Light-Science & Applications最新文献

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Hybrid solar photovoltaic conversion and water desalination via quad-band fano-resonant optical coatings and superwicking cooling 通过四波段扇形谐振光学涂层和超排汗冷却实现太阳能光伏转换和海水淡化混合技术
Light-Science & Applications Pub Date : 2025-04-17 DOI: 10.1038/s41377-025-01796-z
Ran Wei, Tianshu Xu, Mingjiang Ma, Mohamed Elkabbash, Chunlei Guo
{"title":"Hybrid solar photovoltaic conversion and water desalination via quad-band fano-resonant optical coatings and superwicking cooling","authors":"Ran Wei, Tianshu Xu, Mingjiang Ma, Mohamed Elkabbash, Chunlei Guo","doi":"10.1038/s41377-025-01796-z","DOIUrl":"https://doi.org/10.1038/s41377-025-01796-z","url":null,"abstract":"<p>Hybrid Photovoltaic/Thermal (HPT) systems simultaneously convert solar energy into electrical power and thermal energy. These systems are attractive as they enable the thermal management of PV cells to maintain optimal operating temperatures and maximize the overall solar energy conversion. Despite their advantages, HPT systems have been limited to storing solar energy in the form of heat or simple water/space heating, thus restricting the broader application scope of HPT systems, particularly in regions with abundant solar energy. Here, we introduce a device that expands the scope of HPT applications by realizing a hybrid PV/ water desalination system, achieved through the integration of a Fano-resonant optical coating (FROC) onto a silicon substrate, which is turned superwicking via femtosecond laser surface patterning. This configuration allows a single-junction amorphous silicon solar cell to operate under higher solar concentrations with much less heat conversion, achieving a temperature reduction of 101 °C and an efficiency improvement of 335.7% compared to a standalone photovoltaic system under the solar concentration of 5. At the same time, the interfacial water desalination achieves a 2 <span>({kg}{m}^{-2}{h}^{-1})</span> high evaporation rate. Over a 12-hour cycle, our HPT system showed a consistent performance, demonstrating a combined solar conversion efficiency of 79.6%. The demonstrated superwicking-FROC will pave the way for widespread adoption of HPT systems particularly in sunny coastal regions.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"17 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143841467","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Large-scale cluster quantum microcombs 大规模集群量子微梳
Light-Science & Applications Pub Date : 2025-04-16 DOI: 10.1038/s41377-025-01812-2
Ze Wang, Kangkang Li, Yue Wang, Xin Zhou, Yinke Cheng, Boxuan Jing, Fengxiao Sun, Jincheng Li, Zhilin Li, Bingyan Wu, Qihuang Gong, Qiongyi He, Bei-Bei Li, Qi-Fan Yang
{"title":"Large-scale cluster quantum microcombs","authors":"Ze Wang, Kangkang Li, Yue Wang, Xin Zhou, Yinke Cheng, Boxuan Jing, Fengxiao Sun, Jincheng Li, Zhilin Li, Bingyan Wu, Qihuang Gong, Qiongyi He, Bei-Bei Li, Qi-Fan Yang","doi":"10.1038/s41377-025-01812-2","DOIUrl":"https://doi.org/10.1038/s41377-025-01812-2","url":null,"abstract":"<p>An optical frequency comb comprises a cluster of equally spaced, phase-locked spectral lines. Replacing these classical components with correlated quantum light gives rise to cluster quantum frequency combs, providing abundant quantum resources for measurement-based quantum computation, and multi-user quantum networks. We propose and generate cluster quantum microcombs within an on-chip optical microresonator driven by multi-frequency lasers. Through resonantly enhanced four-wave mixing processes, continuous-variable cluster states with 60 qumodes are deterministically created. The graph structures can be programmed into one- and two-dimensional lattices by adjusting the configurations of the pump lines, which are confirmed inseparable based on the measured covariance matrices. Our work demonstrates the largest-scale cluster states with unprecedented raw squeezing levels from a photonic chip, offering a compact and scalable platform for computational and communicational tasks with quantum advantages.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"37 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143836923","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Multi-wavelength optical information processing with deep reinforcement learning 利用深度强化学习进行多波长光学信息处理
Light-Science & Applications Pub Date : 2025-04-15 DOI: 10.1038/s41377-025-01846-6
