npj Clean Water最新文献

{"title":"Machine learning reveals disruptive nutrient pollution shifts in Chinese rivers to 2100","authors":"Xiaoyue Zhang, Hong Zhang, Dingkun Yin, Baojing Gu, Lei Chen","doi":"10.1038/s41545-026-00571-w","DOIUrl":"https://doi.org/10.1038/s41545-026-00571-w","url":null,"abstract":"Anticipating nutrient pollution under changing conditions is urgent for water security. Nonetheless, high-resolution predictive frameworks capturing nonlinear driver responses remain limited. Here, we present a nationwide assessment of China’s water-quality evolution from 2023 to 2100, integrating over 3 million daily records with 41 climatic, landscape, and socioeconomic drivers via regionally tailored Random Forest models (R2 of 0.88–0.92). Our results reveal a disruptive spatiotemporal shift, with projected NPI ranges from –50.9% to +218.1% under SSP5-8.5. Seasonal patterns restructure toward unimodal peaks, with pollution increases in spring/autumn (up to 28.3%) but decreases in summer (up to 27.0%). Spatial homogenization emerges via a westward/southward shift of pollution centers, with localized increases exceeding 200% from coldspots with low baselines (<0.4 vs >1.0 in hotspots). Landscape configuration dominates (64.5% feature importance) over climatic forcing (7.2%–35.5%), reinforced by minimal climatic projection uncertainty. Strategic land-use planning could be a cornerstone of future water security.","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"4 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-03-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147536125","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Haloalkaliphilic archaea-mediated green synthesis of superparamagnetic Fe₃O₄ nanoparticles for electrochemical detection of ibuprofen in saline environments","authors":"Ghada E. Hegazy, Hussein Oraby, Mohamed Elnouby, Nadia A. Soliman, Tarek H. Taha, Yasser R. Abdel-Fattah","doi":"10.1038/s41545-026-00569-4","DOIUrl":"https://doi.org/10.1038/s41545-026-00569-4","url":null,"abstract":"The presence of pharmaceutical residues in aquatic systems poses a growing environmental concern, necessitating the development of sustainable and efficient sensing materials. In this study, haloalkaliphilic archaea were employed as green biocatalysts for the synthesis of magnetite (Fe₃O₄) nanoparticles and their application in the electrochemical detection of ibuprofen under saline conditions. Two archaeal strains produced Fe₃O₄ nanoparticles with well-defined inverse spinel crystal structures, nanoscale dimensions, and superparamagnetic behavior, while exhibiting distinct surface chemistry and magnetic properties. Strain-dependent differences in crystallinity and surface functionalization were found to strongly influence electrochemical performance. RA5-derived nanoparticles exhibited higher crystallinity and enhanced charge-transfer efficiency, achieving a sensitivity of 2.105 µA mg L⁻¹ and a limit of detection of 0.927 mg L⁻¹. In contrast, A6-derived nanoparticles featured a richer organic surface corona that promoted analyte adsorption, resulting in a sensitivity of 2.2186 µA mg L⁻¹ and a detection limit of 1.05 mg L⁻¹. Both modified electrodes enabled reliable ibuprofen detection over a wide linear concentration range of 0–100 mg L⁻¹. These results demonstrate that haloalkaliphilic archaea can function as sustainable nano-factories for producing functional magnetic nanomaterials, offering an eco-friendly strategy for electrochemical monitoring of pharmaceutical contaminants in complex aquatic environments.","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"52 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-03-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147506147","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Waste-to-sensor: high-sensitivity detection of heavy metals in water using Arc-ferrite/N-rGO nanocomposites from industrial and electronic waste","authors":"Aly Reda, Norhan Badr Eldin, Shahdan Abdelkareem, Nada M. Ali, Tamer Shoeib","doi":"10.1038/s41545-026-00567-6","DOIUrl":"https://doi.org/10.1038/s41545-026-00567-6","url":null,"abstract":"The escalating global crises of hazardous waste accumulation and heavy metal contamination demand innovative solutions that simultaneously address environmental remediation and analytical sensing needs. This study presents a sustainable electrochemical platform fabricated from industrial and electronic waste streams for the high-performance detection of notorious heavy metals. Herein, we