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Topological control of chirality and spin with structured light 结构光手性和自旋的拓扑控制
Light-Science & Applications Pub Date : 2026-04-24 DOI: 10.1038/s41377-026-02278-6
Light Mkhumbuza, Pedro Ornelas, Angela Dudley, Isaac Nape, Kayn A. Forbes
{"title":"Topological control of chirality and spin with structured light","authors":"Light Mkhumbuza, Pedro Ornelas, Angela Dudley, Isaac Nape, Kayn A. Forbes","doi":"10.1038/s41377-026-02278-6","DOIUrl":"https://doi.org/10.1038/s41377-026-02278-6","url":null,"abstract":"Structured light beams with engineered topological properties offer a powerful means to control spin angular momentum (SAM) and optical chirality, key quantities shaped by spin-orbit interaction (SOI) in light. Such effects are commonly associated with non-paraxial focusing or light-matter interfaces. Here, we demonstrate that higher-order Poincaré modes carrying a tunable Pancharatnam topological charge ℓp enable deterministic control of SOI entirely in free space and within the paraxial regime. We show that modulation of ℓp drives a measurable radial separation of circular polarization components - a free-space optical Hall effect arising from propagation-induced mechanisms alone. The effect originates from differential Gouy-phase evolution and radial divergence between the two circular components of an initially spin-balanced vector beam. This identifies ℓp as a single, tunable parameter linking Pancharatnam topology to paraxial spin-orbit coupling, establishing a simple and material-independent route to generate and control optical chirality and SAM. This approach provides new opportunities for tunable optical manipulation, chiral sensing, and high-dimensional photonic information processing.\u0000\u0000The alternative text for this image may have been generated using AI.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"40 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147751816","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Deformation engineering enables precise dispersion control in an optical microcavity. 变形工程使光学微腔中的精确色散控制成为可能。
Light-Science & Applications Pub Date : 2026-04-23 DOI: 10.1038/s41377-026-02297-3
Julius Kullig,Jan Wiersig
{"title":"Deformation engineering enables precise dispersion control in an optical microcavity.","authors":"Julius Kullig,Jan Wiersig","doi":"10.1038/s41377-026-02297-3","DOIUrl":"https://doi.org/10.1038/s41377-026-02297-3","url":null,"abstract":"Efficient nonlinear optical processes require the maintenance of frequency matching across a broad spectral range. Recent research demonstrates that this can be realized by tailoring the shape of an optical microdisk.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"42 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147735336","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Editors at the frontier: exploring advanced optical engineering in the UK. 编辑在前沿:探索先进的光学工程在英国。
Light-Science & Applications Pub Date : 2026-04-20 DOI: 10.1038/s41377-026-02292-8
Siqiu Guo,Xiangqian Jiang
{"title":"Editors at the frontier: exploring advanced optical engineering in the UK.","authors":"Siqiu Guo,Xiangqian Jiang","doi":"10.1038/s41377-026-02292-8","DOIUrl":"https://doi.org/10.1038/s41377-026-02292-8","url":null,"abstract":"","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"24 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147726122","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Space-time-coding metasurfaces for high-dimensional communications with OAM-, polarization-, and frequency-division multiplexing. 使用OAM、极化和频分复用的高维通信的空时编码元表面。
Light-Science & Applications Pub Date : 2026-04-20 DOI: 10.1038/s41377-026-02282-w
Lei Zhang,Tie Jun Cui
{"title":"Space-time-coding metasurfaces for high-dimensional communications with OAM-, polarization-, and frequency-division multiplexing.","authors":"Lei Zhang,Tie Jun Cui","doi":"10.1038/s41377-026-02282-w","DOIUrl":"https://doi.org/10.1038/s41377-026-02282-w","url":null,"abstract":"Recent advances in high-dimensional multiplexing have enabled the concurrent operation of multiple independent communication channels through orbital angular momentum, polarization, and frequency division multiplexing, all implemented on a compact space-time-coding metasurface platform. These developments provide a streamlined and high-efficiency approach to optimizing multiplexing performance and enhancing channel capacity in wireless communication systems.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"93 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147726139","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High-performance thermally-evaporated light-emitting diodes via one-step vapor purification. 通过一步蒸汽净化的高性能热蒸发发光二极管。
