Energy & Environmental Science最新文献

{"title":"Unraveling Structure-performance Relationship in Hard Carbon for Sodium-ion Battery by Coupling Key Structural Parameters","authors":"Chun Wu, Yunrui Yang, Yifan Li, Xiangxi He, Yinghao Zhang, Wenjie Huang, Qinghang Chen, Xiaohao Liu, Shuangqiang Chen, Qinfen Gu, Lin Li, Sean C. Smith, Xin Tan, Yan Yu, Xingqiao Wu, Shulei Chou","doi":"10.1039/d5ee00278h","DOIUrl":"https://doi.org/10.1039/d5ee00278h","url":null,"abstract":"The electrochemical performance of hard carbon anode for sodium-ion batteries is primarily determined by the microstructure of materials, and the challenge lies in establishing structure-performance relationship at molecular level. So far, the understanding of intricate relationship between structure and performance in hard carbon remains piecemeal, with research efforts scattered across various aspects, thereby numerous controversies have arisen in this field. Here, we provide new insights into structure-performance relationship in hard carbon by coupling key structural parameters based on integrating theoretical computations and experimental data. Density functional theory calculations show that interlayer spacing determines diffusion behavior of sodium ions in hard carbon, while appropriate defect and curvature secure high-quality intercalation capacity. Inspired by these theoretical results, we successfully produce high-performance hard carbon with optimal microstructures through in-situ molecular reconfiguration of biomass via thermodynamically-driven approach, which is demonstrated as an effective strategy to rationally regulate the microstructure of hard carbon by comprehensive physical characterizations from macroscopic to atomic level. More importantly, cylindrical batteries (18650 and 33140 types) fabricated from industrial-scale hard carbon exhibit fabulous sodium storage behaviors with excellent wide-range temperature performance (-40-100 oC), demonstrating great potential for achieving practical sodium-ion batteries with high energy density and durability in the future.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"33 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143872286","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Designing multi-tentacle electrolytes to enable fast and deep cycling of aqueous Zn batteries at low temperatures","authors":"Huimin Wang, Mingzi Sun, Yongqiang Yang, Junhua Zhou, Lingtao Fang, Qiyao Huang, Bolong Huang, Zijian Zheng","doi":"10.1039/d5ee01316j","DOIUrl":"https://doi.org/10.1039/d5ee01316j","url":null,"abstract":"Rechargeable aqueous zinc batteries (AZBs) offer a safe and sustainable solution for large-scale energy storage, but the freezing of electrolytes prevents AZBs from working at low temperatures. Recent research shows that the freezing point can be effectively lowered by using either concentrated salt or organic-rich electrolytes. However, these strategies result in either low oxidation stability or sluggish mass transport at low temperatures. Here, we report a multi-tentacle electrolyte (MTE) strategy that enables stable, fast and deep running of AZBs at −40 °C. MTE leverages the abundant hydrogen-bonding sites of multi-tentacle salts and organics. Adding small amounts of multi-tentacle moieties not only effectively confines water molecules’ movement and prevents their icing even at −60 °C, but also maintains low viscosity and high ionic conductivity of the electrolyte at low temperatures. At −40 °C, Zn metal anodes could stably cycle for more than 1100 hours at a high current density of 2 mA cm−2 and a high capacity of 2 mAh cm−2; high-capacity AZBs (3.4 mAh cm−2) sustain 1000 stable cycling with 99.99% retention per cycle in MTE. MTE strategy is also versatile to high-voltage LiMn2O4 cathodes, which further enhances the energy density of AZBs to 154.4 Wh kgLMO−1 at −40 °C.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"1 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143872288","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Identifying the role of Zn self-dissolution in the anode corrosion process in Zn-ion batteries","authors":"Yi Yuan, Zixuan Li, Rongyu Deng, Shengda D. Pu, Marc Walker, Mingzhi Cai, Feixiang Wu, Peter G. Bruce, Alex Robertson","doi":"10.1039/d5ee00485c","DOIUrl":"https://doi.org/10.1039/d5ee00485c","url":null,"abstract":"Zn-ion batteries for practical applications face several challenges, some of which arise from the inevitable degradation of the Zn metal anode. The intrinsic thermodynamic instability of Zn metal anodes in mildly acidic Zn-ion batteries can trigger spontaneous interfacial corrosion, which leads to hydrogen evolution, the formation of byproducts, and the irreversible loss of active species during both storage and operation. Here, we delve into the intricate corrosion processes of the Zn metal anode in mildly acidic electrolytes. With the help of operando electrochemical liquid cell transmission electron microscopy, the self-dissolution of Zn is observed, and the capacity loss due to such corrosion behaviour during the cell rest period is quantified. This dissolution of Zn is found to be closely related to the initial pH value of the electrolyte and can be mitigated by pH adjustment through the slight addition of a pH buffer additive. The self-dissolution of Zn, which causes an increase in the local pH, is a prelude to the formation of corrosion byproducts that continues throughout the entire storage and cycling period. These corrosion issues are exacerbated by the presence of excess Zn metal in the system, suggesting that the feasibility of using excess Zn metal in Zn-ion batteries should be carefully evaluated. These findings further emphasise the importance of considering electrolyte pH in future electrolyte modification research, as well as its potential impacts on the stability of both the anode and cathode, and the shelf life of the entire battery.