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Facile Access to N ‐Substituted Pyridyl Ligands N -取代吡啶配体的易得性
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-24 DOI: 10.1002/adsc.70417
Adam Petrik, Aleksander R. Bena, Haralds Baunis, Riley M. Kelch, Tehshik P. Yoon, Bartholomäus Pieber
{"title":"Facile Access to N ‐Substituted Pyridyl Ligands","authors":"Adam Petrik, Aleksander R. Bena, Haralds Baunis, Riley M. Kelch, Tehshik P. Yoon, Bartholomäus Pieber","doi":"10.1002/adsc.70417","DOIUrl":"https://doi.org/10.1002/adsc.70417","url":null,"abstract":"Pyridyl motifs equipped with <jats:italic>N</jats:italic> ‐substituents can be powerful ligands for catalysis, yet their broader adoption is limited by the lack of a practical method to prepare these scaffolds. We report a modular, robust, and versatile Buchwald–Hartwig amination protocol that enables the rapid synthesis of bipyridine, phenanthroline, terpyridine, and pybox ligands bearing dialkylamine, diarylamine, and heteroaromatic <jats:italic>N</jats:italic> ‐substituents. These conditions streamline ligand library synthesis and will facilitate systematic studies in catalysis and related applications.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"13 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147739231","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dual Ligand Enabled Pd‐Catalyzed Deuteration of Indole 双配体激活Pd催化吲哚氘化反应
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-24 DOI: 10.1002/adsc.70466
Zhiwei Yu, Liping Chen, Xin Huang, XinYing Li, Hailong Yang, Juan Yang, Jinquan Zhang
{"title":"Dual Ligand Enabled Pd‐Catalyzed Deuteration of Indole","authors":"Zhiwei Yu, Liping Chen, Xin Huang, XinYing Li, Hailong Yang, Juan Yang, Jinquan Zhang","doi":"10.1002/adsc.70466","DOIUrl":"https://doi.org/10.1002/adsc.70466","url":null,"abstract":"The critical importance of deuterium labeling, from mechanistic studies to drug discovery, has spurred the development of efficient deuteration methods. We herein describe a palladium‐catalyzed strategy for indole derivatives based on a synergistic dual‐ligand (6‐(1H‐indazol‐1‐yl)pyridin‐2(1H)‐one and pyridone) system. This method achieves efficient and regioselective deuteration across all positions of indole scaffolds—including the challenging C4–C7 sites—without directing groups, while exhibiting broad functional group tolerance. This work provides a practical tool for deuterated indole synthesis and establishes a new paradigm for dual‐ligand design in demanding CH functionalization.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"26 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147739228","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Electrochemical Synthesis of Phosphorothiolated Isocoumarins and Benzothiophenes 磷硫代异香豆素和苯并噻吩的电化学合成
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-24 DOI: 10.1002/adsc.70458
Chao Ma, Qiaoli Zhou, Nan Jiang, Mengshuai Zhang, Huiting Xu, Hualiang Shen, Faliang Gou, Tao Cai, Runpu Shen
{"title":"Electrochemical Synthesis of Phosphorothiolated Isocoumarins and Benzothiophenes","authors":"Chao Ma, Qiaoli Zhou, Nan Jiang, Mengshuai Zhang, Huiting Xu, Hualiang Shen, Faliang Gou, Tao Cai, Runpu Shen","doi":"10.1002/adsc.70458","DOIUrl":"https://doi.org/10.1002/adsc.70458","url":null,"abstract":"A new electrochemically driven radical annulation of <jats:italic>o</jats:italic> ‐alkynylbenzoates and <jats:italic>o</jats:italic> ‐alkynylthioanisoles with <jats:italic>S</jats:italic> ‐hydrogen phosphorothioates has been developed, offering an environmentally friendly and atom‐efficient approach to synthesize structurally diverse phosphorothiolated isocoumarins and benzothiophenes. Compared with previous methods, this transformation uses electrons as traceless reagents to oxidize S‐hydrogen phosphorothioates, circumventing the need for stoichiometric initiators and avoiding the formation of equivalent waste. Acetone is employed as a sustainable solvent, and green methanol is produced as the sole by‐product, further highlighting its sustainability. Moreover, the high efficiency and broad substrate scope are demonstrated by 47 total examples and up to 85% yield.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"9 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147739232","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Toward Activity Prediction: Unveiling the Role of Intra/Intermolecular Balance in Fe–N–C Catalysts for Hydrogen Evolution 活性预测：揭示分子内/分子间平衡在Fe-N-C催化剂析氢中的作用