Light-Science & Applications Pub Date : 2026-04-20 DOI: 10.1038/s41377-026-02226-4
Xiang Zhang,Yuanwu Wu,Jianfeng Ou,Zixi Shen,Nian Liu,Thamraa Alshahrani,Abd Rashid Bin Mohd Yusoff,Jiang Tang,Jiajun Luo
{"title":"High-performance thermally-evaporated light-emitting diodes via one-step vapor purification.","authors":"Xiang Zhang,Yuanwu Wu,Jianfeng Ou,Zixi Shen,Nian Liu,Thamraa Alshahrani,Abd Rashid Bin Mohd Yusoff,Jiang Tang,Jiajun Luo","doi":"10.1038/s41377-026-02226-4","DOIUrl":"https://doi.org/10.1038/s41377-026-02226-4","url":null,"abstract":"Purity has been fundamental to the fabrication of high-performance semiconductors, spanning from precursors to reaction atmospheres. Emerging thermally evaporated perovskites involving precise control impose even stricter requirements on the purity of the vapor atmosphere. Compared to the purified solvent for the reaction atmosphere in the solution-based method, efficient and effective vapor purification remains unexplored. Here, we report one-step vapor purification for a pure atmosphere with less than one percent detrimental impurity. The in-situ residual gas analysis was employed to emphasize the complexity of the gas-phase composition and reveal the impurity reaction competition during the purification. The pre-control of the vapor atmosphere enabled a record external quantum efficiency over 20% for a thermally-evaporated perovskite light-emitting diode (PeLED) based on defect-suppressed FAxCs1-xPbBr3 films. Moreover, the PeLED display panels exhibit over 5-fold and 2-fold magnification in operational and storage stability. The stability extension in OLEDs by this strategy demonstrates its universal effectiveness and commercialization potential for other types of thermally evaporated optoelectronic devices.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"207 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147726121","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Multifunctional ligand engineering for pure-blue halide perovskite nanocrystal LEDs. 纯蓝色卤化物钙钛矿纳米晶体led的多功能配体工程。
Light-Science & Applications Pub Date : 2026-04-20 DOI: 10.1038/s41377-026-02288-4
Mark T Swihart
{"title":"Multifunctional ligand engineering for pure-blue halide perovskite nanocrystal LEDs.","authors":"Mark T Swihart","doi":"10.1038/s41377-026-02288-4","DOIUrl":"https://doi.org/10.1038/s41377-026-02288-4","url":null,"abstract":"More efficient and stable blue LEDs are essential for achieving the full potential of halide perovskite-based displays, but defect formation and ion migration limit both external quantum efficiency and lifetime of these devices. Now, a multifunctional fluorinated ligand is shown to mitigate both factors, dramatically enhancing brightness, efficiency and lifetime.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"16 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147726140","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
NIR-II-triggered plasmonic catalysis with tip-localized enhancement: a strategy for hypoxic biofilm eradication on orthopedic implants. nir - ii触发的等离子体催化与尖端局部增强:矫形植入物缺氧生物膜根除的策略。
Light-Science & Applications Pub Date : 2026-04-17 DOI: 10.1038/s41377-026-02279-5
Yu Sun,Fanglin Sheng,Yi Liang,Jinhui Meng,Ke Huang,Sanmao Liu,Yingfeng Qin,Maolin He,Jin-Wen Liu