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"1 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143872290","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Mechanisms and Scale-up Potential of 3D Solar Interfacial-Evaporators","authors":"James Han Zhang, Rohith Mittapally, Abimbola Oluwade, Gang Chen","doi":"10.1039/d5ee01104c","DOIUrl":"https://doi.org/10.1039/d5ee01104c","url":null,"abstract":"Evaporation fluxes from porous evaporators under sunlight have been reported to exceed the solar-thermal limit, determined by relating the incoming solar energy to the latent and sensible heat of water, for applications in desalination and brine pond drying. Although flat two-dimensional (2D) evaporators exceeding the solar limit implies a non-thermal process, tall three-dimensional (3D) solar evaporators can exceed it by absorbing additional environmental heat into its cold sidewalls. Through modeling, we explain the physics and identify the critical heights in which a fin transitions from 2D to 3D evaporation and exceeds the solar-thermal limit. Our analyses illustrate that environmental heat absorption in 3D evaporators is determined by the ambient relative humidity and the airflow velocity. The model is then coarse-grained into a large-scale fin array device on the meters scale to analyze their scalability. We identify that these devices are unlikely to scale favorably in closed environment settings such as solar stills. Our modeling clearly illustrates the benefits and limitations of 3D evaporating arrays and pinpoints design choices in previous works that hinder the device’s overall performance. This work illustrates the importance in distinguishing 2D from 3D evaporation for mechanisms underlying interfacial evaporation exceeding the solar-thermal limit.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"31 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143866905","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Techno-Economic and Life-Cycle Assessment for Syngas Production Using Sustainable Plasma-Assisted Methane Reforming Technologies","authors":"Marc Escribà-Gelonch, Jose Luis Osorio-Tejada, Le Yu, Bart Wanten, Annemie Bogaerts, Volker Hessel","doi":"10.1039/d4ee05129g","DOIUrl":"https://doi.org/10.1039/d4ee05129g","url":null,"abstract":"This study combines for the first time techno-economic and life-cycle assessment metrics to evaluate the economic and environmental viability of plasma-assisted dry reforming of methane (DRM) for producing syngas from methane-rich natural gas. The study compares three different processes (plasma-assisted dry reforming (CO<small><sub>2</sub></small>/CH<small><sub>4</sub></small>), oxi-CO<small><sub>2</sub></small> reforming (CO<small><sub>2</sub></small>/CH<small><sub>4</sub></small>/O<small><sub>2</sub></small>) and bi-reforming (CO<small><sub>2</sub></small>/CH<small><sub>4</sub></small>/H<small><sub>2</sub></small>O)), as well as with current state-of-the-art steam reforming technology. Advancements in cost reduction and environmental performance are highlighted. While comparative studies on different plasma processing concepts have been published, their number is not large; meaning this study is bespoke in this aspect. Our study is also bespoken in extensive consideration of industrial gas separation, to provide a holistic view on sustainability with industrial viewpoint. Three different production design scenarios were considered in the analysis: DRM (scenario 1), oxy-CO<small><sub>2</sub></small> reforming of CH<small><sub>4</sub></small> (OCRM) (scenario 2), and bi-reforming of CH<small><sub>4</sub></small> (BRM) (scenario 3). This evaluation was carried out through a techno-economic analysis and a cradle-to-gate life cycle assessment (LCA). Among the scenarios analysed, OCRM demonstrates the most favourable economic performance, leading to a unitary cost of production of 549 $/tonne syngas, followed by DRM and BRM. However, when operating at large scale, the syngas production cost of BRM could compete with the benchmark if 20% reduction in plasma power consumption can be achieved, so in the near future, plasma-based BRM could be competitive against other more mature electric-powered technologies. When assessing environmental performance across 10 environmental categories of LCA metrics, OCRM is again preferred, followed by DRM and BRM. Key impact categories identified include freshwater eutrophication potential and energy consumption, which are significant contributors to environmental impacts. A study