repurposed arc furnace dust into ferrite nanoparticles and converted spent battery graphite into highly conductive nitrogen-doped reduced graphene oxide (N-rGO) through controlled synthesis processes. The resulting Arc-ferrite/N-rGO nanocomposite was integrated into a carbon paste electrode, demonstrating exceptional electrochemical performance with a 3.5-fold increase in faradaic current and significantly improved electron transfer kinetics compared to bare electrodes. Through comprehensive optimization of differential pulse voltammetry parameters, the optimal conditions were established as follows: an acetate-KCl buffer (pH 4.5), a deposition potential of -1.1 V, a scan rate of 50 mV/s, and a 180 s accumulation time. The sensor achieved remarkable analytical performance for simultaneous detection of cadmium (II), lead (II), and mercury (II) with detection limits of 1.01 – 1.13 ppb, well below WHO guidelines for drinking water. Excellent linearity (R² > 0.995) across a 10.0 – 150.0 ppb concentration range and superior selectivity against a 100-fold excess of eleven common interfering cations demonstrated the sensor’s robustness for real-world applications. The sensor enabled the simultaneous detection of Pb²⁺, Cd²⁺, and Hg²⁺ in industrial wastewater, with results cross-validated by microwave plasma atomic emission spectroscopy. This work establishes a powerful circular economy paradigm, transforming environmental liabilities into valuable analytical assets while addressing the dual challenges of waste management and environmental monitoring. The Arc-ferrite/N-rGO sensor represents a scalable, economically viable, and environmentally responsible solution for next-generation heavy metal detection systems.","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"27 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-03-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147496852","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Implementing wastewater surveillance for viral pathogens: lessons learned from SARS-CoV-2, monkeypox virus, norovirus and influenza A viruses","authors":"Aidan M. Nikiforuk, Muhammad Zohaib Anwar, James Kwan, Michael A. Irvine, Natalie A. Prystajecky, David A. McVea","doi":"10.1038/s41545-026-00570-x","DOIUrl":"https://doi.org/10.1038/s41545-026-00570-x","url":null,"abstract":"","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"55 37 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-03-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147506480","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Speciation of inorganic arsenic in oxic and in reducing groundwaters using the As(V)-selective ImpAs resin","authors":"Martijn Eikelboom, Jay Bullen, Peter S. K. Knappett, Trevor Ferris, Matthieu Carriere, Alexandra Alvarez, Dario Omanović, Subhamoy Bhowmick, Aaron Torres Huerta, Ramon Vilar, Jack N Turney, Paul Lewtas, Dominik Weiss, Pascal Salaün","doi":"10.1038/s41545-026-00564-9","DOIUrl":"https://doi.org/10.1038/s41545-026-00564-9","url":null,"abstract":"Knowledge of arsenic inorganic speciation in groundwaters is critical for optimising water treatment approaches. Here, we characterise the on-site analytical performance of the As(V)-selective ImpAs ion-exchange resin to separate As(V) from As(III) in groundwater with contrasting redox conditions. Field speciation results obtained by ImpAs in the oxic, Fe-poor groundwaters of Guanajuato (Mexico) and in the reducing, Fe-rich groundwaters of West Bengal (India) agreed with voltammetry (slope of 0.91 ± 0.03, r = 0.99, p < 0.001, n = 21). Like for arsenic, oxyanions of Mo, V, U and Cr are retained by ImpAs but their reduced hydroxy forms are not. High As(V) extraction by ImpAs (>95%) was obtained in synthetic groundwater for hundreds of samples without any regeneration, highlighting negligible interactions of major anions such as sulfate, a major advantage over common solid phase extraction resins. However, in Fe rich waters, ImpAs reusability is likely constrained by Fe accumulation in the resin and dissolved organic matter. This study demonstrates the successful application of ImpAs resin as a safe and easy to use analytical device for on-site separation of As(V) and As(III) in groundwaters, which opens the potential for including As inorganic speciation analysis into large scale monitoring programs.","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"60 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-03-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147496720","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"From