Qiuquan Yan, Hao Ouyang, Zilong Tao, Meili Shen, Shiyin Du, Jun Zhang, Hengzhu Liu, Hao Hao, Tian Jiang
{"title":"Multi-wavelength optical information processing with deep reinforcement learning","authors":"Qiuquan Yan, Hao Ouyang, Zilong Tao, Meili Shen, Shiyin Du, Jun Zhang, Hengzhu Liu, Hao Hao, Tian Jiang","doi":"10.1038/s41377-025-01846-6","DOIUrl":"https://doi.org/10.1038/s41377-025-01846-6","url":null,"abstract":"<p>Multi-wavelength optical information processing systems are commonly utilized in optical neural networks and broadband signal processing. However, their effectiveness is often compromised by frequency-selective responses caused by fabrication, transmission, and environmental factors. To mitigate these issues, this study introduces a deep reinforcement learning calibration (DRC) method inspired by the deep deterministic policy gradient training strategy. This method continuously and autonomously learns from the system, effectively accumulating experiential knowledge for calibration strategies and demonstrating superior adaptability compared to traditional methods. In systems based on dispersion compensating fiber, micro-ring resonator array, and Mach-Zehnder interferometer array that use multi-wavelength optical carriers as the light source, the DRC method enables the completion of the corresponding signal processing functions within 21 iterations. This method provides efficient and accurate control, making it suitable for applications such as optical convolution computation acceleration, microwave photonic signal processing, and optical network routing.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"26 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143831687","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
J-type assembled Pt(IV)-coordinated carbon dots for near-infrared light-triggered pyroptosis 近红外光触发的j型组装Pt(IV)配位碳点
Light-Science & Applications Pub Date : 2025-04-15 DOI: 10.1038/s41377-025-01834-w
Dongbo Guo, Yijie Hou, Qin Xu, Bingzhe Wang, Tesen Zhang, Quansheng Cheng, Maohua Chen, Linxuan Huang, Guichuan Xing, Songnan Qu
{"title":"J-type assembled Pt(IV)-coordinated carbon dots for near-infrared light-triggered pyroptosis","authors":"Dongbo Guo, Yijie Hou, Qin Xu, Bingzhe Wang, Tesen Zhang, Quansheng Cheng, Maohua Chen, Linxuan Huang, Guichuan Xing, Songnan Qu","doi":"10.1038/s41377-025-01834-w","DOIUrl":"https://doi.org/10.1038/s41377-025-01834-w","url":null,"abstract":"<p>Near-infrared (NIR) light-triggered pyroptosis based on biocompatible Pt(IV)-coordinated nanomedicine for tumor precision therapy is challenging. Here, we disclose a supramolecular approach to construct a hollow-spherical supra-(carbon dots) (HS-Pt-CDs) via ultrasound-assisted J-type assembly of Pt(IV)-coordinated carbon dots (Pt-CDs). The peculiar assembling behaviors arise from the steric hindrance and lattice distortion in the bowl-like Pt-CDs caused by the coordination of Pt(IV) atoms among the sp<sup>2</sup> domains, which result in around 240 nm red-shifted absorption bands and promoting charge separation in the NIR region due to strong inter-molecular charge transfer (CT) in HS-Pt-CDs. The results reveal that HS-Pt-CDs exhibit excellent NIR light-activated photocatalytic capacities, involving the release of Pt(II) species, the generation of hydroxyl radicals, and acidification under 690 nm laser irradiation. Combined with the effective cellular uptake and tumor accumulation, HS-Pt-CDs can efficiently trigger cancer cell pyroptosis under 690 nm laser irradiation, resulting in the destruction of the primary tumor and effectively induction of strong immunogenic cell death (ICD), thereby evoking anti-tumor immune responses to suppress distant tumor and prevent cancer metastasis. Taken these merits, an important perspective of Pt(IV)-contained supra-CDs with outstanding NIR-triggered photocatalytic behaviors can be of great significance toward precision tumor phototherapy.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"24 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143831688","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Versatile optoelectronic memristor based on wide-bandgap Ga2O3 for artificial synapses and neuromorphic computing 基于Ga2O3的多功能光电忆阻器,用于人工突触和神经形态计算
Light-Science & Applications Pub Date : 2025-04-15 DOI: 10.1038/s41377-025-01773-6
Dongsheng Cui, Mengjiao Pei, Zhenhua Lin, Hong Zhang, Mengyang Kang, Yifei Wang, Xiangxiang Gao, Jie Su, Jinshui Miao, Yun Li, Jincheng Zhang, Yue Hao, Jingjing Chang
