Shengguo Hu, Mingyi Li, Jiawen Xu, Hongrui Zhang, Shanghang Zhang, Tie Jun Cui, Philipp del Hougne, Lianlin Li
{"title":"Electromagnetic metamaterial agent","authors":"Shengguo Hu, Mingyi Li, Jiawen Xu, Hongrui Zhang, Shanghang Zhang, Tie Jun Cui, Philipp del Hougne, Lianlin Li","doi":"10.1038/s41377-024-01678-w","DOIUrl":"https://doi.org/10.1038/s41377-024-01678-w","url":null,"abstract":"<p>Metamaterials have revolutionized wave control; in the last two decades, they evolved from passive devices via programmable devices to sensor-endowed self-adaptive devices realizing a user-specified functionality. Although deep-learning techniques play an increasingly important role in metamaterial inverse design, measurement post-processing and end-to-end optimization, their role is ultimately still limited to approximating specific mathematical relations; the metamaterial is still limited to serving as proxy of a human operator, realizing a predefined functionality. Here, we propose and experimentally prototype a paradigm shift toward a metamaterial agent (coined metaAgent) endowed with reasoning and cognitive capabilities enabling the autonomous planning and successful execution of diverse long-horizon tasks, including electromagnetic (EM) field manipulations and interactions with robots and humans. Leveraging recently released foundation models, metaAgent reasons in high-level natural language, acting upon diverse prompts from an evolving complex environment. Specifically, metaAgent’s cerebrum performs high-level task planning in natural language via a multi-agent discussion mechanism, where agents are domain experts in sensing, planning, grounding, and coding. In response to live environmental feedback within a real-world setting emulating an ambient-assisted living context (including human requests in natural language), our metaAgent prototype self-organizes a hierarchy of EM manipulation tasks in conjunction with commanding a robot. metaAgent masters foundational EM manipulation skills related to wireless communications and sensing, and it memorizes and learns from past experience based on human feedback.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"41 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142908264","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Midya Parto, Christian Leefmans, James Williams, Robert M. Gray, Alireza Marandi
{"title":"Enhanced sensitivity via non-Hermitian topology","authors":"Midya Parto, Christian Leefmans, James Williams, Robert M. Gray, Alireza Marandi","doi":"10.1038/s41377-024-01667-z","DOIUrl":"https://doi.org/10.1038/s41377-024-01667-z","url":null,"abstract":"<p>Sensors are indispensable tools of modern life that are ubiquitously used in diverse settings ranging from smartphones and autonomous vehicles to the healthcare industry and space technology. By interfacing multiple sensors that collectively interact with the signal to be measured, one can go beyond the signal-to-noise ratios (SNR) attainable by the individual constituting elements. Such techniques have also been implemented in the quantum regime, where a linear increase in the SNR has been achieved via using entangled states. Along similar lines, coupled non-Hermitian systems have provided yet additional degrees of freedom to obtain better sensors via higher-order exceptional points. Quite recently, a new class of non-Hermitian systems, known as non-Hermitian topological sensors (NTOS) has been theoretically proposed. Remarkably, the synergistic interplay between non-Hermiticity and topology is expected to bestow such sensors with an enhanced sensitivity that grows exponentially with the size of the sensor network. Here, we experimentally demonstrate NTOS using a network of photonic time-multiplexed resonators in the synthetic dimension represented by optical pulses. By judiciously programming the delay lines in such a network, we realize the archetypal Hatano-Nelson model for our non-Hermitian topological sensing scheme. Our experimentally measured sensitivities for different lattice sizes confirm the characteristic exponential enhancement of NTOS. We show that this peculiar response arises due to the combined synergy between non-Hermiticity and topology, something that is absent in Hermitian topological lattices. Our demonstration of NTOS paves the way for realizing sensors with unprecedented sensitivities.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"34 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142908266","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Mingjian Cheng, Wenjie Jiang, Lixin Guo, Jiangting Li, Andrew Forbes