data to policy: a systematic review of AI in water regulations and compliance","authors":"Yingjie Wang, Matthew Wilchek, Feras A. Batarseh","doi":"10.1038/s41545-026-00555-w","DOIUrl":"https://doi.org/10.1038/s41545-026-00555-w","url":null,"abstract":"Artificial intelligence (AI) algorithms are increasingly recognized for their transformative potential in water regulation and management. This systematic survey reviews 100+ peer-reviewed studies that applied AI-driven techniques to advance water policy across three critical policy domains: water pollution, drinking water, and infrastructure regulation. Using a novel multi-dimensional evaluation framework, this systematic review assesses the methodological rigor, policy integration, real-world applicability, AI assurance, and the socioeconomic or ethical impact of each reviewed study. The results reveal that AI applications in water governance are primarily dominated by machine-learning and neural-network methods, focusing on pollution control and infrastructure optimization. In contrast, far fewer studies employ causal, reinforcement-learning, or decision-support approaches that directly engage with policy evaluation. Despite technical advancements, only 18% incorporated assurance elements such as explainability, fairness, or trustworthiness, underscoring the need for more transparent and deployable AI in water governance. This review synthesizes global research efforts and outlines key opportunities and challenges. In response, it outlines future research directions that emphasize policy-aware decision-support systems, the advancement of trustworthy and explainable AI assurance frameworks, and the systematic incorporation of socioeconomic and ethical considerations to strengthen accountability and equity in water governance.","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"33 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-03-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147454758","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Temporal insights into electromagnetic field-tuned scaling pathways of CaCO3 and CaSO4•2H2O during reverse osmosis desalination of real brackish water","authors":"Xuewei Du, Helani Perera, Thilini Ranasinghe, Wenbin Jiang, Yanxing Wang, Fangjun Shu, Huiyao Wang, Ke Yuan, Lawrence M. Anovitz, Paul Ben Ishai, Pei Xu","doi":"10.1038/s41545-026-00565-8","DOIUrl":"https://doi.org/10.1038/s41545-026-00565-8","url":null,"abstract":"Electromagnetic field (EMF) treatment is a promising nonchemical strategy for scale control in reverse osmosis (RO) desalination; however, the mechanisms by which it influences polymorph selection and competitive precipitation in multi-ionic waters remain poorly understood. Here, we present the first detailed temporal analysis of scale formation, elucidating how EMF alters CaCO₃ and gypsum scaling in multi-ionic, Mg-bearing brackish groundwater (Mg/Ca = 0.67). Without EMF, aragonite and Mg-calcite co-precipitated, consistent with Mg²⁺-mediated inhibition of calcite growth. EMF accelerated bulk crystallization, amplified Mg²⁺ suppression of calcite, and drove an almost complete shift toward aragonite precipitation while maintaining elevated Mg/Ca ratios. EMF also mitigated gypsum scaling by promoting early, uniform CaCO₃ precipitation, reducing free Ca²⁺ availability, and delaying gypsum nucleation during initial concentration stages. At high gypsum supersaturation, precipitation occurred under both EMF and control conditions; however, EMF produced more porous and loosely adherent gypsum deposits. This dual effect—favoring aragonite formation and delaying or modifying gypsum deposition—resulted in more uniform, easily removable scaling layers. Although short-term flux improvements were modest, these mechanistic shifts enhance long-term membrane performance and cleanability, particularly when combined with hydraulic flushing.","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"226 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-03-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147381755","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Recirculation of powdered activated carbon improves the adsorption of organic micropollutants in membrane hybrid processes","authors":"Max Zimmermann, Christian Staaks, Michael Hoffmann, Thomas Wintgens, Benedikt M. Aumeier","doi":"10.1038/s41545-026-00561-y","DOIUrl":"https://doi.org/10.1038/s41545-026-00561-y","url":null,"abstract":"In