Advanced Materials最新文献

Recent Progress on Liquid Superspreading and Its Applications. 液体超扩散及其应用研究进展。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202501734

Lan Liu,Xinyu Gao,Shuangshuang Zheng,Xi Yao,Jie Ju,Lei Jiang

{"title":"Recent Progress on Liquid Superspreading and Its Applications.","authors":"Lan Liu,Xinyu Gao,Shuangshuang Zheng,Xi Yao,Jie Ju,Lei Jiang","doi":"10.1002/adma.202501734","DOIUrl":"https://doi.org/10.1002/adma.202501734","url":null,"abstract":"The dynamic spreading of liquids on solid surfaces is essential across numerous daily and industrial processes. Surfaces that enable liquid superspreading, characterized by rapid or extensive spreading, are particularly valuable due to their implications in functional film fabrication, heat management, liquid/liquid separation, and more. Recently, significant research is conducted on liquid superspreading surfaces, with microstructure-regulated surfaces gaining increasing attention. However, the deeper correlations between microstructural physical factors and the superspreading behaviors, along with the relevant applications, remain inadequately understood. This review aims to consolidate the existing knowledge from published results and stimulate further investigation by detailing structures, functionalities, and principles for constructing liquid superspreading surfaces. Examining is began by the energy balance between input and dissipation that underpins droplet spreading dynamics. Then current designs are reviewed for superspreading surfaces, with a focus on chemical and physical aspects, giving greater emphasis to the physical perspective. Additionally, several typical applications are categorized based on liquid superspreading behaviors across various fields. Finally, the prevailing challenges are highlighted and provide insights into future research directions.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"32 1","pages":"e2501734"},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144065681","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Multiplex Methionine Modulating Hydrogel for Cancer Metabolic Therapy. 多重蛋氨酸调节水凝胶用于癌症代谢治疗。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202420445

Siyu Ma,Wen Zhu,Xiaoyuan Ji,Chang Liu,Nan Chen,Daoxia Guo,Haiyun Song

{"title":"Multiplex Methionine Modulating Hydrogel for Cancer Metabolic Therapy.","authors":"Siyu Ma,Wen Zhu,Xiaoyuan Ji,Chang Liu,Nan Chen,Daoxia Guo,Haiyun Song","doi":"10.1002/adma.202420445","DOIUrl":"https://doi.org/10.1002/adma.202420445","url":null,"abstract":"The reliance on high levels of methionine by tumor cells provides an attractive target for cancer treatment. However, systemic methionine blockade may raise concerns about potential side effects given the broad and essential functions of methionine in cellular metabolism. Here, a combined drug delivery platform for multilayered constraint of methionine within tumor lesions is developed. Small molecule inhibitors PF9366 and adenosine dialdehyde are encapsulated by tumor cell-targeting nanoparticles (NPs) to achieve a cascaded blockage of intracellular methionine metabolism. These NPs are further co-loaded with the extracellular methionine uptake inhibitor JPH203 into a type of reactive oxygen species-sensitive hydrogel, assembling the multiplex methionine modulating hydrogel (3 M Gel). In murine models of triple-negative breast cancer (TNBC), hepatocellular carcinoma, and colorectal cancer, the in situ formed 3 M Gel exhibits superior efficacy in restricting S-adenosyl methionine generation and histone methylation, stimulating immunogenic cell death in tumor cells, thereby eliciting potent innate and adaptive immune responses to restrain tumor progression. Moreover, remodeling of the tumor microenvironment by 3 M Gel overcomes immune checkpoint blockade resistance in TNBC. This study presents a localized triple regulation strategy and paves a new path for amino acid starvation-based cancer therapy.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"152 1","pages":"e2420445"},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144065682","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Biomimetic Intelligent Thermal Management Materials: From Nature-Inspired Design to Machine-Learning-Driven Discovery. 仿生智能热管理材料：从自然启发设计到机器学习驱动的发现。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202503140