{"title":"Metrology with a twist: probing and sensing with vortex light","authors":"Mingjian Cheng, Wenjie Jiang, Lixin Guo, Jiangting Li, Andrew Forbes","doi":"10.1038/s41377-024-01665-1","DOIUrl":"https://doi.org/10.1038/s41377-024-01665-1","url":null,"abstract":"<p>Optical metrology is a well-established subject, dating back to early interferometry techniques utilizing light’s linear momentum through fringes. In recent years, significant interest has arisen in using vortex light with orbital angular momentum (OAM), where the phase twists around a singular vortex in space or time. This has expanded metrology’s boundaries to encompass highly sensitive chiral interactions between light and matter, three-dimensional motion detection via linear and rotational Doppler effects, and modal approaches surpassing the resolution limit for improved profiling and quantification. The intricate structure of vortex light, combined with the integration of artificial intelligence into optical metrology, unlocks new paradigms for expanding measurement frameworks through additional degrees of freedom, offering the potential for more efficient and accurate sensing and metrological advancements. This review aims to provide a comprehensive overview of recent advances and future trends in optical metrology with structured light, specifically focusing on how utilizing vortex beams has revolutionized metrology and remote sensing, transitioning from classical to quantum approaches.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"3 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142908258","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Jianli Wang, Yongting Deng, Chengmiao Wang, Yu Lin, Yeming Han, Junchi Liu, Xiufeng Liu, Hongwen Li, Jan G. Korvink, Yongbo Deng
{"title":"Portable astronomical observation system based on large-aperture concentric-ring metalens","authors":"Jianli Wang, Yongting Deng, Chengmiao Wang, Yu Lin, Yeming Han, Junchi Liu, Xiufeng Liu, Hongwen Li, Jan G. Korvink, Yongbo Deng","doi":"10.1038/s41377-024-01656-2","DOIUrl":"https://doi.org/10.1038/s41377-024-01656-2","url":null,"abstract":"<p>The core advantage of metalenses over traditional bulky lenses lies in their thin volume and lightweight. Nevertheless, as the application scenarios of metalenses extend to the macro-scale optical imaging field, a contradiction arises between the increasing demand for large-aperture metalenses and the synchronous rise in design and processing costs. In response to the application requirements of metalens with diameter reaching the order of 10<sup>4</sup><i>λ</i> or even 10<sup>5</sup><i>λ</i>, this paper proposes a novel design method for fixed-height concentric-ring metalenses, wherein, under the constraints of the processing technology, a subwavelength 2D building unit library is constructed based on different topological structures, and the overall cross-section of the metalens is assembled. Compared to global structural optimization, this approach reduces computational resources and time consumption by several orders of magnitude while maintaining nearly identical focusing efficiency. As a result, a concentric-ring metalens with a designed wavelength of 632.8 nm and a diameter of 46.8 mm was developed, and a quasi-telecentric telescope system composed of aperture stop and metalens was constructed, achieving high-resolution detection within a 20° field of view. In the subsequent experiments, the unique weak polarization dependence and narrowband adaptability of the meta-camera are quantitatively analyzed and tested, and excellent imaging results were finally obtained. Our work not only ensures the narrowband optical performance but also promotes the simplicity and light weight of the metalens based telescopic system, which further advances the deep application of large-diameter metalenses in the field of astronomical observation.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"14 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142908260","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Jianwei Qiao, Dehong Li, Qiufeng Shi, Haijie Guo, Ping Huang, Lei Wang
{"title":"Compositional engineering of phase-stable and highly efficient deep-red emitting phosphor for advanced plant lighting systems","authors":"Jianwei Qiao, Dehong Li, Qiufeng Shi, Haijie Guo, Ping Huang, Lei Wang","doi":"10.1038/s41377-024-01679-9","DOIUrl":"https://doi.org/10.1038/s41377-024-01679-9","url":null,"abstract":"<p>Inorganic luminescent materials hold great promise for optoelectronic device applications, yet the limited efficiency and poor thermal stability of oxide-based deep-red emitting phosphors hinder the advancement of plant lighting technologies. Herein, a simple compositional engineering strategy is proposed to stabilize the phase, boost external quantum efficiency (EQE) and enhance thermal stability. The chemical modification of the PO<sub>4</sub> tetrahedron in NaMgPO<sub>4</sub>:Eu by incorporating SiO<sub>4</sub> lowers the formation energy, leading to the generation of pure olivine phase and increasing the EQE from 27% to 52%, setting a record for oxide deep-red phosphors. In parallel, the introduced deep defect level improves thermal stability at 150 °C from 62.5% to 85.4%. Besides, the excitation and emission peaks shifted to 440 nm and 675 nm, respectively, aligning precisely with the specific spectral absorption requirements of plant phytochromes. Moreover, the luminescent intensity showed nearly no decay after being exposed to 80% relative humidity and 80 <sup>o</sup>C for 6 h, and the pc-LED utilizing Na<sub>1.06</sub>MgP<sub>0.94</sub>Si<sub>0.06</sub>O<sub>4</sub>:Eu achieves a high output power of 780 mW at 300 mA. Our research demonstrates a facile method for optimizing the performance of inorganic luminescent materials and provides alternative solutions for low-cost plant lighting.