this pilot study, we investigated how the counter-current of powdered activated carbon (PAC) improved the removal of organic micropollutants in two membrane hybrid processes. Comparing an inline-dosing process with fine or conventional PAC with a state-of-the-art contact reactor process that uses conventionally sized PAC. Recirculation of partially loaded fine PAC from the inline-dosing membrane hybrid process to the upstream biological treatment reduced the necessary carbon dosage to meet EU requirements for organic micropollutant removal from 1.4 mgPAC/mgDOC down to 0.7 mgPAC/mgDOC. Therefore, the counter-current flow reduced the carbon demand of the inline-dosing process by 50%. At the same time, the fine PAC inline-dosing process reached an even lower carbon demand than the reference process, which required dosages of 1.0 mgPAC/mgDOC. We also determined where and at what timescale adsorption takes place with and without PAC recirculation. The reduction of micropollutants in PAC counter-current schemes is shifting toward the activated sludge process. In this study, we demonstrated the relevance of process configuration as compared to material selection, and particularly the importance of recirculation of PAC in real applications. We also proposed a way to transfer previous lab- or pilot-scale results (without PAC recirculation) to real applications with PAC recirculation.","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"129 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-02-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147320159","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Agricultural water use efficiency and land-use intensity dominate the water-food-ecology nexus coupling coordination in the Lake Victoria Basin","authors":"Tengwen Wang, Jiayao Shu, Maurice Mugabowindekwe, Yifan Lin, Danfei Zhong, Jiansheng Wu, Gaspard Rwanyiziri, Jian Peng","doi":"10.1038/s41545-026-00563-w","DOIUrl":"https://doi.org/10.1038/s41545-026-00563-w","url":null,"abstract":"Water, food, and ecology are closely interconnected and are essential for regional development and human well-being, forming the water-food-ecology (WFE) nexus. However, knowledge about progress towards sustainable development of the WFE nexus at the basin scale remains largely unavailable. This study constructed an evaluation system to assess the WFE nexus in the Lake Victoria Basin (LVB) aligning with the Sustainable Development Goals (SDGs). The spatio-temporal dynamics of WFE nexus coupling coordination were revealed using coupling coordination degree (CCD) model and spatial autocorrelation analysis. Then, the random forest algorithm was employed to identify key factors dominating the evolutionary patterns of CCD. The results showed that the water subsystem index decreased 4.55%, accompanied by growing spatial imbalance. In contrast, the food and ecology subsystem indices increased 45.45% and 33.33%, respectively, with reduced spatial imbalance. Besides, the mean coupling coordination level of WFE nexus improved from intermediate discoordination (CCD = 0.36) to basic coordination (CCD = 0.405), while the proportion of area reaching coordination increased from 36.34% to 51.66%. A cluster of high coupling coordination was maintained in the relatively more developed northeastern sub-basins of the LVB. In addition, social influencing factors dominated CCD across the basin, with agricultural water use efficiency and land-use intensity consistently ranking higher in importance than climate and vegetation variables, highlighting the closer association between human activities and WFE nexus coupling coordination. This study provided a feasible evaluation framework and improved understanding of the WFE nexus in great lake basins.","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"15 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-02-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147320188","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Beyond the flush: a review of wastewater circular systems","authors":"Mahesh Ganesapillai, Anil Kumar Vinayak, Aditya Tiwari, Anushka Darda, Kasvi Chindalia, Thangapandi Chellapandi","doi":"10.1038/s41545-026-00557-8","DOIUrl":"https://doi.org/10.1038/s41545-026-00557-8","url":null,"abstract":"","PeriodicalId":19375,"journal":{"name":"npj Clean Water","volume":"38 1","pages":""},"PeriodicalIF":11.4,"publicationDate":"2026-02-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146205412","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}