{"title":"Versatile optoelectronic memristor based on wide-bandgap Ga2O3 for artificial synapses and neuromorphic computing","authors":"Dongsheng Cui, Mengjiao Pei, Zhenhua Lin, Hong Zhang, Mengyang Kang, Yifei Wang, Xiangxiang Gao, Jie Su, Jinshui Miao, Yun Li, Jincheng Zhang, Yue Hao, Jingjing Chang","doi":"10.1038/s41377-025-01773-6","DOIUrl":"https://doi.org/10.1038/s41377-025-01773-6","url":null,"abstract":"<p>Optoelectronic memristors possess capabilities of data storage and mimicking human visual perception. They hold great promise in neuromorphic visual systems (NVs). This study introduces the amorphous wide-bandgap Ga<sub>2</sub>O<sub>3</sub> photoelectric synaptic memristor, which achieves 3-bit data storage through the adjustment of current compliance (<i>I</i><sub>cc</sub>) and the utilization of variable ultraviolet (UV-254 nm) light intensities. The “AND” and “OR” logic gates in memristor-aided logic (MAGIC) are implemented by utilizing voltage polarity and UV light as input signals. The device also exhibits highly stable synaptic characteristics such as paired-pulse facilitation (PPF), spike-intensity dependent plasticity (SIDP), spike-number dependent plasticity (SNDP), spike-time dependent plasticity (STDP), spike-frequency dependent plasticity (SFDP) and the learning experience behavior. Finally, when integrated into an artificial neural network (ANN), the Ag/Ga<sub>2</sub>O<sub>3</sub>/Pt memristive device mimicked optical pulse potentiation and electrical pulse depression with high pattern accuracy (90.7%). The single memristive cells with multifunctional features are promising candidates for optoelectronic memory storage, neuromorphic computing, and artificial visual perception applications.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"108 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143831689","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Physical twinning for joint encoding-decoding optimization in computational optics: a review 计算光学中编码-解码联合优化的物理孪生:综述
Light-Science & Applications Pub Date : 2025-04-15 DOI: 10.1038/s41377-025-01810-4
Liheng Bian, Xinrui Zhan, Rong Yan, Xuyang Chang, Hua Huang, Jun Zhang
{"title":"Physical twinning for joint encoding-decoding optimization in computational optics: a review","authors":"Liheng Bian, Xinrui Zhan, Rong Yan, Xuyang Chang, Hua Huang, Jun Zhang","doi":"10.1038/s41377-025-01810-4","DOIUrl":"https://doi.org/10.1038/s41377-025-01810-4","url":null,"abstract":"<p>Computational optics introduces computation into optics and consequently helps overcome traditional optical limitations such as low sensing dimension, low light throughput, low resolution, and so on. The combination of optical encoding and computational decoding offers enhanced imaging and sensing capabilities with diverse applications in biomedicine, astronomy, agriculture, etc. With the great advance of artificial intelligence in the last decade, deep learning has further boosted computational optics with higher precision and efficiency. Recently, there developed an end-to-end joint optimization technique that digitally twins optical encoding to neural network layers, and then facilitates simultaneous optimization with the decoding process. This framework offers effective performance enhancement over conventional techniques. However, the reverse physical twinning from optimized encoding parameters to practical modulation elements faces a serious challenge, due to the discrepant gap in such as bit depth, numerical range, and stability. In this regard, this review explores various optical modulation elements across spatial, phase, and spectral dimensions in the digital twin model for joint encoding-decoding optimization. Our analysis offers constructive guidance for finding the most appropriate modulation element in diverse imaging and sensing tasks concerning various requirements of precision, speed, and robustness. The review may help tackle the above twinning challenge and pave the way for next-generation computational optics.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"359 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143831911","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Tsang’s resolution enhancement method for imaging with focused illumination Tsang的聚焦照明成像分辨率增强方法
Light-Science & Applications Pub Date : 2025-04-11 DOI: 10.1038/s41377-025-01791-4
