic polystyrene beads, despite polystyrene constituting only 4.5% of global plastic production. Real-world NPs exist as hetero-aggregates with eco-corona layers, significantly altering their reactivity and toxicity. Furthermore, NPs interact with heavy metals and organic pollutants, modifying their fate and altering transport and remediation outcomes.</div><div>This perspective discusses the limitations of current water treatment plant (WTP) processes, highlighting emerging mitigation technologies, associated challenges, and the possibility of their incorporation into existing treatment settings. Enhanced adsorption, nano-enabled membrane filtration, photocatalytic degradation, magnetic microrobots, emulsions, deep eutectic solvents, and plasma technology show initial promise but face challenges like integration in existing treatment setups, high costs, regeneration difficulties, and potential for secondary pollution. Future research should focus on adapting mitigation techniques to diverse environmental matrices and their integration into existing setups, ensuring sustainability and resource recovery while achieving complete mineralization or recovery of NPs.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101107"},"PeriodicalIF":8.0,"publicationDate":"2025-03-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143578856","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A review of the application and future directions of high-power ultrasonic technology in environmental protection
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-03-04 DOI: 10.1016/j.coche.2025.101105
JunJie Ma , Juanjuan Wang , Fulei Xu , Xiaoge Wu
{"title":"A review of the application and future directions of high-power ultrasonic technology in environmental protection","authors":"JunJie Ma ,&nbsp;Juanjuan Wang ,&nbsp;Fulei Xu ,&nbsp;Xiaoge Wu","doi":"10.1016/j.coche.2025.101105","DOIUrl":"10.1016/j.coche.2025.101105","url":null,"abstract":"<div><div>This review delves into the growing importance of power ultrasonic technology in the field of environmental protection, with a focus on its applications in wastewater treatment. It discusses various commercial transducer types, including piezoelectric, MEMS-based, air-coupled, high-frequency thin-film, magnetostrictive, and hybrid transducers, each with distinct characteristics and specific applications. The paper further assesses the effectiveness of power ultrasound in water treatment and resource recycling. Although power ultrasonic technology is still in the developmental stage and faces challenges such as high initial costs and energy consumption, this review looks to the future by identifying potential directions, such as the combination of power ultrasound with other advanced processes like catalytic oxidation and ozonation to further enhance treatment efficiency. It also emphasizes the integration of artificial intelligence and machine learning for process optimization.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101105"},"PeriodicalIF":8.0,"publicationDate":"2025-03-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143550202","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Editorial overview: Digital design of pharmaceutical manufacturing processes
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-03-04 DOI: 10.1016/j.coche.2025.101108
Kimberley B McAuley , Jonathan P McMullen , Salvador Garcia Muñoz
{"title":"Editorial overview: Digital design of pharmaceutical manufacturing processes","authors":"Kimberley B McAuley ,&nbsp;Jonathan P McMullen ,&nbsp;Salvador Garcia Muñoz","doi":"10.1016/j.coche.2025.101108","DOIUrl":"10.1016/j.coche.2025.101108","url":null,"abstract":"","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101108"},"PeriodicalIF":8.0,"publicationDate":"2025-03-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143550312","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Membranes from upcycled waste plastics: current status, challenges, and future outlook
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-02-22 DOI: 10.1016/j.coche.2025.101106
Milad R Esfahani , Steven T Weinman
{"title":"Membranes from upcycled waste plastics: current status, challenges, and future outlook","authors":"Milad R Esfahani ,&nbsp;Steven T Weinman","doi":"10.1016/j.coche.2025.101106","DOIUrl":"10.1016/j.coche.2025.101106","url":null,"abstract":"<div><div>Plastic is ubiquitous across all aspects of modern life. Despite its usefulness, only 9% of all plastic waste ever produced has been recycled, leaving a tremendous amount that ends up in landfills and the environment. New strategies need to investigate using this waste plastic. This report analyzes upcycling waste plastics into membranes for water and gas separations. Polyethylene terephthalate, polystyrene, poly(vinyl chloride), polyethylene, polypropylene, and tire rubber have been studied for use as membranes. Future work needs to investigate greener solvents, health and safety aspects, costs, supply and demand, and life cycle assessments for upcycling plastic waste into membranes.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101106"},"PeriodicalIF":8.0,"publicationDate":"2025-02-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143464542","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Using advanced X-ray spectroscopy to reveal molecular level insights into water treatment