Heng Zhang,Qingxia He,Fei Zhang,Yanshuai Duan,Mengmeng Qin,Wei Feng

引用次数: 0

Scaling Up Purcell-Enhanced Self-Assembled Nanoplasmonic Perovskite Scintillators into the Bulk Regime 放大purcell增强的自组装纳米等离子体钙钛矿闪烁体

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202417874

Michal Makowski, Wenzheng Ye, Dominik Kowal, Francesco Maddalena, Somnath Mahato, Yudhistira Tirtayasri Amrillah, Weronika Zajac, Marcin Eugeniusz Witkowski, Konrad Jacek Drozdowski, Nathaniel, Cuong Dang, Joanna Cybinska, Winicjusz Drozdowski, Ferry Anggoro Ardy Nugroho, Christophe Dujardin, Liang Jie Wong, Muhammad Danang Birowosuto

{"title":"Scaling Up Purcell-Enhanced Self-Assembled Nanoplasmonic Perovskite Scintillators into the Bulk Regime","authors":"Michal Makowski, Wenzheng Ye, Dominik Kowal, Francesco Maddalena, Somnath Mahato, Yudhistira Tirtayasri Amrillah, Weronika Zajac, Marcin Eugeniusz Witkowski, Konrad Jacek Drozdowski, Nathaniel, Cuong Dang, Joanna Cybinska, Winicjusz Drozdowski, Ferry Anggoro Ardy Nugroho, Christophe Dujardin, Liang Jie Wong, Muhammad Danang Birowosuto","doi":"10.1002/adma.202417874","DOIUrl":"https://doi.org/10.1002/adma.202417874","url":null,"abstract":"Scintillators convert high-energy radiation into detectable photons and play a crucial role in medical imaging and security applications. The enhancement of scintillator performance through nanophotonics and nanoplasmonics, specifically using the Purcell effect, has shown promise but has so far been limited to ultrathin scintillator films because of the localized nature of this effect. This study introduces a method to expand the application of nanoplasmonic scintillators to the bulk regime. By integrating 100-nm-sized plasmonic spheroid and cuboid nanoparticles with perovskite scintillator nanocrystals, nanoplasmonic scintillators are enabled to function effectively within bulk-scale devices. Power and decay rate enhancements of up to (3.20 ± 0.20) and (4.20 ± 0.31) folds are experimentally demonstrated for plasmonic spheroid and cuboid nanoparticles, respectively, in a 5-mm thick CsPbBr<sub>3</sub> nanocrystal-polymer scintillator at RT. Theoretical modeling also predicts similar enhancements of up to (2.26 ± 0.31) and (3.02 ± 0.69) folds for the same nanoparticle shapes and dimensions. Moreover, a (2.07 ± 0.39) fold increase in light yield under <sup>241</sup>Am γ-excitation is demonstrated. These findings provide a viable pathway for utilizing nanoplasmonics to enhance bulk scintillator devices, advancing radiation detection technology.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"141 1","pages":""},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144066077","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Revealing the Degradation Mechanism of Lithium-Ion Batteries for Electric Aircraft. 揭示电动飞机用锂离子电池的退化机理。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202502363

Shihai Tang,Fu Sun,Hailong Wang,Qinlang Rong,Nuo Sun,Liang Zhang,Yuan Zhao,Qianjin Xiong,Bingxuan Huang,Linyu Hu,Jan-Philipp Hoffknecht,Zhimeng Liu,Xin He

