Advanced Materials最新文献

{"title":"Heterogeneous Polymer Multilayers Enabling Photoresponsive Nonreciprocal Patterns for Information Encryption.","authors":"Chenrui Yuan, Dachuan Zhang, Zhulu Xie, Wen-Cong Xu, Shuofeng Liang, Si Wu","doi":"10.1002/adma.202506950","DOIUrl":"https://doi.org/10.1002/adma.202506950","url":null,"abstract":"<p><p>Society has a growing demand for information security. The development of nonreciprocal patterns is a new approach for high-security information encryption, but it is difficult to achieve due to its complexity in material design. Herein, heterogeneous polymer multilayers are designed to prepare nonreciprocal patterns for information encryption. The heterogeneous polymer multilayers are constructed by gluing polyvinyl alcohol (PVA) polarizers and photoresponsive azobenzene-containing polymers (azopolymers) via photocontrolled adhesion. Nonreciprocal optical patterns are fabricated via photopatterning of the azopolymer layer with polarized light. The information can only be decrypted from one direction of the nonreciprocal optical patterns. The nonreciprocal optical patterns are dynamic, which can be erased and rewritten with updated information via light irradiation. The nonreciprocal optical patterns can be further imprinted with diffraction elements, showing dual-mode optical signals. The nonreciprocal optical patterns with dynamic, dual-mode features enable high-security information encryption. Moreover, the heterogeneous polymer multilayers are flexible, bendable, and foldable, enabling the design of devices with nonreciprocal optical patterns for encryption in 3D space. The heterogeneous polymer multilayers with photoresponsive nonreciprocal patterns offer a solution for designing secure, updatable, and mechanically robust information encryption materials for flexible photonics, portable electronics, new anti-counterfeiting technologies, and wearable devices.</p>","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":" ","pages":"e2506950"},"PeriodicalIF":27.4,"publicationDate":"2025-06-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144525601","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Bioinspired Adaptive Sensors: A Review on Current Developments in Theory and Application.","authors":"Guodong Gong, You Zhou, Qingxiu Li, Wenyu Zhao, Sunyingyue Geng, Hangfei Li, Yan-Bing Leng, Shirui Zhu, Guanglong Ding, Yongbiao Zhai, Ziyu Lv, Ye Zhou, Su-Ting Han","doi":"10.1002/adma.202505420","DOIUrl":"https://doi.org/10.1002/adma.202505420","url":null,"abstract":"<p><p>The human perception system features many dynamic functional mechanisms that efficiently process the large amount of sensory information available in the surrounding environment. In this system, sensory adaptation operates as a core mechanism that seamlessly filters familiar and inconsequential external stimuli at sensory endpoints. Such adaptive filtering minimizes redundant data movement between sensory terminals and cortical processing units and contributes to a lower communication bandwidth requirement and lower energy consumption at the system level. Recreating the behavior of sensory adaptation using electronic devices has garnered significant research interest owing to its promising prospects in next-generation intelligent perception platforms. Herein, the recent progress in bioinspired adaptive device engineering is systematically examined, and its valuable applications in electronic skins, wearable electronics, and machine vision are highlighted. The rapid development of bioinspired adaptive sensors can be attributed not only to the recent advances in emerging neuromorphic electronic elements, including piezoelectric and triboelectric sensors, memristive devices, and neuromorphic transistors, but also to the improved understanding of biological sensory adaptation. Existing challenges hindering device performance optimization, multimodal adaptive sensor development, and system-level integration are also discussed, providing insights for the development of high-performance neuromorphic sensing systems.