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-24 DOI: 10.1002/adsc.70464
Tengyi Liu, Xiaofan Hou, Kosuke Ishibashi, Yutaro Hirai, Shimpei Ono, Hiroshi Yabu
{"title":"Toward Activity Prediction: Unveiling the Role of Intra/Intermolecular Balance in Fe–N–C Catalysts for Hydrogen Evolution","authors":"Tengyi Liu, Xiaofan Hou, Kosuke Ishibashi, Yutaro Hirai, Shimpei Ono, Hiroshi Yabu","doi":"10.1002/adsc.70464","DOIUrl":"https://doi.org/10.1002/adsc.70464","url":null,"abstract":"Metal–nitrogen–carbon (M–N–C) molecular catalysts attract attention for the hydrogen evolution reaction (HER) owing to their well‐defined active sites and structural tunability. However, previous studies prioritize intramolecular regulation, leaving the cooperative role of intermolecular interactions insufficiently understood. Herein, we design and synthesize three Fe–N–C molecules, including iron phthalocyanine (FePc) and two pyridinic‐N–incorporated FePc derivatives (FeTAP and FeOM), and elucidate their structure–activity relationships via integrated structural and electronic analyses to enable performance prediction. We demonstrate that pyridinic‐N incorporation drives Fe centers from Fe <jats:sup>2+</jats:sup> to a more positively charged Fe <jats:sup>2+δ</jats:sup> state, creating an “oxidation‐state reservoir” that promotes rapid electron transfer and proton adsorption for HER. Moreover, overall activity is governed by the balance between intramolecular electronic regulation and intermolecular π–π interactions: FePc is limited by weak intramolecular regulation; FeOM exhibits strong intramolecular effects but weakened intermolecular coupling; and FeTAP optimizes this balance, delivering the highest HER activity. Electrochemical measurements corroborate the predictions and further reveal that an optimal level of pyridinic‐N achieves the intra‐/intermolecular balance, thereby accelerating HER kinetics on these Fe–N–C catalysts. These findings provide a predictive basis and a clear design guideline centered on intra‐/intermolecular balance for molecular electrocatalysts.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"34 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147739229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
One‐Pot Two‐Step Synthesis of 1,4,5,6‐Tetrahydropyridazines Through a Three‐Component Reaction of 2,5‐Dimethoxytetrahydrofuran, Hydrazides, and Aromatic Nucleophiles 2,5 -二甲氧基四氢呋喃、肼和芳香亲核试剂三组分反应一锅两步合成1,4,5,6 -四氢吡啶
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-24 DOI: 10.1002/adsc.70457
Muhammad Noman Haider Tariq, Gul Khanda Sajjad, Guoqiang Tang, Tianjian Zhang, Rongxian Bai, Yanlong Gu
{"title":"One‐Pot Two‐Step Synthesis of 1,4,5,6‐Tetrahydropyridazines Through a Three‐Component Reaction of 2,5‐Dimethoxytetrahydrofuran, Hydrazides, and Aromatic Nucleophiles","authors":"Muhammad Noman Haider Tariq, Gul Khanda Sajjad, Guoqiang Tang, Tianjian Zhang, Rongxian Bai, Yanlong Gu","doi":"10.1002/adsc.70457","DOIUrl":"https://doi.org/10.1002/adsc.70457","url":null,"abstract":"A one‐pot two‐step method for the synthesis of heteroaryl‐substituted 1,4,5,6‐tetrahydropyridazines was developed using 2,5‐dimethoxytetrahydrofuran (2,5‐DMTHF), hydrazides, and arene nucleophile as substrates. In the first step, condensation of 2,5‐DMTHF and tosyl hydrazide generates a 2‐tosyl‐2,3,4,5‐tetrahydropyridazin‐3‐ol intermediate, which undergoes in the second step a nucleophilic substitution with indole, with the aid of Al(OTf) <jats:sub>3</jats:sub> catalyst, to give an (indol‐3‐yl)‐substituted tosyl‐tetrahydropyridazine in good yield. Thiophenes and electron‐rich benzenes can also be used as nucleophiles in the synthesis. This operationally simple and efficient protocol offers a straightforward route to access 6‐heteroaryl‐substituted 1,4,5,6‐tetrahydropyridazines.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"1 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147739230","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Recent Advances in Enantioselective C‐H Functionalization via Electrochemical/Transition‐Metal Cooperative Catalysis 电化学/过渡金属协同催化对映选择性C - H功能化研究进展
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-23 DOI: 10.1002/adsc.70394
Ming‐Shuang Li, Teck‐Peng Loh, Tong Li, Xu‐Hong Hu