{"title":"NIR-II-triggered plasmonic catalysis with tip-localized enhancement: a strategy for hypoxic biofilm eradication on orthopedic implants.","authors":"Yu Sun,Fanglin Sheng,Yi Liang,Jinhui Meng,Ke Huang,Sanmao Liu,Yingfeng Qin,Maolin He,Jin-Wen Liu","doi":"10.1038/s41377-026-02279-5","DOIUrl":"https://doi.org/10.1038/s41377-026-02279-5","url":null,"abstract":"The utilization of light as an external stimulus to promote the generation of hot electrons in plasmonic heterostructures and thus augment their catalytic efficacy presents significant potential for bacterial biofilm eradication. However, the inefficient harnessing of photoinduced hot electrons in conventional developed strategies greatly impede their therapeutic application in bone tissues. To overcome these challenges, we herein engineered a near-infrared II (NIR-II)-triggered plasmonic catalysis, which was fabricated through the integration of gold nanobipyramids (Au NBPs) with tip-deposited platinum nanoparticles (Pt NPs), for effective elimination of hypoxic bacterial biofilms on bone implants. The strategic deposition of Pt NPs at the tip of Au NBPs (ePt-Au NBPs) not only brought the redshift of the NIR absorption peak, but also accelerated charge separation and electromagnetic field localization, which endowed the ePt-Au NBPs plasmonic heterostructures with enhanced catalytic activity. Under NIR-II laser irradiation, the plasmonic catalysis with tip-localized enhancement enabled robust generation of hydroxyl radicals (•OH), thereby facilitating the cleavage of extracellular DNA (eDNA) within biofilms, disrupting biofilm integrity, and ultimately sensitizing bacteria to thermal ablation. These attributes collectively contribute to the effective elimination of hypoxic bacterial biofilms. Furthermore, surface functionalization with RGDC peptides conferred the implant with superior biocompatibility and osteogenic integration capabilities. This rationally designed plasmonic catalysis, combining the NIR-II-triggered simultaneous production of enhanced catalytic activity and localized hyperthermia, demonstrates significant potential for translational applications in light-responsive therapeutic strategies for implant-associated infections.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"29 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147702278","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Electrically switchable continuous phase liquid crystal Fresnel zone plate. 电开关连续相液晶菲涅耳带板。
Light-Science & Applications Pub Date : 2026-04-17 DOI: 10.1038/s41377-026-02251-3
Zhiyu Xu,Camron Nourshargh,Tianxin Wang,Alec Xu,Nathan Spiller,Urban Mur,Martin J Booth,Steve J Elston,Stephen M Morris
{"title":"Electrically switchable continuous phase liquid crystal Fresnel zone plate.","authors":"Zhiyu Xu,Camron Nourshargh,Tianxin Wang,Alec Xu,Nathan Spiller,Urban Mur,Martin J Booth,Steve J Elston,Stephen M Morris","doi":"10.1038/s41377-026-02251-3","DOIUrl":"https://doi.org/10.1038/s41377-026-02251-3","url":null,"abstract":"We present the design, fabrication, and characterization of continuous phase Fresnel zone plates (FZPs) using two-photon polymerization direct laser writing in a polymerizable nematic liquid crystal (LC) confined between glass substrates. Unlike conventional binary LC diffractive elements, our devices exhibit a smooth, continuous three-dimensional phase profile. Two devices were demonstrated with wrapped phase profiles of 2π and 4π radians, respectively. Polarized optical microscopy and digital holographic microscopy confirm that the polymerized regions follow the intended spatially varying phase distribution. Far field measurements show that the 2π rad FZP generates a strong focal spot at 0 Vpp and switches off at higher voltages. In contrast, the 4π rad FZP exhibits varifocal behavior, switching between two focal lengths: 24 mm at 0 Vpp and 48 mm at an intermediate voltage of 2.1 Vpp. At higher voltages, the focus disappears entirely. Compared to a binary FZP of equal size and focal length, the continuous phase design nearly doubles the focusing efficiency and enables switchable, compact, vari-focal, and energy-efficient optical components. This approach offers new opportunities for advanced applications such as augmented and virtual reality, adaptive optics, and other next-generation photonic systems.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"18 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147695034","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Minimalist optical system for achromatic imaging within extended field of view based on monolithic integrated meta-axicon cluster. 基于单片集成元轴子簇的扩展视场消色差最小光学系统。
Light-Science & Applications Pub Date : 2026-04-16 DOI: 10.1038/s41377-026-02272-y
Jianli Wang,Chengmiao Wang,Bin Wang,Yongting Deng,Yu Lin,Yeming Han,Lu Yao,Long Zhang,Dayu Li,Dejia Meng,Xiufeng Liu,Xiyu Li,Jan G Korvink,Yongbo Deng