</p>","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":" ","pages":"e2505420"},"PeriodicalIF":27.4,"publicationDate":"2025-06-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144525596","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Van der Waals Welding of Carbon Nanotubes with Near‐Limit High Strength","authors":"Yunxiang Bai, Hongjie Yue, Yukang Zhu, Jun Gao, Mengxiong Liu, Shijun Wang, Rufan Zhang, Fei Wei","doi":"10.1002/adma.202502638","DOIUrl":"https://doi.org/10.1002/adma.202502638","url":null,"abstract":"The strength of carbon nanotube (CNT) bundles and fibers is generally much lower than that of single CNTs, the short length of CNT components results in the assembly strength can only be contributed by the weak shearing interaction between CNTs. Here, the welding of CNTs by a fast chemical‐vapor‐deposition self‐assembly (FCVDS) technique using TiO<jats:sub>2</jats:sub> nanoparticles as the solder is reported. It is simple, fast, pressure‐free, applicable to ambient conditions, and can weld samples with macroscale length. The welded junctions have a mechanical strength approaching the tensile strength of a single CNT. Whereas the interface interaction between TiO<jats:sub>2</jats:sub> and CNTs is only contributed by Van der Waals forces, avoiding the destruction of the defect‐free structure of CNTs. The solder mass can be only ≈1 wt% of welded CNTs.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"23 1","pages":""},"PeriodicalIF":29.4,"publicationDate":"2025-06-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144515253","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Fine-Tuning of Molecular Self-Assembly Morphology via Synergistic Ternary Copolymerization and Side Chain Optimization of Low-Cost Polymer Donors Toward Efficient Organic Solar Cells.","authors":"Xixi Zhang, Xinrui Li, Xiaolei Kong, Jinyuan Zhang, Jing Li, Aoxiang Li, Chuanjun Song, Yongfang Li, Chenkai Sun","doi":"10.1002/adma.202503325","DOIUrl":"https://doi.org/10.1002/adma.202503325","url":null,"abstract":"<p><p>Self-assembly morphology optimization of organic photovoltaic materials is crucial to improve the performance of organic solar cells (OSCs). Herein, three low-cost PTQ derivative donors, PTQ17, PTQ18, and PTQ19 are developed by synergistic ternary copolymerization and side chain optimization of utilizing different benzothiadiazole (BT) units, to fine-tune molecular self-assembly morphology. PTQ17, containing difluorinated BT, shows the tightest π-π packing and strongest molecular crystallinity, leading to excessive molecular aggregation and phase separation morphology in active layer. In contrast, PTQ19, containing dialkoxy-substituted BT, has the weakest molecular crystallinity, resulting in the worst long-range ordered molecular packing and the smallest phase domains in active layer. Remarkably, PTQ18, containing monofluorinated and monoalkoxy-substituted BT, has moderate molecular crystallinity and the best compatibility with acceptor, resulting in the most ideal microscopic morphology of active layer with desirable domain size and phase separation features. In result, the PTQ18-based binary OSC achieves an outstanding efficiency of 19.68%; and further optimized energy level alignment leads to an enhanced PCE of 20.06% in the PTQ18-based ternary device. This work demonstrates the importance of self-assembly morphology modification of organic photovoltaic molecules in improving performance of OSCs, and it has guiding role in design of high-performance organic photovoltaic materials.</p>","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":" ","pages":"e2503325"},"PeriodicalIF":27.4,"publicationDate":"2025-06-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144525599","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Ultrathin-Film Small Molecule Mixed Conductors Exhibiting Ion-Tunable Ambipolarity for High-Performance Organic Electrochemical Transistors and Multivalued Logic Inverters.","authors":"Liuyuan Lan, Yiming Wang, Xiuyuan Zhu, Iain McCulloch, Wan Yue","doi":"10.1002/adma.202501041","DOIUrl":"https://doi.org/10.1002/adma.202501041","url":null,"abstract":"<p><p>Single-component, ultrathin ambipolar organic electrochemical transistors (OECTs) combined with multivalued logic (MVL) circuits offer new opportunities for advancing next-generation bioelectronic systems due to their low-power consumption, manufacturing simplicity, and high-density integration, central to which is the evolution of ambipolar organic mixed ionic-electronic conductors (OMIECs) as channel materials. However, small-molecule analogues remain unexplored