on the transition of energy sources indicates a substantial decrease in global environmental impact in the range of 50% when shifting from current electricity generation methods to wind energy sources. Comparative benchmarking reveals that the technologies evaluated in all three plasma scenarios perform better in environmental metrics across 7 over 9 categories assessed, when compared with current state-of-the-art steam reforming technologies. A material circularity indicator around 0.7 is obtained in all scenarios with slight differences, reflecting a medium-high level of circularity. Sectors such as chemicals, and recycling manufacturing could greatly benefit from our findings on plasma-assisted methane reforming. By leveraging these techn","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"13 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143866908","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Screening thermoelectric materials for high output performance in wearable electronics","authors":"Xinjie Yuan, Pengfei Qiu, Chuanyao Sun, Shiqi Yang, Yi Wu, Yumeng Wang, Ming Gu, Lidong Chen, Xun Shi","doi":"10.1039/d5ee00216h","DOIUrl":"https://doi.org/10.1039/d5ee00216h","url":null,"abstract":"Thermoelectric (TE) technology provides a promising self-powered solution to the wearable electronics and Internet of Things (IoT), but the output voltage density and power density of current TE devices are still far below the target values for practical use. In this work, instead of the commonly used TE figure-of-merit (zT = S2σ/κT, where S is the Seebeck coefficient, σ is the electrical conductivity, κ is the thermal conductivity, and T is the absolute temperature), we propose that |S|/κ and S2σ/κ2are more effective indicators to screen the TE materials for the development of powerful TE devices used in the exacting working conditions (e.g. windless indoor environment and extremely limited space) for wearable electronics and IoT. As a case study, both the simulation and experiment well prove that the TE device consisting of n-type Ag1.995Au0.005Te0.7S0.3 and p-type Ag0.9Sb1.1Te2.1 with high |S|/κ and S2σ/κ2 can achieve higher output performance than the Bi2Te3-based TE device. When the Ag1.995Au0.005Te0.7S0.3/Ag0.9Sb1.1Te2.1 TE device is worn on human wrist, record-high voltage density and power density are achieved. This work brings a new insight to the development of advanced TE devices used for the wearable electronics and IoT.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"18 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143862365","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Unlocking High-Performance Photocapacitors for Edge Computing in Low-Light Environments","authors":"Natalie Flores Diaz, Francesca De Rossi, Timo Keller, George Harvey Morritt, Zaida Perez- Bassart, A. Lopez-Rubio, Maria Fabra Rovira, Richard Freitag, Alessio Gagliardi, Francesca Fasulo, Ana Belen Munoz-Garcia, Michele Pavone, Hamed Javanbakht Lomeri, Sandy Sánchez, Michael Grätzel, Francesca Brunetti, Marina Freitag","doi":"10.1039/d5ee01052g","DOIUrl":"https://doi.org/10.1039/d5ee01052g","url":null,"abstract":"Driving continuous, low-power artificial intelligence (AI) in the Internet of Things (IoT) requires reliable energy harvesting and storage under indoor or low-light conditions, where batteries face constraints such as finite lifetimes and increased environmental impact. Here, we demonstrate an integrated three-terminal dye-sensitized photocapacitor that unites a dye-sensitized solar cell (DSC) with an asymmetric supercapacitor, leveraging molecularly engi- neered polyviologen electrodes and bioderived chitosan membranes. Under 1000 lux ambient illumination, the photocapacitor delivers photocharging voltages of 920 mV, achieving power conversion efficiencies exceeding 30% and photocharging efficiencies up to 18%. Density Functional Theory calculations reveal low reorganization energies (0.1–0.2 eV) for polyviologen radical cations, promoting efficient charge transfer and stable cycling performance over 3000 charge-discharge cycles. The system reliably powers a multilayer IoT network at 500 lux for 72 hours, surpassing commercial amorphous-silicon modules by a factor of 3.5 in inference throughput. Critically, the photocapacitor driven edge microcontroller achieves 93% accuracy on CIFAR-10 classification with an energy requirement of only 0.81 mJ per inference. By eliminating the need for batteries or grid connection, this work offers a proof of concept for high-efficiency, long-lived indoor power solutions that merge advanced materials chemistry with edge AI, demonstrating a practical route toward self-sustaining, data-driven IoT devices.