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"9 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142804797","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Unlocking high-performance near-infrared photodetection: polaron-assisted organic integer charge transfer hybrids","authors":"Muhammad Ahsan Iqbal, Xueqian Fang, Yasir Abbas, Xiaoliang Weng, Tingchao He, Yu-Jia Zeng","doi":"10.1038/s41377-024-01695-9","DOIUrl":"https://doi.org/10.1038/s41377-024-01695-9","url":null,"abstract":"<p>Room temperature femtowatt sensitivity remains a sought-after attribute, even among commercial inorganic infrared (IR) photodetectors (PDs). While organic IR PDs are poised to emerge as a pivotal sensor technology in the forthcoming Fourth-Generation Industrial Era, their performance lags behind that of their inorganic counterparts. This discrepancy primarily stems from poor external quantum efficiencies (<i>EQE</i>), driven by inadequate exciton dissociation (high exciton binding energy) within organic IR materials, exacerbated by pronounced non-radiative recombination at narrow bandgaps. Here, we unveil a high-performance organic Near-IR (NIR) PD via integer charge transfer between Poly[2,5-bis(3-tetradecylthiophen-2-yl)thieno[3,2-b]thiophene] (C-14PBTTT) donor (D) and Tetrafluorotetracyanoquinodimethane (TCNQF4) acceptor (A) molecules, showcasing strong low-energy subgap absorptions up to 2.5 µm. We observe that specifically, polaron excitation in these radical and neutral D-A blended molecules enables bound charges to exceed the Coulombic attraction to their counterions, leading to an elevated <i>EQE</i> (polaron absorption region) compared to Frenkel excitons. As a result, our devices achieve a high <i>EQE</i> of <span>∼</span>10<sup>7</sup>%, femtowatt sensitivity (<i>NEP)</i> of ~0.12 fW Hz<sup>-1/2</sup> along a response time of ~81 ms, at room temperature for a wavelength of 1.0 µm. Our innovative utilization of polarons highlights their potential as alternatives to Frenkel excitons in high-performance organic IR PDs.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"82 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-12-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142793312","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"A bright future for micro-LED displays","authors":"Vineeth K. Bandari, Oliver G. Schmidt","doi":"10.1038/s41377-024-01683-z","DOIUrl":"https://doi.org/10.1038/s41377-024-01683-z","url":null,"abstract":"<p>The development of GaN-based Micro-LED arrays achieving brightnesses exceeding 10<sup>7</sup> nits and high-density micro-displays with up to 1080×780 pixels marks a true breakthrough in the field. This breakthrough is a result of mastering a combination of long-standing challenges comprising wafer-scale high-quality epitaxial growth, sidewall passivation, efficient photon extraction, and elegant bonding technologies, and promises significant advantages for augmented and virtual reality devices, wearables, and next-generation consumer electronics.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"27 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-12-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142782497","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Advancing wavefront sensing: meta Shack-Hartmann sensor enhances phase imaging","authors":"Xiaoyuan Liu, Zihan Geng, Mu Ku Chen","doi":"10.1038/s41377-024-01646-4","DOIUrl":"https://doi.org/10.1038/s41377-024-01646-4","url":null,"abstract":"<p>A meta-lens array-based Shack-Hartmann wavefront sensor has been developed to break the limits imposed by the size and curvature of traditional micro-lenses, which significantly improves both sampling density and angular resolution of phase measurement. Metasurface advances the field of optical phase measurement to smaller-scale complex wavefront characterization.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"7 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-12-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142758450","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Huifang Jiang, Huifang Ji, Zhuangzhuang Ma, Dongwen Yang, Jingli Ma, Mengyao Zhang, Xu Li, Meng Wang, Ying Li, Xu Chen, Di Wu, Xinjian Li, Chongxin Shan, Zhifeng Shi