to date for lack of well-defined molecular strategies. Herein, first two acceptor-donor-acceptor-donor-acceptor-type vinyl-linked bis-diketopyrrolopyrrole-core ambipolar small-molecule OMIECs are developed featuring multiple conformational locks. It is discovered that grafting shortened glycolated sidechains produces stronger solid-state aggregation, tighter lamellar stacking, and higher crystallinity, consequently elevating the ambipolar µC* figure-of-merit by over fourfold. Furthermore, the skillful manipulation of anionic species to facilitate oxidation doping enables significant increasement in p-type µC* (170 F cm^-1 V^-1 s^-1) and a record-high n-type µC* of 360 F cm^-1 V^-1 s^-1, especially at a channel thickness of sub-10 nm. Crucially, single-component OECT-based inverters constructed therefrom are for the first time demonstrated to accommodate ternary/quaternary logic, achieving a remarkable gain of 135 V/V. This work not only provides an effective molecular design strategy for creating high-performing ultrathin-film ambipolar small-molecule OMIECs, highlighting ionic doping effect on ambipolarity, but also demonstrates their potential in MVL circuits for organic bioelectronics applications.</p>","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":" ","pages":"e2501041"},"PeriodicalIF":27.4,"publicationDate":"2025-06-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144525606","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A Light‐Driven Closed‐Loop Chemical Recycling System for Polypinacols","authors":"Ahsen Sare Yalin, Patrick Schara, Željko Tomović, Fabian Eisenreich","doi":"10.1002/adma.202506733","DOIUrl":"https://doi.org/10.1002/adma.202506733","url":null,"abstract":"The development of innovative recycling strategies for polymers is crucial to addressing the rapidly growing plastic waste challenge. While thermal ground‐state chemistry is the standard for closed‐loop chemical recycling, the potential of photochemical excited‐state chemistry remains largely unexplored. This study bridges this gap by investigating light‐driven polymerization and depolymerization processes for hydroxyl‐rich polymers. Through consecutive pinacol coupling reactions, a range of simple bis‐aldehyde monomers is photopolymerized into well‐defined polypinacols on a gram scale. These polymers exhibit excellent thermal stability, retaining their integrity up to 306 °C, with glass transition temperatures ranging from 72 to 137 °C. Using an earth‐abundant cerium photocatalyst, selective cleavage of stable C─C bonds within the polypinacol backbone is achieved under visible light, efficiently regenerating the original monomer. As this approach tolerates the presence of standard commodity plastics, it presents an opportunity for orthogonal recycling methods that could help recover specific polymers from diverse plastic waste streams. The successful completion of one recycling cycle, resulting in a polymer with comparable properties to the original, highlights the significant potential and advantages of (photo)chemical recycling.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"18 1","pages":""},"PeriodicalIF":29.4,"publicationDate":"2025-06-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144515322","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Fundamental Chemistry and Functional Mechanisms of Nitrile‐Based Electrolyte in Advanced Battery Systems","authors":"Chang Che, Ripeng Zhang, Yu Li, Huanyu Li, Shuqiang Li, Ji Qian, Yuteng Gong, Hanyang Li, Ying Bai, Feng Wu, Chuan Wu","doi":"10.1002/adma.202506504","DOIUrl":"https://doi.org/10.1002/adma.202506504","url":null,"abstract":"Nitriles have gained attention as promising candidates for secondary battery electrolytes due to the high polarity of cyano groups, excellent cathode compatibility, remarkable oxidation resistance, and broad thermal stability. As additives, nitriles effectively stabilize cathode surfaces and inhibit the dissolution of transition metals. Besides, as the electrolyte solvent, the characteristics of a wide liquidus range, excellent high‐voltage tolerance, and superior conductivity endow it with outstanding performance. Moreover, nitriles are also beneficially applied in solid‐state electrolytes, offering advantages such as strong cation coordination, excellent thermal and electrochemical stability, and