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"24 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143862363","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Multi-H-Bonded Self-Assembled Superstructures for Ultrahigh-Capacity and Ultralong-Life All-Organic Ammonium-Ion Batteries","authors":"Pingxuan Liu, Ziyang Song, Qi Huang, Ling Miao, Yaokang Lv, Lihua Gan, Mingxian Liu","doi":"10.1039/d5ee00823a","DOIUrl":"https://doi.org/10.1039/d5ee00823a","url":null,"abstract":"All-organic ammonium-ion batteries (AOBs) with light organic electrodes and small-hydrated-sized NH4+ charge carriers are up-and-coming for next-generation energy storage. However, the low NH4+-accessible redox-active motifs of organics with high coordination barriers pose significant challenges for advancing AOBs. Here we design multi-H-bonded donor-acceptor self-assembled ultralow-coordination-barrier organic superstructures (OSs) by fusing six-electron melem modules (H-bond donor) and three-electron cyanuric acid units (H-bond acceptor) via in-plane H-bonding and out-of-plane π-π stacking. OSs with low-energy-bandgap conjugated planar configuration and long-range π-electron delocalization paths promise full utilization (99.3%) of built-in redox-active carbonyl/imine motifs with an ultralow activation energy (0.16 eV). Consequently, a high-kinetics and ultrastable 15 e− NH4+ coordination mechanism within OSs cathode is initiated, liberating ultrahigh capacity (393 mAh g−1cathode) and ultralong stability (60,000 cycles). Significantly, the superior metrics of OSs electrode enable the state-of-the-art AOBs with record capacity (213 mAh g−1) and unprecedented lifespan (100,000 cycles). This work offers new insights into the structural engineering of multi-active low-coordination-barrier OSs for advanced aqueous batteries.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"126 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143862366","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A Large Conjugated Rigid Dimer Acceptor Enables 20.19% Efficiency in Organic Solar Cells","authors":"Wendi Shi, Qiansai Han, Wenkai Zhao, Ruohan Wang, Longyu Li, Guangkun Song, Xin Chen, Guankui Long, Zhaoyang Yao, Yan Lu, Chenxi Li, Xiangjian Wan, Yongsheng Chen","doi":"10.1039/d5ee00878f","DOIUrl":"https://doi.org/10.1039/d5ee00878f","url":null,"abstract":"Non-fullerene acceptors with a large conjugated rigid skeleton are conducive to promoting low disorder and reducing non-radiative recombination loss (ΔEnr), thereby improving open voltage(Voc) in organic solar cells (OSCs). However, an unfavorable active layer morphology is often formed due to excessive aggregation of these acceptors, which leads to a low short-circuit current density (Jsc) and fill factor (FF), and significantly lower device efficiencies. In this study, we report a dimer acceptor, QD-1, featuring a large conjugated rigid skeleton, which exhibits low energy disorder, small reorganization energy and weakened electro-photon coupling. All of these contribute to a reduction in ΔEnr and improved charge mobility. Benefiting from the above advantages as well as favorable fibrillar morphology, the binary OSC based on PM6:QD-1 showed high and balanced device parameters in Voc , Jsc, and FF, resulting in a high power conversion efficiency (PCE) of 19.46%, which is highest reported for binary OSCs utilizing dimer acceptors. Furthermore, by incorporating QD-1 into the PM6:BTP-eC9 system, a remarkable PCE of 20.19% is achieved, accompanied by all three photovoltaic parameters improved, thanks to the optimized morphology of the active layer. Additionally, a module (13.5cm2) based on the ternary system achieves a high PCE of 17.33%.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"37 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143862558","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Dual strain regulated RhNiAu trimetallene for efficient plasmonic-promoted acidic nitrate electroreduction","authors":"Wei Zhong, Qing-Ling Hong, Qiu-Yu Du, Bao Yu Xia, Xuan Ai, Fumin Li, Yu Chen","doi":"10.1039/d5ee00788g","DOIUrl":"https://doi.org/10.1039/d5ee00788g","url":null,"abstract":"Nitrate electroreduction reaction (NO3ERR) under acidic conditions provides a green and sustainable pathway for acidic industrial wastewater treatment and ammonia (NH3) synthesis. As a typical multi-electron transfer and proton-coupled reaction, acidic NO3ERR is hindered by competing hydrogen evolution reaction (HER) and intrinsically slow kinetics. Herein, we report a strategy to regulate the electronic structure of Rh by introducing coupled in-plane and out-of-plane compressive strain into RhNiAu trimetallene (RhNiAu-TML), thereby suppressing HER and accelerating NO3ERR kinetics. The surface Rh-Au single-atom alloy and subsurface Rh-Ni alloy impart a total compressive strain of 4.1% to RhNiAu-TML. The significantly compressed Rh atoms effectively decrease the formation of underpotentially deposited hydrogen to suppress the Volmer step of HER and reduce the adsorption energy of *NO intermediate to promote its hydrogenation during NO3ERR, resulting in improved NO3ERR performance with a high NH3 Faradaic efficiency of 97.9 ± 2%, a remarkable NH3 yield rate of 21.6 ± 0.35 mg h−1 mgcat−1 and outstanding stability for 120 h at +0.05 V versus reversible hydrogen electrode. Additionally, the Au nanocrystal anchored on RhNiAu-TML can result in plasmon-enhanced NO3ERR, which is further validated in the zinc-nitrate battery, achieving a power density of up to 22.1 mW cm−2 under light illumination.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"41 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143862364","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}