{"title":"Simultaneous achieving negative photoconductivity response and volatile resistive switching in Cs2CoCl4 single crystals towards artificial optoelectronic synapse","authors":"Huifang Jiang, Huifang Ji, Zhuangzhuang Ma, Dongwen Yang, Jingli Ma, Mengyao Zhang, Xu Li, Meng Wang, Ying Li, Xu Chen, Di Wu, Xinjian Li, Chongxin Shan, Zhifeng Shi","doi":"10.1038/s41377-024-01642-8","DOIUrl":"https://doi.org/10.1038/s41377-024-01642-8","url":null,"abstract":"<p>The development of negative photoconductivity (NPC)-related devices is of great significance for numerous applications, such as optoelectronic detection, neuromorphic computing, and optoelectronic synapses. Here, an unusual but interesting NPC phenomenon in the novel cesium cobalt chlorine (Cs<sub>2</sub>CoCl<sub>4</sub>) single crystal-based optoelectronic devices is reported, which simultaneously possess volatile resistive switching (RS) memory behavior. Joint experiment−theory characterizations reveal that the NPC behavior is derived from the intrinsic vacancy defects of Cs<sub>2</sub>CoCl<sub>4</sub>, which could trap photogenerated charge carriers and produce an internal electric field opposite to the applied electric field. Such NPC effect enables an abnormal photodetection performance with a decrease in electrical conductivity to illumination. Also, a large specific detectivity of 2.7 × 10<sup>12</sup> Jones and broadband NPC detection wavelength from 265 to 780 nm were achieved. In addition to the NPC response, the resulting devices demonstrate a volatile RS performance with a record-low electric field of 5 × 10<sup>4 </sup>V m<sup>−1</sup>. By integrating the characteristics of electric-pulse enhancement from RS and light-pulse depression from NPC, an artificial optoelectronic synapse was successfully demonstrated, and based on the simulation of artificial neural network algorithm, the recognition application of handwritten digital images was realized. These pioneer findings are anticipated to contribute significantly to the practical advancement of metal halides in the fields of in-memory technologies and artificial intelligence.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"18 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-12-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142758449","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yue Wang, Wen Xu, Haichun Liu, Yuhan Jing, Donglei Zhou, Yanan Ji, Jerker Widengren, Xue Bai, Hongwei Song
{"title":"A multiband NIR upconversion core-shell design for enhanced light harvesting of silicon solar cells","authors":"Yue Wang, Wen Xu, Haichun Liu, Yuhan Jing, Donglei Zhou, Yanan Ji, Jerker Widengren, Xue Bai, Hongwei Song","doi":"10.1038/s41377-024-01661-5","DOIUrl":"https://doi.org/10.1038/s41377-024-01661-5","url":null,"abstract":"<p>Exploring lanthanide light upconversion (UC) has emerged as a promising strategy to enhance the near-infrared (NIR) responsive region of silicon solar cells (SSCs). However, its practical application under normal sunlight conditions has been hindered by the narrow NIR excitation bandwidth and the low UC efficiency of conventional materials. Here, we report the design of an efficient multiband UC system based on Ln<sup>3+</sup>/Yb<sup>3+</sup>-doped core-shell upconversion nanoparticles (Ln/Yb-UCNPs, Ln<sup>3+ </sup>= Ho<sup>3+</sup>, Er<sup>3+</sup>, Tm<sup>3+</sup>). In our design, Ln<sup>3+</sup> ions are incorporated into distinct layers of Ln/Yb-UCNPs to function as near-infrared (NIR) absorbers across different spectral ranges. This design achieves broad multiband absorption withtin the 1100 to 2200 nm range, with an aggregated bandwidth of ~500 nm. We have identified a synthetic electron pumping (SEP) effect involving Yb<sup>3+</sup> ions, facilitated by the synergistic interplay of energy transfer and cross-relaxation between Yb<sup>3+</sup> and other ions Ln<sup>3+</sup> (Ho<sup>3+</sup>, Er<sup>3+</sup>, Tm<sup>3+</sup>). This SEP effect enhances the UC efficiency of the nanomaterials by effectively transferring electrons from the low-excited states of Ln<sup>3+</sup> to the excited state of Yb<sup>3+</sup>, resulting in intense Yb<sup>3+</sup> luminescence at ~980 nm within the optimal response region for SSCs, thus markedly improving their overall performance. The SSCs integrated with Ln/Yb-UCNPs with multiband excitation demonstrate the largest reported NIR response range up to 2200 nm, while enabling the highest improvement in absolute photovoltaic efficiency reported, with an increase of 0.87% (resulting in a total efficiency of 19.37%) under standard AM 1.5 G irradiation. Our work tackles the bottlenecks in UCNP-coupled SSCs and introduces a viable approach to extend the NIR response of SSCs.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"7 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-11-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142696880","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}