enhanced ionic conductivity. However, obstacles such as side reactions with anodes, the formation of non‐robust SEI layers, and inherent toxicity hinder their broader application. Herein, the mechanism of nitriles as additives, and the application progress of nitriles in liquid electrolytes and solid‐state electrolytes are introduced in detail. Furthermore, the current challenges faced by nitriles are in depth analyzed, and the advanced modification strategies of nitriles as secondary battery electrolytes are thoroughly summarized and discussed. Additionally, the future development of nitriles in the field of secondary batteries is prospected. This review provides important references for the future development of nitrile‐based electrolytes, with guiding significance for other electrolyte solvents and additives.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"18 1","pages":""},"PeriodicalIF":29.4,"publicationDate":"2025-06-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144515309","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Bilateral Anchoring for Enhanced Mechanical Stability and Efficiency in Flexible all-Perovskite Tandem Solar Cells.","authors":"Le Geng, Yinyi Ma, Yinqing Sun, Zhuolin Cai, Lan Lan, Haochen Ma, Hao Zhang, Lin Mao, Faming Li, Mingzhen Liu","doi":"10.1002/adma.202419018","DOIUrl":"https://doi.org/10.1002/adma.202419018","url":null,"abstract":"<p><p>Flexible all-perovskite tandem solar cells (TSCs) feature an outstanding power-to-weight ratio, rendering them perfect for building-integrated photovoltaic, wearable electronics, and aerospace applications, owing to their adaptability to flexible and lightweight substrates. However, the weak mechanical adhesion between the perovskite and adjacent functional layers, combined with tin (Sn) oxidation at the buried interface in tin-lead (Sn-Pb) narrow-bandgap (NBG) perovskites solar cells (PSCs), substantially hampers the durability and performance of device. Herein, a bilateral anchoring strategy is proposed by employing 2-bromoethylamine hydrobromide (2-BH) at the NBG perovskite/ hole transporting layer (PEDOT:PSS) interface. The incorporation of 2-BH establishes robust bonds with both PEDOT:PSS and the perovskite layer, thereby enhancing interfacial adhesion and charge transfer. Meanwhile, the morphology and crystallinity of the perovskite films are also improved due to the mitigated oxidation of Sn²⁺. Thus, this approach yields flexible single-junction NBG  with a power conversion efficiency (PCE) of 18.5%, maintaining its 95% efficiency after 3000 bending cycles. When integrated into monolithic flexible all-perovskite TSCs, a certified PCE of 24.01% is achieved.</p>","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":" ","pages":"e2419018"},"PeriodicalIF":27.4,"publicationDate":"2025-06-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144525595","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Xolography for Rapid Volumetric Production of Objects from the Nanoscopic to Macroscopic Length Scales.","authors":"Xichuan Li, Yuan Xiu, Kenny Lee, Jin Zhang, Nathaniel Corrigan, Cyrille Boyer","doi":"10.1002/adma.202503245","DOIUrl":"https://doi.org/10.1002/adma.202503245","url":null,"abstract":"<p><p>Light-mediated 3D printing has revolutionized additive manufacturing, progressing from pointwise stereolithography, to layer-by-layer digital light processing, and most recently to volumetric 3D printing. Xolography, a novel light-sheet-based volumetric 3D printing approach, offers high-speed and high-precision fabrication of complex geometries unattainable with traditional methods. However, achieving nanoscale control (<100 nm) within these 3D printing systems remains unexplored. This work leverages polymerization-induced microphase separation (PIMS) within the xolography process to prepare network polymer materials with simultaneous control over feature sizes at the nano-, micro-, and macro-scale. By controlling the chain length and mass fraction of macromolecular chain transfer agents used in the PIMS process, precise manipulation of nanodomain size within 3D printed materials is demonstrated, while optimization of the other resin components enables the fabrication of rigid materials with feature sizes of 80 µm. Critically, the rapid one-step fabrication of complex and multi-component structures such as a functional waterwheel with interlocking parts, at high volume-building rates is showcased. This combined approach expands the design space for functional nanomaterials, opening new avenues for applications in diverse fields such as polymer electrolyte membranes, biomedical delivery systems, and semi-permeable microcapsules.