{"title":"Revealing the Degradation Mechanism of Lithium-Ion Batteries for Electric Aircraft.","authors":"Shihai Tang,Fu Sun,Hailong Wang,Qinlang Rong,Nuo Sun,Liang Zhang,Yuan Zhao,Qianjin Xiong,Bingxuan Huang,Linyu Hu,Jan-Philipp Hoffknecht,Zhimeng Liu,Xin He","doi":"10.1002/adma.202502363","DOIUrl":"https://doi.org/10.1002/adma.202502363","url":null,"abstract":"The widespread adoption of electric vehicles has spurred the exploration of airworthy lithium-ion batteries (LIBs) for electric-powered aircraft. However, LIBs used for aviation exhibit rapid aging and shortened service life due to the harsh conditions of aviation, posing significant risks to flight safety. In this study, a comprehensive analysis is conducted under simulated flight conditions to reveal the degradation mechanism of aviation batteries. Low-temperature and low-pressure lead to a sluggish kinetics and hinder thermodynamic process. As the reversibility of Li-ions insertion and extraction is deteriorates, residual Li-ions accumulate and plated-Li on the anode, accelerating the aging process and arising the issue of internal short circuits. Additionally, the interatomic distance of Ni-coordination induces significant stress variations, which drives an expanded occupation of porosity in the electrode under flight conditions, with 2.13% void spaces of cathode and 13.39% of anode. The formation and growth of cracks elongate the charge transfer pathway, increasing resistance and reducing rate capability. As a result, this study quantifies the degradation mechanisms of aviation batteries and establishes the relative impact weights of temperature and pressure factors, offering critical insights for optimizing future electric aircraft power battery designs.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"232 1","pages":"e2502363"},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144065679","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Harnessing Photo-Energy Conversion in Nanomaterials for Precision Theranostics. 利用纳米材料中的光能转换进行精密治疗。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202501623

Jingyu Shi,Yadi Fan,Qin Zhang,Yingying Huang,Mo Yang

{"title":"Harnessing Photo-Energy Conversion in Nanomaterials for Precision Theranostics.","authors":"Jingyu Shi,Yadi Fan,Qin Zhang,Yingying Huang,Mo Yang","doi":"10.1002/adma.202501623","DOIUrl":"https://doi.org/10.1002/adma.202501623","url":null,"abstract":"The rapidly advancing field of theranostics aims to integrate therapeutic and diagnostic functionalities into a single platform for precision medicine, enabling the simultaneous treatment and monitoring of diseases. Photo-energy conversion-based nanomaterials have emerged as a versatile platform that utilizes the unique properties of light to activate theranostics with high spatial and temporal precision. This review provides a comprehensive overview of recent developments in photo-energy conversion using nanomaterials, highlighting their applications in disease theranostics. The discussion begins by exploring the fundamental principles of photo-energy conversion in nanomaterials, including the types of materials used and various light-triggered mechanisms, such as photoluminescence, photothermal, photoelectric, photoacoustic, photo-triggered SERS, and photodynamic processes. Following this, the review delves into the broad spectrum of applications of photo-energy conversion in nanomaterials, emphasizing their role in the diagnosis and treatment of major diseases, including cancer, neurodegenerative disorders, retinal degeneration, and osteoarthritis. Finally, the challenges and opportunities of photo-energy conversion-based technologies for precision theranostics are discussed, aiming to advance personalized medicine.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"71 1","pages":"e2501623"},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144065683","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Multi-Generational Frontal Curing and Chemical Recycling of Polydicyclopentadiene Thermosets. 聚双环戊二烯热固性材料的多代正面固化及化学回收。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202505141

Xuyi Luo,Yong Min Kim,M J Lee,Edgar B Mejia,Yuran Shi,Nancy R Sottos,Jeffery W Baur,Yan Xia