Alexander Duplinskiy, Jernej Frank, Kaden Bearne, A. I. Lvovsky
{"title":"Tsang’s resolution enhancement method for imaging with focused illumination","authors":"Alexander Duplinskiy, Jernej Frank, Kaden Bearne, A. I. Lvovsky","doi":"10.1038/s41377-025-01791-4","DOIUrl":"https://doi.org/10.1038/s41377-025-01791-4","url":null,"abstract":"<p>A widely tested approach to overcoming the diffraction limit in microscopy without disturbing the sample relies on substituting widefield sample illumination with a structured light beam. This gives rise to confocal, image scanning, and structured illumination microscopy methods. On the other hand, as shown recently by Tsang and others, subdiffractional resolution at the detection end of the microscope can be achieved by replacing the intensity measurement in the image plane with spatial mode demultiplexing. In this work, we study the combined action of Tsang’s method with image scanning. We experimentally demonstrate superior lateral resolution and enhanced image quality compared to either method alone. This result paves the way for integrating spatial demultiplexing into existing microscopes, contributing to further pushing the boundaries of optical resolution.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"3 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143819091","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
End-to-end design of multicolor scintillators for enhanced energy resolution in X-ray imaging 多色闪烁体的端到端设计,用于增强x射线成像中的能量分辨率
Light-Science & Applications Pub Date : 2025-04-11 DOI: 10.1038/s41377-025-01836-8
Seokhwan Min, Seou Choi, Simo Pajovic, Sachin Vaidya, Nicholas Rivera, Shanhui Fan, Marin Soljačić, Charles Roques-Carmes
{"title":"End-to-end design of multicolor scintillators for enhanced energy resolution in X-ray imaging","authors":"Seokhwan Min, Seou Choi, Simo Pajovic, Sachin Vaidya, Nicholas Rivera, Shanhui Fan, Marin Soljačić, Charles Roques-Carmes","doi":"10.1038/s41377-025-01836-8","DOIUrl":"https://doi.org/10.1038/s41377-025-01836-8","url":null,"abstract":"<p>Scintillators have been widely used in X-ray imaging due to their ability to convert high-energy radiation into visible light, making them essential for applications such as medical imaging and high-energy physics. Recent advances in the artificial structuring of scintillators offer new opportunities for improving the energy resolution of scintillator-based X-ray detectors. Here, we present a three-bin energy-resolved X-ray imaging framework based on a three-layer multicolor scintillator used in conjunction with a physics-aware image postprocessing algorithm. The multicolor scintillator is able to preserve X-ray energy information through the combination of emission wavelength multiplexing and energy-dependent isolation of X-ray absorption in specific layers. The dominant emission color and the radius of the spot measured by the detector are used to infer the incident X-ray energy based on prior knowledge of the energy-dependent absorption profiles of the scintillator stack. Through ab initio Monte Carlo simulations, we show that our approach can achieve an energy reconstruction accuracy of 49.7%, which is only 2% below the maximum accuracy achievable with realistic scintillators. We apply our framework to medical phantom imaging simulations where we demonstrate that it can effectively differentiate iodine and gadolinium-based contrast agents from bone, muscle, and soft tissue.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"39 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143819090","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Non-reciprocal response in silicon photonic resonators integrated with 2D CuCrP2S6 at short-wave infrared 硅光子谐振器中与二维 CuCrP2S6 集成的短波红外非互惠响应
Light-Science & Applications Pub Date : 2025-04-09 DOI: 10.1038/s41377-025-01826-w
Ghada Dushaq, Solomon Serunjogi, Srinivasa R. Tamalampudi, Mahmoud Rasras