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-02-20 DOI: 10.1016/j.coche.2025.101103
Hande Demir , Pinar Aydogan Gokturk , Ethan J Crumlin
{"title":"Using advanced X-ray spectroscopy to reveal molecular level insights into water treatment","authors":"Hande Demir ,&nbsp;Pinar Aydogan Gokturk ,&nbsp;Ethan J Crumlin","doi":"10.1016/j.coche.2025.101103","DOIUrl":"10.1016/j.coche.2025.101103","url":null,"abstract":"<div><div>Water treatment technologies separate relevant solutes from water resources for water reuse, valuable resource recovery, and increasing the equity and availability of clean water worldwide. Although a variety of treatment methods exist, their performance needs to be improved to enable selective separation with increased durability and fouling resistance. To achieve this, we need to gain a better understanding of how molecular-level physics and chemistry impact integrated systems. Regarding current research on water treatment techniques, there is a clear need to study such systems under realistic environmental conditions. In this review, we aim to show that X-ray spectroscopic techniques are uniquely positioned to provide such information by obtaining detailed molecular insight into phenomena relevant to water research. By doing so, we hope to accelerate the rational design of novel treatment materials and processes. Specifically, a deeper understanding of the complex and interconnected phenomena that impact multilevel water treatment processes will lead to the successful development of next-generation water purification technologies.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101103"},"PeriodicalIF":8.0,"publicationDate":"2025-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143446075","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Tackling micro(nano)plastic pollution in aquaculture systems
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-02-19 DOI: 10.1016/j.coche.2025.101104
Camilla Mossotto , Alessandra Maganza , Alice Gabetti , Giuseppe Esposito , Caterina Faggio , Monia Renzi , Syed Shabi Ul Hassan Kazmi , Elena Bozzetta , Marino Prearo , Paolo Pastorino
{"title":"Tackling micro(nano)plastic pollution in aquaculture systems","authors":"Camilla Mossotto ,&nbsp;Alessandra Maganza ,&nbsp;Alice Gabetti ,&nbsp;Giuseppe Esposito ,&nbsp;Caterina Faggio ,&nbsp;Monia Renzi ,&nbsp;Syed Shabi Ul Hassan Kazmi ,&nbsp;Elena Bozzetta ,&nbsp;Marino Prearo ,&nbsp;Paolo Pastorino","doi":"10.1016/j.coche.2025.101104","DOIUrl":"10.1016/j.coche.2025.101104","url":null,"abstract":"<div><div>Micro(nano)plastics (MNPs) are emerging contaminants affecting aquaculture, a key global protein source. Their presence poses significant risks to aquatic ecosystems, farmed species, and human health through consumption of contaminated products. This mini-review highlights MNP contamination in aquaculture, focusing on detection methods, mitigation strategies, and future solutions. Aquaculture-derived MNPs are significant contributors to pollution, requiring innovative countermeasures such as biodegradable materials, advanced real-time detection technologies, and strengthened filtration systems. Future perspectives emphasize the urgent need for standardized, cost-effective MNP detection methods and the adoption of bio-based materials, balancing ecological benefits and environmental impacts. Nature-based solutions, such as plant-based filters, and eco-engineered strategies offer promising avenues to improve ecosystem resilience. Policymakers must establish regulatory frameworks to limit MNP pollution, integrate microplastics into food safety protocols, and promote sustainable practices. Long-term studies on human health risks are also critical to inform actionable interventions. Addressing MNP pollution in aquaculture requires global collaboration and technological innovation to ensure seafood safety, protect ecosystems, and reduce the industry’s environmental footprint.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101104"},"PeriodicalIF":8.0,"publicationDate":"2025-02-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143446076","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Prediction and assessment methods for sustainable solar energy systems within our planetary boundaries: how reliable are they?