{"title":"Multi-Generational Frontal Curing and Chemical Recycling of Polydicyclopentadiene Thermosets.","authors":"Xuyi Luo,Yong Min Kim,M J Lee,Edgar B Mejia,Yuran Shi,Nancy R Sottos,Jeffery W Baur,Yan Xia","doi":"10.1002/adma.202505141","DOIUrl":"https://doi.org/10.1002/adma.202505141","url":null,"abstract":"Polydicyclopentadiene (pDCPD) is a high-performance thermoset with lightweight and exceptional thermomechanical properties. However, its traditional thermal curing process is energy-intensive and lacks chemical recyclability. Frontal Ring-Opening Metathesis Polymerization (FROMP) is an energy-efficient curing process and allows additive manufacturing of pDCPD. 2,3-Dihydrofuran (DHF) has been shown as an effective comonomer to allow the deconstruction of pDCPD thermosets when incorporated at a small fraction in pDCPD. Herein, a simple strategy for chemical recycling of pDCPD thermosets is reported, and maintaining FROMP characteristics and thermomechanical properties of the thermosets over five life cycles. Norbornadiene (NBD) is a key additive in resins containing recycled pDCPD to enhance polymerization kinetics and sustain FROMP characteristics. A one-pot strategy is also developed to deconstruct pDCPD thermosets and simultaneously functionalize the chain ends with norbornenes for reincorporating deconstructed oligomers back to the next generation thermoset. Using these strategies, five generations of recycling pDCPD thermosets with invariable thermomechanical properties are demonstrated. This work highlights a scalable and energy-efficient process to produce chemically recyclable pDCPD thermosets, significantly improving the circularity of this class of high-performance thermosets.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"35 1","pages":"e2505141"},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144065952","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Optogenetics-Inspired Nanofluidic Artificial Dendrite with Spatiotemporal Integration Functions. 具有时空集成功能的光遗传学启发纳米流体人工树突。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202502438

Zhuangzhuang Li,Ya Lin,Xuanyu Shan,Zhongqiang Wang,Xiaoning Zhao,Ye Tao,Haiyang Xu,Yichun Liu

{"title":"Optogenetics-Inspired Nanofluidic Artificial Dendrite with Spatiotemporal Integration Functions.","authors":"Zhuangzhuang Li,Ya Lin,Xuanyu Shan,Zhongqiang Wang,Xiaoning Zhao,Ye Tao,Haiyang Xu,Yichun Liu","doi":"10.1002/adma.202502438","DOIUrl":"https://doi.org/10.1002/adma.202502438","url":null,"abstract":"Dendrites play an essential role in processing functions by facilitating the integration of spatial and temporal information in biological system. Nanofluidic memristors, which harness ions for signal transmission within electrolyte solutions, closely resemble biological neuronal ion channels and hold the potential for the development of biorealistic neuromorphic devices. Herein, inspired by the optogenetic technique that utilized light to tune the ions dynamic, an optical-controlled nanofluidic artificial dendrite by embedding layered graphene oxide (GO) within a polydimethylsiloxane (PDMS) elastomer is developed. Taking advantage of the confinement effect of ions in the nanochannel, it has demonstrated optically-modulated ionic currents, which can effectively replicate dendritic functions. The mechanism can be attributed to the migration of Na+ ions, driven by the electric potential difference light illumination. The dendritic spatial and temporal multiport integrations are realized, including the dendritic sublinear/superlinear integrations and spike-rate-dependent plasticity (SRDP). Moreover, the hand withdrawal reflex, as a crucial mode of neuroregulation governed by central nerve and brain control signals, is replicated in the nanofluidic dendrite-based neuromorphic system, capable of managing a range of withdrawal states of a mechanical arm. This work offers a new strategy for developing nanofluidic artificial dendrite and paves the way toward developing advanced neuromorphic sensorimotor systems.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"40 1","pages":"e2502438"},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144065903","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Traceless Photopolymerization with Non-Pulsed Red Light Enables 3D-Printable Cell-Laden Hydrogels. 无痕迹光聚合与非脉冲红光使3d打印细胞负载水凝胶。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202502386

Ali Eftekhari,Kelsey Rianne de Graaf,Ekaterina Takmakova,Hatai Jongprasitkul,Alexander Efimov,Sanna Turunen,Andrew Kerr,Minna Kellomäki,Robert Luxenhofer,Timo Laaksonen,Nikita Durandin