{"title":"Recent Advances in Enantioselective C‐H Functionalization via Electrochemical/Transition‐Metal Cooperative Catalysis","authors":"Ming‐Shuang Li, Teck‐Peng Loh, Tong Li, Xu‐Hong Hu","doi":"10.1002/adsc.70394","DOIUrl":"https://doi.org/10.1002/adsc.70394","url":null,"abstract":"Enantioselective C‐H functionalization has emerged as a key strategy for constructing chiral molecules, as it enables direct and precise chiral modification of inert C‐H bonds while significantly improving atom economy in synthetic processes. Traditional asymmetric C‐H functionalization relies on chemical oxidants to drive catalytic cycles, which suffers from limitations such as high toxicity of reagents, excessive byproduct formation, and harsh reaction conditions. Electrochemical/transition metal cooperative catalysis offers an innovative pathway by replacing chemical oxidants with electrical energy, utilizing electrode reactions to precisely regulate the valence cycle of metal catalysts. By integrating the C‐H bond activation capability and chiral induction ability of transition metals, this approach provides a green and efficient route for constructing chiral molecules. This review systematically summarizes the research progress over the past 5 years in electrochemical/transition metal cooperative catalysis for asymmetric C‐H functionalization toward chiral compounds. It highlights the cooperative mechanisms between different transition metals (palladium, rhodium, nickel, copper, cobalt) and electrochemistry. We believe this review will serve as an important reference for scientists interested in advances in asymmetric C‐H functionalization via electrochemical/metal cooperative catalysis.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"20 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147733497","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Copper‐Mediated ortho ‐C–H Etherification of Arylaldehydes Enabled by a Transient Directing Group 铜介导的芳醛邻C-H醚化反应的瞬时导向基团
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-23 DOI: 10.1002/adsc.70465
Qingbo Ma, Huijian Zhou, Zijin Luo, Chengrong Ding, Jinghui Lyu, Yiyong Zhao, Guofu Zhang
{"title":"Copper‐Mediated ortho ‐C–H Etherification of Arylaldehydes Enabled by a Transient Directing Group","authors":"Qingbo Ma, Huijian Zhou, Zijin Luo, Chengrong Ding, Jinghui Lyu, Yiyong Zhao, Guofu Zhang","doi":"10.1002/adsc.70465","DOIUrl":"https://doi.org/10.1002/adsc.70465","url":null,"abstract":"Transient directing groups (TDGs) have been demonstrated to promote the in situ generation and elimination of directing groups, thereby providing an efficient strategy for C–H functionalization. This study utilizes the in situ formation of imines between amino acids and aromatic aldehydes. Under copper‐mediated conditions, an <jats:italic>ortho</jats:italic> ‐C–H etherification reaction between aromatic aldehydes and phenols/alcohols was achieved. To the best of our knowledge, this represents the first example of a TDG‐mediated reaction involving phenol substrates. The utility of this strategy has been demonstrated through multiple applications, including the late‐stage diversification of drug analogs.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"25 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147733501","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ce‐Incorporation‐Induced Crystal and Electronic Structure Regulation of Amorphous NiP Alloy to Boost Hydrogen Evolution in Anion Exchange Membrane Water Electrolysis 非晶态NiP合金在阴离子交换膜电解中促进析氢的晶体和电子结构调控
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-23 DOI: 10.1002/adsc.70461
Yongchao Cheng, Ningbo Fan, Cong Chen, Junxia Shen, Zhihe Wei, Wen Dong, Yang Peng, Ronglei Fan, Mingrong Shen
{"title":"Ce‐Incorporation‐Induced Crystal and Electronic Structure Regulation of Amorphous NiP Alloy to Boost Hydrogen Evolution in Anion Exchange Membrane Water Electrolysis","authors":"Yongchao Cheng, Ningbo Fan, Cong Chen, Junxia Shen, Zhihe Wei, Wen Dong, Yang Peng, Ronglei Fan, Mingrong Shen","doi":"10.1002/adsc.70461","DOIUrl":"https://doi.org/10.1002/adsc.70461","url":null,"abstract":"Anion exchange membrane water electrolysis (AEMWE) driven by intermittent renewable energy is one of the optimal solutions for producing green hydrogen gas; however, its further development is limited by highly active and long‐lived hydrogen evolution reaction (HER) catalysts. Herein, a cerium (Ce) incorporated amorphous NiP alloy grown on nickel foam is proposed to meet these challenges, which