</p>","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":" ","pages":"e2503245"},"PeriodicalIF":27.4,"publicationDate":"2025-06-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144525608","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Over a Decade of Progress in Metal-Halide Perovskite Light-Emitting Diodes","authors":"Tae-Woo Lee","doi":"10.1002/adma.202508542","DOIUrl":"https://doi.org/10.1002/adma.202508542","url":null,"abstract":"&lt;p&gt;Metal-halide perovskites have emerged as a highly promising material for light-emitting diodes (LEDs), driving significant progress in the performance of perovskite LEDs (PeLEDs), particularly in terms of external quantum efficiency (EQE), which has reached as high as 30% due to rapid progress over the past 10 years. This marks a dramatic improvement from the low EQEs of ≈0.1% observed using bulk polycrystalline films with large grains, as reported online in August 2014&lt;sup&gt;[&lt;/sup&gt;&lt;span&gt;&lt;sup&gt;1&lt;/sup&gt;&lt;/span&gt;&lt;sup&gt;]&lt;/sup&gt; and November 2014&lt;sup&gt;[&lt;/sup&gt;&lt;span&gt;&lt;sup&gt;2&lt;/sup&gt;&lt;/span&gt;&lt;sup&gt;]&lt;/sup&gt; at room temperature. Despite the inherent challenges posed by the low exciton binding energy and long exciton diffusion length of bulk perovskites,&lt;sup&gt;[&lt;/sup&gt;&lt;span&gt;&lt;sup&gt;1, 2&lt;/sup&gt;&lt;/span&gt;&lt;sup&gt;]&lt;/sup&gt; which hinder efficient radiative recombination, material strategies to overcome those limitations have been developed to confine charge carriers within nanoscale structures, referred to as nanocrystalline perovskites.&lt;sup&gt;[&lt;/sup&gt;&lt;span&gt;&lt;sup&gt;3&lt;/sup&gt;&lt;/span&gt;&lt;sup&gt;]&lt;/sup&gt; This approach enabled the first high-efficiency PeLEDs, thereby triggering a surge in research by demonstrating the potential for achieving commercially viable efficiencies comparable to those exhibited by organic light-emitting diodes (OLEDs) or inorganic quantum dot light-emitting diodes (QLEDs). Three main categories of nanocrystalline perovskites have been identified: nanoscale polycrystalline perovskites, quasi-2D perovskites, and perovskite nanocrystals (PNCs). Each perovskite has undergone distinct material engineering strategies, contributing significantly to improved device efficiencies (&lt;b&gt;Figure&lt;/b&gt; &lt;b&gt;1&lt;/b&gt;A).&lt;/p&gt;&lt;p&gt;Simultaneously, significant progress has been made in the development of charge-transporting layers (CTLs) specifically designed for perovskite materials. Research has extensively focused on optimizing the band alignment and charge mobility of CTLs, as well as their interactions with perovskite crystallization and chemical properties, leading to improved device efficiency. Additionally, several strategies have been explored to enhance the outcoupling efficiency. Perovskites, in particular, offer the unique advantage of photon recycling and scattering structures, which further contribute to increasing outcoupling efficiency (Figure 1A).&lt;/p&gt;&lt;p&gt;While the efficiency and operational lifetime of PeLEDs have improved, several challenges persist. Notably, the operational lifetime must exceed 10&lt;sup&gt;6&lt;/sup&gt; h, but the current status remains below 10&lt;sup&gt;5&lt;/sup&gt; h only for green PeLEDs. In response to concerns about lead toxicity, lead-free perovskite LEDs have achieved EQE over 20% recently, but their emissions are mainly focused on red, and their brightness and stability are still limited. Additionally, achieving high efficiency in the deep-blue emission region (&lt;465 nm) remains an ongoing challenge. Furthermore, PeLEDs emitting in the short-wave infrared (SWIR) range are still relativel","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"37 25","pages":""},"PeriodicalIF":27.4,"publicationDate":"2025-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adma.202508542","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144503015","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}