{"title":"Minimalist optical system for achromatic imaging within extended field of view based on monolithic integrated meta-axicon cluster.","authors":"Jianli Wang,Chengmiao Wang,Bin Wang,Yongting Deng,Yu Lin,Yeming Han,Lu Yao,Long Zhang,Dayu Li,Dejia Meng,Xiufeng Liu,Xiyu Li,Jan G Korvink,Yongbo Deng","doi":"10.1038/s41377-026-02272-y","DOIUrl":"https://doi.org/10.1038/s41377-026-02272-y","url":null,"abstract":"Achromatic metalenses face stringent aperture and numerical aperture (NA) constraints, which have become a key bottleneck in metasurface imaging. To this end, a novel achromatic imaging method was first proposed, utilizing the unique wideband consistency of diffracted Bessel spots combined with non-blind image restoration techniques. To address the off-axis aberration issue, off-axis achromatic meta-axicons with eccentric conical phases were further designed to convert oblique plane waves into wideband uniform off-axis Bessel beams. Ultimately, a single metasurface integrating 9 meta-axicons with different design field angles was developed, and a meta-camera was constructed accordingly. After image restoration, the meta-camera achieves achromatic imaging within a 10° stitched field of view (FOV), and an angular resolution close to that of near-diffraction-limit lens with the same aperture throughout the entire FOV. The core idea of achieving achromatic imaging based on natural dispersion laws in this study enables the wideband minimalist optical system based on metasurface to completely circumvent the aperture limitation, providing a highly valuable solution for large-aperture meta-camera design that can simultaneously accommodate wideband and off-axis FOV.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"3 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147695191","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Self-recoverable mechanoluminescence in simple oxides: Al2O3:Cr. 在简单氧化物:Al2O3:Cr中的自恢复机械发光。
Light-Science & Applications Pub Date : 2026-04-15 DOI: 10.1038/s41377-026-02274-w
Ziyi Fang,Xiaofeng Pan,Qi'an Zhang,Mingzhi Wu,Yang Liu,Qidong Ma,Biyun Ren,Yanze Wang,Shengqiang Liu,Maryam Zulfiqar,Ming-Gang Ju,Jiulin Gan,Leipeng Li,Feng Wang,Dengfeng Peng
{"title":"Self-recoverable mechanoluminescence in simple oxides: Al2O3:Cr.","authors":"Ziyi Fang,Xiaofeng Pan,Qi'an Zhang,Mingzhi Wu,Yang Liu,Qidong Ma,Biyun Ren,Yanze Wang,Shengqiang Liu,Maryam Zulfiqar,Ming-Gang Ju,Jiulin Gan,Leipeng Li,Feng Wang,Dengfeng Peng","doi":"10.1038/s41377-026-02274-w","DOIUrl":"https://doi.org/10.1038/s41377-026-02274-w","url":null,"abstract":"Materials exhibiting mechanoluminescence (ML) that directly convert mechanical stimuli into light hold significant potential for real-time stress sensing and intelligent photonic systems. However, most high-performance ML systems rely on complex multicomponent compounds that often suffer from limited intensity, stability, and scalability, largely due to poorly understood mechanisms. Herein, we report a simple Al2O3:Cr3+ oxide that exhibits unprecedented ML intensity, enabled by a well-defined mechanical-to-optical energy conversion process. The self-recoverable ML arises from stress-induced ionization of electrons from luminescence centers, followed by their recapture upon stress release. By precisely tuning the doping levels, annealing conditions, and heterojunction interfaces, Al2O3:Cr3+ phosphors achieved intense, reproducible, and thermally stable near-infrared emission. Notably, high-temperature annealing dramatically enhanced the ML intensity, with thermodynamic and kinetic analyses revealing increases in the carrier and defect concentrations by several orders of magnitude, accounting for the exceptional brightness. By leveraging the chemical robustness, abundance, and low cost of alumina, we demonstrated the flexible ML paper for stress visualization and multi-level anti-counterfeiting, as well as in-situ grown Al2O3:Cr3+ luminescent layers on Cr-Al alloys for passive, real-time stress monitoring. This study establishes Al2O3 as a durable and scalable oxide platform for next-generation self-recoverable ML materials, bridging fundamental research and practical sensing technologies.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"441 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2026-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147684981","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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