{"title":"Traceless Photopolymerization with Non-Pulsed Red Light Enables 3D-Printable Cell-Laden Hydrogels.","authors":"Ali Eftekhari,Kelsey Rianne de Graaf,Ekaterina Takmakova,Hatai Jongprasitkul,Alexander Efimov,Sanna Turunen,Andrew Kerr,Minna Kellomäki,Robert Luxenhofer,Timo Laaksonen,Nikita Durandin","doi":"10.1002/adma.202502386","DOIUrl":"https://doi.org/10.1002/adma.202502386","url":null,"abstract":"Photocrosslinking of hydrogels with non-pulsed red light offers improved biocompatibility and deep tissue penetration in contrast to traditional UV-initiated methods. However, hydrogels fabricated upon red-light excitation are always colored by a photoinitiator, limiting their use in applications requiring high optical transparency, such as (bio)sensors, ophthalmological applications, or wound dressings. Additionally, the cytotoxicity of a photoinitiator is always a concern, especially in bioapplications. Herein, a photoinitiating system composed of an FDA-approved methylene blue photosensitizer and cytocompatible triethanolamine is introduced. The system can induce photopolymerization upon 625 nm irradiation and leaves no visible trace of the methylene blue color afterward, thus named \"traceless\". With this approach, gelatine methacrylate hydrogel is successfully polymerized under ambient conditions. The hydrogel is permanently colorless with well-controlled stiffness due to the light-dependent nature of the polymerization process. The system is further successfully applied in extrusion-based 3D-bioprinting with NIH-3T3 fibroblasts, followed by photocuring to produce cell-laden 3D structures, indicating its potential for tissue engineering. Upon culturing the cell-laden constructs, the fibroblasts are able to proliferate and adhere to the hydrogel material. The red-light excitation enables polymerization through at least 5 mm of biological tissue, projecting, inter alia, its use for transdermal photopolymerization in minimally invasive implantation.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"5 1","pages":"e2502386"},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144065912","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

4D-Printed Adaptive and Programmable Shape-Morphing Batteries. 4d打印自适应和可编程变形电池。

IF 29.4 1区材料科学

Advanced Materials Pub Date : 2025-05-16 DOI: 10.1002/adma.202505018

Shaoshuai Ma,Pan Xue,Cristian Valenzuela,Yuan Liu,Yuanhao Chen,Yufan Feng,Ran Bi,Xinnuo Yang,Yanzhao Yang,CaiXia Sun,Xinhua Xu,Ling Wang

{"title":"4D-Printed Adaptive and Programmable Shape-Morphing Batteries.","authors":"Shaoshuai Ma,Pan Xue,Cristian Valenzuela,Yuan Liu,Yuanhao Chen,Yufan Feng,Ran Bi,Xinnuo Yang,Yanzhao Yang,CaiXia Sun,Xinhua Xu,Ling Wang","doi":"10.1002/adma.202505018","DOIUrl":"https://doi.org/10.1002/adma.202505018","url":null,"abstract":"Shape-morphing batteries that can reconfigure their shape to adapt to different tasks are highly desirable for emerging soft electronics in diverse fields. However, it is a challenging task to develop advanced shape-morphing batteries with on-demand programmability and adaptive responsiveness. Here, 4D-printed programmable shape-morphing batteries by sequentially direct-ink-writing of shape-programmable liquid crystal elastomers (LCEs) and in-situ covalent crosslinked flexible zinc-ion microbatteries, where tough covalent bonding is built at the interface, are reported. The resulting shape-morphing batteries exhibit controllable, reversible, and programmable shape-morphing by controlling sophisticated molecular alignment of LCEs, which enables them to adaptively alter configurations to accommodate different functionalities. Importantly, diverse origami batteries with excellent spatiotemporal controllability are demonstrated by precisely designing active hinges to achieve adaptive transformations from folded to deployed configurations. The programmable shape-morphing mechanisms of the batteries are revealed by finite element analyses. As a proof-of-concept illustration, adaptive shape-morphing battery systems capable of interactive communication and controllable sensing are developed through the incorporation of an elaborate all-MXene-printed near-field-communication antenna, which can adaptively tune its deployment configuration according to variations in environmental humidity or dust content. This work brings new insights for the development of next-generation shape-morphing power sources, human-machine interactive electronics, and swarm intelligence.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"30 1","pages":"e2505018"},"PeriodicalIF":29.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144065908","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0