shows an industrial‐level current density of −1000 mA/cm <jats:sup>2</jats:sup> under 255 mV overpotential and maintains excellent stability under intermittent start‐shutdown operation for 10k cycles in 1 M KOH. The experimental results reveal that the incorporation of Ce can optimize the electronic structure and endow appropriate OH binding energy during HER, thereby significantly accelerating HER kinetics. Moreover, the optimization of NiP crystal structure induced by Ce incorporation can adjust the surface microstructure and release the interfacial stress between the catalytic layer and substrate, resulting in accelerated charge and mass transfer and enhanced stability during the HER process. When integrated into an AEMWE, the optimized NiCeP catalyst displays a low cell voltage of 1.79 V at 1000 mA/cm <jats:sup>2</jats:sup> and maintains stable operation up to 200 h under industrial conditions. This work highlights the importance of modification in the crystal and electronic structure of catalysts in advancing AEMWE under fluctuating renewable energy driving conditions.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"136 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147733436","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Base‐Promoted Multicomponent Reaction of Phthalaldehyde With Amines and Sulfur: Access to 3‐Iminoisoindoline‐1‐Thiones 碱促进邻苯二醛与胺和硫的多组分反应：获得3 -亚氨基异吲哚- 1 -硫酮
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-23 DOI: 10.1002/adsc.70435
Le Anh Nguyen, Quoc Anh Ngo, Dinh Hung Mac, Thi Thu Tram Nguyen, Pascal Retailleau, Thanh Binh Nguyen
{"title":"Base‐Promoted Multicomponent Reaction of Phthalaldehyde With Amines and Sulfur: Access to 3‐Iminoisoindoline‐1‐Thiones","authors":"Le Anh Nguyen, Quoc Anh Ngo, Dinh Hung Mac, Thi Thu Tram Nguyen, Pascal Retailleau, Thanh Binh Nguyen","doi":"10.1002/adsc.70435","DOIUrl":"https://doi.org/10.1002/adsc.70435","url":null,"abstract":"A base‐catalyzed, oxidative multicomponent condensation involving primary anilines, elemental sulfur, and phthalaldehyde is reported. Utilizing readily available starting materials, this protocol affords a novel series of structurally diverse 3‐iminoisoindoline‐1‐thiones in satisfactory yields under mild reaction conditions. Furthermore, the methodology was successfully extended to 1,8‐diaminonaphthalene, yielding the photosensitizer 12 <jats:italic>H</jats:italic> ‐isoindolo[2,1‐ <jats:italic>a</jats:italic> ]perimidine‐12‐thione in excellent yields with a simplified purification process via filtration.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"19 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147733498","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Recent Advances in Electrochemical Nucleophilic Introduction of Azide and Functionalization 叠氮化物的电化学亲核引入及其功能化研究进展
IF 5.4 2区 化学
Advanced Synthesis & Catalysis Pub Date : 2026-04-23 DOI: 10.1002/adsc.70460
Bin Song, Chong Zhang
{"title":"Recent Advances in Electrochemical Nucleophilic Introduction of Azide and Functionalization","authors":"Bin Song, Chong Zhang","doi":"10.1002/adsc.70460","DOIUrl":"https://doi.org/10.1002/adsc.70460","url":null,"abstract":"Azides, as multifunctional nitrogen‐containing molecules, are significant precursors in various chemical transformations, especially for the preparation of amines, amides, nitriles, triazoles, tetrazoles, and pyrrolines by subsequent redox, cycloaddition, click chemistry, and rearrangement processes. Organic electrochemistry has garnered increasing attention due to its essential potential to promote the development of sustainable organic synthesis, enabling the new avenues to introduce the azide group or directly realize the functionalization in the past decade. In this review, the research progress on the nucleophilic incorporation and direct functionalization of azide groups through electrochemical methodologies is critically summarized based on the electrophilic species involved. The representative scopes and electrochemical mechanism are emphatically described, aiming to inspire innovations in the development of azide chemistry.","PeriodicalId":118,"journal":{"name":"Advanced Synthesis & Catalysis","volume":"24 1","pages":""},"PeriodicalIF":5.4,"publicationDate":"2026-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147733499","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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