{"title":"Non-reciprocal response in silicon photonic resonators integrated with 2D CuCrP2S6 at short-wave infrared","authors":"Ghada Dushaq, Solomon Serunjogi, Srinivasa R. Tamalampudi, Mahmoud Rasras","doi":"10.1038/s41377-025-01826-w","DOIUrl":"https://doi.org/10.1038/s41377-025-01826-w","url":null,"abstract":"<p>Achieving non-reciprocal optical behavior in integrated photonics with high efficiency has long been a challenge. Here, we demonstrate a non-reciprocal magneto-optic response by integrating multilayer 2D CuCrP<sub>2</sub>S<sub>6</sub> (CCPS) onto silicon microring resonators (MRRs). Under an applied magnetic field, the CCPS intralayer ferromagnetic ordering, characterized by easy-plane magneto-crystalline anisotropy, induces asymmetrical modal responses in the clockwise (CW) and counterclockwise (CCW) light propagation directions. The proposed configuration achieves a low insertion loss ranging from 0.15 dB to 1.8 dB and a high isolation ratio of 28 dB at 1550 nm. Notably, it exhibits a significant resonance wavelength splitting of 0.4 nm between the counter propagation directions, supporting a 50 GHz optical bandwidth. Operating directly in the transverse electric (TE) mode, it aligns with the main polarization used in silicon photonics circuits, eliminating the need for additional polarization management. The device is ultra-compact, with a 2D flake interaction length ranging from 22 µm to 55 µm and a thickness between 39 nm and 62 nm. Its operation range covers the entire C-band with a bandwidth of up to 100 nm. These attributes make our hybrid CCPS/Si device ideal for advanced non-reciprocal optical applications in the short-wave infrared (SWIR) spectrum, crucial for enhancing the resilience of optical systems against back-reflections.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"394 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143805871","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Exceptionally high brightness and long lifetime of efficient blue OLEDs for programmable active-matrix display 高亮度和长寿命的高效蓝色oled可编程有源矩阵显示
Light-Science & Applications Pub Date : 2025-04-09 DOI: 10.1038/s41377-025-01817-x
Chengcheng Wu, Kai-Ning Tong, Kefei Shi, Wei He, Manli Huang, Jie Yan, Siqi Li, Zhaoyun Jin, Xin Wang, Sinyeong Jung, Jingrui Ma, Yixi Zhuang, Rong-Jun Xie, Cunjiang Yu, Hong Meng, Xiao Wei Sun, Chuluo Yang, Yun Chi, Feiyu Kang, Guodan Wei
{"title":"Exceptionally high brightness and long lifetime of efficient blue OLEDs for programmable active-matrix display","authors":"Chengcheng Wu, Kai-Ning Tong, Kefei Shi, Wei He, Manli Huang, Jie Yan, Siqi Li, Zhaoyun Jin, Xin Wang, Sinyeong Jung, Jingrui Ma, Yixi Zhuang, Rong-Jun Xie, Cunjiang Yu, Hong Meng, Xiao Wei Sun, Chuluo Yang, Yun Chi, Feiyu Kang, Guodan Wei","doi":"10.1038/s41377-025-01817-x","DOIUrl":"https://doi.org/10.1038/s41377-025-01817-x","url":null,"abstract":"<p>Blue phosphorescent OLEDs (Ph-OLEDs) have long faced critical challenges in efficiency, stability and brightness, which are crucial for advanced display. Herein, we introduce two novel Ir(III) emitters featuring a 3,6-di(<i>tert</i>-butyl)-9H-carbazolyl (tBuCz) substituted tridentate carbene pincer ligand, significantly improving efficiency and stability. The <b>tBuCz-</b><b><i>m</i></b><b>-CF3</b> and <b>tBuCz-</b><b><i>p</i></b><b>-CF3</b> complexes are designed to enhance steric encumbrance and minimize exciton accumulation. These innovations lead to exceptional photoluminescence quantum yields (PLQY) of 98% and an impressive decay rate constant of 7.97 × 10<sup>5</sup> s<sup>−1</sup> in doped thin films. The Ph-OLEDs emit blue light with a peak wavelength of 485 nm and CIE coordinates of (0.175, 0.446), exhibiting a peak external quantum efficiencies (EQE) of 31.62% and brightness up to 214,255 cd m<sup>−2</sup>. Notably, they shown minimal efficiency roll-off, retaining an EQE of 27.76% at 10,000 cd m<sup>−2</sup>, and 20.58% at 100,000 cd m<sup>−2</sup>. These consistent performances across various brightness levels represent a significant milestone for blue Ph-OLED technology. The devices also exhibit impressive stability, with an operational lifetime (LT<sub>50</sub>, the time taken for luminance to decrease by 50%) reaching 1237 h at 1000 cd m<sup>−2</sup>, setting new benchmarks for blue Ph-OLEDs. To enhance the color purity, hyper-OLEDs were developed with a full width at half maximum (FWHM) of 20 nm and the CIEy of 0.233, achieving an EQE<sub>m</sub> of 29.78% and LT<sub>50</sub> of 318 h at 1000 cd m<sup>−2</sup>. We also fabricated the active-matrix (AM) blue Hyper-OLEDs with 400 pixels per inch to demonstrate their application in AM displays.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"112 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-04-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143805873","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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