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-02-18 DOI: 10.1016/j.coche.2025.101100
Natalia A. Cano-Londoño , Rebecca Saive , Tim Bekius , Laura Franco-García
{"title":"Prediction and assessment methods for sustainable solar energy systems within our planetary boundaries: how reliable are they?","authors":"Natalia A. Cano-Londoño ,&nbsp;Rebecca Saive ,&nbsp;Tim Bekius ,&nbsp;Laura Franco-García","doi":"10.1016/j.coche.2025.101100","DOIUrl":"10.1016/j.coche.2025.101100","url":null,"abstract":"<div><div>This study presents a critical analysis of the sustainability of solar energy systems within the planetary boundaries framework, which sets the limits within which humanity can safely operate. Given the substantial contribution of the energy sector to global greenhouse gas emissions, solar energy has emerged as a crucial element in the shift toward a sustainable energy future. Nevertheless, numerous challenges impede solar energy systems reaching optimal effectiveness, encompassing technological and methodological sustainable tools constraints, environmental impacts, and socioeconomic implications. This research aims to comprehensively assess these challenges and propose strategies to surmount them through applying a Life Cycle Sustainability Assessment approach. The primary research question addressed is, \"How reliable are the predictive and anticipatory assessment methods for sustainable solar energy systems within our planetary boundaries?\" The study integrated circular economy principles, criticality evaluation, and advanced technological tools to enhance solar energy systems’ efficiency, environmental performance, and socioeconomic benefits. By addressing the entire life cycle of solar technologies — from material extraction to end-of-life (cradle-to-grave) — this work seeks to contribute to developing more sustainable solar energy systems that operate within the safe limits of our planet’s boundaries. The findings highlight the need for a holistic approach that not only focuses on technological advancements but also considers the broader environmental and socioeconomic impacts to ensure a truly sustainable energy transition.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"48 ","pages":"Article 101100"},"PeriodicalIF":8.0,"publicationDate":"2025-02-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143436433","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Paving the way for green cross-linker substances for the fabrication of polymer membranes — a review
IF 8 2区 工程技术
Current Opinion in Chemical Engineering Pub Date : 2025-02-13 DOI: 10.1016/j.coche.2025.101097
Roberto Castro-Muñoz , Grzegorz Boczkaj
{"title":"Paving the way for green cross-linker substances for the fabrication of polymer membranes — a review","authors":"Roberto Castro-Muñoz ,&nbsp;Grzegorz Boczkaj","doi":"10.1016/j.coche.2025.101097","DOIUrl":"10.1016/j.coche.2025.101097","url":null,"abstract":"<div><div>Chemical cross-linking in membrane fabrication aims to face limitations of polymer membranes, including poor chemical resistance, low mechanical stability, swelling, etc. Typical cross-linkers do not fit green chemistry and sustainable principles due to their toxicity. Thus, this article discusses the successful application of green cross-linkers (including organic acids — citric, gallic, ferulic, and tannic acid, calcium chloride, deep eutectic solvents, pectin) and less toxic substances in polymer membranes (including biopolymeric ones based on chitosan or cellulose) fabrication. This article also mentions how to make it ‘greener’. Important areas for these developments include food biopackaging materials, 3D printing materials, and biomedical items.</div></div>","PeriodicalId":292,"journal":{"name":"Current Opinion in Chemical Engineering","volume":"47 ","pages":"Article 101097"},"PeriodicalIF":8.0,"publicationDate":"2025-02-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143403072","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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